arXiv subjects

W. A. Coish

Publications and source records attributed to W. A. Coish.

At least 37 records · Page 2Linked to original sources

arXiv2020

First-principles hyperfine tensors for electrons and holes in GaAs and silicon

Understanding (and controlling) hyperfine interactions in semiconductor nanostructures is important for fundamental studies of material properties as well as for quantum information processing with electron, hole, and nuclear-spin states. Through a combination of first-principles density-functional theory (DFT) and $\mathbf{k}\cdot\mathbf{p}$ theory, we have calculated hyperfine tensors for electrons and holes in GaAs and crystalline silicon. Accounting for relativistic effects near the nuclear core, we find contact hyperfine interactions for electrons in GaAs that are consistent with Knight-shift measurements performed on GaAs quantum wells and are roughly consistent with prior estimates extrapolated from measurements on InSb. We find that a combination of DFT and $\mathbf{k}\cdot\mathbf{p}$ theory is necessary to accurately determine the contact hyperfine interaction for electrons at a conduction-band minimum in silicon that is consistent with bulk Knight-shift measurements. For hole spins in GaAs, the overall magnitude of the hyperfine couplings we find from DFT is consistent with previous theory based on free-atom properties, and with heavy-hole Overhauser shifts measured in GaAs (and InGaAs) quantum dots. In addition, we theoretically predict that the heavy-hole hyperfine coupling to the As nuclear spins is stronger and almost purely Ising-like, while the (weaker) coupling to the Ga nuclear spins has significant non-Ising corrections. In the case of hole spins in silicon, we find (surprisingly) that the strength of the hyperfine interaction in the valence band is comparable to that in the conduction band and that the hyperfine tensors are highly anisotropic (Ising-like) in the heavy-hole subspace. These results suggest that the hyperfine coupling cannot be ruled out as a limiting mechanism for coherence ($T_2^{\ast}$) times recently measured for heavy holes in silicon quantum dots.

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arXiv2019

Tunable skyrmion-skyrmion binding on the surface of a topological insulator

We show that skyrmions on the surface of a magnetic topological insulator may experience an attractive interaction that leads to the formation of a skyrmion-skyrmion bound state. This is in contrast to the case of skyrmions in a conventional chiral ferromagnet, for which the intrinsic interaction is repulsive. The origin of skyrmion binding in our model is the molecular hybridization of topologically protected electronic orbitals associated with each skyrmion. Attraction between the skyrmions can therefore be controlled by tuning a chemical potential that populates/depopulates the lowest-energy molecular orbital. We find that the skyrmion-skyrmion bound state can be made stable, unstable, or metastable depending on the chemical potential, magnetic field, and easy-axis anisotropy of the underlying ferromagnet, resulting in a rich phase diagram. Finally, we discuss the possibility to realize this effect in a recently synthesized Cr doped ${\left(\mathrm{Bi}_{2-y}\mathrm{Sb}_{y}\right)}_{2}\mathrm{Te}_3$ heterostructure.

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arXiv2019

Hole-Spin-Echo Envelope Modulations

Hole spins in semiconductor quantum dots or bound to acceptor impurities show promise as potential qubits, partly because of their weak and anisotropic hyperfine couplings to proximal nuclear spins. Since the hyperfine coupling is weak, it can be difficult to measure. However, an anisotropic hyperfine coupling can give rise to a substantial spin-echo envelope modulation that can be Fourier-analyzed to accurately reveal the hyperfine tensor. Here, we give a general theoretical analysis for hole-spin-echo envelope modulation (HSEEM), and apply this analysis to the specific case of a boron-acceptor hole spin in silicon. For boron acceptor spins in unstrained silicon, both the hyperfine and Zeeman Hamiltonians are approximately isotropic leading to negligible envelope modulations. In contrast, in strained silicon, where light-hole spin qubits can be energetically isolated, we find the hyperfine Hamiltonian and $g$-tensor are sufficiently anisotropic to give spin-echo-envelope modulations. We show that there is an optimal magnetic-field orientation that maximizes the visibility of envelope modulations in this case. Based on microscopic estimates of the hyperfine coupling, we find that the maximum modulation depth can be substantial, reaching $\sim 10\%$, at a moderate laboratory magnetic field, $B\lesssim 200\,\mathrm{mT}$.

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arXiv2017

Magnetoconductance signatures of chiral domain-wall bound states in magnetic topological insulators

Recent magnetoconductance measurements performed on magnetic topological insulator candidates have revealed butterfly-shaped hysteresis. This hysteresis has been attributed to the formation of gapless chiral domain-wall bound states during a magnetic field sweep. We treat this phenomenon theoretically, providing a link between microscopic magnetization dynamics and butterfly hysteresis in magnetoconductance. Further, we illustrate how a spatially resolved conductance measurement can probe the most striking feature of the domain-wall bound states: their chirality. This work establishes a regime where a definitive link between butterfly hysteresis in longitudinal magneto-conductance and domain-wall bound states can be made. This analysis provides an important tool for the identification of magnetic topological insulators.

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arXiv2017

Hamiltonian engineering for robust quantum state transfer and qubit readout in cavity QED

Quantum state transfer into a memory, state shuttling over long distances via a quantum bus, and high-fidelity readout are important tasks for quantum technology. Realizing these tasks is challenging in the presence of realistic couplings to an environment. Here, we introduce and assess protocols that can be used in cavity QED to perform high-fidelity quantum state transfer and fast quantum nondemolition qubit readout through Hamiltonian engineering. We show that high-fidelity state transfer between a cavity and a single qubit can be performed, even in the limit of strong dephasing due to inhomogeneous broadening. We generalize this result to state transfer between a cavity and a logical qubit encoded in a collective mode of a large ensemble of $N$ physical qubits. Under a decoupling sequence, we show that inhomogeneity in the ensemble couples two collective bright states to only two other collective modes, leaving the remaining $N-3$ single-excitation states dark. Moreover, we show that large signal-to-noise and high single-shot fidelity can be achieved in a cavity-based qubit readout, even in the weak-coupling limit. These ideas may be important for novel systems coupling single spins to a microwave cavity.

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arXiv2016

Coupling a single electron spin to a microwave resonator: Controlling transverse and longitudinal couplings

Microwave-frequency superconducting resonators are ideally suited to perform dispersive qubit readout, to mediate two-qubit gates, and to shuttle states between distant quantum systems. A prerequisite for these applications is a strong qubit-resonator coupling. Strong coupling between an electron-spin qubit and a microwave resonator can be achieved by correlating spin- and orbital degrees of freedom. This correlation can be achieved through the Zeeman coupling of a single electron in a double quantum dot to a spatially inhomogeneous magnetic field generated by a nearby nanomagnet. In this paper, we consider such a device and estimate spin-resonator couplings of order ~ 1 MHz with realistic parameters. Further, through realistic simulations, we show that precise placement of the double dot relative to the nanomagnet allows to select between a purely longitudinal coupling (commuting with the bare spin Hamiltonian) and a purely transverse (spin non-conserving) coupling. Additionally, we suggest methods to mitigate dephasing and relaxation channels that are introduced in this coupling scheme. This analysis gives a clear route toward the realization of coherent state transfer between a microwave resonator and a single electron spin in a GaAs double quantum dot with a fidelity above 90%. Improved dynamical decoupling sequences, low-noise environments, and longer-lived microwave cavity modes may lead to substantially higher fidelities in the near future.

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arXiv2016

Maximal adaptive-decision speedups in quantum-state readout

The average time $T$ required for high-fidelity readout of quantum states can be significantly reduced via a real-time adaptive decision rule. An adaptive decision rule stops the readout as soon as a desired level of confidence has been achieved, as opposed to setting a fixed readout time $t_f$. The performance of the adaptive decision is characterized by the "adaptive-decision speedup," $t_f/T$. In this work, we reformulate this readout problem in terms of the first-passage time of a particle undergoing stochastic motion. This formalism allows us to theoretically establish the maximum achievable adaptive-decision speedups for several physical two-state readout implementations. We show that for two common readout schemes (the Gaussian latching readout and a readout relying on state-dependent decay), the speedup is bounded by $4$ and $2$, respectively, in the limit of high single-shot readout fidelity. We experimentally study the achievable speedup in a real-world scenario by applying the adaptive decision rule to a readout of the nitrogen-vacancy-center (NV-center) charge state. We find a speedup of $\approx 2$ with our experimental parameters. In addition, we propose a simple readout scheme for which the speedup can, in principle, be increased without bound as the fidelity is increased. Our results should lead to immediate improvements in nanoscale magnetometry based on spin-to-charge conversion of the NV-center spin, and provide a theoretical framework for further optimization of the bandwidth of quantum measurements.

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arXiv2015

Theory of box-model hyperfine couplings and transport signatures of long-range nuclear-spin coherence in a quantum-dot spin valve

We have theoretically analyzed coherent nuclear-spin dynamics induced by electron transport through a quantum-dot spin valve. The hyperfine interaction between electron and nuclear spins in a quantum dot allows for the transfer of angular momentum from spin-polarized electrons injected from ferromagnetic or half-metal leads to the nuclear spin system under a finite voltage bias. Accounting for a local nuclear-spin dephasing process prevents the system from becoming stuck in collective dark states, allowing a large nuclear polarization to be built up in the long-time limit. After reaching a steady state, reversing the voltage bias induces a transient current response as the nuclear polarization is reversed. Long-range nuclear-spin coherence leads to a strong enhancement of spin-flip transition rates (by an amount proportional to the number of nuclear spins) and is revealed by an intense current burst, analogous to superradiant light emission. The crossover to a regime with incoherent spin flips occurs on a relatively long time scale, on the order of the single-nuclear-spin dephasing time, which can be much longer than the time scale for the superradiant current burst. This conclusion is confirmed through a general master equation. For the two limiting regimes (coherent/incoherent spin flips) the general master equation recovers our simpler treatment based on rate equations, but is also applicable at intermediate dephasing. Throughout this work we assume uniform hyperfine couplings, which yield the strongest coherent enhancement. We propose realistic strategies, based on isotopic modulation and wavefunction engineering in core-shell nanowires, to realize this analytically solvable "box-model" of hyperfine couplings.

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arXiv2015

Maximizing the purity of a qubit evolving in an anisotropic environment

We provide a general method to calculate and maximize the purity of a qubit interacting with an anisotropic non-Markovian environment. Counter to intuition, we find that the purity is often maximized by preparing and storing the qubit in a superposition of non-interacting eigenstates. For a model relevant to decoherence of a heavy-hole spin qubit in a quantum dot or for a singlet-triplet qubit for two electrons in a double quantum dot, we show that preparation of the qubit in its non-interacting ground state can actually be the worst choice to maximize purity. We further give analytical results for spin-echo envelope modulations of arbitrary spin components of a hole spin in a quantum dot, going beyond a standard secular approximation. We account for general dynamics in the presence of a pure-dephasing process and identify a crossover timescale at which it is again advantageous to initialize the qubit in the non-interacting ground state. Finally, we consider a general two-axis dynamical decoupling sequence and determine initial conditions that maximize purity, minimizing leakage to the environment.

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arXiv2015

Microscopic models for charge-noise-induced dephasing of solid-state qubits

Several experiments have shown qubit coherence decay of the form $\mathrm{exp}[-(t/T_2)^α]$ due to environmental charge-noise fluctuations. We present a microscopic description for temperature dependences of the parameters $T_2$ and $α$. Our description is appropriate to qubits in semiconductors interacting with spurious two-level charge fluctuators coupled to a thermal bath. We find distinct power-law dependences of $T_2$ and $α$ on temperature depending on the nature of the interaction of the fluctuators with the associated bath. We consider fluctuator dynamics induced by first- and second-order tunneling with a continuum of delocalized electron states. We also study one- and two-phonon processes for fluctuators in either GaAs or Si. These results can be used to identify dominant charge-dephasing mechanisms and suppress them.

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arXiv2014

Soft Decoding of a Qubit Readout Apparatus

Qubit readout is commonly performed by thresholding a collection of analog detector signals to obtain a sequence of single-shot bit values. The intrinsic irreversibility of the mapping from analog to digital signals discards soft information associated with an \emph{a posteriori} confidence that can be assigned to each bit value when a detector is well characterized. Accounting for soft information, we show significant improvements in enhanced state detection with the quantum repetition code as well as quantum state or parameter estimation. These advantages persist in spite of non-Gaussian features of realistic readout models, experimentally relevant small numbers of qubits, and finite encoding errors. These results show useful and achievable advantages for a wide range of current experiments on quantum state tomography, parameter estimation, and qubit readout.

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arXiv2014

Controlling hole spins in quantum dots and wells

We review recent theoretical results for hole spins influenced by spin-orbit coupling and Coulomb interaction in two-dimensional quantum wells as well as the decoherence of single hole spins in quantum dots due to hyperfine interaction with surrounding nuclear spins. After reviewing the different forms of spin-orbit coupling that are relevant for electrons and heavy holes in III-V semiconductor quantum wells, we illustrate the combined effect of spin-orbit coupling and Coulomb interactions for hole systems on spin-dependent quasiparticle group velocities. We further analyze spin-echo decay for a single hole spin in a nuclear-spin bath, demonstrating that this decoherence source can be controlled in these systems by entering a motional-averaging regime. Throughout this review, we emphasize physical effects that are unique to hole spins (rather than electrons) in nanoscale systems.

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arXiv2014

Enhanced hyperfine-induced spin dephasing in a magnetic-field gradient

Magnetic-field gradients are important for single-site addressability and electric-dipole spin resonance of spin qubits in semiconductor devices. We show that these advantages are offset by a potential reduction in coherence time due to the non-uniformity of the magnetic field experienced by a nuclear-spin bath interacting with the spin qubit. We theoretically study spins confined to quantum dots or at single donor impurities, considering both free-induction and spin-echo decay. For quantum dots in GaAs, we find that, in a realistic setting, a magnetic-field gradient can reduce the Hahn-echo coherence time by almost an order of magnitude. This problem can, however, be resolved by applying a moderate external magnetic field to enter a motional averaging regime. For quantum dots in silicon, we predict a cross-over from non-Markovian to Markovian behavior that is unique to these devices. Finally, for very small systems such as single phosphorus donors in silicon, we predict a breakdown of the common Gaussian approximation due to finite-size effects.

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arXiv2013

Optimal post-processing for a generic single-shot qubit readout

We analyze three different post-processing methods applied to a single-shot qubit readout: the average-signal (boxcar filter), peak-signal, and maximum-likelihood methods. In contrast to previous work, we account for a stochastic turn-on time $t_i$ associated with the leading edge of a pulse signaling one of the qubit states. This model is relevant to spin-qubit readouts based on spin-to-charge conversion and would be generically reached in the limit of large signal-to-noise ratio $r$ for several other physical systems, including fluorescence-based readouts of ion-trap qubits and nitrogen-vacancy center spins. We derive analytical closed-form expressions for the conditional probability distributions associated with the peak-signal and boxcar filters. For the boxcar filter, we find an asymptotic scaling of the single-shot error rate $\varepsilon \sim \ln r/\sqrt{r}$ when $t_i$ is stochastic, in contrast to the result $\varepsilon \sim \ln r/ r$ for deterministic $t_i$. Consequently, the peak-signal method outperforms the boxcar filter significantly when $t_i$ is stochastic, but is only marginally better for deterministic $t_i$ (a result that is consistent with the widespread use of the boxcar filter for fluorescence-based readouts and the peak-signal for spin-to-charge conversion). We generalize the theoretically optimal maximum-likelihood method to stochastic $t_i$ and show numerically that a stochastic turn-on time $t_i$ will always result in a larger single-shot error rate. Based on this observation, we propose a general strategy to improve the quality of single-shot readouts by forcing $t_i$ to be deterministic.

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arXiv2013

Anomalous magnetotransport through reflection-symmetric artificial molecules

We calculate magnetotransport oscillations in current through a triple-quantum-dot molecule, accounting for higher harmonics (having flux period h/ne, with n an integer). For a reflection-symmetric triple quantum dot, we find that harmonics with n odd can dominate over those with n even. This is opposite to the behavior theoretically predicted due to `dark-state' localization, but has been observed in recent experiments [L. Gaudreau et al., Phys. Rev. B, 80, 075415 (2009)], albeit in a triple-dot that may not exhibit reflection symmetry. This feature arises from a more general result: In the weak-coupling limit, we find that the current is flux-independent for an arbitrary reflection-symmetric Aharonov-Bohm network. We further show that these effects are observable in nanoscale systems even in the presence of typical dephasing sources.

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arXiv2012

Quasiparticle velocities in 2D electron/hole liquids with spin-orbit coupling

We study the influence of spin-orbit interactions on quasiparticle dispersions in two-dimensional electron and heavy-hole liquids in III-V semiconductors. To obtain closed-form analytical results, we restrict ourselves to spin-orbit interactions with isotropic spectrum and work within the screened Hartree-Fock approximation, valid in the high-density limit. For electrons having a linear-in-momentum Rashba (or, equivalently, Dresselhaus) spin-orbit interaction, we show that the screened Hartree-Fock approximation recovers known results based on the random-phase approximation and we extend those results to higher order in the spin-orbit coupling. While the well-studied case of electrons leads only to a weak modification of quasiparticle properties in the presence of the linear-in-momentum spin-orbit interaction, we find two important distinctions for hole systems (with a leading nonlinear-in-momentum spin-orbit interaction). First, the group velocities associated with the two hole-spin branches acquire a significant difference in the presence of spin-orbit interactions, allowing for the creation of spin-polarized wavepackets in zero magnetic field. Second, we find that the interplay of Coulomb and spin-orbit interactions is significantly more important for holes than for electrons and can be probed through the quasiparticle group velocities. These effects should be directly observable in magnetotransport, Raman scattering, and femtosecond-resolved Faraday rotation measurements. Our results are in agreement with a general argument on the velocities, which we formulate for an arbitrary choice of the spin-orbit coupling.

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arXiv2011

Leakage-current lineshapes from inelastic cotunneling in the Pauli spin blockade regime

We find the leakage current through a double quantum dot in the Pauli spin blockade regime accounting for inelastic (spin-flip) cotunneling processes. Taking the energy-dependence of this spin-flip mechanism into account allows for an accurate description of the current as a function of applied magnetic fields, gate voltages, and an inter-dot tunnel coupling. In the presence of an additional local dephasing process or nonuniform magnetic field, we obtain a simple closed-form analytical expression for the leakage current giving the full dependence on an applied magnetic field and energy detuning. This work is important for understanding the nature of leakage, especially in systems where other spin-flip mechanisms (due, e.g., to hyperfine coupling to nuclear spins or spin-orbit coupling) are weak, including silicon and carbon-nanotube or graphene quantum dots.

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arXiv2011

Pauli Spin Blockade in a Highly Tunable Silicon Double Quantum Dot

Double quantum dots are convenient solid-state platforms to encode quantum information. Two-electron spin states can be conveniently detected and manipulated using strong quantum selection rules based on the Pauli exclusion principle, leading to the well-know Pauli spin blockade of electron transport for triplet states. Coherent spin states would be optimally preserved in an environment free of nuclear spins, which is achievable in silicon by isotopic purification. Here we report on a deliberately engineered, gate-defined silicon metal-oxide-semiconductor double quantum dot system. The electron occupancy of each dot and the inter-dot tunnel coupling are independently tunable by electrostatic gates. At weak inter-dot coupling we clearly observe Pauli spin blockade and measure a large intra-dot singlet-triplet splitting $>$ 1 meV. The leakage current in spin blockade has a peculiar magnetic field dependence, unrelated to electron-nuclear effects and consistent with the effect of spin-flip cotunneling processes. The results obtained here provide excellent prospects for realizing singlet-triplet qubits in silicon.

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