arXiv subjects

W. K. Park

Publications and source records attributed to W. K. Park.

At least 19 recordsLinked to original sources

arXiv2023

Topological surface states in the Kondo insulator YbB$_{12}$ revealed via planar tunneling spectroscopy

Planar tunneling spectroscopy of the Kondo insulator SmB$_6$ suggests that an interaction between the surface Dirac fermions and the bulk spin excitons results in incompletely protected topological surface states. To gain further insight into their true nature, it is necessary to study other topological Kondo insulator candidates. Calculations of electronic energy bands predict that the Kondo insulator YbB$_{12}$ hosts topological surface states protected by crystalline mirror symmetry. In this study, we present tunneling conductance spectra obtained from the (001) surface of YbB$_{12}$ single crystals and discuss them in comparison to SmB$_6$. The linear conductance at low bias provides strong evidence for the existence of surface Dirac fermions. The double-hump structure in the negative bias region is associated with hybridized band edges, in agreement with a calculated band structure. While these similarities with SmB6 are suggestive of the existence of topological surface states in YbB$_{12}$, in agreement with other experiments, some discrepancies are also observed, which we attribute to a difference in their exact nature from those in SmB$_6$.

cond-mat.str-el↗

arXiv2021

Spectroscopic Evidence for the Direct Involvement of Local Moments in the Pairing Process of the Heavy-Fermion Superconductor CeCoIn$_5$

The microscopic mechanism for electron pairing in heavy-fermion superconductors remains a major challenge in quantum materials. Some form of magnetic mediation is widely accepted with spin fluctuations as a prime candidate. A novel mechanism, 'composite pairing' based on the cooperative two-channel Kondo effect directly involving the f-electron moments has also been proposed for some heavy fermion compounds including CeCoIn$_5$. The origin of the spin resonance peak observed in neutron scattering measurements on CeCoIn$_5$ is still controversial and the corresponding hump-dip structure in the tunneling conductance is missing. This is in contrast to the cuprate and Fe-based high-temperature superconductors, where both characteristic signatures are observed, indicating spin fluctuations are likely involved in the pairing process. Here, we report results from planar tunneling spectroscopy along three major crystallographic orientations of CeCoIn5 over wide ranges of temperature and magnetic field. The pairing gap opens at T$_p$ ~ 5 K, well above the bulk T$_c$ = 2.3 K, and its directional dependence is consistent with d$_{x^2-y^2}$ symmetry. With increasing magnetic field, this pairing gap is suppressed as expected but, intriguingly, a gaplike structure emerges smoothly, increasing linearly up to the highest field applied. This field-induced gaplike feature is only observed below T$_p$. The concomitant appearance of the pairing gap and the field-induced gaplike feature, along with its linear increase with field, indicates that the f-electron local moments are directly involved in the pairing process in CeCoIn$_5$.

cond-mat.supr-con↗

arXiv2021

Topological nature of the Kondo insulator SmB$_6$ and its sensitiveness to Sm vacancy

The true topological nature of the Kondo insulator SmB$_6$ remains to be unveiled. Our previous tunneling study not only found evidence for the existence of surface Dirac fermions, but it also uncovered that they inherently interact with the spin excitons, collective excitations in the bulk. We have extended such a spectroscopic investigation into crystals containing a Sm deficiency. The bulk hybridization gap is found to be insensitive to the deficiency up to 1% studied here, but the surface states in Sm-deficient crystals exhibit quite different temperature evolutions from those in stoichiometric ones. We attribute this to the topological surface states remaining incoherent down to the lowest measurement temperature due to their continued interaction with the spin excitons that remain uncondensed. This result shows that the detailed topological nature of SmB$_6$ could vary drastically in the presence of disorder in the lattice. This sensitiveness to disorder is seemingly contradictory to the celebrated topological protection, but it can be understood as being due to the intimate interplay between strong correlations and topological effects.

cond-mat.str-el↗

arXiv2020

Origin of gap-like behaviors in URu$_2$Si$_2$: Combined study via quasiparticle scattering spectroscopy and resistivity measurements

We address two long-standing questions regarding the hidden order in URu2Si2: Is it associated with the hybridization process, and what are the distinct roles played by the localized and itinerant electrons? Our quasiparticle scattering spectroscopy reveals a hybridization gap ubiquitous in the entire phase space spanned by P and Fe substitutions in URu2Si2, including the no-order and antiferromagnetic regions, with minimal change upon crossing the phase boundary. This indicates its opening isn't associated with the ordering, and thus localized electrons must be the major player. Towards a consistent understanding of all the other gap-like behaviors observed only below transition temperatures, we analyze the electrical resistivity using a model in which gapped bosonic excitations are the dominant scattering source. With their stiffness set to follow an unusual temperature dependence (decreasing with decreasing temperature), this model fits all of our resistivity data well including the jump at the transition. Remarkably, the extracted gap increases slowly with increasing Fe content, similarly to the gap detected by inelastic neutron scattering at Q1 = (1.4, 0, 0), suggesting a common origin. Such a model can also naturally explain the Hall effect temperature dependence without invoking Fermi surface gapping.

cond-mat.str-el↗

arXiv2017

Planar tunneling spectroscopy of the topological Kondo insulator SmB$_6$

Several technical issues and challenges are identified and investigated for the planar tunneling spectroscopy of the topological Kondo insulator SmB$_6$. Contrasting behaviors of the tunnel junctions prepared in two different ways are analyzed and explained in detail. The conventional approach based on an AlO$_\text{x}$ tunnel barrier results in unsatisfactory results due to the inter-diffusion between SmB$_6$ and deposited Al. On the contrary, plasma oxidation of SmB$_6$ crystals produces high-quality tunnel barriers on both (001) and (011) surfaces. Resultant conductance spectra are highly reproducible with clear signatures for the predicted surface Dirac fermions and the bulk hybridization gap as well. The surface states are identified to reside on two or one {\it distinguishable} Dirac cone(s) on the (001) and (011) surface, respectively, in good agreement with the recent literature. However, their topological protection is found to be limited within the low energy region due to their inevitable interaction with the bulk excitations, called spin excitons, consistent with a recent theoretical prediction. Implications of our findings on other physical properties in SmB$_6$ and also other correlated topological materials are remarked.

cond-mat.str-el↗

arXiv2017

Hybridization gap in the heavy-fermion compound UPd$_2$Al$_3$ via quasiparticle scattering spectroscopy

We present results from point-contact spectroscopy of the antiferromagnetic heavy-fermion superconductor UPd$_2$Al$_3$: conductance spectra are taken from single crystals with two major surface orientations as a function of temperature and magnetic field, and analyzed using a theory of co-tunneling into an Anderson lattice. Spectroscopic signatures are clearly identified including the distinct asymmetric double-peak structure arising from the opening of a hybridization gap when a coherent heavy Fermi liquid is formed. Both the hybridization gap, found to be 7.2 $\pm$ 0.3 meV at 4 K, and the conductance enhancement above a flat background decrease upon increasing temperature. While the hybridization gap is extrapolated to remain finite up to $\sim$28 K, close to the temperature around which the magnetic susceptibility displays a broad peak, the conductance enhancement vanishes at $\sim$18 K, slightly above the antiferromagnetic transition temperature ($T_\textrm{N}$ $\approx$ 14 K). This rapid decrease of the conductance enhancement is understood as a consequence of the junction drifting away from the ballistic regime due to increased scattering off magnons associated with the localized U 5$f$ electrons. This shows that while the hybridization gap opening is not directly associated with the antiferromagnetic ordering, its visibility in the conductance is greatly affected by the temperature-dependent magnetic excitations. Our findings are not only consistent with the 5$f$ dual-nature picture in the literature but also shed new light on the interplay between the itinerant and localized electrons in UPd$_2$Al$_3$.

cond-mat.str-el↗

arXiv2016

Design and construction of a point-contact spectroscopy rig with lateral scanning capability

The design and realization of a cryogenic rig for point-contact spectroscopy measurements in the needle-anvil configuration is presented. Thanks to the use of two piezoelectric nano-positioners, the tip can move along the vertical ($z$) and horizontal ($x$) direction and thus the rig is suitable to probe different regions of a sample \textit{in situ}. Moreover, it can also form double point-contacts on different facets of a single crystal for achieving, e.g., an interferometer configuration for phase-sensitive measurements. For the latter purpose, the sample holder can also host a Helmholtz coil for applying a small transverse magnetic field to the junction. A semi-rigid coaxial cable can be easily added for studying the behavior of Josephson junctions under microwave irradiation. The rig can be detached from the probe and thus used with different cryostats. The performance of this new probe has been tested in a Quantum Design PPMS system by conducting point-contact Andreev reflection measurements on Nb thin films over large areas as a function of temperature and magnetic field.

cond-mat.supr-con↗

arXiv2014

Automated fabrication technique of gold tips for use in point-contact spectroscopy

For a successful point-contact spectroscopy (PCS) measurement, metallic tips of proper shape and smoothness are essential to ensure the ballistic nature of a point-contact junction. Until recently, the fabrication of Au tips suitable for use in point-contact spectroscopy has remained more of an art involving a trial and error method rather than an automated scientific process. To address these issues, we have developed a technique with which one can prepare high quality Au tips reproducibly and systematically. It involves an electronic control of the driving voltages used for an electrochemical etching of a gold wire in an HCl-glycerol mixture or an HCl solution. We find that a stopping current, below which the circuit is set to shut off, is a single very important parameter to produce an Au tip of desired shape. We present detailed descriptions for a two-step etching process for Au tips and also test results from PCS measurements using them.

physics.ins-det↗

arXiv2014

Hybridization and Slow Coherence Crossover in the Intermediate Valence Compound YbAl$_3$ via Quasiparticle Scattering Spectroscopy

The intermediate valence compound YbAl$_3$ is known to undergo a hybridization process between itinerant and localized electrons. The resulting heavy Fermi liquid remains non-magnetic and non-superconducting. A microscopic understanding of the hybridization process in YbAl$_3$ is still lacking although some characteristic temperature and energy scales have been identified. Here we report results from novel spectroscopic measurements based on quasiparticle scattering. From the conductance spectra taken over a wide temperature range, we deduce that the band renormalization and hybridization process begins around 110 K, causing the conductance enhancement with a Fano background. This temperature, a new scale found in this work, is much higher than the coherence temperature (34 K). Our observation is in agreement with the slow crossover scenario discussed recently in the literature. The indirect hybridization gap appears to open concomitantly with the emergence of a coherent Fermi liquid. Thus, we suggest its measurement as a more rigorous way to define the coherence temperature than just taking the temperature for a resistivity peak.

cond-mat.str-el↗

arXiv2012

Detection of Orbital Fluctuations Above the Structural Transition Temperature in the Iron-Pnictides and Chalcogenides

We use point contact spectroscopy to probe $\rm{AEFe_2As_2}$ ($\rm{AE=Ca, Sr, Ba}$) and $\rm{Fe_{1+y}Te}$. For $\rm{AE=Sr, Ba}$ we detect orbital fluctuations above $T_S$ while for AE=Ca these fluctuations start below $T_S$. Co doping preserves the orbital fluctuations while K doping suppresses it. The fluctuations are only seen at those dopings and temperatures where an in-plane resistive anisotropy is known to exist. We predict an in-plane resistive anisotropy of $\rm{Fe_{1+y}Te}$ above $T_S$. Our data are examined in light of the recent work by W.-C. Lee and P. Phillips (arXiv:1110.5917v2). We also study how joule heating in the PCS junctions impacts the spectra. Spectroscopic information is only obtained from those PCS junctions that are free of heating effects while those PCS junctions that are in the thermal regime display bulk resistivity phenomenon.

cond-mat.supr-con↗

arXiv2012

Observation of the hybridization gap and Fano resonance in the Kondo lattice URu2Si2

The nature of the second order phase transition that occurs in URu2Si2 at 17.5 K remains puzzling despite intensive research over the past two and half decades. A key question emerging in the field is whether a hybridization gap between the renormalized bands can be identified as the long-sought 'hidden' order parameter. We report on the measurement of a hybridization gap in URu2Si2 employing a spectroscopic technique based on quasiparticle scattering across a ballistic metallic junction. The differential conductance exhibits an asymmetric double-peak structure, a clear signature for a Fano resonance in a Kondo lattice. The extracted hybridization gap opens well above the transition temperature, indicating that it is not the hidden order parameter. Our results put stringent constraints on the origin of the hidden order transition in URu2Si2 and demonstrate that quasiparticle scattering spectroscopy can probe the band renormalizations in a Kondo lattice via detection of a novel type of Fano resonance.

cond-mat.str-el↗

arXiv2011

Gap-like feature in the normal state of $\bf{X(Fe_{1-x}Co_x)_2As_2}$, $\bf{X=Ba,Sr}$ and $\bf{Fe_{1+y}Te}$ revealed by Point Contact Spectroscopy

Point contact spectroscopy reveals a gap-like feature above the magnetic and structural transition temperatures for underdoped $Ba(Fe_{1-x}Co_x)_2As_2$, $SrFe_2As_2$ and $Fe_{1+y}Te$. The conductance spectrum starts showing an enhancement at temperatures as high as 177 K for $BaFe_2As_2$ ($T_N$ $\sim$ 132 K) and 250 K for $SrFe_2As_2$ ($T_N$ $\sim$ 192 K). Possible origins for this enhancement are discussed in light of recent experimental claims of nematicity in these materials. We construct a modified phase diagram for Co-doped Ba122 showing a gap-like feature existing above $T_N$ and $T_S$ for the underdoped regime.

cond-mat.supr-con↗

arXiv2010

Phase Separation and Chemical Inhomogeneity in the Iron Chalcogenide Superconductor Fe1+yTexSe1-x

We report investigation on Fe1+yTexSe1-x single crystals by using scanning transmission electron microscopy (STEM) and electron energy loss spectroscopy (EELS). Both nonsuperconducting samples with excess iron and superconducting samples demonstrate nanoscale phase separation and chemical inhomogeneity of Te/Se content, which we attribute to a miscibility gap. The line scan EELS technique indicates ~20% or less fluctuation of Te concentration from the nominal compositions.

cond-mat.supr-con↗

arXiv2010

Point-contact spectroscopy in heavy-fermion superconductors

We develop a minimal model to calculate point-contact spectra between a metallic tip and a superconducting heavy-fermion system. We apply our tunneling model to the heavy fermion CeCoIn5, both in the normal and superconducting state. In point-contact and scanning tunneling spectroscopy many heavy-fermion materials, like CeCoIn5, exhibit an asymmetric differential conductance, dI/dV, combined with a strongly suppressed Andreev reflection signal in the superconducting state. We argue that both features may be explained in terms of a multichannel tunneling model in the presence of localized states near the interface. We find that it is not sufficient to tunnel into two itinerant bands of light and heavy electrons to explain the Fano line shape of the differential conductance. Localized states in the bulk or near the interface are an essential component for quantum interference to occur when an electron tunnels from the metallic tip of the point contact into the heavy-fermion system.

cond-mat.supr-con↗

arXiv2010

Strong Coupling Superconductivity in Iron-Chalcogenide FeTe$_{0.55}$Se$_{0.45}$

The superconducting order parameter in the iron-chalcogenide superconductor FeTe$_{0.55}$Se$_{0.45}$ ($T_\textrm{c}$ = 14.2 K) is investigated by point-contact Andreev reflection spectroscopy. The energy gap magnitude (3.8 meV at 1.70 K) and temperature dependence as extracted from the Andreev conductance spectra reveal strong-coupling superconductivity and is consistent with $s$-wave order parameter symmetry. No clear evidence for multiple order parameters or interference from multiple bands is observed. A conductance enhancement persists above $T_\textrm{c}$ to $\sim 18-20$ K and possible origins, including novel quasiparticle scattering due to strong antiferromagnetic spin fluctuations, are discussed.

cond-mat.supr-con↗

arXiv2010

Superconducting order parameter in nonmagnetic borocarbides RNi$_{2}$B$_{2}$C (R=Y, Lu) probed by point-contact Andreev reflection spectroscopy

We report on the measurements of the superconducting order parameter in the nonmagnetic borocarbides LuNi$_2$B$_2$C and YNi$_2$B$_2$C. Andreev conductance spectra are obtained from nanoscale metallic junctions on single crystal surfaces prepared along three major crystallographic orientations: [001], [110], and [100]. The gap values extracted by the single-gap Blonder-Tinkham-Klapwijk model follow the BCS predictions as a function of temperature and magnetic field and exhibit a small anisotropy. These observations are robust and reproducible among all the measurements on two different sets of LuNi$_2$B$_2$C crystals and one set of YNi$_2$B$_2$C crystals. We suggest possible explanations for the small gap anisotropy based on the recent detailed gap measurements by angle-resolved photoemission spectroscopy and the tunneling cone effect. Our results provide a consistent picture of the superconducting gap structure in these materials, addressing the controversy particularly in the reported results of point-contact Andreev reflection spectroscopy.

cond-mat.supr-con↗

arXiv2009

Point-contact spectroscopic studies on normal and superconducting AFe_2As_2-type iron-pnictide single crystals

Point-contact Andreev reflection spectroscopy (PCARS) is applied to investigate the gap structure in iron pnictide single crystal superconductors of the AFe_2As_2 (A=Ba, Sr) family ("Fe-122"). The observed point-contact junction conductance curves, G(V), can be divided into two categories: one where Andreev reflection is present for both (Ba_{0.6}K_{0.4})Fe_2As_2 and Ba(Fe_{0.9}Co_{0.1})_2As_2, and the other with a V^{2/3} background conductance universally observed extending even up to 100 meV for Sr_{0.6}Na_{0.4}Fe_2As_2 and Sr(Fe_{0.9}Co_{0.1})_2As_2. The latter is also observed in point-contact junctions on the nonsuperconducting parent compound BaFe_2As_2. Mesoscopic phase-separated coexistence of magnetic and superconducting orders is considered to explain distinct behaviors in the superconducting samples. For Ba_{0.6}K_{0.4}Fe_2As_2, double peaks due to Andreev reflection with strongly-sloping background are frequently observed for point-contacts on freshly-cleaved c-axis surfaces. If normalized by a background baseline and analyzed by the Blonder-Tinkham-Klapwijk model, the data show a gap size ~3.0-4.0 meV with 2Δ_0/k_BT_c ~ 2.0-2.6, consistent with the smaller gap size reported in the LnFeAsO family ("Fe-1111"). For the Ba(Fe_{0.9}Co_{0.1})_2As_2, G(V) curves typically display a zero-bias conductance peak.

cond-mat.supr-con↗

arXiv2008

Andreev Reflection in Heavy-Fermion Superconductors and Order Parameter Symmetry in CeCoIn_5

Differential conductance spectra are obtained from nanoscale junctions on the heavy-fermion superconductor CeCoIn$_5$ along three major crystallographic orientations. Consistency and reproducibility of characteristic features among the junctions ensure their spectroscopic nature. All junctions show a similar conductance asymmetry and Andreev reflection-like conductance with reduced signal (~ 10%-13%), both commonly observed in heavy-fermion superconductor junctions. Analysis using the extended Blonder-Tinkham-Klapwijk model indicates that our data provide the first spectroscopic evidence for $d_{x^2-y^2}$ symmetry. To quantify our conductance spectra, we propose a model by considering the general phenomenology in heavy fermions, the two-fluid behavior, and an energy-dependent density of states. Our model fits to the experimental data remarkably well and should invigorate further investigations.

cond-mat.supr-con↗