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W. B. Walters

Publications and source records attributed to W. B. Walters.

31 records · Page 2Linked to original sources
arXiv2010

Coulomb excitation of 73Ga

The B(E2; Ii -> If) values for transitions in 71Ga and 73Ga were deduced from a Coulomb excitation experiment at the safe energy of 2.95 MeV/nucleon using post-accelerated beams of 71,73Ga at the REX-ISOLDE on-line isotope mass separator facility. The emitted gamma rays were detected by the MINIBALL-detector array and B(E2; Ii->If) values were obtained from the yields normalized to the known strength of the 2+ -> 0+ transition in the 120Sn target. The comparison of these new results with the data of less neutron-rich gallium isotopes shows a shift of the E2 collectivity towards lower excitation energy when adding neutrons beyond N = 40. This supports conclusions from previous studies of the gallium isotopes which indicated a structural change in this isotopical chain between N = 40 and N = 42. Combined with recent measurements from collinear laser spectroscopy showing a 1/2- spin and parity for the ground state, the extracted results revealed evidence for a 1/2-; 3/2- doublet near the ground state in 73 31Ga42 differing by at most 0.8 keV in energy.

nucl-ex↗
arXiv2010

Half-lives and branchings for β-delayed neutron emission for neutron-rich Co-Cu isotopes in the r-process

The β decays of very neutron-rich nuclides in the Co-Zn region were studied experimentally at the National Superconducting Cyclotron Laboratory using the NSCL β-counting station in conjunction with the neutron detector NERO. We measured the branchings for β-delayed neutron emission (Pn values) for 74Co (18 +/- 15%) and 75-77Ni (10 +/- 2.8%, 14 +/- 3.6%, and 30 +/- 24%, respectively) for the first time, and remeasured the Pn values of 77-79Cu, 79,81Zn, and 82Ga. For 77-79Cu and for 81Zn we obtain significantly larger Pn values compared to previous work. While the new half-lives for the Ni isotopes from this experiment had been reported before, we present here in addition the first half-life measurements of 75Co (30 +/- 11 ms) and 80Cu (170+110 -50 ms). Our results are compared with theoretical predictions, and their impact on various types of models for the astrophysical rapid neutron-capture process (r-process) is explored. We find that with our new data, the classical r-process model is better able to reproduce the A = 78-80 abundance pattern inferred from the solar abundances. The new data also influence r-process models based on the neutrino-driven high-entropy winds in core collapse supernovae.

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arXiv2010

$β$ Decay and Isomeric Properties of Neutron-Rich Ca and Sc Isotopes

The isomeric and $β$-decay properties of neutron-rich $^{53-57}$Sc and $^{53,54}$Ca nuclei near neutron number $N$=32 are reported, and the low-energy level schemes of $^{53,54,56}$Sc and $^{53-57}$Ti are presented. The low-energy level structures of the $_{21}$Sc isotopes are discussed in terms of the coupling of the valence $1f_{7/2}$ proton to states in the corresponding $_{20}$Ca cores. Implications with respect to the robustness of the $N$=32 subshell closure are discussed, as well as the repercussions for a possible $N$=34 subshell closure.

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arXiv2009

Low-energy structure of 61Mn populated following $β$ decay of 61Cr

$β$ decay of the $^{61}$Cr$_{37}$ ground state has been studied. A new half-life of 233 +/- 11 ms has been deduced, and seven delayed $γ$ rays have been assigned to the daughter, $^{61}$Mn$_{36}$. The low-energy level structure of $^{61}$Mn$_{36}$ is similar to that of the less neutron-rich $^{57,59}$Mn nuclei. The odd-A $_{25}$Mn isotopes follow the systematic trend in the yrast states of the even-even, Z + 1 $_{26}$Fe isotopes, and not that of the Z - 1 $_{24}$Cr isotopes, where a possible onset of collectivity has been suggested to occur already at N = 36.

nucl-ex↗
arXiv2009

Evidence for a beta-decaying 1/2- isomer in 71Ni

We report on the investigation of the population mechanism for the 454-KeV level in 71Cu. This level was identified for the first time in a recent Coulomb excitation measurement with a radioactive beam of 71Cu. The selective nature of the Coulomb-excitation process as well as nuclear-structure considerations constrain the possible spin values for the newly observed state to Ipi=1/2-. A re-examination of the data set obtained in a beta-decay study at the LISOL separator revealed that this state is also populated in the decay of 71Ni, most probably by direct feeding from a newly identified 1/2- beta-decaying isomer having a T1/2=2.34(25) s. In this paper we investigate the proposed scenario by reanalyzing the beta-gamma and gamma-gamma coincidences obtained in the beta-decay study at LISOL.

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arXiv2009

Structure of 65,67Co studied through the beta decay of 65,67Fe and a deep-inelastic reaction

The neutron-rich isotopes 65,67Fe and 65Co have been produced at the LISOL facility, Louvain-La-Neuve, in the proton-induced fission of 238U. Beams of these isotopes have been extracted with high selectivity by means of resonant laser ionization combined with mass separation. Yrast and near-yrast levels of 65Co have also been populated in the 64Ni+238U reaction at Argonne National Laboratory. The level structure of 65Co could be investigated by combining all the information from both the 65Fe and 65Co beta decay and the deep-inelastic reaction. The 65Fe, 65Co and 67Fe decay schemes and the 65Co yrast structure are fully established. The 65,67Co level structures can be interpreted as resulting from the coexistence of core-coupled states with levels based on a low-energy proton-intruder configuration.

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arXiv2009

Beta-decay half-lives and beta-delayed neutron emission probabilities of nuclei in the region below A=110, relevant for the r-process

Measurements of the beta-decay properties of r-process nuclei below A=110 have been completed at the National Superconducting Cyclotron Laboratory, at Michigan State University. Beta-decay half-lives for Y-105, Zr-106,107 and Mo-111, along with beta-delayed neutron emission probabilities of Y-104, Mo-109,110 and upper limits for Y-105, Zr-103,104,105,106,107 and Mo-108,111 have been measured for the first time. Studies on the basis of the quasi-random phase approximation are used to analyze the ground-state deformation of these nuclei.

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arXiv2008

Shape Isomerism at N = 40: Discovery of a Proton Intruder in 67Co

The nuclear structure of 67Co has been investigated through 67Fe beta-decay. The 67Fe isotopes were produced at the LISOL facility in proton-induced fission of 238U and selected using resonant laser ionization combined with mass separation. The application of a new correlation technique unambiguously revealed a 496(33) ms isomeric state in 67Co at an unexpected low energy of 492 keV. A 67Co level scheme has been deduced. Proposed spin and parities suggest a spherical (7/2-) 67Co ground state and a deformed first excited (1/2-) state at 492 keV, interpreted as a proton 1p-2h prolate intruder state.

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arXiv2008

Beta decay of Neutron-Rich 53-56Ca

Beta-decay properties of neutron-rich Ca isotopes have been obtained. Half-life values were determined for the first time for 54Ca [86(7) ms], 55Ca [22(2) ms], and 56Ca [11(2) ms]. The half-life of 230(6) ms deduced for 53Ca is significantly longer than reported previously, where the decay chain 53K -> 53Ca -> 53Sc was considered. A delayed gamma ray with energy 247 keV as identified following beta decay of 54Ca, and is proposed to depopulate the first 1+ level in 54Sc. The beta-decay properties compare favorably with the results of shell model calculations completed in the full pf-space with the GXPF1 interaction. The half-lives of the neutron-rich Ca isotopes are also compared with gross beta-decay theory. The systematic trend of the neutron-rich Ca half-lives is consistent with the presence of a subshell gap at N=32.

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arXiv2005

Half Life of the Doubly-magic r-Process Nucleus 78Ni

Nuclei with magic numbers serve as important benchmarks in nuclear theory. In addition, neutron-rich nuclei play an important role in the astrophysical rapid neutron-capture process (r-process). 78Ni is the only doubly-magic nucleus that is also an important waiting point in the r-process, and serves as a major bottleneck in the synthesis of heavier elements. The half-life of 78Ni has been experimentally deduced for the first time at the Coupled Cyclotron Facility of the National Superconducting Cyclotron Laboratory at Michigan State University, and was found to be 110 (+100 -60) ms. In the same experiment, a first half-life was deduced for 77Ni of 128 (+27 -33) ms, and more precise half-lives were deduced for 75Ni and 76Ni of 344 (+20 -24) ms and 238 (+15 -18) ms respectively.

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arXiv1999

Nuclear Structure Studies at ISOLDE and their Impact on the Astrophysical r-Process

The focus of the present review is the production of the heaviest elements in nature via the r-process. A correct understanding and modeling requires the knowledge of nuclear properties far from stability and a detailed prescription of the astrophysical environment. Experiments at CERN/ISOLDE have played a pioneering role in exploring the characteristics of nuclear structure in terms of masses and beta-decay properties. Initial examinations paid attention to far unstable nuclei with magic neutron numbers related to r-process peaks, while present activities are centered on the evolution of shell effects with the distance from the valley of stability. We first show in site-independent applications the effect of both types of nuclear properties on r-process abundances. Then, we explore the results of calculations related to two different `realistic' astrophysical sites, (i) the supernova neutrino wind and (ii) neutron star mergers. We close with a list of remaining theoretical and experimental challenges needed to overcome for a full understanding of the nature of the r-process, and the role CERN/ISOLDE can play in this process.

astro-ph↗
arXiv1998

Decay of neutron-rich Mn nuclides and deformation of heavy Fe isotopes

The use of chemically selective laser ionization combined with beta-delayed neutron counting at CERN/ISOLDE has permitted identification and half-life measurements for 623-ms Mn-61 up through 14-ms Mn-69. The measured half-lives are found to be significantly longer near N=40 than the values calculated with a QRPA shell model using ground-state deformations from the FRDM and ETFSI models. Gamma-ray singles and coincidence spectroscopy has been performed for Mn-64 and Mn-66 decays to levels of Fe-64 and Fe-66, revealing a significant drop in the energy of the first 2+ state in these nuclides that suggests an unanticipated increase in collectivity near N=40.

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