arXiv subjects

W. Langbein

Publications and source records attributed to W. Langbein.

At least 19 recordsLinked to original sources

arXiv2024

Controlling dephasing of coupled qubits via shared-bath coherence

The interaction of a quantum system with its environment limits its coherence time. This, in particular, restricts the utility of qubits in quantum information processing applications. In this paper, we show that the decoherence of a coupled qubit system can be minimized, or even eliminated, by exploiting the quantum coherence of the bath itself. We investigate the dephasing in a system of two spatially separated, electronically decoupled qubits, with direct or mediated coupling, interacting with a shared bath. For illustration, we treat Förster or cavity-mediated coupling between semiconductor quantum dots interacting with acoustic phonons. Using the rigorous method of Trotter's decomposition with cumulant expansion, we demonstrate a reduction in the dephasing rates at specific distances between the dots. The control of dephasing with distance is a coherent effect of the shared bath and is absent for independent baths. It can be understood in terms of phonon-assisted transitions between the entangled qubit states of the coupled system.

cond-mat.mes-hall↗

arXiv2021

Influence of disorder on a Bragg microcavity

Using the resonant-state expansion for leaky optical modes of a planar Bragg microcavity, we investigate the influence of disorder on its fundamental cavity mode. We model the disorder by randomly varying the thickness of the Bragg-pair slabs (composing the mirrors) and the cavity, and calculate the resonant energy and linewidth of each disordered microcavity exactly, comparing the results with the resonant-state expansion for a large basis set and within its first and second orders of perturbation theory. We show that random shifts of interfaces cause a growth of the inhomogeneous broadening of the fundamental mode that is proportional to the magnitude of disorder. Simultaneously, the quality factor of the microcavity decreases inversely proportional to the square of the magnitude of disorder. We also find that first-order perturbation theory works very accurately up to a reasonably large disorder magnitude, especially for calculating the resonance energy, which allows us to derive qualitatively the scaling of the microcavity properties with disorder strength.

cond-mat.dis-nn↗

arXiv2019

Resonant-state expansion applied to three-dimensional open optical systems: A complete set of static modes

We present two alternative complete sets of static modes of a homogeneous dielectric sphere, for their use in the resonant-state expansion (RSE), a rigorous perturbative method in electrodynamics. Physically, these modes are needed to correctly describe the static electric field of a charge redistribution within the optical system due to a perturbation of the permittivity. We demonstrate the convergence of the RSE towards the exact result for a perturbation describing a size reduction of the basis sphere. We then revisit the quarter-sphere perturbation treated in [Doost {\it et al.}, Phys. Rev. A {\bf 90}, 013834 (2014)], where only a single static mode per each angular momentum was introduced, and show that using a complete set of static modes leads to a small, though non-negligible correction of the RSE result, improving the agreement with finite-element simulations. As another example of applying the RSE with a complete set of static modes, we calculate the resonant states of a dielectric cylinder, also comparing the result with a finite-element simulation.

physics.optics↗

arXiv2019

99% beta factor and directional coupling of quantum dots to fast light in photonic crystal waveguides determined by hyperspectral imaging

Spontaneous emission from excitonic transitions in InAs/GaAs quantum dots embedded in photonic crystal waveguides at 5K into non-guided and guided modes is determined by direct hyperspectral imaging. This enables measurement of the absolute coupling efficiency into the guided modes, the beta-factor, directly, without assumptions on decay rates used previously. Notably, we found beta-factors above 90% over a wide spectral range of 40meV in the fast light regime, reaching a maximum of (99 $\pm$ 1)%. We measure the directional emission of the circularly polarized transitions in a magnetic field into counter-propagating guided modes, to deduce the mode circularity at the quantum dot sites. We find that points of high directionality, up to 97%, correlate with a reduced beta-factor, consistent with their positions away from the mode field antinode. By comparison with calibrated finite-difference time-domain simulations, we use the emission energy, mode circularity and beta-factor to estimate the quantum dot position inside the photonic crystal waveguide unit cell.

cond-mat.mes-hall↗

arXiv2018

Resonant-state expansion of three-dimensional open optical systems: Light scattering

A rigorous method of calculating the electromagnetic field, the scattering matrix, and scattering cross-sections of an arbitrary finite three-dimensional optical system described by its permittivity distribution is presented. The method is based on the expansion of the Green's function into the resonant states of the system. These can be calculated by any means, including the popular finite element and finite-difference time-domain methods. However, using the resonant-state expansion with a spherically-symmetric analytical basis, such as that of a homogeneous sphere, allows to determine a complete set of the resonant states of the system within a given frequency range. Furthermore, it enables to take full advantage of the expansion of the field outside the system into vector spherical harmonics, resulting in simple analytic expressions. We verify and illustrate the developed approach on an example of a dielectric sphere in vacuum, which has an exact analytic solution known as Mie scattering.

physics.optics↗

arXiv2018

No exceptional precision of exceptional point sensors

Recently, sensors with resonances at exceptional points (EPs) have been suggested to have a vastly improved sensitivity due to the extraordinary scaling of the complex frequency splitting of the $n$ initially degenerate modes with the $n$-th root of the perturbation. We show here that the resulting quantum-limited signal to noise at EPs is proportional to the perturbation, and comparable to other sensors, thus providing the same precision. The complex frequency splitting close to EPs is therefore not suited to estimate the precision of EP sensors. The underlying reason of this counter-intuitive result is that the mode fields, described by the eigenvectors, are equal for all modes at the EP, and are strongly changing with the perturbation.

physics.app-ph↗

arXiv2018

Quantitative chemical imaging of amyloid-β plaques with Raman micro-spectroscopy in human Alzheimer's diseased brains

Alzheimer's disease (AD) is a neurodegenerative disorder and the most common cause of dementia in the elderly. The extracellular accumulation of amyloid-$β$ (A$β$) in senile plaques is a principal event in the pathogenesis and there is growing evidence that the dysregulation of lipid pathways is implicated in the disease, however the link between these two is still under study. In this work, we investigated human brain samples, from 11 AD patients and a control cohort of age-matched subjects without AD, using label-free chemically-specific Raman micro-spectroscopy. The collected image data were quantitatively analysed using an efficient quantitative unsupervised/partially supervised non-negative matrix factorization method, to retrieve the concentration maps and spectra of the samples' chemical constituents. Significant changes in lipid composition as well as increased concentrations of oxidative stress bio-markers were observed in AD tissues compared to the control. In particular, the analysis revealed accumulations of cholesteryl esters with saturated long-chain fatty acids (FAs), A$β$ fibrils, arachidic acid, fibrin, collagen-like amyloidogenic component (CLAC), $β$-carotene and magnetite, co-localising in A$β$ plaques of AD human brains and exhibiting concentrations highest at the fibrillar core and lowest at the rim. This finding opens perspectives for new anti-inflammatory and antioxidant drug strategies, designed to restore brain homeostasis as potential therapeutics of AD. We also demonstrate by the means of spatial concentration histograms that these identified species separate AD from non-demented control brains, beneficial for AD diagnosis.

physics.med-ph↗

arXiv2017

Impact of environment on dynamics of exciton complexes in a WS$_2$ monolayer

Scientific curiosity to uncover original optical properties and functionalities of atomically thin semiconductors, stemming from unusual Coulomb interactions in the two-dimensional geometry and multi-valley band structure, drives the research on monolayers of transition metal dichalcogenides (TMDs). While recent works ascertained the exotic energetic schemes of exciton complexes in TMDs, we here employ four-wave mixing microscopy to indicate that their subpicosecond dynamics is determined by the surrounding disorder. Focusing on a monolayer WS$_2$, we observe that exciton coherence is lost primarily due to interaction with phonons and relaxation processes towards optically dark excitonic states. Notably, when temperature is low and disorder weak excitons large coherence volume results in huge oscillator strength, allowing to reach the regime of radiatively limited dephasing and we observe long valley coherence. We thus elucidate the crucial role of exciton environment in the TMDs on its dynamics and show that revealed mechanisms are ubiquitous within that family.

cond-mat.mes-hall↗

arXiv2017

Optimizing the Drude-Lorentz model for material permittivity - method, program, and examples for gold, silver, and copper

Approximating the frequency dispersion of the permittivity of materials with simple analytical functions is of fundamental importance for understanding and modeling the optical response of materials and resulting structures. In the generalized Drude-Lorentz model, the permittivity is described in the complex frequency plane by a number of simple poles having complex weights, which is a physically relevant and mathematically simple approach: By construction, it respects causality represents physical resonances of the material, and can be implemented easily in numerical simulations. We report here an efficient method of optimizing the fit of measured data with the Drude-Lorentz model having an arbitrary number of poles. We show examples of such optimizations for gold, silver, and copper, for different frequency ranges and up to four pairs of Lorentz poles taken into account. We also provide a program implementing the method for general use.

physics.optics↗

arXiv2017

Resonantly excited exciton dynamics in two-dimensional MoSe$_2$ monolayers

We report on the exciton and trion density dynamics in a single layer of MoSe$_2$, resonantly excited and probed using three-pulse four-wave mixing (FWM), at temperatures from 300K to 77K . A multi-exponential third-order response function for amplitude and phase of the heterodyne-detected FWM signal including four decay processes is used to model the data. We provide a consistent interpretation within the intrinsic band structure, not requiring the inclusion of extrinsic effects. We find an exciton radiative lifetime in the sub-picosecond range consistent to what has been recently reported. After the dominating radiative decay, the remaining exciton density, which has been scattered from the initially excited bright radiative state into dark states of different nature by exciton-phonon scattering or disorder scattering, shows a slower dynamics, covering 10ps to 10ns timescales. This includes direct bright transitions with larger in-plane momentum, as well as indirect dark transitions to indirect dark states. We find that exciton-exciton annihilation is not relevant in the observed dynamics, in variance from previous finding under non-resonant excitation. The trion density at 77K reveals a decay of the order of 1ps, similar to what is observed for the exciton. After few tens of picoseconds, the trion dynamics resembles the one of the exciton, indicating that trion ionization occurs on this timescale.

cond-mat.mes-hall↗

arXiv2017

Resonant-state expansion of light propagation in non-uniform waveguides

A new rigorous approach for precise and efficient calculation of light propagation along non-uniform waveguides is presented. Resonant states of a uniform waveguide, which satisfy outgoing-wave boundary conditions, form a natural basis for expansion of the local electromagnetic field. Using such an expansion at fixed frequency, we convert the wave equation for light propagation in a non-uniform waveguide into an ordinary second-order matrix differential equation for the expansion coefficients depending on the coordinate along the waveguide. We illustrate the method on several examples of non-uniform planar waveguides and evaluate its efficiency compared to the aperiodic Fourier modal method and the finite element method, showing improvements of one to four orders of magnitude. A similar improvement can be expected also for applications in other fields of physics showing wave phenomena, such as acoustics and quantum mechanics.

physics.optics↗

arXiv2016

Impact of phonons on dephasing of individual excitons in deterministic quantum dot microlenses

Optimized light-matter coupling in semiconductor nanostructures is a key to understand their optical properties and can be enabled by advanced fabrication techniques. Using in-situ electron beam lithography combined with a low-temperature cathodoluminescence imaging, we deterministically fabricate microlenses above selected InAs quantum dots (QDs) achieving their efficient coupling to the external light field. This enables to perform four-wave mixing micro-spectroscopy of single QD excitons, revealing the exciton population and coherence dynamics. We infer the temperature dependence of the dephasing in order to address the impact of phonons on the decoherence of confined excitons. The loss of the coherence over the first picoseconds is associated with the emission of a phonon wave packet, also governing the phonon background in photoluminescence (PL) spectra. Using theory based on the independent boson model, we consistently explain the initial coherence decay, the zero-phonon line fraction, and the lineshape of the phonon-assisted PL using realistic quantum dot geometries.

cond-mat.mes-hall↗

arXiv2016

Dynamics of excitons in individual InAs quantum dots revealed in four-wave mixing spectroscopy

A detailed understanding of the population and coherence dynamics in optically driven individual emitters in solids and their signatures in ultrafast nonlinear-optical signals is of prime importance for their applications in future quantum and optical technologies. In a combined experimental and theoretical study on exciton complexes in single semiconductor quantum dots we reveal a detailed picture of the dynamics employing three-beam polarization-resolved four-wave mixing (FWM) micro-spectroscopy. The oscillatory dynamics of the FWM signals in the exciton-biexciton system is governed by the fine-structure splitting and the biexciton binding energy in an excellent quantitative agreement between measurement and analytical description. The analysis of the excitation conditions exhibits a dependence of the dynamics on the specific choice of polarization configuration, pulse areas and temporal ordering of driving fields. The interplay between the transitions in the four-level exciton system leads to rich evolution of coherence and population. Using two-dimensional FWM spectroscopy we elucidate the exciton-biexciton coupling and identify neutral and charged exciton complexes in a single quantum dot. Our investigations thus clearly reveal that FWM spectroscopy is a powerful tool to characterize spectral and dynamical properties of single quantum structures.

cond-mat.mes-hall↗

arXiv2016

Comment on "Normalization of quasinormal modes in leaky optical cavities and plasmonic resonators"

Recently, Kristensen, Ge and Hughes have compared [Phys. Rev. A 92, 053810 (2015)] three different methods for normalization of quasinormal modes in open optical systems, and concluded that they all provide the same result. We show here that this conclusion is incorrect and illustrate that the normalization of [Opt. Lett. 37, 1649 (2012)] is divergent for any optical mode having a finite quality factor, and that the Silver-Mueller radiation condition is not fulfilled for quasinormal modes.

cond-mat.mes-hall↗

arXiv2015

Exact mode volume and Purcell factor of open optical systems

The Purcell factor quantifies the change of the radiative decay of a dipole in an electromagnetic environment relative to free space. Designing this factor is at the heart of photonics technology, striving to develop ever smaller or less lossy optical resonators. The Purcell factor can be expressed using the electromagnetic eigenmodes of the resonators, introducing the notion of a mode volume for each mode. This approach allows to use an analytic treatment, consisting only of sums over eigenmode resonances, a so-called spectral representation. We show in the present work that the expressions for the mode volumes known and used in literature are only approximately valid for modes of high quality factor, while in general they are incorrect. We rectify this issue, introducing the exact normalization of modes. We present an analytic theory of the Purcell effect based on the exact mode normalization and resulting effective mode volume. We use a homogeneous dielectric sphere in vacuum, which is analytically solvable, to exemplify these findings.

cond-mat.mes-hall↗

arXiv2015

Multi-Wave Coherent Control of a Solid State Single Emitter

Coherent control of individual two-level systems (TLSs) is at the basis of any implementation of quantum information. An impressive level of control is now achieved using nuclear, vacancies and charge spins. Manipulation of bright exciton transitions in semiconductor quantum dots (QDs) is less advanced, principally due to the sub-nanosecond dephasing. Conversely, owing to their robust coupling to light, one can apply tools of nonlinear spectroscopy to achieve all-optical command. Here, we report on the coherent manipulation of an exciton via multi-wave mixing. Specifically, we employ three resonant pulses driving a single InAs QD. The first two induce a four-wave mixing (FWM) transient, which is projected onto a six-wave mixing (SWM) depending on the delay and area of the third pulse, in agreement with analytical predictions. Such a switch enables to demonstrate the generation of SWM on a single emitter and to engineer the spectro-temporal shape of the coherent response originating from a TLS. These results pave the way toward multi-pulse manipulations of solid state qubits via implementing the NMR-like control schemes in the optical domain.

cond-mat.mes-hall↗

arXiv2015

Resonant-state expansion of dispersive open optical systems

A resonant-state expansion (RSE) for open optical systems with a general frequency dispersion of the relative permittivity, described by a finite number of simple poles, is presented. As in the non-dispersive case, the RSE of dispersive systems converts Maxwell's wave equation into a linear matrix eigenvalue problem in the basis of unperturbed resonant states, in this way numerically exactly determining all relevant eigenmodes of the optical system. This dispersive RSE is verified by application to the analytically solvable system of a sphere in vacuum, with a dispersion of the dielectric constant described by the Drude and Drude-Lorentz models. We calculate the change of the optical modes when converting the sphere material from gold to non-dispersive silica and back to gold, and evaluate the accuracy using the exact solutions.

cond-mat.mes-hall↗

arXiv2015

Resonant-state expansion for a simple dispersive medium

The resonant-state expansion (RSE), a rigorous perturbative method developed in electrodynamics for non-dispersive optical systems is applied to media with an Ohm's law dispersion, in which the frequency dependent part of the permittivity scales inversely with the frequency, corresponding to a frequency-independent conductivity. This dispersion has only a single pole at zero frequency, which is already present in the non-dispersive RSE, allowing to maintain not only the linearity of the eigenvalue problem of the RSE but also its size. Media which can be described by this dispersion over the relevant frequency range, such as optical glass or doped semiconductors, can be treated in the RSE without additional complexity. Results are presented using analytically solvable homogeneous spheres, for doped silicon and BK7 glass, both for a perturbation of the system going from non-dispersive to dispersive media and the reverse, from dispersive to non-dispersive media.

physics.optics↗