arXiv subjects

W. C. Mei

Publications and source records attributed to W. C. Mei.

5 recordsLinked to original sources

arXiv2026

Towards Collinear Laser Spectroscopy of Radioactive Molecules Utilizing In-trap Produced Molecular Ion Beam

Molecules containing short-lived isotopes, namely radioactive molecules, are among the most promising candidates for probing new physics beyond the Standard Model, although their production and spectroscopic measurements remain technically challenging. Here, we demonstrate an integrated methodology that combines formation of molecular ion beams in a radiofrequency quadrupole cooler-buncher with collinear laser spectroscopy. As a proof-of-principle experiment, we successfully produce molecular ions such as $\rm BaF^+$ and $\rm YbF^+$ via in-trap ion-molecule reactions and perform high-resolution laser spectroscopy of the target molecule $\rm ^{138}BaF$. Vibrational and rotational structures of $\rm ^{138}BaF$ across different electronic states are obtained using resonance-enhanced multiphoton ionization schemes, confirming the feasibility of the proposed methodology. This work establishes a practical route for future formation and spectroscopic studies of short-lived radioactive molecules, such as those containing $\rm ^{225}Ra$, at radioactive ion beam facilities.

physics.atom-ph↗

arXiv2026

Commissioning and Full Realization of the PLASEN System at BRIF

A PLASEN (Precision LAser Spectroscopy for Exotic Nuclei) system, consisting of a compact radio-frequency quadrupole cooler-buncher (RFQ-cb) and a collinear resonance ionization spectroscopy setup, has now been fully commissioned with radioactive ion beams at the Beijing Radioactive Ion-beam Facility (BRIF). Using both stable and radioactive Rb ion beams from BRIF, we demonstrated that the large beam energy spread observed at BRIF has been successfully handled by employing the RFQ-cb, enabling the delivery of high-quality bunched radioactive ion beams for collinear resonance ionization spectroscopy experiments. Under these conditions, we performed laser spectroscopy of exotic nuclei, achieving high resolution (about 100 MHz spectral linewidth) and high sensitivity (up to 1:200 efficiency). This fully operational PLASEN system will serve as a state-of-the-art experimental platform at BRIF for research in multiple fields such as nuclear, atomic and molecular physics.

physics.ins-det↗

arXiv2025

Development and Characterization of a High-Resolution and High-Sensitivity Collinear Resonance Ionization Spectroscopy Setup

With the recent implementation of a radio-frequency quadrupole (RFQ) cooler-buncher and a multi-step laser resonance ionization technique, our previously developed collinear laser spectroscopy setup has been successfully upgraded into a fully functional collinear resonance ionization spectroscopy system. The new system was fully characterized using a bunched ion beam at 30~keV, during which hyperfine structure spectra of $^{85,87}$Rb isotopes were measured. An overall efficiency exceeding 1:200 (one resonant ion detected for every 200 ions after the RFQ cooler-buncher) was achieved while maintaining a spectral resolution of 100 MHz. Under these conditions, the extracted hyperfine structure parameters and isotope shift for $^{85,87}$Rb show excellent agreement with the literature values. These results demonstrate the system's capability to perform high-resolution and high-sensitivity laser spectroscopy of neutron-rich Rb isotopes, which are expected to be produced at the Beijing Radioactive Ion-beam Facility at a rate of approximately 100 particles per second.

physics.ins-det↗

arXiv2024

Pinning down electron correlations in RaF via spectroscopy of excited states and high-accuracy relativistic quantum chemistry

We report the spectroscopy of the 14 lowest excited electronic states in the radioactive molecule radium monofluoride (RaF). The observed excitation energies are compared with fully relativistic state-of-the-art Fock-space coupled cluster (FS-RCC) calculations, which achieve an agreement of >=99.64% (within ~12 meV) with experiment for all states. Guided by theory, a firm assignment of the angular momentum and term symbol is made for 10 states and a tentative assignment for 4 states. The role of high-order electron correlation and quantum electrodynamics effects in the excitation energy of excited states is studied, found to be important for all states. Establishing the simultaneous accuracy and precision of calculations is an important step for research at the intersection of particle, nuclear, and chemical physics, including searches of physics beyond the Standard Model, for which RaF is a promising probe.

physics.atom-ph↗

arXiv2024

Radiative lifetime of the A 2Π1/2 state in RaF with relevance to laser cooling

The radiative lifetime of the $A$ $^2 Π_{1/2}$ (v=0) state in radium monofluoride (RaF) is measured to be 35(1) ns. The lifetime of this state and the related decay rate $Γ= 2.86(8) \times 10^7$ $s^{-1}$ are of relevance to the laser cooling of RaF via the optically closed $A$ $^2 Π_{1/2} \leftarrow X$ $^2Σ_{1/2}$ transition, which makes the molecule a promising probe to search for new physics. RaF is found to have a comparable photon-scattering rate to homoelectronic laser-coolable molecules. Thanks to its highly diagonal Franck-Condon matrix, it is expected to scatter an order of magnitude more photons than other molecules when using just 3 cooling lasers, before it decays to a dark state. The lifetime measurement in RaF is benchmarked by measuring the lifetime of the $8P_{3/2}$ state in Fr to be 83(3) ns, in agreement with literature.

physics.atom-ph↗