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Vitaly N. Golovach

Publications and source records attributed to Vitaly N. Golovach.

At least 19 recordsLinked to original sources

Theory of Spin-splitter Magnetoresistance in Altermagnets

We develop a theory of angular-dependent magnetoresistance (ADMR) in metallic altermagnets coupled to ferromagnetic insulators and establish criteria that distinguish them from conventional compensated magnets with spin-orbit coupling. We show that, once its full set of angular dependencies is established, the spin-splitter magnetoresistance (SSMR)-- recently reported in the bilayer geometry of H. Chen et al. [Adv. Mater. 37, 2507764 (2025)] -- would constitute a smoking-gun signature of collinear d-wave altermagnetism in metallic systems. Although SSMR has been regarded as a close analogue of spin Hall magnetoresistance (SMR), we demonstrate that the two differ qualitatively in three key respects: SSMR depends solely on the relative orientation between the ferromagnetic magnetization and the altermagnetic Néel vector, yields a longitudinal ADMR response of opposite sign, and features a direct proportionality between longitudinal and transverse ADMR signals, absent in SMR. Building on these distinctions, we further show that the full angular dependence of the SSMR provides a practical recipe to extract the direction of the Néel vector from customary magnetoresistance measurements. These results provide a clear route to unambiguously identify altermagnets in transport.

cond-mat.mes-hall↗

Surface States in Strain-Induced Nodal-Line Topological Semiconductors

This work explores the topological phase diagram of inverted-band-gap semiconductors under strain and spin-orbit coupling. Using a minimalistic Luttinger Hamiltonian model, we follow the transitions between a 3D topological insulator, a Dirac semimetal, a nodal-line semimetal, and a Weyl semimetal. Analytical and exact solutions for surface states are derived for high-symmetry directions as well as in several limiting cases. We demonstrate the continuous evolution of these surface states across phase boundaries, providing a unified picture that synthesizes previous literature. Specifically, we detail the progression from a Dirac to a nodal-line and then to a Weyl semimetal as spin-orbit coupling originating from bulk inversion asymmetry is introduced. A hierarchy of energy scales is established, defining the criteria for realizing these phases. Finally, we reveal a non-analyticity in the surface-state dispersion at the projected nodal line, originating from distinct, terminating patches of surface states with unique spin textures in momentum space.

cond-mat.mes-hall↗

Weak-anti-localization-to-spin-dependent scattering at a proximity-magnetized heavy metal interface

A change in a materials electrical resistance with magnetic field (magnetoresistance) results from quantum interference effects and, or spin-dependent transport, depending on materials properties and dimensionality. In disordered conductors, electron interference leads to weak localization or anti-localization; in contrast, ferromagnetic conductors support spin-dependent scattering, leading to giant magnetoresistance (GMR). By varying the thickness of Au between 4 and 28 nm in a EuS/Au/EuS spin-switches, we observe a crossover from weak anti-localization to interfacial GMR. The crossover is related to a magnetic proximity effect in Au due to electron scattering at the insulating EuS interface. The proximity-induced exchange field in Au suppresses weak anti-localization, consistent with Maekawa-Fukuyama theory. With increasing Au thickness, GMR emerges along with spin Hall magnetoresistance. These findings demonstrate spin transport governed by interfacial exchange fields, building a framework for spintronic functionality without metallic magnetism.

cond-mat.mtrl-sci↗

Quasiparticle density of states and triplet correlations in superconductor/ferromagnetic-insulator structures across a sharp domain wall

A ferromagnetic insulator (FI) in contact with a superconductor (S) is known to induce a spin splitting of the BCS density of states at the FI/S interface. This spin splitting causes the Cooper pairs to reduce their singlet-state correlations and acquire odd-in-frequency triplet correlations. We consider a diffusive FI/S bilayer with a sharp magnetic domain wall in the FI and study the local quasiparticle density of states and triplet superconducting correlations. In the case of collinear alignment of the domains, we obtain analytical results by solving the Usadel equation. For a small enough exchange field or weak superconductivity, we also find an analytical expression for arbitrary magnetic textures, which reveals how the triplet component vector depends on the local magnetization of the FI. For an arbitrary angle between the magnetizations and the strength of the exchange field, we numerically solve the problem of a sharp domain wall. We finally propose two different setups based on FI/S/F stacks, where F is a ferromagnetic layer, to filter out singlet pairs and detect the presence of triplet correlations via tunneling differential conductance measurements.

cond-mat.supr-con↗

Paramagnetic spin Hall magnetoresistance

Spin Hall magnetoresistance (SMR) refers to a resistance change in a metallic film reflecting the magnetization direction of a magnet attached to the film. The mechanism of this phenomenon is spin exchange between conduction-electron spins and magnetization at the interface. SMR has been used to read out information written in a small magnet and to detect magnetization dynamics, but it has been limited to magnets; magnetic ordered phases or instability of magnetic phase transition has been believed to be indispensable. Here, we report the observation of SMR in a paramagnetic insulator Gd$_{3}$Ga$_{5}$O$_{12}$ (GGG) without spontaneous magnetization combined with a Pt film. The paramagnetic SMR can be attributed to spin-transfer torque acting on localized spins in GGG. We determine the efficiencies of spin torque and spin-flip scattering at the Pt/GGG interface, and demonstrate these quantities can be tuned with external magnetic fields. The results clarify the mechanism of spin-transport at a metal/paramagnetic insulator interface, which gives new insight into the spintronic manipulation of spin states in paramagnetic systems.

cond-mat.mtrl-sci↗

Strong interfacial exchange field in a heavy metal/ferromagnetic insulator system determined by spin Hall magnetoresistance

Spin-dependent transport at heavy metal/magnetic insulator interfaces is at the origin of many phenomena at the forefront of spintronics research. A proper quantification of the different interfacial spin conductances is crucial for many applications. Here, we report the first measurement of the spin Hall magnetoresistance (SMR) of Pt on a purely ferromagnetic insulator (EuS). We perform SMR measurements in a wide range of temperatures and fit the results by using a microscopic model. From this fitting procedure we obtain the temperature dependence of the spin conductances ($G_s$, $G_r$ and $G_i$), disentangling the contribution of field-like torque ($G_i$), damping-like torque ($G_r$), and spin-flip scattering ($G_s$). An interfacial exchange field of the order of 1 meV acting upon the conduction electrons of Pt can be estimated from $G_i$, which is at least three times larger than $G_r$ below the Curie temperature. Our work provides an easy method to quantify this interfacial spin-splitting field, which play a key role in emerging fields such as superconducting spintronics and caloritronics, and topological quantum computation.

cond-mat.mes-hall↗

Spin-Hall magnetoresistance in a low-dimensional magnetic insulator

We observe an unusual behavior of the spin Hall magnetoresistance (SMR) measured in a Pt ultra-thin film deposited on a ferromagnetic insulator, which is a tensile-strained LaCoO3 (LCO) thin film with the Curie temperature Tc=85K. The SMR displays a strong magnetic-field dependence below Tc, with the SMR amplitude continuing to increase (linearly) with increasing the field far beyond the saturation value of the ferromagnet. The SMR amplitude decreases gradually with raising the temperature across Tc and remains measurable even above Tc. Moreover, no hysteresis is observed in the field dependence of the SMR. These results indicate that a novel low-dimensional magnetic system forms on the surface of LCO and that the Pt/LCO interface decouples magnetically from the rest of the LCO thin film. To explain the experiment, we revisit the derivation of the SMR corrections and relate the spin-mixing conductances to the microscopic quantities describing the magnetism at the interface. Our results can be used as a technique to probe quantum magnetism on the surface of a magnetic insulator.

cond-mat.mes-hall↗

Magnetic properties of metal-organic coordination networks based on 3d transition metal atoms

The magnetic anisotropy and exchange coupling between spins localized at the positions of 3d transition metal atoms forming two-dimensional metal-organic coordination networks (MOCNs) grown on the Au(111) metal surface are studied. In particular, we consider MOCNs made of Ni or Mn metal centers linked by TCNQ (7,7,8,8-tetracyanoquinodimethane) organic ligands, which form rectangular networks with 1:1 stoichiometry. Based on the analysis of X-ray magnetic circular dichroism (XMCD) data taken at T= 2.5 K, we find that Ni atoms in the Ni-TCNQ MOCNs are coupled ferromagnetically and do not show any significant magnetic anisotropy, while Mn atoms in the Mn-TCNQ MOCNs are coupled antiferromagnetically and do show a weak magnetic anisotropy with in-planemagnetization. We explain these observations using both amodelHamiltonian based on mean-fieldWeiss theory and density functional theory calculations that include spin-orbit coupling. Our main conclusion is that the antiferromagnetic coupling between Mn spins and the in-plane magnetization of the Mn spins can be explained neglecting effects due to the presence of the Au(111) surface, while for Ni-TCNQ the metal surface plays a role in determining the absence of magnetic anisotropy in the system.

cond-mat.mes-hall↗

Hanle Magnetoresistance in Thin Metal Films with Strong Spin-Orbit Coupling

We report measurements of a new type of magnetoresistance in Pt and Ta thin films. The spin accumulation created at the surfaces of the film by the spin Hall effect decreases in a magnetic field because of the Hanle effect, resulting in an increase of the electrical resistance as predicted by Dyakonov [PRL 99, 126601 (2007)]. The angular dependence of this magnetoresistance resembles the recently discovered spin Hall magnetoresistance in Pt/Y3Fe5O12 bilayers, although the presence of a ferromagnetic insulator is not required. We show that this Hanle magnetoresistance is an alternative, simple way to quantitatively study the coupling between charge and spin currents in metals with strong spin-orbit coupling.

cond-mat.mes-hall↗

Modeling Ferro- and Antiferromagnetic Interactions in Metal-Organic Coordination Networks

Magnetization curves of two rectangular metal-organic coordination networks formed by the organic ligand TCNQ (7,7,8,8-tetracyanoquinodimethane) and two different (Mn and Ni) 3d transition metal atoms [M(3d)] show marked differences that are explained using first principles density functional theory and model calculations. We find that the existence of a weakly dispersive hybrid band with M(3d) and TCNQ character crossing the Fermi level is determinant for the appearance of ferromagnetic coupling between metal centers, as it is the case of the metallic system Ni-TCNQ but not of the insulating system Mn-TCNQ. The spin magnetic moment localized at the Ni atoms induces a significant spin polarization in the organic molecule; the corresponding spin density being delocalized along the whole system. The exchange interaction between localized spins at Ni centers and the itinerant spin density is ferromagnetic. Based on two different model Hamiltonians, we estimate the strength of exchange couplings between magnetic atoms for both Ni- and Mn-TCNQ networks that results in weak ferromagnetic and very weak antiferromagnetic correlations for Ni- and Mn-TCNQ networks, respectively.

physics.chem-ph↗

Holonomic Quantum Computation with Electron Spins in Quantum Dots

With the help of the spin-orbit interaction, we propose a scheme to perform holonomic single qubit gates on the electron spin confined to a quantum dot. The manipulation is done in the absence (or presence) of an applied magnetic field. By adiabatic changing the position of the confinement potential, one can rotate the spin state of the electron around the Bloch sphere in semiconductor heterostructures. The dynamics of the system is equivalent to employing an effective non-Abelian gauge potential whose structure depends on the type of the spin-orbit interaction. As an example, we find an analytic expression for the electron spin dynamics when the dot is moved around a circular path (with radius R) on the two dimensional electron gas (2DEG), and show that all single qubit gates can be realized by tuning the radius and orientation of the circular paths. Moreover, using the Heisenberg exchange interaction, we demonstrate how one can generate two-qubit gates by bringing two quantum dots near each other, yielding a scalable scheme to perform quantum computing on arbitrary N qubits. This proposal shows a way of realizing holonomic quantum computers in solid-state systems.

cond-mat.mes-hall↗

Dynamic response of 1D bosons in a trap

We calculate the dynamic structure factor S(q,omega) of a one-dimensional (1D) interacting Bose gas confined in a harmonic trap. The effective interaction depends on the strength of the confinement enforcing the 1D motion of atoms; interaction may be further enhanced by superimposing an optical lattice on the trap potential. In the compressible state, we find that the smooth variation of the gas density around the trap center leads to softening of the singular behavior of S(q,omega) at Lieb-1 mode compared to the behavior predicted for homogeneous 1D systems. Nevertheless, the density-averaged response remains a non-analytic function of q and omega at Lieb-1 mode in the limit of weak trap confinement. The exponent of the power-law non-analyticity is modified due to the inhomogeneity in a universal way, and thus, bears unambiguously the information about the (homogeneous) Lieb-Liniger model. A strong optical lattice causes formation of Mott phases. Deep in the Mott regime, we predict a semi-circular peak in S(q,ω) centered at the on-site repulsion energy, omega=U. Similar peaks of smaller amplitudes exist at multiples of U as well. We explain the suppression of the dynamic response with entering into the Mott regime, observed recently by D. Clement et al., Phys. Rev. Lett. v. 102, p. 155301 (2009), based on an f-sum rule for the Bose-Hubbard model.

cond-mat.quant-gas↗

Spin relaxation at the singlet-triplet crossing in a quantum dot

We study spin relaxation in a two-electron quantum dot in the vicinity of the singlet-triplet crossing. The spin relaxation occurs due to a combined effect of the spin-orbit, Zeeman, and electron-phonon interactions. The singlet-triplet relaxation rates exhibit strong variations as a function of the singlet-triplet splitting. We show that the Coulomb interaction between the electrons has two competing effects on the singlet-triplet spin relaxation. One effect is to enhance the relative strength of spin-orbit coupling in the quantum dot, resulting in larger spin-orbit splittings and thus in a stronger coupling of spin to charge. The other effect is to make the charge density profiles of the singlet and triplet look similar to each other, thus diminishing the ability of charge environments to discriminate between singlet and triplet states. We thus find essentially different channels of singlet-triplet relaxation for the case of strong and weak Coulomb interaction. Finally, for the linear in momentum Dresselhaus and Rashba spin-orbit interactions, we calculate the singlet-triplet relaxation rates to leading order in the spin-orbit interaction, and find that they are proportional to the second power of the Zeeman energy, in agreement with recent experiments on triplet-to-singlet relaxation in quantum dots.

cond-mat.mes-hall↗

Spin dynamics in InAs-nanowire quantum-dots coupled to a transmission line

We study theoretically electron spins in nanowire quantum dots placed inside a transmission line resonator. Because of the spin-orbit interaction, the spins couple to the electric component of the resonator electromagnetic field and enable coherent manipulation, storage, and read-out of quantum information in an all-electrical fashion. Coupling between distant quantum-dot spins, in one and the same or different nanowires, can be efficiently performed via the resonator mode either in real time or through virtual processes. For the latter case we derive an effective spin-entangling interaction and suggest means to turn it on and off. We consider both transverse and longitudinal types of nanowire quantum-dots and compare their manipulation timescales against the spin relaxation times. For this, we evaluate the rates for spin relaxation induced by the nanowire vibrations (phonons) and show that, as a result of phonon confinement in the nanowire, this rate is a strongly varying function of the spin operation frequency and thus can be drastically reduced compared to lateral quantum dots in GaAs. Our scheme is a step forward to the formation of hybrid structures where qubits of different nature can be integrated in a single device.

cond-mat.mes-hall↗

Direct Measurement of the Spin-Orbit Interaction in a Two-Electron InAs Nanowire Quantum Dot

We demonstrate control of the electron number down to the last electron in tunable few-electron quantum dots defined in catalytically grown InAs nanowires. Using low temperature transport spectroscopy in the Coulomb blockade regime we propose a simple method to directly determine the magnitude of the spin-orbit interaction in a two-electron artificial atom with strong spin-orbit coupling. Due to a large effective g-factor |g*|=8+/-1 the transition from singlet S to triplet T+ groundstate with increasing magnetic field is dominated by the Zeeman energy rather than by orbital effects. We find that the spin-orbit coupling mixes the T+ and S states and thus induces an avoided crossing with magnitude $Δ_{SO}$=0.25+/-0.05 meV. This allows us to calculate the spin-orbit length $λ_{SO}\approx$127 nm in such systems using a simple model.

cond-mat.mes-hall↗

Measurement, control, and decay of quantum-dot spins

In this review we discuss a recent proposal to perform partial Bell-state (parity) measurements on two-electron spin states for electrons confined to quantum dots. The realization of this proposal would allow for a physical implementation of measurement-based quantum computing. In addition, we consider the primary sources of energy relaxation and decoherence which provide the ultimate limit to all proposals for quantum information processing using electron spins in quantum dots. We give an account of the Hamiltonians used for the most important interactions (spin-orbit and hyperfine) and survey some of the recent work done to understand dynamics, control, and decoherence under the action of these Hamiltonians. We conclude the review with a table of important decay times found in experiment, and relate these time scales to the potential viability of measurement-based quantum computing.

cond-mat.mes-hall↗

Electric Dipole Induced Spin Resonance in Quantum Dots

An alternating electric field, applied to a quantum dot, couples to the electron spin via the spin-orbit interaction. We analyze different types of spin-orbit coupling known in the literature and find two efficient mechanisms of spin control in quantum dots. The linear in momentum Dresselhaus and Rashba spin-orbit couplings give rise to a fully transverse effective magnetic field in the presence of a Zeeman splitting at lowest order in the spin-orbit interaction. The cubic in momentum Dresselhaus terms are efficient in a quantum dot with non-harmonic confining potential and give rise to a spin-electric coupling proportional to the orbital magnetic field. We derive an effective spin Hamiltonian, which can be used to implement spin manipulation on a timescale of $10 {\rm ns}$ with the current experimental setups.

cond-mat.mes-hall↗

Spin-spin coupling in electrostatically coupled quantum dots

We study the spin-spin coupling between two single-electron quantum dots due to the Coulomb and spin-orbit interactions, in the absence of tunneling between the dots. We find an anisotropic XY spin-spin interaction that is proportional to the Zeeman splitting produced by the external magnetic field. This interaction is studied both in the limit of weak and strong Coulomb repulsion with respect to the level spacing of the dot. The interaction is found to be a non-monotonic function of inter-dot distance $a_0$ and external magnetic field, and, moreover, vanishes for some special values of $a_0$ and/or magnetic field orientation. This mechanism thus provides a new way to generate and tune spin interaction between quantum dots. We propose a scheme to measure this spin-spin interaction based on the spin-relaxation-measurement technique.

cond-mat.mes-hall↗