arXiv subjects

W. Gawlik

Publications and source records attributed to W. Gawlik.

At least 19 recordsLinked to original sources

arXiv2022

Wide-field magnetometry with nitrogen-vacancy centers in randomly oriented micro-diamonds

Magnetometry with nitrogen-vacancy color centers in diamond has gained significant interest among researchers in recent years. Absolute knowledge of the three-dimensional orientation of the magnetic field is necessary for many applications. Conventional magnetometry measurements are usually performed with NV ensembles in a bulk diamond with a thin NV layer or a scanning probe in the form of a diamond tip, which requires a smooth sample surface and proximity of the probing device, often limiting the sensing capabilities. Here, we present a method for determining the three-dimensional orientation of the magnetic field vector relative to the diamond crystal lattice. We demonstrate that NV centers in arbitrarily oriented submicrometer-sized diamond powder deposited on a planar surface can be used for sensing the magnetic field. Our work can be extended to irregular surfaces, which shows a promising path for nanodiamond-based photonic sensors.

quant-ph↗

arXiv2022

Role of high nitrogen-vacancy concentration on the photoluminescence and Raman spectra of diamond

We present a photoluminescence (PL) and Raman spectroscopy study of various diamond samples that have high concentrations of nitrogen-vacancy (NV) color centers up to multiple parts per million (ppm). With green red, and near infrared (NIR) light excitation, we demonstrate that while for samples with a low density of NV centers the signals are primarily dominated by Raman scattering from the diamond lattice, for higher density of NVs we observe a combination of Raman scattering from the diamond lattice and fluorescence from the NV centers, while for the highest NV densities the Raman signals from diamond are completely overwhelmed by the intense NVs fluorescence. However, under NIR excitation, Raman diamond signatures can be observed for some diamonds. These observations reveal different roles of two mechanisms of light emission and contradict the naive belief that Raman scattering enables complete characterisation of a diamond crystalline sample.

physics.atom-ph↗

arXiv2016

Coherent population oscillations with nitrogen-vacancy color centers in diamond

We present results of our research on two-field (two-frequency) microwave spectroscopy in nitrogen-vacancy (NV-) color centers in a diamond. Both fields are tuned to transitions between the spin sublevels of the NV- ensemble in the 3A2 ground state (one field has a fixed frequency while the second one is scanned). Particular attention is focused on the case where two microwaves fields drive the same transition between two NV- ground state sublevels (ms=0 -> ms=+1). In this case, the observed spectra exhibit a complex narrow structure composed of three Lorentzian resonances positioned at the pump-field frequency. The resonance widths and amplitudes depend on the lifetimes of the levels involved in the transition. We attribute the spectra to coherent population oscillations induced by the two nearly degenerate microwave fields, which we have also observed in real time. The observations agree well with a theoretical model and can be useful for investigation of the NV relaxation mechanisms.

physics.atom-ph↗

arXiv2015

Strontium optical lattice clocks for practical realization of the metre and secondary representation of the second

We present a system of two independent strontium optical lattice standards probed with a single shared ultra-narrow laser. The absolute frequency of the clocks can be verified by the use of Er:fiber optical frequency comb with the GPS-disciplined Rb frequency standard. We report hertz-level spectroscopy of the clock line and measurements of frequency stability of the two strontium optical lattice clocks.

physics.atom-ph↗

arXiv2015

Longitudinal spin relaxation in nitrogen-vacancy ensembles in diamond

We present an experimental study of the longitudinal electron-spin relaxation of ensembles of negatively charged nitrogen-vacancy (NV ) centers in diamond. The measurements were performed with samples having different NV- concentrations and at different temperatures and magnetic fields. We found that the relaxation rate T1-1 increases when transition frequencies in NV- centers with different orientations become degenerate and interpret this as cross-relaxation caused by dipole-dipole interaction.

physics.atom-ph↗

arXiv2014

Microwave saturation spectroscopy of nitrogen-vacancy ensembles in diamond

Negatively-charged nitrogen-vacancy (NV$^-$) centers in diamond have generated much recent interest for their use in sensing. The sensitivity improves when the NV ground-state microwave transitions are narrow, but these transitions suffer from inhomogeneous broadening, especially in high-density NV ensembles. To better understand and remove the sources of broadening, we demonstrate room-temperature spectral "hole burning" of the NV ground-state transitions. We find that hole burning removes the broadening caused by magnetic fields from $^{13}$C nuclei and demonstrate that it can be used for magnetic-field-insensitive thermometry.

physics.optics↗

arXiv2014

Saturated-absorption spectroscopy revisited: atomic transitions in strong magnetic fields ($>$20 mT) with a micrometer-thin cell

The existence of cross-over resonances makes saturated-absorption spectra very complicated when external magnetic field B is applied. It is demonstrated for the first time that the use of micrometric-thin cells (MTC, $L\approx40\,μ$m) allows application of SA for quantitative studies of frequency splittings and shifts of the Rb atomic transitions in a wide range of external magnetic fields, from 0.2 up to 6 kG (20-600 mT). We compare the SA spectra obtained with the MTC with those obtained with other techniques, and present applications for optical magnetometry with micrometer spatial resolution and a broadly tunable optical frequency reference.

physics.atom-ph↗

arXiv2013

Global Network of Optical Magnetometers for Exotic (GNOME): Physics Novel scheme for exotic physics searches

A novel experimental scheme enabling investigation of transient exotic spin couplings is discussed. The scheme is based on synchronous measurements of optical-magnetometer signals of several devices operating in magnetically shielded environments in distant locations ($\gtrsim100$ km). Although signatures of such exotic couplings may be present in the signal from a single magnetometer, it would be challenging to distinguish them from noise. By analyzing the correlation between signals from multiple, geographically separated magnetometers, it is not only possible to identify the exotic transient but also to investigate its nature. The ability of the network to probe presently unconstrained physics beyond the Standard Model is examined by considering the spin coupling to stable topological defects (e.g., domain walls) of axion-like fields. In the spirit of this research, a brief ($\sim 2$ hours) demonstration experiment involving two magnetometers located in Kraków and Berkeley ($\sim 9000$ km separation) is presented and discussion of the data-analysis approaches that may allow for the transient signal identification is provided. The prospects of the network are outlined in the last part of the paper.

physics.atom-ph↗

arXiv2012

How do you know if you ran through a wall?

Stable topological defects of light (pseudo)scalar fields can contribute to the Universe's dark energy and dark matter. Currently the combination of gravitational and cosmological constraints provides the best limits on such a possibility. We take an example of domain walls generated by an axion-like field with a coupling to the spins of standard-model particles, and show that if the galactic environment contains a network of such walls, terrestrial experiments aimed at detection of wall-crossing events are realistic. In particular, a geographically separated but time-synchronized network of sensitive atomic magnetometers can detect a wall crossing and probe a range of model parameters currently unconstrained by astrophysical observations and gravitational experiments.

hep-ph↗

arXiv2011

All-optical atomic magnetometers based on nonlinear magneto-optical rotation with amplitude modulated light

We demonstrate a magnetometric technique based on nonlinear magneto-optical rotation using amplitude modulated light. The magnetometers can be operated in either open-loop (typical nonlinear magneto-optical rotation with amplitude-modulated light) or closed-loop (self-oscillating) modes. The latter mode is particularly well suited for conditions where the magnetic field is changing by large amounts over a relatively short timescale.

physics.atom-ph↗

arXiv2010

Tailoring quantum superpositions with linearly polarized amplitude-modulated light

Amplitude-modulated nonlinear magneto-optical rotation is a powerful technique that offers a possibility of controllable generation of given quantum states. In this paper, we demonstrate creation and detection of specific ground-state magnetic-sublevel superpositions in $^{87}$Rb. By appropriate tuning of the modulation frequency and magnetic-field induction the efficiency of a given coherence generation is controlled. The processes are analyzed versus different experimental parameters.S

physics.atom-ph↗

arXiv2009

High nitrogen-vacancy density diamonds for magnetometry applications

Nitrogen-vacancy (NV) centers in millimeter-scale diamond samples were produced by irradiation and subsequent annealing under varied conditions. The optical and spin relaxation properties of these samples were characterized using confocal microscopy, visible and infrared absorption, and optically detected magnetic resonance. The sample with the highest NV- concentration, approximately 16 ppm = 2.8 x 10^{18} cm^{-3}, was prepared with no observable traces of neutrally-charged vacancy defects. The effective transverse spin relaxation time for this sample was T2* = 118(48) ns, predominately limited by residual paramagnetic nitrogen which was determined to have a concentration of 52(7) ppm. Under ideal conditions, the shot-noise limited sensitivity is projected to be ~150 fT/\sqrt{Hz} for a 100 micron-scale magnetometer based on this sample. Other samples with NV- concentrations from .007 to 12 ppm and effective relaxation times ranging from 27 to 291 ns were prepared and characterized.

cond-mat.mtrl-sci↗

arXiv2009

Electromagnetically Induced Transparency versus Nonlinear Faraday Effect. Coherent Control of the Light Beam Polarization

We report on experimental and theoretical study of the nonlinear Faraday effect under conditions of electromagnetically induced transparency at the 5$S_{1/2} \to 5P_{3/2} \to 5D_{5/2}$ two-photon transition in rubidium vapors. These transitions realize the inverted Y model which combines the $Λ$ and ladder systems. Strong nonlinearity allowing for large rotation angles of a probe beam tuned to the $S\to P$ transition was obtained by creation of quantum superpositions of magnetic sublevels (Zeeman coherences) in the rubidium ground state ($Λ$ scheme). Additionally, electromagnetically induced transparency was accomplished in a ladder scheme by acting with an additional strong coupling laser on the $P\to D$ transition. Under conditions of a two-photon resonance the rotation was significantly reduced, which is interpreted as a competition between the two processes. The effect was observed in sub-Gauss magnetic fields and could be used for efficient coherent control of generation of the ground-state coherences, e.g. for controlling the polarization state of the probe light.

physics.optics↗

arXiv2008

Analysis and calibration of absorptive images of Bose-Einstein condensate at non-zero temperatures

We describe the method allowing quantitative interpretation of absorptive images of mixtures of BEC and thermal atoms which reduces possible systematic errors associated with evaluation of the contribution of each fraction. By using known temperature dependence of the BEC fraction, the analysis allows precise calibration of the fitting results. The developed method is verified in two different measurements and compares well with theoretical calculations and with measurements performed by another group.

cond-mat.other↗

arXiv2008

Free-fall expansion of finite-temperature Bose-Einstein condensed gas in the non Thomas-Fermi regime

We report on our study of the free-fall expansion of a finite-temperature Bose-Einstein condensed cloud of 87Rb. The experiments are performed with a variable total number of atoms while keeping constant the number of atoms in the condensate. The results provide evidence that the BEC dynamics depends on the interaction with thermal fraction. In particular, they provide experimental evidence that thermal cloud compresses the condensate.

cond-mat.other↗

arXiv2007

Magnetometry Based on Nonlinear Magneto-Optical Rotation with Amplitude-Modulated Light

We report on an all-optical magnetometric technique based on nonlinear magneto-optical rotation with amplitude-modulated light. The method enables sensitive magnetic-field measurements in a broad dynamic range. We demonstrate the sensitivity of $4.3\times10^{-9}$ G/$\sqrt{\text{Hz}}$ at 10 mG and the magnetic field tracking in a range of 40 mG. The fundamental limits of the method sensitivity and factors determining current performance of the magnetometer are discussed.

physics.atom-ph↗

arXiv2007

Production and detection of atomic hexadecapole at Earth's magnetic field

Anisotropy of atomic states is characterized by population differences and coherences between Zeeman sublevels. It can be efficiently created and probed via resonant interactions with light, the technique which is at the heart of modern atomic clocks and magnetometers. Recently, nonlinear magneto-optical techniques have been developed for selective production and detection of higher polarization moments, hexadecapole and hexacontatetrapole, in the ground states of the alkali atoms. Extension of these techniques into the range of geomagnetic fields is important for practical applications. This is because hexadecapole polarization corresponding to the $ΔM=4$ Zeeman coherence, with maximum possible $ΔM$ for electronic angular momentum $J=1/2$ and nuclear spin $I=3/2$, is insensitive to the nonlinear Zeeman effect (NLZ). This is of particular interest because NLZ normally leads to resonance splitting and systematic errors in atomic magnetometers. However, optical signals due to the hexadecapole moment decline sharply as a function of magnetic field. We report a novel method that allows selective creation of a macroscopic long-lived ground-state hexadecapole polarization. The immunity of the hexadecapole signal to NLZ is demonstrated with F=2 $^{87}$Rb atoms at Earth's field.

physics.atom-ph↗

arXiv2006

Nonlinear magneto-optical rotation with modulated light in tilted magnetic fields

Larmor precession of laser-polarized atoms contained in anti-relaxation-coated cells, detected via nonlinear magneto-optical rotation (NMOR) is a promising technique for a new generation of ultra-sensitive atomic magnetometers. For magnetic fields directed along the light propagation direction, resonances in NMOR appear when linearly polarized light is frequency- or amplitude-modulated at twice the Larmor frequency. Because the frequency of these resonances depends on the magnitude but not the direction of the field, they are useful for scalar magnetometry. New NMOR resonances at the Larmor frequency appear when the magnetic field is tilted away from the light propagation direction in the plane defined by the light propagation and polarization vectors. These new resonances, studied both experimentally and with a density matrix calculation in the present work, offer a convenient method for NMOR-based vector magnetometry.

physics.atom-ph↗