arXiv subjects

Vladimir A. Sidorov

Publications and source records attributed to Vladimir A. Sidorov.

7 recordsLinked to original sources

arXiv2022

Quasi-uniaxial pressure induced superconductivity in stoichiometric compound UTe$_2$

The recent discovery of superconductivity in heavy Fermion compound UTe2, a candidate topological and triplet-paired superconductor, has aroused widespread interest. However, to date, there is no consensus on whether the stoichiometric sample of UTe2 is superconducting or not due to lack of reliable evidence to distinguish the difference between the nominal and real compositions of samples. Here, we are the first to clarify that the stoichiometric UT2 is non-superconducting at ambient pressure and under hydrostatic pressure up to 6 GPa, however we find that it can be compressed into superconductivity by application of quasi-uniaxial pressure. Measurements of resistivity, magnetoresistance and susceptibility reveal that the quasi-uniaxial pressure results in a suppression of the Kondo coherent state seen at ambient pressure, and then leads to a superconductivity initially emerged on the ab-plane at 1.5 GPa. At 4.8 GPa, the superconductivity is developed in three crystallographic directions. The superconducting state coexists with an exotic magnetic ordered state that develops just below the onset temperature of the superconducting transition. The discovery of the quasi-uniaxial-pressure-induced superconductivity with exotic magnetic state in the stoichiometric UTe2 not only provide new understandings on this compound, but also highlight the vital role of Te deficiency in developing the superconductivity at ambient pressures.

cond-mat.supr-con↗

arXiv2020

Quantum phases of SrCu2(BO3)2 from high-pressure thermodynamics

We report heat capacity measurements of SrCu$_2$(BO$_3$)$_2$ under high pressure along with simulations of relevant quantum spin models and map out the $(P,T)$ phase diagram of the material. We find a first-order quantum phase transition between the low-pressure quantum dimer paramagnet and a phase with signatures of a plaquette-singlet state below T = $2$ K. At higher pressures, we observe a transition into a previously unknown antiferromagnetic state below $4$ K. Our findings can be explained within the two-dimensional Shastry-Sutherland quantum spin model supplemented by weak inter-layer couplings. The possibility to tune SrCu$_2$(BO$_3$)$_2$ between the plaquette-singlet and antiferromagnetic states opens opportunities for experimental tests of quantum field theories and lattice models involving fractionalized excitations, emergent symmetries, and gauge fluctuations.

cond-mat.str-el↗

arXiv2018

Universal superconductivity phase diagram for pressurized tetradymite topological insulators

We show that two different superconducting phases exist at high pressures in the optimized tetradymite topological insulators Bi2Te2Se (BTS) and Bi1.1Sb0.9Te2S (BSTS). The superconducting phases emerge at structural phase transitions, the first at 8.4 GPa for BTS and 12.4 GPa for BSTS, and the second at 13.6 GPa for BTS and 20.4 GPa, for BSTS. Electronic structure calculations show that these phases do not have topological character. Comparison of our results with prior work on Bi2Se3, Bi2Te3 and (Bi,Sb)2(Se,Te)3 allows us to uncover a universal phase diagram for pressure-induced superconductivity in tetradymites, providing a basis for understanding the relationships between topological behavior, crystal structure, and superconductivity for these materials.

cond-mat.supr-con↗

arXiv2018

Independence of topological surface state and bulk conductances in three-dimensional topological insulators

The archetypical 3D topological insulators Bi2Se3, Bi2Te3 and Sb2Te3 commonly exhibit high bulk conductivities, hindering the characterization of the surface state charge transport. The optimally doped topological insulators Bi2Te2Se and Bi2-xSbxTe2S, however, allow for such characterizations to be made. Here we report the first experimental comparison of the topological surface states and bulk conductances of Bi2Te2Se and Bi1.1Sb0.9Te2S, based on temperature-dependent high-pressure measurements. We find that the surface state conductance at low temperatures remains constant in the face of orders of magnitude increase in the bulk state conductance, revealing in a straightforward way that the topological surface states and bulk states are decoupled at low temperatures, consistent with theoretical models, and confirming topological insulators to be an excellent venue for studying charge transport in 2D Dirac electron systems.

cond-mat.str-el↗

arXiv2017

Anomalous connection between antiferromagnetic and superconducting phases in pressurized non-centrosymmetric heavy fermion compound CeRhGe3

Unconventional superconductivity frequently emerges as the transition temperature of a magnetic phase, typically antiferromagnetic, is suppressed continuously toward zero temperature. Here, we report contrary behavior in pressurized CeRhGe3, a non-centrosymmetric heavy fermion compound. We find that its pressure-tuned antiferromagnetic transition temperature (TN) appears to avoid a continuous decrease to zero temperature by terminating abruptly above a dome of pressure-induced superconductivity. Near 21.5 GPa, evidence for TN suddenly vanishes, the electrical resistance becomes linear in temperature and the superconducting transition reaches a maximum. In light of X-ray absorption spectroscopy measurements, these characteristics appear to be related to a pressured-induced Ce valence instability, which reveals as a sharp increase in the rate of change of Ce valence with applied pressure.

cond-mat.supr-con↗

arXiv2016

Discovery of a bi-critical point between antiferromagnetic and superconducting phases in pressurized single crystal Ca0.73La0.27FeAs2

One of the most strikingly universal features of the high temperature superconductors is that the superconducting phase emerges in the close proximity of the antiferromagnetic phase, and the interplay between these two phases poses a long standing challenge. It is commonly believed that,as the antiferromagnetic transition temperature is continuously suppressed to zero, there appears a quantum critical point, around which the existence of antiferromagnetic fluctuation is responsible for the development of the superconductivity. In contrast to this scenario, we report the discovery of a bi-critical point identified at 2.88 GPa and 26.02 K in the pressurized high quality single crystal Ca0.73La0.27FeAs2 by complementary in situ high pressure measurements. At the critical pressure, we find that the antiferromagnetism suddenly disappears and superconductivity simultaneously emerges at almost the same temperature, and that the external magnetic field suppresses the superconducting transition temperature but hardly affects the antiferromagnetic transition temperature.

cond-mat.supr-con↗

arXiv2016

Correlation between non-centrosymmetry and superconductivity in quasi-one-dimensional compounds A2Cr3As3 (A=K, Rb)

Non-centrosymmetric superconductors, whose crystal structure is absent of inversion symmetry, have recently received special attentions due to the expectation of unconventional pairings and exotic physics associated with such pairings. The newly discovered superconductors A2Cr3As3 (A=K, Rb), featured by the quasi-one dimensional structure with conducting CrAs chains, belongs to such kind of superconductor. In this study, we are the first to report the finding that the superconductivity of A2Cr3As3 (A=K, Rb) has a positive correlation with the extent of non-centrosymmetry. Our in-situ high pressure ac susceptibility and synchrotron x-ray diffraction measurements reveal that the larger bond angle of As-Cr-As in the CrAs chains can be taken as a key factor controlling superconductivity. While the smaller bond angle and the distance between the CrAs chains also affect the superconductivity due to their structural connections with the angle. We find that the larger value of the difference between the larger and samller angles, which is associated with the extent of the non-centrosymmetry of the lattice structure, is in favor of superconductivity. These results are expected to shed a new light on the underlying mechanism of the superconductivity in these Q1D superconductors and also to provide new perspective in understanding other non-centrosymmetric superconductors.

cond-mat.supr-con↗