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W. Helml

Publications and source records attributed to W. Helml.

5 recordsLinked to original sources

Laser-driven bunch compression for ultrashort free-electron laser pulses

Generation of ultrashort X-ray pulses in a free-electron laser relies on high-density electron bunches with a precisely adjusted current and energy distribution. To this end, robust and flexible electron bunch manipulation techniques are required that allow a high degree of control over the phase space density of the bunch. This paper reports on the demonstration of ultrashort current spikes with femtosecond duration, created by compressing an electron bunch after a laser-induced energy modulation with linearly varying envelope. This scheme is implemented at the free-electron laser FLASH, where the energy modulation is created early in the linear accelerator before the bunch is accelerated to its final energy. Formation of the spikes is observed in measurements of the longitudinal phase space density. It is demonstrated that, in conjunction with conventional compression techniques, this laser-based scheme allows to create two spikes with variable temporal separation. Therefore, the demonstrated compression scheme shows great potential of enabling flexible ultrashort single- and double-pulse operation modes of free-electron lasers.

physics.acc-ph

Clocking Auger Electrons

Intense X-ray free-electron lasers (XFELs) can rapidly excite matter, leaving it in inherently unstable states that decay on femtosecond timescales. As the relaxation occurs primarily via Auger emission, excited state observations are constrained by Auger decay. In situ measurement of this process is therefore crucial, yet it has thus far remained elusive at XFELs due to inherent timing and phase jitter, which can be orders of magnitude larger than the timescale of Auger decay. Here, we develop a new approach termed self-referenced attosecond streaking, based upon simultaneous measurements of streaked photo- and Auger electrons. Our technique enables sub-femtosecond resolution in spite of jitter. We exploit this method to make the first XFEL time-domain measurement of the Auger decay lifetime in atomic neon, and, by using a fully quantum-mechanical description, retrieve a lifetime of $2.2^{ + 0.2}_{ - 0.3}$ fs for the KLL decay channel. Importantly, our technique can be generalised to permit the extension of attosecond time-resolved experiments to all current and future FEL facilities.

physics.atom-ph

Dual-energy electron beams from a compact laser-driven accelerator

Ultrafast pump-probe experiments open the possibility to track fundamental material behaviour like changes in its electronic configuration in real time. To date, most of these experiments are performed using an electron or a high-energy photon beam, which is synchronized to an infrared laser pulse. Entirely new opportunities can be explored if not only a single, but multiple synchronized, ultra-short, high-energy beams are used. However, this requires advanced radiation sources that are capable of producing dual-energy electron beams, for example. Here, we demonstrate simultaneous generation of twin-electron beams from a single compact laser wakefield accelerator. The energy of each beam can be individually adjusted over a wide range and our analysis shows that the bunch lengths and their delay inherently amount to femtoseconds. Our proof-of-concept results demonstrate an elegant way to perform multi-beam experiments in future on a laboratory scale.

physics.acc-ph

Femtosecond profiling of shaped X-ray pulses

Arbitrary manipulation of the temporal and spectral properties of X-ray pulses at free-electron lasers (FELs) would revolutionize many experimental applications. At the Linac Coherent Light Source at Stanford National Accelerator Laboratory, the momentum phase-space of the FEL driving electron bunch can be tuned to emit a pair of X-ray pulses with independently variable photon energy and femtosecond delay. However, while accelerator parameters can easily be adjusted to tune the electron bunch phase-space, the final impact of these actuators on the X-ray pulse cannot be predicted with sufficient precision. Furthermore, shot-to-shot instabilities that distort the pulse shape unpredictably cannot be fully suppressed. Therefore, the ability to directly characterize the X-rays is essential to ensure precise and consistent control. In this work, we have generated X-ray pulse pairs and characterized them on a single-shot basis with femtosecond resolution through time-resolved photoelectron streaking spectroscopy. This achievement completes an important step toward future X-ray pulse shaping techniques.

physics.acc-ph

Machine learning applied to single-shot x-ray diagnostics in an XFEL

X-ray free-electron lasers (XFELs) are the only sources currently able to produce bright few-fs pulses with tunable photon energies from 100 eV to more than 10 keV. Due to the stochastic SASE operating principles and other technical issues the output pulses are subject to large fluctuations, making it necessary to characterize the x-ray pulses on every shot for data sorting purposes. We present a technique that applies machine learning tools to predict x-ray pulse properties using simple electron beam and x-ray parameters as input. Using this technique at the Linac Coherent Light Source (LCLS), we report mean errors below 0.3 eV for the prediction of the photon energy at 530 eV and below 1.6 fs for the prediction of the delay between two x-ray pulses. We also demonstrate spectral shape prediction with a mean agreement of 97%. This approach could potentially be used at the next generation of high-repetition-rate XFELs to provide accurate knowledge of complex x-ray pulses at the full repetition rate.

physics.data-an