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Vincenzo Giannini

Publications and source records attributed to Vincenzo Giannini.

At least 19 recordsLinked to original sources

Far-field radiation of bulk, edge and corner eigenmodes from a finite 2D Su-Schrieffer-Heeger plasmonic lattice

Subwavelength arrays of plasmonic nanoparticles allow us to control the behaviour of light at the nanoscale. Here, we develop an eigenmode analysis, employing a coupled electromagnetic dipole formalism, which permits us to isolate the contribution to the far-field radiation of each array mode. Specifically, we calculate the far-field radiation patterns by bulk, edge and corner out-of-plane eigenmodes in a finite 2D Su-Schrieffer-Heeger (SSH) array of plasmonic nanoparticles with out-of-plane dipolar resonances. The breaking of symmetries in multipartite unit cells is exploited to tailor the optical properties and far-field radiation of the resonant modes. We prove that the antisymmetric modes are darker and have higher Q-factors than their symmetric counterparts. Also, the out-of-plane nature of the dipolar resonances imposes that all bulk $Γ$-modes are dark, while corner and edge states need extra in-plane symmetries to cancel the far-field radiation; radiation patterns in turn become more complex and concentrated along the array plane with increasing array size.

cond-mat.mes-hall↗

Long-range molecular energy transfer mediated by strong coupling to plasmonic topological edge states

Strong coupling between light and molecular matter is currently attracting interest both in chemistry and physics, in the fast-growing field of molecular polaritonics. The large near-field enhancement of the electric field of plasmonic surfaces and their high tunability make arrays of metallic nanoparticles an interesting platform to achieve and control strong coupling. Two dimensional plasmonic arrays with several nanoparticles per unit cell and crystalline symmetries can host topological edge and corner states. Here we explore the coupling of molecular materials to these edge states using a coupled-dipole framework including long-range interactions. We study both the weak and strong coupling regimes and demonstrate that coupling to topological edge states can be employed to enhance highly-directional long-range energy transfer between molecules.

cond-mat.mes-hall↗

Casimir nanoparticle levitation in vacuum with broadband perfect magnetic conductor metamaterials

The levitation of nanoparticles is essential in various branches of research. Casimir forces are natural candidates to tackle it but the lack of broadband metamaterials precluded repulsive forces in vacuum. We show sub-micron nanoparticle levitation in vacuum only based on the design of a broadband metamaterial perfect magnetic conductor surface, where the force is mostly given by the (quantum) zero-point contribution. In the harmonic regime of the center of mass dynamics, the characteristic frequency depends linearly on Planck's constant $\hbar$ while independent of the nanoparticle's volume.

quant-ph↗

Exploiting oriented field projectors to open topological gaps in plasmonic nanoparticle arrays

In the last years there have been multiple proposals in nanophotonics to mimic topological condensed matter systems. However, nanoparticles have degrees of freedom that atoms lack of, like dimensions or shape, which can be exploited to explore topology beyond electronics. Elongated nanoparticles can act like projectors of the electric field in the direction of the major axis. Then, by orienting them in an array the coupling between them can be tuned, allowing to open a gap in an otherwise gapless system. As a proof of the potential of the use of orientation of nanoparticles for topology, we study 1D chains of prolate spheroidal silver nanoparticles. We show that in these arrays spatial modulation of the polarization allows to open gaps, engineer hidden crystalline symmetries and to switch on/off or left/right edge states depending on the polarization of the incident electric field. This opens a path towards exploiting features of nanoparticles for topology to go beyond analogues of condensed matter systems.

physics.optics↗

High temperature nanocomposites with photonic group velocity suppression of thermal emission

Quenching of thermal emission above 0 K is an unusual material property, essential for future energy, transportation, and space technologies. Despite the great effort invested, nearly complete quenching of thermal radiation rather than some reduction of its flux has only been achieved at low temperatures (below 373 K) and in narrow spectral windows using complex techniques suitable only for small scale objects. In this work, we present a light and flexible composite material that can suppress propagating photonic modes and, in this way, quench thermal radiation while preserving heat transfer (by thermal conduction) at a room and higher temperature below 600 K. This has been achieved by altering the local photonic density of states and consequentially the thermal properties of carbon nanotubes forming a percolating nanofiber network with a thermostable polymeric matrix.

physics.optics↗

Engineering bound states in the continuum at telecom wavelengths with non-Bravais lattices

Various optical phenomena can be induced in periodic arrays of nanoparticles by the radiative coupling of the local dipoles in each particle. Probably the most impressive example is bound states in the continuum (BICs), which are electromagnetic modes with a dispersion inside the light cone but infinite lifetime, i.e., modes that cannot leak to the continuum. Symmetry-protected BICs appear at highly symmetric points in the dispersion of periodic systems. Although the addition of nonequivalent lattice points in a unit cell is an easy and straightforward way of tuning the symmetry, BICs in such particle lattice, i.e., non-Bravais lattice, are less explored among periodic systems. Starting from a periodic square lattice of Si nanodisks, we have prepared three non-Bravais lattices by detuning size and position of the second disk in the unit cell. Diffraction-induced coupling excites magnetic/electric dipoles in each nanodisk, producing two surface lattice resonances at the $Γ$ point with a band gap in between. %of $\sim$ 41 meV. The high/low energy branch becomes a BIC for the size/position-detuned array, respectively, while both branches are bright (or leaky) when both size and position are detuned simultaneously. The role of magnetic and electric resonances in dielectric nanoparticles and the change of BIC to bright character of the modes is explained by the two different origins of BICs in the detuned arrays, which is further discussed with the aid of a coupled electric and magnetic dipole model. This study gives a simple way of tuning BICs at telecom wavelengths in non-Bravais lattices, including both plasmonic and dielectric systems, thus scalable to a wide range of frequencies.

physics.optics↗

Negative reflection of polaritons at the nanoscale in a low-loss natural medium

Negative reflection occurs when light is reflected towards the same side of the normal to the boundary from which it is incident. This exotic optical phenomenon, which provides a new avenue towards light manipulation, is not only yet to be visualized in real space but remains largely unexplored both at the nanoscale and in natural media. Here, we directly visualize nanoscale-confined polaritons negatively reflecting on subwavelength mirrors fabricated in a low-loss van der Waals crystal. Our near-field nanoimaging results unveil an unconventional and broad tunability of both the polaritonic wavelength and direction of propagation upon negative reflection. Based on these findings, we introduce a novel device in nano-optics: a hyperbolic nanoresonator, in which hyperbolic polaritons with different momenta reflect back to a common point source, enhancing its intensity. These results pave the way to realize nanophotonics in low-loss natural media, providing a novel and efficient route to confine and control the flow of light at the nanoscale, key for future optical on-chip nanotechnologies.

physics.optics↗

Proposal for THz lasing from a topological quantum dot

Topological quantum dots (TQDs) are 3D topological insulator nanoparticles with radius below 100 nm, which display symmetry-protected surface states with discretized energies. We propose a scheme which harnesses these energy levels in a closed lasing scheme, in which a single TQD, when pumped with incoherent THz light, lases from its surface states in the THz regime. The time scales associated with the system are unusually slow, and lasing occurs with a very low threshold. Due to the low threshold, we predict that blackbody radiation at room-temperature provides enough photons to pump the system, providing a route to room-temperature THz lasing with blackbody radiation as the pump.

cond-mat.mes-hall↗

Ultrabroad-Band Direct Digital Refractive Index Imaging Based on Suspended Graphene Plasmon Cavities

Mid-infrared spectroscopy is essential for chemical identification and compositional analysis, due to the existence of characteristic molecular absorption fingerprints. However, it is very challenging to determine the refractive index of an analyte at low concentrations using current photonic systems in a broad mid-infrared spectral range. We propose an imaging-based nanophotonic technique for refractive index determination. The technique is based on deeply subwavelength graphene plasmon cavities and allows for the retrieval of molecular concentration. This method features a two-dimensional array of suspended graphene plasmon cavities, in which the extremely high field enhancement and extraordinary compression of graphene plasmons can be realized simultaneously by combining shallow and deep cavities. This enables resonant unit cells to be read out in the spatial absorption pattern of the array at multiple spectral points, and the resulting information is then translated into the refractive index of the analytes. The proposed technique gives complementary information compared with the current nanophotonic techniques based on molecular absorption, including the ability of the refractive index measurement, the ultra-broadband measurable spectral range, and the small volume of the analyte required, thereby pushing the potential for refractometric sensing technologies into the infrared frequencies.

physics.optics↗

Tuning the period of femtosecond laser induced surface structures in steel: from angled incidence to quill writing

Exposure of metal surfaces to multiple ultrashort laser pulses under certain conditions leads to the formation of well-defined periodic surface structures. We show how the period of such structures in steel can be tuned over a wide range by controlling the complex interaction mechanisms triggered in the material. Amongst the different irradiation parameters that influence the properties of the induced structures, the angle of incidence of the laser beam occupies a prominent role. We present an experimental and theoretical investigation of this angle dependence in steel upon irradiation with laser pulses of 120 fs duration and 800 nm wavelength, while moving the sample at constant speed. Our findings can be grouped into two blocks. First, we observe the spatial coexistence of two different ripple periods at the steel surface, both featuring inverse scaling upon angle increase, which are related to forward and backward propagation of surface plasmon polaritons. To understand the underlying physical phenomena, we extend a recently developed model that takes into account quantitative properties of the surface roughness to the case of absorbing metals (large imaginary part of the dielectric function), and obtain an excellent match with the experimentally observed angle dependence. As second important finding, we observe a quill writing effect, also termed non-reciprocal writing, in form of a significant change of the ripple period upon reversing the sample movement direction. This remarkable phenomenon has been observed so far only inside dielectric materials and our work underlines its importance also in laser surface processing. We attribute the origin of symmetry breaking to the non-symmetric micro- and nanoscale roughness induced upon static multiple pulse irradiation, leading to non-symmetric modification of the wavevector of the coupled surface plasmon polariton.

physics.app-ph↗

Berry bands and pseudo-spin of topological photonic phases

Realising photonic analogues of the robust, unidirectional edge states of electronic topological insulators would improve our control of light on the nanoscale and revolutionise the performance of photonic devices. Here we show that new symmetry protected topological phases can be detected by reformulating energy eigenproblems as Berry curvature eigenproblems. The "Berry bands" span the same eigenspace as the original valence energy bands, but separate into pseudo-spinful and pseudo-spinless subspaces in $\mathrm{C}_2\mathcal{T}$-symmetric crystals. We demonstrate the method on the well-known case of Wu & Hu [Phys. Rev. Lett. 114, 223901 (2015)] and a recently discovered fragilely topological crystal, and show that both crystals belong to the same $\mathrm{C}_2\mathcal{T}$-protected $\mathbb{Z}_2$ topological phase. This work helps unite theory and numerics, and is useful in defining and identifying new symmetry-protected phases in photonics and electronics.

physics.optics↗

Near- and Far-Field Excitation of Topological Plasmonic Metasurfaces

The breathing honeycomb lattice hosts a topologically non-trivial bulk phase due to the crystalline-symmetry of the system. Pseudospin-dependent edge states which emerge at the interface between trivial and non-trivial regions can be used for directional propagation of energy. Using the plasmonic metasurface as an example system, we probe these states in the near and far-field using a semi-analytical model. We give the conditions under which directionality is observed and show that it is source position dependent. By probing with circularly-polarized magnetic dipoles out of the plane, we first characterize modes along the interface in terms of the enhancement of source emission due to the metasurface. We then excite from the far-field with non-zero orbital angular momentum beams. The position dependent directionality holds true for all classical wave systems with a breathing honeycomb lattice. Our results show that a metasurface in combination with a chiral two-dimensional material could be used to guide light effectively on the nanoscale.

cond-mat.mes-hall↗

Exciting Pseudospin Dependent Edge States in Plasmonic Metasurfaces

We study a plasmonic metasurface that supports pseudospin dependent edge states confined at a subwavelength scale, considering full electrodynamic interactions including retardation and radiative effects. The spatial symmetry of the lattice of plasmonic nanoparticles gives rise to edge states with properties reminiscent of the quantum spin Hall effect in topological insulators. However, unlike the spin-momentum locking characteristic of topological insulators, these modes are not purely unidirectional and their propagation properties can be understood by analysing the spin angular momentum of the electromagnetic field, which is inhomogenous in the plane of the lattice. The local sign of the spin angular momentum determines the propagation direction of the mode under a near-field excitation source. We also study the optical response under far-field excitation and discuss in detail the effects of radiation and retardation.

cond-mat.mes-hall↗

Laser-plasma accelerated protons: energy increase in gas-mixtures using high mass number atomic species

The idea of using a gas-mixture comprising atoms with high mass number in order to increase proton energies in laser induced plasma acceleration at under critical density is investigated by means of 2D PIC (Particle-In-Cell) simulations. Comparing and discussing the case of a pure hydrogen plasma, and that of a plasma containing higher mass number species with a small percentage of hydrogen, we demonstrated that the mixture enhances the energies of the accelerated protons. We also show that using a gas-mixture introduces the possibility of using the densities ratio to change the relative acceleration of the species.

physics.plasm-ph↗

Experimental signature of a topological quantum dot

Topological insulators (TIs) present a neoteric class of materials, which support delocalised, conducting surface states despite an insulating bulk. Due to their intriguing electronic properties, their optical properties have received relatively less attention. Even less well studied is their behaviour in the nanoregime, with most studies thus far focusing on bulk samples - in part due to the technical challenges of synthesizing TI nanostructures. We study topological insulator nanoparticles (TINPs), for which quantum effects dominate the behaviour of the surface states and quantum confinement results in a discretized Dirac cone, whose energy levels can be tuned with the nanoparticle size. The presence of these discretized energy levels in turn leads to a new electron-mediated phonon-light coupling in the THz range. We present the experimental realisation of Bi$_2$Te$_3$ TINPs and strong evidence of this new quantum phenomenon, remarkably observed at room temperature. This system can be considered a topological quantum dot, with applications to room temperature THz quantum optics and quantum information technologies.

cond-mat.mes-hall↗

Bulk-edge correspondence and long range hopping in the topological plasmonic chain

The existence of topologically protected edge modes is often cited as a highly desirable trait of topological insulators. However, these edge states are not always present. A realistic physical treatment of long range hopping in a one-dimensional dipolar system can break the symmetry that protects the edge modes without affecting the bulk topological number, leading to a breakdown in bulk-edge correspondence. It is important to find a better understanding of where and how this occurs, as well as how to measure it. Here we examine the behaviour of the bulk and edge modes in a dimerised chain of metallic nanoparticles and in a simpler non-Hermitian next-nearest-neighbour model to provide some insight into the phenomena of bulk-edge breakdown. We construct bulk-edge correspondence phase diagrams for the simpler case and use these ideas to devise a measure of symmetry-breaking for the plasmonic system based on its bulk properties. This provides a parameter regime for which bulk-edge correspondence is preserved in the topological plasmonic chain, as well as a framework for assessing this phenomenon in other systems.

cond-mat.mes-hall↗

A perspective on topological nanophotonics: current status and future challenges

Topological photonic systems, with their ability to host states protected against disorder and perturbation, allow us to do with photons what topological insulators do with electrons. Topological photonics can refer to electronic systems coupled with light or purely photonic setups. By shrinking these systems to the nanoscale, we can harness the enhanced sensitivity observed in nanoscale structures and combine this with the protection of the topological photonic states, allowing us to design photonic local density of states and to push towards one of the ultimate goals of modern science: the precise control of photons at the nanoscale. This is paramount for both nano-technological applications and also for fundamental research in light matter problems. For purely photonic systems, we work with bosonic rather than fermionic states, so the implementation of topology in these systems requires new paradigms. Trying to face these challenges has helped in the creation of the exciting new field of topological nanophotonics, with far-reaching applications. In this prospective article we review milestones in topological photonics and discuss how they can be built upon at the nanoscale.

cond-mat.mes-hall↗

Extraordinarily transparent compact metallic metamaterials

Metals are highly opaque, yet we show that densely packed arrays of metallic nanoparticles can be more transparent to infrared radiation than dielectrics such as germanium, even for arrays that are over 75% metal by volume. Despite strong interactions between the metallic particles, these arrays form effective dielectrics that are virtually dispersion-free, making possible the design of optical components that are achromatic over ultra-broadband ranges of wavelengths from a few microns up to millimetres or more. Furthermore, the local refractive indices may be tuned by altering the size, shape, and spacing of the nanoparticles, allowing the design of gradient-index lenses that guide and focus light on the microscale. The electric field is also strongly concentrated in the gaps between the metallic nanoparticles, and the simultaneous focusing and squeezing of the electric field produces strong `doubly-enhanced' hotspots which could boost measurements made using infrared spectroscopy and other non-linear processes over a broad range of frequencies, with minimal heat production.

physics.optics↗