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W. N. Hardy

Publications and source records attributed to W. N. Hardy.

187 records · Page 11Linked to original sources

Oxygen Ordering Superstructures and Structural Phase Diagram of YBa_2Cu_3O_{6+x} Studied by Hard X-ray Diffraction

High energy x-ray diffraction is used to investigate the bulk oxygen ordering properties of YBa_2Cu_3O_{6+x}. Superstructures of Cu-O chains aligned along the b axis and ordered with periodicity ma, along the a axis have been observed. For $x < 0.62$ the only observed superstructure is ortho-II with m=2. At room temperature we find ortho-III (m=3) for $0.72\le x\le 0.82$, ortho-V (m=5) in a mixed state with ortho-II at x=0.62, and ortho-VIII (m=8) at x=0.67. Ortho-II is a 3D ordered structural phase, the remaining ones are essentially 2D. None of the superstructures develops long range ordering. Studies of the ortho-II ordering properties in samples prepared with x=0.5 but by different methods show that finite size domains with internal thermodynamic equilibrium are formed. The crystal perfection as well as the thermal annealing history determine the domain size. The temperature dependence of the observed superstructure ordering is investigated explicitly and a structural phase diagram is presented.

cond-mat.supr-con↗

Microwave Spectroscopy of Thermally Excited Quasiparticles in YBa_2Cu_3O_{6.99}

We present here the microwave surface impedance of a high purity crystal of $YBa_2Cu_3O_{6.99}$ measured at 5 frequencies between 1 and 75 GHz. This data set reveals the main features of the conductivity spectrum of the thermally excited quasiparticles in the superconducting state. Below 20 K there is a regime of extremely long quasiparticle lifetimes, due to both the collapse of inelastic scattering below $T_c$ and the very weak impurity scattering in the high purity $BaZrO_3$-grown crystal used in this study. Above 20 K, the scattering increases dramatically, initially at least as fast as $T^4$.

cond-mat.supr-con↗

Measurements of the Magnetic Field Dependence of Lambda in YBa_2Cu_3O_6.95: Results as a Function of Temperature and Field Orientation

We present measurements of the magnetic field dependence of the penetration depth Lambda(H) for untwinned YBa_2Cu_3O_6.95 for temperatures from 1.2 to 70 K in dc fields up to 42 gauss and directions 0, 45 and 90 degrees with respect to the crystal b-axis. The experiment uses an ac susceptometer with fields applied parallel to the ab-plane of thin platelet samples. The resolution is about 0.15 Angstroms in zero dc field, degrading to 0.2 or 0.3 Angstroms at the higher fields. At low temperatures the field dependencies are essentially linear in H, ranging from 0.04 Angstroms/gauss for Delta-Lambda_a to 0.10 Angstroms/gauss for Delta-Lambda_b, values comparable to the T=0 Yip and Sauls prediction for a d-wave superconductor. However, the systematics versus temperature and orientation do not agree with the d-wave scenario probably due, in part, to residual sample problems.

cond-mat.supr-con↗

Magnetic Penetration Depth and Surface Resistance in YBa_2Cu_3O_{7-delta}: New Results for Ultra High Purity Crystals

We have succeeded in growing very high purity (99.995%) YBa_2Cu_3O_{7-delta} crystals in BaZrO_3 crucibles and have measured Delta-lambda(T) and R_s(T) at 1 GHz in crystals with various oxygen treatments. For an oxygen vacancy level of delta=0.007, Delta-lambda and R_s essentially reproduce our previous results and show no sign of the existence of the two order parameter components as recently reported by Srikanth et al. on BaZrO_3-grown crystals. For other oxygen concentrations, we have in some cases observed deviations from the linear low T dependence of Delta-lambda, but never any sign of a second transition.

cond-mat.supr-con↗

c-axis electrodynamics of ybco

New measurements of surface impedance in ybco show that the c-axis penetration depth and conductivity below Tc exhibit behaviour different from that observed in the planes. The c-axis penetration depth never has the linear temperature dependence seen in the ab-plane. Instead of the conductivity peak seen in the planes, the c-axis microwave conductivity falls to low values in the superconducting state, then rises slightly below 20K. These results show that c-axis transport remains incoherent below Tc, even though this is one of the least anisotropic cuprate superconductors.

cond-mat.supr-con↗

Muon spin rotation measurement of the fundamental length scales in the vortex state of YBa2Cu3O6.60

The internal field distribution in the vortex state of YBa2Cu3O6.60 is shown to be a sensitive measure of both the magnetic penetration depth and the vortex-core radius. The temperature dependence of the vortex core radius is found to be weaker than in the conventional superconductor NbSe2 and much weaker than theoretical predictions for an isolated vortex. The effective vortex-core radius decreases sharply with increasing H, whereas the penetration depth is found to be much stronger than in NbSe2.

cond-mat.supr-con↗

Optical properties along the c axis of YBa_2Cu_3O_{6+x}, for x=0.50 -> 0.95: evolution of the pseudogap

The reflectance of high-quality, unpolished single crystals of YBa_2Cu_3O_{6+x}, for the doping range x=0.50 -> 0.95, has been measured with radiation polarized along the c axis from approx 50 cm^{-1} to 5000 cm^{-1} between 10 K and 300 K. In highly doped (x=0.95) material, the normal-state conductivity shows a metallic response. For intermediate dopings (x=0.85 -> 0.90) the conductivity is no longer metallic, increasing with temperature, and for low dopings (x=0.50 -> 0.80) this behavior is clearly seen to be caused by a pseudogap at approx 280 cm^{-1}, which develops well above T_c. In the superconducting state, in the optimally-doped material, a gap-like depression develops below T_c but there is residual conductivity to very low frequency indicating either an anisotropic gap, or a gap with nodes. In the underdoped materials the superconductivity-induced changes to the conductivity are harder to see, but it appears that the weight of the condensate originates at frequencies much higher than the conventional weak-coupling value of 3.5k_BT_c.

cond-mat↗