arXiv subjects

Vyacheslavs Kashcheyevs

Publications and source records attributed to Vyacheslavs Kashcheyevs.

33 records · Page 2Linked to original sources

arXiv2013

Nonlinear thermovoltage and thermocurrent in quantum dots

Quantum dots are model systems for quantum thermoelectric behavior because of the ability to control and measure the effects of electron-energy filtering and quantum confinement on thermoelectric properties. Interestingly, nonlinear thermoelectric properties of such small systems can modify the efficiency of thermoelectric power conversion. Using quantum dots embedded in semiconductor nanowires, we measure thermovoltage and thermocurrent that are strongly nonlinear in the applied thermal bias. We show that most of the observed nonlinear effects can be understood in terms of a renormalization of the quantum-dot energy levels as a function of applied thermal bias and provide a theoretical model of the nonlinear thermovoltage taking renormalization into account. Furthermore, we propose a theory that explains a possible source of the observed, pronounced renormalization effect by the melting of Kondo correlations in the mixed-valence regime. The ability to control nonlinear thermoelectric behavior expands the range in which quantum thermoelectric effects may be used for efficient energy conversion.

cond-mat.mes-hall↗

arXiv2012

Quantum fluctuations and coherence in high-precision single-electron capture

The phase of a single quantum state is undefined unless the history of its creation provides a reference point. Thus quantum interference may seem hardly relevant for the design of deterministic single-electron sources which strive to isolate individual charge carriers quickly and completely. We provide a counterexample by analyzing the non-adiabatic separation of a localized quantum state from a Fermi sea due to a closing tunnel barrier. We identify the relevant energy scales and suggest ways to separate the contributions of quantum non-adiabatic excitation and backtunneling to the rare non-capture events. In the optimal regime of balanced decay and non-adiabaticity, our simple electron trap turns into a single-lead Landau-Zener-backtunneling interferometer, revealing the dynamical phase accumulated between the particle capture and leakage. The predicted "quantum beats in backtunneling" may turn the error of a single-electron source into a valuable signal revealing essentially non-adiabatic energy scales of a dynamic quantum dot.

cond-mat.mes-hall↗

arXiv2012

Counting statistics for electron capture in a dynamic quantum dot

We report non-invasive single-charge detection of the full probability distribution $P_n$ of the initialization of a quantum dot with $n$ electrons for rapid decoupling from an electron reservoir. We analyze the data in the context of a model for sequential tunneling pinch-off, which has generic solutions corresponding to two opposing mechanisms. One limit considers sequential "freeze out" of an adiabatically evolving grand canonical distribution, the other one is an athermal limit equivalent to the solution of a generalized decay cascade model. We identify the athermal capturing mechanism in our sample, testifying to the high precision of our combined theoretical and experimental methods. The distinction between the capturing mechanisms allows to derive efficient experimental strategies for improving the initialization.

cond-mat.mes-hall↗

arXiv2012

Electronic charge redistribution in LaAlO$_3$(001) thin films deposited at SrTiO$_3$(001) substrate: First principles analysis and the role of stoichiometry

We present a comprehensive first-principles study of the electronic charge redistribution in atomically sharp LaAlO$_3$/SrTiO$_3$(001) heterointerfaces of both n- and p-types allowing for non-stoichiometric composition. Using two different computational methods within the framework of the density functional theory (linear combination of atomic orbitals and plane waves) we demonstrate that conducting properties of LaAlO$_3$/SrTiO$_3$(001) heterointerfaces strongly depend on termination of LaAlO$_3$ (001) surface. We argue that both the polar "catastrophe" and the polar distortion scenarios may be realized depending on the interface stoichiometry. Our calculations predict that heterointerfaces with a non-stoichiometrc film---either LaO-terminated n-type or AlO$_2$-terminated p-type---may exhibit the conductivity of n- or p-type, respectively, independently of LaAlO$_3$(001) film thickness.

cond-mat.mtrl-sci↗

arXiv2011

Exact canonical occupation numbers in a Fermi gas with finite level spacing and a q-analog of Fermi-Dirac distribution

We consider equilibrium level occupation numbers in a Fermi gas with a fixed number of particles, n, and finite level spacing. Using the method of generating functions and the cumulant expansion we derive a recurrence relation for canonical partition function and an explicit formula for occupation numbers in terms of single-particle partition function at n different temperatures. We apply this result to a model with equidistant non-degenerate spectrum and obtain close-form expressions in terms of q-polynomials and Rogers-Ramanujan partial theta function. Deviations from the standard Fermi-Dirac distribution can be interpreted in terms of a gap in the chemical potential between the particle and the hole excitations with additional correlations at temperatures comparable to the level spacing.

cond-mat.stat-mech↗

arXiv2011

A quantized current source with mesoscopic feedback

We study a mesoscopic circuit of two quantized current sources, realized by non-adiabatic single- electron pumps connected in series with a small micron-sized island in between. We find that quantum transport through the second pump can be locked onto the quantized current of the first one by a feedback due to charging of the mesoscopic island. This is confirmed by a measurement of the charge variation on the island using a nearby charge detector. Finally, the charge feedback signal clearly evidences loading into excited states of the dynamic quantum dot during single-electron pump operation.

cond-mat.mes-hall↗

arXiv2011

Exact non-Hookean scaling of cylindrically bent elastic sheets and the large-amplitude pendulum

A sheet of elastic foil rolled into a cylinder and deformed between two parallel plates acts as a non-Hookean spring if deformed normally to the axis. For large deformations the elastic force shows an interesting inverse squares dependence on the interplate distance [Siber and Buljan, arXiv:1007.4699 (2010)]. The phenomenon has been used as a basis for an experimental problem at the 41st International Physics Olympiad. We show that the corresponding variational problem for the equilibrium energy of the deformed cylinder is equivalent to a minimum action description of a simple gravitational pendulum with an amplitude of 90 degrees. We use this analogy to show that the power-law of the force is exact for distances less than a critical value. An analytical solution for the elastic force is found and confirmed by measurements over a range of deformations covering both linear and non-Hookean behavior.

physics.class-ph↗

arXiv2010

Universal decay cascade model for dynamic quantum dot initialization

Dynamic quantum dots can be formed by time-dependent electrostatic potentials in nanoelectronic devices, such as gate- or surface-acoustic-wave-driven electron pumps. Ability to control the number of captured electrons with high precision is required for applications in fundamental metrology and quantum information processing. In this work we propose and quantify a scheme to initialize quantum dots with a controllable number of electrons. It is based on the stochastic decrease in the electron number of a shrinking dynamic quantum dot and is described by a nuclear decay cascade model with "isotopes" being different charge states of the dot. Unlike the natural nuclei, the artificial confinement is time-dependent and tunable, so the probability distribution for the final "stable isotopes" depends on the external gate voltage. We derive an explicit fitting formula to extract the sequence of decay rate ratios from the measurements of averaged current in a periodically driven device. This provides a device-specific fingerprint which allows to compare different devices and architectures, and predict the upper limits of initialization accuracy from low precision measurements.

cond-mat.mes-hall↗

arXiv2009

Non-adiabatic pumping of single electrons affected by magnetic fields

Non-adiabatic pumping of discrete charges, realized by a dynamical quantum dot in an AlGaAs/GaAs heterostructure, is studied under influence of a perpendicular magnetic field. Application of an oscillating voltage in the GHz-range to one of two top gates, crossing a narrow wire and confining a quantum dot, leads to quantized pumped current plateaus in the gate characteristics. The regime of pumping one single electron is traced back to the diverse tunneling processes into and out-of the dot. Extending the theory to multiple electrons allows to investigate conveniently the pumping characteristics in an applied magnetic field. In this way, a qualitatively different behavior between pumping even or odd numbers of electrons is extracted.

cond-mat.mes-hall↗

arXiv2008

Low-frequency excitation of double quantum dots

We address theoretically adiabatic regime of charge transport for a model of two tunnel-coupled quantum dots connected in series. The energy levels of the two dots are harmonically modulated by an external potential with a constant phase shift between the two. Motivated by recent experiments with surface-acoustic-wave excitation, we consider two situations: (a) pure pumping in the absence of external voltage (also at finite temperature), and (b) adiabatic modulation of the current driven by large external bias. In both cases we derive results consistent with published experimental data. For the case (b) we explicitly derive the adiabatic limit of Tien-Gordon formula for photon-assisted tunneling and compare it to the outcome of simple conductance modulation. A tutorial for adiabatic pumping current calculations with the Green function formalism is included.

cond-mat.mes-hall↗

arXiv2006

Unified description of correlations in double quantum dots

The two-level model for a double quantum dot coupled to two leads, which is ubiquitously used to describe charge oscillations, transmission-phase lapses and correlation-induced resonances, is considered in its general form. The model features arbitrary tunnelling matrix elements among the two levels and the leads and between the levels themselves (including the effect of Aharonov-Bohm fluxes), as well as inter-level repulsive interactions. We show that this model is exactly mapped onto a generalized Anderson model of a single impurity, where the electrons acquire a pseudo-spin degree of freedom, which is conserved by the tunnelling but not within the dot. Focusing on the local-moment regime where the dot is singly occupied, we show that the effective low-energy Hamiltonian is that of the anisotropic Kondo model in the presence of a tilted magnetic field. For moderate values of the (renormalized) field, the Bethe ansatz solution of the isotropic Kondo model allows us to derive accurate expressions for the dot occupation numbers, and henceforth its zero-temperature transmission. Our results are in excellent agreement with those obtained from the Bethe ansatz for the isotropic Anderson model, and with the functional and numerical renormalization-group calculations of Meden and Marquardt [Phys. Rev. Lett. 96, 146801 (2006)], which are valid for the general anisotropic case. In addition we present highly accurate estimates for the validity of the Schrieffer-Wolff transformation (which maps the Anderson Hamiltonian onto the low-energy Kondo model) at both the high- and low-magnetic field limits. Perhaps most importantly, we provide a single coherent picture for the host of phenomena to which this model has been applied.

cond-mat.mes-hall↗

arXiv2005

On the applicability of the equations-of-motion technique for quantum dots

The equations-of-motion (EOM) hierarchy satisfied by the Green functions of a quantum dot embedded in an external mesoscopic network is considered within a high-order decoupling approximation scheme. Exact analytic solutions of the resulting coupled integral equations are presented in several limits. In particular, it is found that at the particle-hole symmetric point the EOM Green function is temperature-independent due to a discontinuous change in the imaginary part of the interacting self-energy. However, this imaginary part obeys the Fermi liquid unitarity requirement away from this special point, at zero temperature. Results for the occupation numbers, the density of states and the local spin susceptibility are compared with exact Fermi liquid relations and the Bethe ansatz solution. The approximation is found to be very accurate far from the Kondo regime. In contrast, the description of the Kondo effect is valid on a qualitative level only. In particular, we find that the Friedel sum rule is considerably violated, up to 30%, and the spin susceptibility is underestimated. We show that the widely-used simplified version of the EOM method, which does not account fully for the correlations on the network, fails to produce the Kondo correlations even qualitatively.

cond-mat.mes-hall↗

arXiv2004

Quantized charge pumping by surface acoustic waves in ballistic quasi-1D channels

Adiabatic pumping of electrons induced by surface acoustic waves (SAWs) in a ballistic quasi-1D quantum channel is considered using an exactly solvable tight-binding model for non-interacting electrons. The single-electron degrees of freedom, responsible for acoustoelectric current quantization, are related to the transmission resonances. We study the influence of experimentally controllable parameters (SAW power, gate voltage, source-drain bias, amplitude and phase of a secondary SAW beam) on the plateau-like structure of the acoustoelectric current. The results are consistent with existing experimental observations.

cond-mat.mes-hall↗

arXiv2003

Adiabatic Quantum Pumping of Coherent Electrons

We review recent theoretical calculations of charge transfer through mesoscopic devices in response to slowly-oscillating, spatially-confined, potentials. The discussion is restricted to non-interacting electrons, and emphasizes the role of quantum interference and resonant transmission in producing almost integer values (in units of the electronic charge $e$) of the charge transmitted per cycle, $Q$. The expression for the pumped charge is derived from a systematic expansion of the system scattering states in terms of the temporal derivatives of the instantaneous solutions. This yields the effect of the modulating potential on the Landauer formula for the conductance in response to a constant bias on one hand, and the corrections to the widely-used adiabatic-limit formula (in which the modulation frequency is smaller than any electronic relaxation rate) on the other hand. The expression for $Q$ is used in connection with simple models to exemplify the intimate relationship between resonant transmission through the mesoscopic device and almost integral values of $Q$, and to analyze the charge pumped by a surface acoustic wave coupled to a quantum channel by the piezoelectric effect. \keywords{interference in nanostructures, quantum pumping, surface acoustic waves, resonant transmission.

cond-mat.mes-hall↗

arXiv2003

Resonance approximation and charge loading/unloading in adiabatic quantum pumping

Quantum pumping through mesoscopic quantum dots is known to be enhanced by resonant transmission. The pumped charge is close to an integer number of electrons when the pumping contour surrounds a resonance, but the transmission remains small on the contour. For non-interacting electrons, we give a quantitative account of the detailed exchange of electrons between the dot and the leads (to the electron reservoirs) during a pumping cycle. Near isolated distinct resonances, we use approximate Breit-Wigner expressions for the dot's Green function to discuss the loading/unloading picture of the pumping: the fractional charge exchanged between the dot and each lead through a single resonance point is related to the relative couplings of the dot and the leads at this resonance. If each resonance point along the pumping contour is dominated by the coupling to a single lead (which also implies a very small transmission), then the crossing of each such resonance results in a single electron exchange between the dot and that lead, ending up with a net quantized charge. When the resonance approximation is valid, the fractional charges can also be extracted from the peaks of the transmissions between the various leads.

cond-mat.mes-hall↗