arXiv subjects

Vincent Jacques

Publications and source records attributed to Vincent Jacques.

39 records · Page 3Linked to original sources

arXiv2007

Enhancing single-molecule photostability by optical feedback from quantum-jump detection

We report an optical technique that yields an enhancement of single-molecule photostability, by greatly suppressing photobleaching pathways which involve photoexcitation from the triplet state. This is accomplished by dynamically switching off the excitation laser when a quantum-jump of the molecule to the triplet state is optically detected. This procedure leads to a lengthened single-molecule observation time and an increased total number of detected photons. The resulting improvement in photostability unambiguously confirms the importance of photoexcitation from the triplet state in photobleaching dynamics, and may allow the investigation of new phenomena at the single-molecule level.

quant-ph↗

arXiv2006

Experimental realization of Wheeler's delayed-choice GedankenExperiment

The quantum "mystery which cannot go away" (in Feynman's words) of wave-particle duality is illustrated in a striking way by Wheeler's delayed-choice GedankenExperiment. In this experiment, the configuration of a two-path interferometer is chosen after a single-photon pulse has entered it : either the interferometer is \textit{closed} (\textit{i.e.} the two paths are recombined) and the interference is observed, or the interferometer remains \textit{open} and the path followed by the photon is measured. We report an almost ideal realization of that GedankenExperiment, where the light pulses are true single photons, allowing unambiguous which-way measurements, and the interferometer, which has two spatially separated paths, produces high visibility interference. The choice between measuring either the 'open' or 'closed' configuration is made by a quantum random number generator, and is space-like separated -- in the relativistic sense -- from the entering of the photon into the interferometer. Measurements in the closed configuration show interference with a visibility of 94%, while measurements in the open configuration allow us to determine the followed path with an error probability lower than 1%.

quant-ph↗

arXiv2005

Narrow-band single-photon emission in the near infrared for quantum key distribution

We report on the observation of single colour centers in natural diamond samples emitting in the near infrared region when optically excited. Photoluminescence of these single emitters have several striking features, such as a narrow-band fully polarized emission (FWHM 2 nm) around 780 nm, a short excited-state lifetime of about 2 ns, and perfect photostability at room temperature under our excitation conditions. We present a detailed study of their photophysical properties. Development of a triggered single-photon source relying on this single colour centre is discussed in the prospect of its application to quantum key distribution.

quant-ph↗