arXiv subjects

Vincenzo Macrì

Publications and source records attributed to Vincenzo Macrì.

At least 19 recordsLinked to original sources

arXiv2026

Explanation of the Observed Energy Exchange through the vacuum in Optomechanics

In cavity optomechanics, the standard large-detuning regime is commonly described by retaining only the radiation-pressure interaction, while higher-order mirror--field interactions are assumed to be negligible. This approximation, however, fails to provide a microscopic explanation for the vacuum-mediated heat transfer observed between the mechanical membranes in the experiment of Fong, et.al.,[Nature \textbf{576}, 243 (2019)], whose physical origin has remained under active debate. Here, using a fully quantum model, we show that the neglected higher-order optomechanical interactions naturally generate phonon-phonon coupling and quantitatively account for the observed energy exchange within the standard optomechanical framework. Building on this microscopic description, we further propose a protocol in which phonon-phonon interaction drives a cyclic process enabling net work extraction. Our results establish the fundamental role of higher-order optomechanical interactions and provide a microscopic framework for describing next-generation optomechanical experiments beyond the linear approximation.

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arXiv2026

Dissipative phase transitions and chaos in two-photon driven quantum optomechanics

We investigate nonequilibrium criticality and chaos in a two-photon-driven optomechanical system. The parametric drive preserves a discrete $\mathbb{Z}_2$ symmetry of the optical field, while radiation-pressure coupling transfers the resulting nonlinear dynamics to a mechanical oscillator. Combining semiclassical stability analysis, exact Liouvillian spectra, and stochastic quantum trajectories, we show that this driven-dissipative optomechanical model supports both first- and second-order dissipative phase transitions. At negative detuning a second-order transition yields spontaneous breaking of the cavity-parity symmetry in the thermodynamic limit. At positive detuning the same symmetry breaking coexists with a first-order transition, signaled by metastability and by an additional symmetric Liouvillian mode. At stronger pump power the mean-field dynamics loses all stable fixed points and develops limit cycles and chaotic attractors with positive Lyapunov exponent. Quantum trajectories in this regime display chaotic-like motion, enhanced steady-state entropy, and delocalization over many entropic Liouvillian modes. These results establish two-photon-driven optomechanics as a platform where dissipative criticality, symmetry breaking, and quantum signatures of chaos emerge within the same experimentally accessible setting.

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arXiv2026

Floquet Dissipative Phase Transitions

Dissipative phase transitions (DPTs) are traditionally characterized through the spectrum of a time-independent Liouvillian superoperator. However, this definition does not apply to time-periodic (Floquet) systems that cannot be exactly recast as time-independent problems. Here, we develop a general framework to characterize DPTs in time-periodic open quantum systems through the spectrum of the Floquet propagator. We first study driven-dissipative Kerr resonators, known to display a DPT, showing that counter-rotating terms in the drive shift the critical point and significantly change the time scales associated with the transition. We then investigate DPTs in the driven quantum Rabi model and its time-independent approximation, the driven Jaynes-Cummings model, finding that the Rabi model exhibits distinct critical features as the ultrastrong coupling regime is approached. Moreover, our Floquet analysis unveils the disappearance of the DPT in the deep strong coupling regime, due to light-matter decoupling. Our approach sets the stage for the study of dissipative criticality in a broad class of time-dependent open quantum systems.

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arXiv2026

High-order interactions in quantum optomechanics: fluctuations, dynamics and thermodynamics

Quantum optomechanics describes the interaction between a confined field and a fluctuating wall due to radiation pressure. The dynamics of this system is typically understood using perturbation theory up to second order in the small coupling. Improving beyond this regime can shed light onto new phenomena. In this work we study high-order resonant wall-field interactions characterized by two- and three-phonon scattering processes. We obtain the Hamiltonian, compute the perturbed energy spectrum and explicitly calculate corrections to the ground state. Finally, we study the dynamics of the system when second- and third-order resonance conditions are activated, showing that the presence of high-order terms in the Hamiltonian drastically affects the populations of all particles, as well as the entropy production rate.

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arXiv2026

An asymptotic field approach for the control of dipole emission in integrated structures

We present a general framework to model spontaneous emission in integrated photonic structures by exploiting quantization of the electromagnetic field in terms of asymptotic in/out modes. This approach allows for an efficient and physically meaningful calculation of the emission rate into each radiative channel of an arbitrary structure, without relying on approximations such as Lorentzian lineshapes or point-like system-bath coupling. We show that with this approach one can recover well-known results for dipole emission in waveguides or ring resonators, and that such results can be easily extended to include the effect of backscattering. Finally, as an application, we design a tunable integrated single-photon source that enables full control over both the emission rate and output mode. This flexibility makes our method particularly well-suited for the design and analysis of integrated single-photon sources in various material platforms.

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arXiv2025

Bilateral photon emission from a vibrating mirror and multiphoton entanglement generation

Entanglement plays a crucial role in the development of quantum-enabled devices. One significant objective is the deterministic creation and distribution of entangled states, achieved, for example, through a mechanical oscillator interacting with confined electromagnetic fields. In this study, we explore a cavity resonator containing a two-sided perfect mirror. Although the mirror separates the cavity modes into two independent confined electromagnetic fields, the radiation pressure interaction gives rise to high-order effective interactions across all subsystems. Depending on the chosen resonant conditions, which are also related to the position of the mirror, we study $2n$-photon entanglement generation and bilateral photon pair emission. Demonstrating the non-classical nature of the mechanical oscillator, we provide a pathway to control these phenomena, opening potential applications in quantum technologies. Looking ahead, similar integrated devices could be used to entangle subsystems across vastly different energy scales, such as microwave and optical photons.

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arXiv2023

Phonon-photon conversion as mechanism for cooling and coherence transfer

The dynamical Casimir effect is the physical phenomenon where the mechanical energy of a movable wall of a cavity confining a quantum field can be converted into quanta of the field itself. This effect has been recognized as one of the most astonishing predictions of quantum field theory. At the quantum scale, the energy conversion can also occur incoherently, namely without an physical motion of the wall. We employ quantum thermodynamics to show that this phenomenon can be employed as a tool to cool down the wall when there is a non-vanishing temperature gradient between the wall and the cavity. At the same time, the process of heat-transfer enables to share the coherence from one cavity mode, driven by a laser, to the wall, thereby forcing its coherent oscillation. Finally, we show how to employ one laser drive to cool the entire system including the case when it is composed of other subsystems.

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arXiv2023

Quantum field heat engine powered by phonon-photon interactions

We present a quantum heat engine based on a cavity with two oscillating mirrors that confine a quantum field as the working substance. The engine performs an Otto cycle during which the walls and a field mode interact via a nonlinear Hamiltonian. Resonances between the frequencies of the cavity mode and the walls allow to transfer heat from the hot and the cold bath by exploiting the conversion between phononic and photonic excitations. We study the time evolution of the system and show that net work can be extracted after a full cycle. We evaluate the efficiency of the process.

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arXiv2023

Coherent Resonant Coupling between Atoms and a Mechanical Oscillator Mediated by Cavity-Vacuum Fluctuations

We show that an atom can be coupled to a mechanical oscillator via quantum vacuum fluctuations of a cavity field enabling energy transfer processes between them. In a hybrid quantum system consisting of a cavity resonator with a movable mirror and an atom, these processes are dominated by two pair-creation mechanisms: the counterrotating (atom-cavity system) and dynamical Casimir interaction terms (optomechanical system). Because of these two pair-creation mechanisms, the resonant atom-mirror coupling is the result of high-order virtual processes with different transition paths well described in our theoretical framework. We perform a unitary transformation to the atom-mirror system Hamiltonian, exhibiting two kinds of multiple-order transitions of the pair creation. By tuning the frequency of the atom, we show that photon frequency conversion can be realized within a cavity of multiple modes. Furthermore, when involving two atoms coupled to the same mechanical mode, a single vibrating excitation of the mechanical oscillator can be simultaneously absorbed by the two atoms. Considering recent advances in strong and ultrastrong coupling for cavity optomechanics and other systems, we believe our proposals can be implemented using available technology.

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arXiv2022

Spontaneous Scattering of Raman Photons from Cavity-QED Systems in the Ultrastrong Coupling Regime

We show that spontaneous Raman scattering of incident radiation can be observed in cavity-QED systems without external enhancement or coupling to any vibrational degree of freedom. Raman scattering processes can be evidenced as resonances in the emission spectrum, which become clearly visible as the cavity-QED system approaches the ultrastrong coupling regime. We provide a quantum mechanical description of the effect, and show that ultrastrong light-matter coupling is a necessary condition for the observation of Raman scattering. This effect, and its strong sensitivity to the system parameters, opens new avenues for the characterization of cavity QED setups and the generation of quantum states of light.

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arXiv2022

Pure Dephasing of Light-Matter Systems in the Ultrastrong and Deep-Strong Coupling Regimes

Pure dephasing originates from the non-dissipative information exchange between quantum systems and environments, and plays a key-role in both spectroscopy and quantum information technology. Often pure dephasing constitutes the main mechanism of decay of quantum correlations. Here we investigate how pure dephasing of one of the components of a hybrid quantum system affects the dephasing rate of the system transitions. We find that, in turn, the interaction, in the case of a light-matter system, can significantly affect the form of the stochastic perturbation describing the dephasing of a subsystem, depending on the adopted gauge. Neglecting this issue can lead to wrong and unphysical results when the interaction becomes comparable to the bare resonance frequencies of subsystems, which correspond to the ultrastrong and deep-strong coupling regimes. We present results for two prototypical models of cavity quantun electrodynamics: the quantum Rabi and the Hopfield model.

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arXiv2021

Regimes of Cavity-QED under Incoherent Excitation: From Weak to Deep Strong Coupling

The prototypical system constituted by a two-level atom interacting with a quantized single-mode electromagnetic field is described by the quantum Rabi model (QRM). The QRM is potentially valid at any light-matter interaction regime, ranging from the weak (where the decay rates exceeds the coupling rate) to the deep strong coupling (where the interaction rate exceeds the bare transition frequencies of the subsystems). However, when reaching the ultrastrong coupling regime, several theoretical issues may prevent the correct description of the observable dynamics of such a system: (i) the standard quantum optics master equation fails to correctly describe the interaction of this system with the reservoirs; (ii) the correct output photon rate is no longer proportional to the intracavity photon number; and (iii) the appears to violate gauge invariance. Here, we study the photon flux emission rate of this system under the incoherent excitation of the two-level atom for any light-matter interaction strength, and consider different effective temperatures. The dependence of the emission spectra on the coupling strength is the result of the interplay between energy levels, matrix elements of the observables, and the density of states of the reservoirs. Within this approach, we also study the occurence of light-matter decoupling in the deep strong coupling regime, and show how all of the obtained results are gauge invariant.

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arXiv2021

Dissipative state transfer and Maxwell's demon in single quantum trajectories: Excitation transfer between two noninteracting qubits via unbalanced dissipation rates

We introduce a protocol to transfer excitations between two noninteracting qubits via purely dissipative processes (i.e., in the Lindblad master equation there is no coherent interaction between the qubits). The fundamental ingredients are the presence of collective (i.e. nonlocal) dissipation and unbalanced local dissipation rates (the qubits dissipate at different rates). The resulting quantum trajectories show that the measurement backaction changes the system wave function and induces a passage of the excitation from one qubit to the other. While similar phenomena have been witnessed for a non-Markovian environment, here the dissipative quantum state transfer is induced by an update of the observer knowledge of the wave function in the presence of a Markovian (memoryless) environment -- this is a single quantum trajectory effect. Beyond single quantum trajectories and postselection, such an effect can be observed by histogramming the quantum jumps along several realizations at different times. By investigating the effect of the temperature in the presence of unbalanced local dissipation, we demonstrate that, if appropriately switched on and off, the collective dissipator can act as a Maxwell's demon. These effects are a generalized measure equivalent to the standard projective measure description of quantum teleportation and Maxwell's demon. They can be witnessed in state-of-the-art setups given the extreme experimental control in, e.g., superconducting qubits or Rydberg atoms.

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arXiv2019

Emission of photon pairs by mechanical stimulation of the squeezed vacuum

To observe the dynamical Casimir effect (DCE) induced by a moving mirror is a long-standing challenge because the mirror velocity needs to approach the speed of light. Here, we present an experimentally feasible method for observing this mechanical DCE in an optomechanical system. It employs a detuned, parametric driving to squeeze a cavity mode, so that the mechanical mode, with a typical resonance frequency, can parametrically and resonantly couple to the squeezed cavity mode, thus leading to a resonantly amplified DCE in the squeezed frame. The DCE process can be interpreted as {\it mechanically-induced two-photon hyper-Raman scattering} in the laboratory frame. Specifically, {\it a photon pair} of the parametric driving absorbs a single phonon and then is scattered into an anti-Stokes sideband. We also find that the squeezing, which additionally induces and amplifies the DCE, can be extremely small. Our method requires neither an ultra-high mechanical-oscillation frequency (i.e., a mirror moving at nearly the speed of light) nor an ultrastrong single-photon optomechanical coupling and, thus, could be implemented in a wide range of physical systems.

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arXiv2019

Conversion of Mechanical Noise into Correlated Photon Pairs: Dynamical Casimir effect from an incoherent mechanical drive

We show that the dynamical Casimir effect in an optomechanical system can be achieved under incoherent mechanical pumping. We adopt a fully quantum-mechanical approach for both the cavity field and the oscillating mirror. The dynamics is then evaluated using a recently-developed master equation approach in the dressed picture, including both zero and finite temperature photonic reservoirs. This analysis shows that the dynamical Casimir effect can be observed even when the mean value of the mechanical displacement is zero. This opens up new possibilities for the experimental observation of this effect. We also calculate cavity emission spectra both in the resonant and the dispersive regimes, providing useful information on the emission process.

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arXiv2018

Dissipation and Thermal Noise in Hybrid Quantum Systems in the Ultrastrong Coupling Regime

The interaction among the components of a hybrid quantum system is often neglected when considering the coupling of these components to an environment. However, if the interaction strength is large, this approximation leads to unphysical predictions, as has been shown for cavity-QED and optomechanical systems in the ultrastrong-coupling regime. To deal with these cases, master equations with dissipators retaining the interaction between these components have been derived for the quantum Rabi model and for the standard optomechanical Hamiltonian. In this article, we go beyond these previous derivations and present a general master equation approach for arbitrary hybrid quantum systems interacting with thermal reservoirs. Specifically, our approach can be applied to describe the dynamics of open hybrid systems with harmonic, quasi-harmonic, and anharmonic transitions. We apply our approach to study the influence of temperature on multiphoton vacuum Rabi oscillations in circuit QED. We also analyze the influence of temperature on the conversion of mechanical energy into photon pairs in an optomechanical system, which has been recently described at zero temperature. We compare our results with previous approaches, finding that these sometimes overestimate decoherence rates and understimate excited-state populations.

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arXiv2018

Interaction of Mechanical Oscillators Mediated by the Exchange of Virtual Photon Pairs

Two close parallel mirrors attract due to a small force (Casimir effect) originating from the electromagnetic quantum vacuum uctuations of the electromagnetic field. These vacuum uctuations can also induce motional forces exerted upon one mirror when the other one moves. Here we consider an optomechanical system consisting of two vibrating mirrors coupled to an optical resonator. We find that motional forces can determine noticeable coupling rates between the two spatially separated vibrating mirrors. We show that, by tuning the two mechanical oscillators into resonance, energy is exchanged between them at the quantum level. This coherent motional coupling is enabled by the exchange of virtual photon pairs, originating from the dynamical Casimir effect. The process proposed here shows that the electromagnetic quantum vacuum is able to transfer mechanical energy somewhat like an ordinary uid. We show that this system can also operate as a mechanical parametric down-converter even at very weak excitations. These results demonstrate that vacuuminduced motional forces open up new possibilities for the development of optomechanical quantum technologies.

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arXiv2018

Simple preparation of Bell and GHZ states using ultrastrong-coupling circuit QED

The ability to entangle quantum systems is crucial for many applications in quantum technology, including quantum communication and quantum computing. Here, we propose a new, simple, and versatile setup for deterministically creating Bell and Greenberger-Horne-Zeilinger (GHZ) states between photons of different frequencies in a two-step protocol. The setup consists of a quantum bit (qubit) coupled ultrastrongly to three photonic resonator modes. The only operations needed in our protocol are to put the qubit in a superposition state, and then tune its frequency in and out of resonance with sums of the resonator-mode frequencies. By choosing which frequency we tune the qubit to, we select which entangled state we create. We show that our protocol can be implemented with high fidelity using feasible experimental parameters in state-of-the-art circuit quantum electrodynamics. One possible application of our setup is as a node distributing entanglement in a quantum network.

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