arXiv subjects

Vinay Pramod Majety

Publications and source records attributed to Vinay Pramod Majety.

7 recordsLinked to original sources

arXiv2024

Single-photon and multi-photon Fano lines for helium and neon using tRecX-haCC

Single-photon and multi-photon ionization of helium and neon atoms by ultrashort extreme ultraviolet radiation is studied. The wavelength of radiation is chosen to excite a set of doubly excited states. We analyse the lineshapes arising from the presence of doubly excited states and numerically demonstrate the sensitivity of the Fano $q$ parameter to the order of multi-photon process. The computations were performed using the tRecX-haCC package developed by the authors. The tRecX-haCC package solves the time-dependent Schrödinger equation in the presence of a laser pulse and computes the photoelectron spectra including the narrow resonance peaks using the tSurff and iSurf techniques.

physics.atom-ph↗

arXiv2017

Multielectron effects in strong field ionization of CO$_2$: impact on differential photoelectron spectra

We report fully differential photoelectron spectra from an {\it ab-inito} coupled channels treatment of CO$_2$. Photoionization by laser pulses centered at 400 nm and 800 nm wavelength are considered, with arbitrary molecular alignment and polarization (linear and elliptic). Calculations reveal significant excited state channel contributions that are, at certain molecular orientations, an order of magnitude larger than the ground state channel in the rescattering plateau. Partial wash out of the multiphoton structure in the ATI spectra and of the nodal features in angle resolved spectra is observed due to ionization to excited state channels. The qualitative nature of the spectra is determined by ionization thresholds, orbital symmetries and interchannel coupling in the order of precedence.

physics.atom-ph↗

arXiv2015

Double photo-electron momentum spectra of Helium at infrared wavelength

Double photo-electron momentum spectra of the Helium atom are calculated \textit{ab initio} at extreme ultra-violet and near infrared wavelengths. At short wavelengths two-photon double ionization yields, two-electron energy spectra, and triply differential cross sections agree with results from recent literature. At the near infrared wavelength of $780\,nm$ the experimental single-to-double ionization ratio is reproduced up to intensities of $4\times 10^{14}W/cm^2$, and two-electron energy spectra and joint angular distributions are presented. The time-dependent surface flux (tSurff) approach is extended to full 3+3 spatial dimensions and systematic error control is demonstrated. We analyze our differential spectra in terms of an experimentally accessible quantitative measure of correlation.

physics.comp-ph↗

arXiv2015

Anomalous Fano Profiles in External Fields

We show that external control of Fano resonances in general leads to complex Fano $q$-parameters. Fano line shapes of photo-electron and transient absorption spectra in presence of an infrared control field are investigated. Computed transient absorption spectra are compatible with a recent experiment [C. Ott {\it et al.}, Science 340, 716 (2013)] but suggest a modification of the interpretation proposed there. Control mechanisms for photo-electron spectra are exposed: control pulses applied {\em during} excitation modify the line shapes by momentum boosts of the continuum electrons. Pulses arriving {\em after} excitation generate interference fringes due to infrared two-photon transitions.

physics.atom-ph↗

arXiv2015

Dynamic exchange in the strong field ionization of molecules

We show that dynamic exchange is a dominant effect in strong field ionization of molecules. In $CO_2$ it fixes the peak ionization yield at the experimentally observed angle of $45^\circ$ between polarization direction and the molecular axis. In $N_2$ it changes the alignment dependence of yields by up to a factor of 2. The effect appears on the Hartree-Fock level as well as in full {\it ab initio} solutions of the Schrödinger equation.

physics.atom-ph↗

arXiv2014

Photoionization of few electron systems with a hybrid Coupled Channels approach

We present the hybrid anti-symmetrized coupled channels method for the calculation of fully differential photo-electron spectra of multi-electron atoms and small molecules interacting with strong laser fields. The method unites quantum chemical few-body electronic structure with strong-field dynamics by solving the time dependent Schrödinger equation in a fully anti-symmetrized basis composed of multi-electron states from quantum chemistry and a one-electron numerical basis. Photoelectron spectra are obtained via the time dependent surface flux (tSURFF) method. Performance and accuracy of the approach are demonstrated for spectra from the helium and berryllium atoms and the hydrogen molecule in linearly polarized laser fields at wavelength from 21 nm to 400 nm. At long wavelengths, helium and the hydrogen molecule at equilibrium inter-nuclear distance can be approximated as single channel systems whereas beryllium needs a multi-channel description.

physics.comp-ph↗

arXiv2014

Mixed gauge in strong laser-matter interaction

We show that the description of laser-matter interaction in length gauge at short short and in velocity gauge at longer distances allows for compact physical modeling in terms of field free states, rapidly convergent numerical approximation, and efficient absorption of outgoing flux. The mathematical and numerical framework for using mixed gauge in practice is introduced. We calculate photoelectron spectra generated by a laser field at wavelengths of 400$\sim$800 nm from single-electron systems and from the helium atom and hydrogen molecule. We assess the accuracy of coupled channels calculations by comparison to full two-electron solutions of the time-dependent Schrodinger equation and find substantial advantages of mixed over velocity and length gauges.

physics.comp-ph↗