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W. Hardy

Publications and source records attributed to W. Hardy.

3 recordsLinked to original sources

Persistent short-range charge correlations revealed by ultrafast melting of electronic order in YBa$_2$Cu$_3$O$_{6+x}$

Charge density waves (CDW) are ubiquitous in the complex phase diagram of cuprate superconductors and exhibit both short- and long-range correlations. Using time-resolved resonant X-ray scattering, we investigate the photo-induced dynamics of CDW in YBa$_2$Cu$_3$O$_{6.67}$. We discover an excitation threshold ($\Phi$$_\mathrm{C}$ $\approx$ 65 $\mu$J/cm$^2$) above which long-range CDW disappear, revealing a persistent CDW peak with short-range correlation length. Ultrafast photo-excitation promptly uncovers this residual short-range CDW correlations, appearing within $\approx$ 0.2 ps. Long-range CDW coherence recovers within $\approx$ 0.6 ps, while the peak intensity remains partially suppressed. We rationalize the dichotomic behavior in the fluence and temporal dependencies as the signature of two coexisting CDW peaks, arising from short- and long-range correlations, which we disentangle through their distinct response to photo-excitation. We provide evidence that the collapse of long-range correlations is driven by an electronic process, while short-range correlations are characterized by distinct timescales and stiffness against photo-excitation. This approach establishes ultrafast X-ray scattering as an effective tool for disentangling coexisting density waves and correlations in quantum materials.

cond-mat.supr-con

Enhanced charge density wave coherence in a light-quenched, high-temperature superconductor

Superconductivity and charge density waves (CDW) are competitive, yet coexisting orders in cuprate superconductors. To understand their microscopic interdependence, a probe capable of discerning their interaction on its natural length and time scales is necessary. We use ultrafast resonant soft x-ray scattering to track the transient evolution of CDW correlations in YBa$_{2}$Cu$_{3}$O$_{6+x}$ following the quench of superconductivity by an infrared laser pulse. We observe a non-thermal response of the CDW order characterized by a near doubling of the correlation length within $\approx$ 1 picosecond of the superconducting quench. Our results are consistent with a model in which the interaction between superconductivity and CDW manifests inhomogeneously through disruption of spatial coherence, with superconductivity playing the dominant role in stabilizing CDW topological defects, such as discommensurations.

cond-mat.supr-con

Unusual interplay between superconductivity and field-induced charge order in YBa2Cu3Oy

We present a detailed study of the temperature (T) and magnetic field (H) dependence of the electronic density of states (DOS) at the Fermi level, as deduced from specific heat and Knight shift measurements in underdoped YBa2Cu3Oy. We find that the DOS becomes field-independent above a characteristic field H_{DOS} and that the H_{DOS}(T) line displays an unusual inflection near the onset of the long range 3D charge-density wave order. The unusual S-shape of H_{DOS}(T) is suggestive of two mutually-exclusive orders that eventually establish a form of cooperation in order to coexist at low T. On theoretical grounds, such a collaboration could result from the stabilisation of a pair-density wave state, which calls for further investigations in this region of the phase diagram

cond-mat.supr-con