arXiv subjects

W. N. Catford

Publications and source records attributed to W. N. Catford.

At least 37 records · Page 2Linked to original sources

arXiv2019

Single-Particle Structure of Neutron-Rich Sr Isotopes Via d( 94,95,96 Sr, p) Reactions

The region around neutron number N = 60 in the neutron-rich Sr and Zr nuclei is one of the most dramatic examples of a ground state shape transition from (near) spherical below N = 60 to strongly deformed shapes in the heavier isotopes. The single-particle structure of 95-97Sr approaching the ground state shape transition at 98 Sr has been investigated via single-neutron transfer reactions using the (d, p) reaction in inverse kinematics. These reactions selectively populate states with a large overlap of the projectile ground state coupled to a neutron in a single-particle orbital. Radioactive 94,95,96Sr nuclei with energies of 5.5 AMeV were used to bombard a CD 2 target. Recoiling light charged particles and γ rays were detected using a quasi-4π silicon strip detector array and a 12 element Ge array. The excitation energy of states populated was reconstructed employing the missing mass method combined with γ-ray tagging and differential cross sections for final states were extracted. A reaction model analysis of the angular distributions allowed for firm spin assignments to be made for the low-lying 352, 556 and 681 keV excited states in 95Sr and a constraint has been placed on the spin of the higher-lying 1666 keV state. Angular distributions have been extracted for 10 states populated in the d(95Sr,p)96Sr reaction, and constraints have been provided for the spins and parities of several final states. Results are compared to shell model calculations in several model spaces and the structure of low-lying states in 94Sr and 95Sr is well-described. The spectroscopic strength of the 0+ and 2 states in 96Sr is significantly more fragmented than predicted.

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arXiv2019

Shell evolution approaching the N=20 island of inversion: Structure of 29Mg

The "Island of Inversion" for neutron-rich nuclei in the vicinity of N=20 has become the testing ground par excellence for our understanding and modelling of shell evolution with isospin. In this context, the structure of the transitional nucleus 29Mg is critical. The first quantitative measurements of the single particle structure of 29Mg are reported, using data from the d(28Mg,p gamma)29Mg reaction. Two key states carrying significant ell=3 (f-wave) strength were identified at 2.40 +/- 0.10 (Jpi = 5/2-) and 4.28 +/- 0.04 MeV (7/2-). New state-of-the-art shell model calculations have been performed and the predictions are compared in detail with the experimental results. Whilst the two lowest 7/2- levels are well described, the sharing of single-particle strength disagrees with experiment for both the 3/2- and 5/2- levels and there appear to be general problems with configurations involving the p3/2 neutron orbital and core-excited components. These conclusions are supported by an analysis of the neutron occupancies in the shell model calculations.

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arXiv2019

Chronology of the three-body dissociation of $^8$He

The space and time configurations of the dissociation of $^8$He into $^6$He+$n$+$n$, on C and Pb targets, have been explored simultaneously for the first time. The final-state interactions in the $n$-$n$ and $^6$He-$n$ channels are successfully described within a model that considers independent emission of neutrons from a Gaussian volume with a given lifetime. The dissociation on C target exhibits a dominant sequential decay through the ground state of $^7$He, consistent with neutrons being emitted from a Gaussian volume of $r_{nn}^{\rm{rms}}=7.3\pm0.6$~fm with a $n$-$n$ delay in the sequential channel of $1400\pm400$~fm/$c$, in agreement with the lifetime of $^7$He. The lower-statistics data on Pb target correspond mainly to direct breakup, and are well described using the $n$-$n$ volume measured, without any $n$-$n$ delay. The validity of the phenomenological model used is discussed.

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arXiv2018

Weakly Bound Neutron-Rich Nuclei and Cosmic Phenomena

The single particle and bulk properties of the neutron-rich nuclei constrain fundamental issues in nuclear physics and nuclear astrophysics like the limits of existence of quantum many body systems (atomic nuclei), the equation of state of neutron-rich matter, neutron star, nucleosynthesis, evolution of stars, neutron star merging etc.. The state of the art of Coulomb breakup of the neutron-rich nuclei has been used to explore those properties. Unambiguous information on detailed components of the ground-state wave-function along with quantum numbers of the valence neutron of the nuclei have been obtained from the measurement of threshold strength along with the $γ$-rays spectra of the core following Coulomb breakup. The shape of this threshold strength is a finger-print of the quantum numbers of the nucleon. We investigated the ground-state properties of the neutron-rich Na, Mg, Al nuclei around N $\sim$ 20 using this method at GSI, Darmstadt. Very clear evidence has been observed for melting and merging of long cherished magic shell gaps at N = 20, 28. The evanescent neutron-rich nuclei imprint their existence in stellar explosive scenarios (r-process etc.). Coulomb dissociation (CD) is one of the important indirect measurements of the capture cross-section which may provide valuable input to the model for star evolution process, particularly the r-process. Some valuable bulk properties of the neutron-rich nuclei like the density dependent symmetry energy,neutron skin etc. play a key role in understanding cosmic phenomena and these properties have been studied via electromagnetic excitation. Preliminary results of electromagnetic excitation of the neutron-rich nucleus, $^{32}$Mg are presented.

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arXiv2018

Shape Coexistence and Mixing of Low-Lying $0^+$ States in $^{96}$Sr

The low energy excited $0_{2,3}^+$ states in $^{96}$Sr are amongst the most prominent examples of shape coexistence across the nuclear landscape. In this work, the neutron $[2s_{1/2}]^2$ content of the $0_{1,2,3}^+$ states in $^{96}$Sr was determined by means of the d($^{95}$Sr,p) transfer reaction at the TRIUMF-ISAC2 facility using the SHARC and TIGRESS arrays. Spectroscopic factors of 0.19(3) and 0.22(3) were extracted for the $^{96}$Sr ground and 1229~keV $0^+$ states, respectively, by fitting the experimental angular distributions to DWBA reaction model calculations. A detailed analysis of the $γ$-decay of the isomeric $0_3^+$ state was used to determine a spectroscopic factor of 0.33(13). The experimental results are compared to shell model calculations, which predict negligible spectroscopic strength for the excited $0^+$ states in $^{96}$Sr. The strengths of the excited $0_{2,3}^+$ states were also analyzed within a two-level mixing model and are consistent with a mixing strength of $a^2$=0.40(14) and a difference in intrinsic deformations of $|Δβ|=0.31(3)$. These results suggest coexistence of three different configurations in $^{96}$Sr and strong shape mixing of the two excited $0^+$ states.

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arXiv2018

Strong neutron pairing in core+4n nuclei

The emission of neutron pairs from the neutron-rich $N\!=\!12$ isotones $^{18}$C and $^{20}$O has been studied by high-energy nucleon knockout from $^{19}$N and $^{21}$O secondary beams, populating unbound states of the two isotones up to 15~MeV above their two-neutron emission thresholds. The analysis of triple fragment-$n$-$n$ correlations shows that the decay $^{19}$N$(-1p)^{18}$C$^*\!\rightarrow^{16}$C+$n$+$n$ is clearly dominated by direct pair emission. The two-neutron correlation strength, the largest ever observed, suggests the predominance of a $^{14}$C core surrounded by four valence neutrons arranged in strongly correlated pairs. On the other hand, a significant competition of a sequential branch is found in the decay $^{21}$O$(-1n)^{20}$O$^*\!\rightarrow^{18}$O+$n$+$n$, attributed to its formation through the knockout of a deeply-bound neutron that breaks the $^{16}$O core and reduces the number of pairs.

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arXiv2018

Re-examining the transition into the N=20 island of inversion: structure of $^{30}$Mg

Intermediate energy single-neutron removal from $^{31}$Mg has been employed to investigate the transition into the N=20 island of inversion. Levels up to 5~MeV excitation energy in $^{30}$Mg were populated and spin-parity assignments were inferred from the corresponding longitudinal momentum distributions and $γ$-ray decay scheme. Comparison with eikonal-model calculations also permitted spectroscopic factors to be deduced. Surprisingly, the 0$^{+}_{2}$ level in $^{30}$Mg was found to have a strength much weaker than expected in the conventional picture of a predominantly $2p - 2h$ intruder configuration having a large overlap with the deformed $^{31}$Mg ground state. In addition, negative parity levels were identified for the first time in $^{30}$Mg, one of which is located at low excitation energy. The results are discussed in the light of shell-model calculations employing two newly developed approaches with markedly different descriptions of the structure of $^{30}$Mg. It is concluded that the cross-shell effects in the region of the island of inversion at Z=12 are considerably more complex than previously thought and that $np - nh$ configurations play a major role in the structure of $^{30}$Mg.

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arXiv2018

Direct Measurement of Astrophysically Important Resonances in $^{38}\mathrm{K}(p, γ){}^{39}\mathrm{Ca}$

According to sensitivity studies, the $^{38}\mathrm{K}\left( p, γ\right){}^{39}\mathrm{Ca}$ reaction has a significant influence on $\mathrm{Ar}$, $\mathrm{K}$, and $\mathrm{Ca}$ production in classical novae. In order to constrain the rate of this reaction, we have performed a direct measurement of the strengths of three candidate $\ell = 0$ resonances within the Gamow window, at $386 \pm 10~\mathrm{keV}$, $515 \pm 10~\mathrm{keV}$, and $689 \pm 10~\mathrm{keV}$. The experiment was performed in inverse kinematics using a beam of unstable $^{38}\mathrm{K}$ impinged on a windowless $\mathrm{H}_2$ target. The $^{39}\mathrm{Ca}$ recoils and prompt $γ$ rays from $^{38}\mathrm{K}\left( p, γ\right){}^{39}\mathrm{Ca}$ reactions were detected in coincidence using a recoil mass separator and a BGO array, respectively. For the $689$ keV resonance, we observed a clear recoil-$γ$ coincidence signal and extracted resonance strength and energy values of $120^{+50}_{-30}~\mathrm{(stat.)}^{+20}_{-60}~\mathrm{(sys.)}~\mathrm{meV}$ and $679^{+2}_{-1}~\mathrm{(stat.)} \pm 1~\mathrm{(sys.)}~\mathrm{keV}$, respectively. We also performed a singles analysis, extracting a resonance strength of $120 \pm 20~\mathrm{(stat.)} \pm 15~\mathrm{(sys.)}~\mathrm{meV}$, consistent with the coincidence result. For the $386$ keV and $515$ keV resonances, we extract $90\%$ confidence level upper limits of $2.54$ meV and $18.4$ meV, respectively. We have established a new recommended $^{38}\mathrm{K}(p, γ){}^{39}\mathrm{Ca}$ rate based on experimental information, which reduces overall uncertainties near the peak temperatures of nova burning by a factor of ${\sim} 250$. Using the rate obtained in this work in model calculations of the hottest oxygen-neon novae reduces overall uncertainties on $\mathrm{Ar}$, $\mathrm{K}$, and $\mathrm{Ca}$ synthesis to factors of $15$ or less in all cases.

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arXiv2017

Coulomb breakup of neutron-rich $^{29,30}$Na isotopes near the island of inversion

First results are reported on the ground state configurations of the neutron-rich $^{29,30}$Na isotopes, obtained via Coulomb dissociation (CD) measurements as a method of the direct probe. The invariant mass spectra of those nuclei have been obtained through measurement of the four-momentum of all decay products after Coulomb excitation on a $^{208}Pb$ target at energies of 400-430 MeV/nucleon using FRS-ALADIN-LAND setup at GSI, Darmstadt. Integrated Coulomb-dissociation cross-sections (CD) of 89 $(7)$ mb and 167 $(13)$ mb up to excitation energy of 10 MeV for one neutron removal from $^{29}$Na and $^{30}$Na respectively, have been extracted. The major part of one neutron removal, CD cross-sections of those nuclei populate core, in its' ground state. A comparison with the direct breakup model, suggests the predominant occupation of the valence neutron in the ground state of $^{29}$Na${(3/2^+)}$ and $^{30}$Na${(2^+)}$ is the $d$ orbital with small contribution in the $s$-orbital which are coupled with ground state of the core. The ground state configurations of these nuclei are as $^{28}$Na$_{gs (1^+)\otimesν_{s,d}$ and $^{29}$Na$_{gs}(3/2^+)\otimesν_{ s,d}$, respectively. The ground state spin and parity of these nuclei, obtained from this experiment are in agreement with earlier reported values. The spectroscopic factors for the valence neutron occupying the $s$ and $d$ orbitals for these nuclei in the ground state have been extracted and reported for the first time. A comparison of the experimental findings with the shell model calculation using MCSM suggests a lower limit of around 4.3 MeV of the sd-pf shell gap in $^{30}$Na.

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arXiv2016

Shell evolution approaching the N=20 island of inversion: structure of 26Na

The levels in 26Na with single particle character have been observed for the first time using the d(25Na,p gamma) reaction at 5 MeV/nucleon. The measured excitation energies and the deduced spectroscopic factors are in good overall agreement with (0+1) hbar-omega shell model calculations performed in a complete spsdfp basis and incorporating a reduction in the N=20 gap. Notably, the 1p3/2 neutron configuration was found to play an enhanced role in the structure of the low-lying negative parity states in 26Na, compared to the isotone 28Al. Thus, the lowering of the 1p3/2 orbital relative to the 0f7/2 occurring in the neighbouring Z=10 and 12 nuclei -- 25,27Ne and 27,29Mg -- is seen also to occur at Z=11 and further strengthens the constraints on the modelling of the transition into the island of inversion.

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arXiv2014

Structure of $^{13}$Be probed via secondary beam reactions

The low-lying level structure of the unbound neutron-rich nucleus $^{13}$Be has been investigated via breakup on a carbon target of secondary beams of $^{14,15}$B at 35 MeV/nucleon. The coincident detection of the beam velocity $^{12}$Be fragments and neutrons permitted the invariant mass of the $^{12}$Be+$n$ and $^{12}$Be+$n$+$n$ systems to be reconstructed. In the case of the breakup of $^{15}$B, a very narrow structure at threshold was observed in the $^{12}$Be+$n$ channel. Contrary to earlier stable beam fragmentation studies which identified this as a strongly interacting $s$-wave virtual state in $^{13}$Be, analysis here of the $^{12}$Be+$n$+$n$ events demonstrated that this was an artifact resulting from the sequential-decay of the $^{14}$Be(2$^+$) state. Single-proton removal from $^{14}$B was found to populate a broad low-lying structure some 0.70 MeV above the neutron-decay threshold in addition to a less prominent feature at around 2.4 MeV. Based on the selectivity of the reaction and a comparison with (0-3)$\hbarω$ shell-model calculations, the low-lying structure is concluded to most probably arise from closely spaced J$^π$=1/2$^+$ and 5/2$^+$ resonances (E$_r$=0.40$\pm$0.03 and 0.85$^{+0.15}_{-0.11}$ MeV), whilst the broad higher-lying feature is a second 5/2$^+$ level (E$_r$=2.35$\pm$0.14 MeV). Taken in conjunction with earlier studies, it would appear that the lowest 1/2$^+$ and 1/2$^-$ levels lie relatively close together below 1 MeV.

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arXiv2013

Two-neutron transfer reaction mechanisms in $^{12}$C($^6$He,$^{4}$He)$^{14}$C using a realistic three-body $^{6}$He model

The reaction mechanisms of the two-neutron transfer reaction $^{12}$C($^6$He,$^4$He) have been studied at 30 MeV at the TRIUMF ISAC-II facility using the SHARC charged-particle detector array. Optical potential parameters have been extracted from the analysis of the elastic scattering angular distribution. The new potential has been applied to the study of the transfer angular distribution to the 2$^+_2$ 8.32 MeV state in $^{14}$C, using a realistic 3-body $^6$He model and advanced shell model calculations for the carbon structure, allowing to calculate the relative contributions of the simultaneous and sequential two-neutron transfer. The reaction model provides a good description of the 30 MeV data set and shows that the simultaneous process is the dominant transfer mechanism. Sensitivity tests of optical potential parameters show that the final results can be considerably affected by the choice of optical potentials. A reanalysis of data measured previously at 18 MeV however, is not as well described by the same reaction model, suggesting that one needs to include higher order effects in the reaction mechanism.

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arXiv2013

Clustering in Nuclei from N/Z=1 to N/Z=2

The clustering of nucleons in nuclei is a widespread but elusive phenomenon for study. Here, we wish to highlight the variety of theoretical approaches, and demonstrate how they are mutually supportive and complementary. On the experimental side, we describe recent advances in the study of the classic cluster nucleus 24Mg. Also, recent studies of clustering in nuclei approaching the neutron drip line are described. In the region near N/Z=2, both theory and experiment now suggest that multi-centre cluster structure is important, in particular for the very neutron rich beryllium isotopes.

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arXiv2010

Emergence of the N=16 shell gap in 21O

The spectroscopy of 21O has been investigated using a radioactive 20O beam and the (d,p) reaction in inverse kinematics. The ground and first excited states have been determined to be Jpi=5/2+ and Jpi=1/2+ respectively. Two neutron unbound states were observed at excitation energies of 4.76 +- 0.10 and 6.16 +- 0.11. The spectroscopic factor deduced for the lower of these interpreted as a 3/2+ level, reveals a rather pure 0d3/2 single-particle configuration. The large energy difference between the 3/2+ and 1/2+ states is indicative of the emergence of the N=16 magic number. For the higher lying resonance, which has a character consistent with a spin-parity assignment of 3/2+ or 7/2-, a 71% branching ratio to the first 2+ state in 20O has been observed. The results are compared with new shell model calculations.

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arXiv2010

Clusters in Light Nuclei

A great deal of research work has been undertaken in the alpha-clustering study since the pioneering discovery, half a century ago, of 12C+12C molecular resonances. Our knowledge of the field of the physics of nuclear molecules has increased considerably and nuclear clustering remains one of the most fruitful domains of nuclear physics, facing some of the greatest challenges and opportunities in the years ahead. In this work, the occurence of "exotic" shapes in light N=Z alpha-like nuclei is investigated. Various approaches of superdeformed and hyperdeformed bands associated with quasimolecular resonant structures are presented. Results on clustering aspects are also discussed for light neutron-rich Oxygen isotopes.

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arXiv2010

Migration of nuclear shell gaps studied in the d(24Ne,p gamma)25Ne reaction

The transfer of neutrons onto 24Ne has been measured using a reaccelerated radioactive beam of 24Ne to study the (d,p) reaction in inverse kinematics. The unusual raising of the first 3/2+ level in 25Ne and its significance in terms of the migration of the neutron magic number from N=20 to N=16 is put on a firm footing by confirmation of this state's identity. The raised 3/2+ level is observed simultaneously with the intruder negative parity 7/2- and 3/2- levels, providing evidence for the reduction in the N=20 gap. The coincident gamma-ray decays allowed the assignment of spins as well as the transferred orbital angular momentum. The excitation energy of the 3/2+ state shows that the established USD shell model breaks down well within the sd model space and requires a revised treatment of the proton-neutron monopole interaction.

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arXiv2010

TIARA: a large solid angle silicon array for direct reaction studies with radioactive beams

A compact, quasi-4pi position sensitive silicon array, TIARA, designed to study direct reactions induced by radioactive beams in inverse kinematics is described here. The Transfer and Inelastic All-angle Reaction Array (TIARA) consists of 8 resistive charge division detectors forming an octagonal barrel around the target and a set of double-sided silicon-strip annular detectors positioned at each end of the barrel. The detector was coupled to the -ray array EXOGAM and the spectrometer VAMOS at the GANIL Laboratory to demonstrate the potential of such an apparatus with radioactive beams. The 14N(d,p)15N reaction, well known in direct kinematics, has been carried out in inverse kinematics for that purpose. The observation of the 15N ground state and excited states at 7.16 and 7.86 MeV is presented here as well as the comparison of the measured proton angular distributions with DWBA calculations. Transferred l-values are in very good agreement with both theoretical calculations and previous experimental results obtained in direct kinematics.

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arXiv2009

Spectroscopy of Neutron-Rich 168,170Dy: Yrast Band Evolution Close to the NpNn Valence Maximum

The yrast sequence of the neutron-rich dysprosium isotope 168Dy has been studied using multi-nucleon transfer reactions following collisions between a 460-MeV 82Se beam and a 170Er target. The reaction products were identified using the PRISMA magnetic spectrometer and the gamma rays detected using the CLARA HPGe-detector array. The 2+ and 4+ members of the previously measured ground state rotational band of 168Dy have been confirmed and the yrast band extended up to 10+. A tentative candidate for the 4+ to 2+ transition in 170Dy was also identified. The data on these nuclei and on the lighter even-even dysprosium isotopes are interpreted in terms of Total Routhian Surface calculations and the evolution of collectivity in the vicinity of the proton-neutron valence product maximum is discussed.

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