arXiv subjects

W. N. Hardy

Publications and source records attributed to W. N. Hardy.

At least 127 records · Page 7Linked to original sources

arXiv2009

Magnetic field resonantly enhanced free spins in underdoped YBa$_{2}$Cu$_{3}$O$_{6+x}$

Using neutron scattering, we investigate the effect of a magnetic field on the static and dynamic spin response in heavily underdoped superconducting YBa$_{2}$Cu$_{3}$O$_{6+x}$ (YBCO$_{6+x}$) with x=0.33 (T$_{c}$=8 K) and 0.35 (T$_{c}$=18 K). In contrast to the heavily doped and superconducting monolayer cuprates, the elastic central peak characterizing static spin correlations does not respond observably to a magnetic field which suppresses superconductivity. Instead, we find a magnetic field induced resonant enhancement of the spin fluctuations. The energy scale of the enhanced fluctuations matches the Zeeman energy within both the normal and vortex phases while the momentum dependence is the same as the zero field bilayer response. The magnitude of the enhancement is very similar in both phases with a fractional intensity change of $(I/I_{0}-1) \sim 0.1$. We suggest that the enhancement is not directly correlated with superconductivity but is the result of almost free spins located near hole rich regions.

cond-mat.supr-con↗

arXiv2008

Stability of nodal quasiparticles in underdoped YBa2Cu3O6+y probed by penetration depth and microwave spectroscopy

High resolution measurements of superfluid density and broadband quasiparticle conductivity have been used to probe the low energy excitation spectrum of nodal quasiparticles in underdoped YBCO. Penetration depth is measured to temperatures as low as 0.05 K. Microwave conductivity is measured from 0.1 to 20 GHz and is a direct probe of zero-energy quasiparticles. The data are compared with predictions for a number of theoretical scenarios that compete with or otherwise modify pure d-wave superconductivity, in particular commensurate and incommensurate spin and charge density waves; d + i s and d + i d superconductivity; circulating current phases; and the BCS--BEC crossover. We conclude that the data are consistent with a pure d-wave state in the presence of a small amount of strong scattering disorder, and are able to rule out most candidate competing states either completely, or to a level set by the energy scale of the disorder, ~ 4 K. Commensurate spin and charge density orders, however, are not expected to alter the nodal spectrum and therefore cannot be excluded.

cond-mat.supr-con↗

arXiv2008

Inhomogeneous Magnetic-Field Response of YBa2Cu3Oy and La2-xSrxCuO4 Persisting above the Bulk Superconducting Transition Temperature

We report that in YBa2Cu3Oy and La2-xSrxCuO4 there is a spatially inhomogeneous response to magnetic field for temperatures T extending well above the bulk superconducting transition temperature Tc. An inhomogeneous magnetic response is observed above Tc even in ortho-II YBa2Cu3O6.50, which has highly ordered doping. The degree of the field inhomogeneity above Tc tracks the hole doping dependences of both Tc and the density of the superconducting carriers below Tc, and therefore is apparently coupled to superconductivity.

cond-mat.supr-con↗

arXiv2008

A novel antiproton radial diagnostic based on octupole induced ballistic loss

We report results from a novel diagnostic that probes the outer radial profile of trapped antiproton clouds. The diagnostic allows us to determine the profile by monitoring the time-history of antiproton losses that occur as an octupole field in the antiproton confinement region is increased. We show several examples of how this diagnostic helps us to understand the radial dynamics of antiprotons in normal and nested Penning-Malmberg traps. Better understanding of these dynamics may aid current attempts to trap antihydrogen atoms.

physics.atom-ph↗

arXiv2008

Compression of Antiproton Clouds for Antihydrogen Trapping

Control of the radial profile of trapped antiproton clouds is critical to trapping antihydrogen. We report the first detailed measurements of the radial manipulation of antiproton clouds, including areal density compressions by factors as large as ten, by manipulating spatially overlapped electron plasmas. We show detailed measurements of the near-axis antiproton radial profile and its relation to that of the electron plasma.

nucl-ex↗

arXiv2008

Electron pockets in the Fermi surface of hole-doped high-Tc superconductors

High-temperature superconductivity occurs as copper oxides are chemically tuned to have a carrier concentration intermediate between their metallic state at high doping and their insulating state at zero doping. The underlying evolution of the electron system in the absence of superconductivity is still unclear and a question of central importance is whether it involves any intermediate phase with broken symmetry. The Fermi surface of underdoped YBa2Cu3Oy and YBa2Cu4O8 was recently shown to include small pockets in contrast with the large cylinder characteristic of the overdoped regime1, pointing to a topological change in the Fermi surface. Here we report the observation of a negative Hall resistance in the magnetic field-induced normal state of YBa2Cu3Oy and YBa2Cu4O8, which reveals that these pockets are electron-like. We propose that electron pockets arise most likely from a reconstruction of the Fermi surface caused by the onset of a density-wave phase, as is thought to occur in the electron-doped materials near the onset of antiferromagnetic order Comparison with materials of the La2CuO4 family that exhibit spin/charge density-wave order suggests that a Fermi surface reconstruction also occurs in those materials, pointing to a generic property of high-Tc superconductors.

cond-mat.supr-con↗

arXiv2008

Particle Physics Aspects of Antihydrogen Studies with ALPHA at CERN

We discuss aspects of antihydrogen studies, that relate to particle physics ideas and techniques, within the context of the ALPHA experiment at CERN's Antiproton Decelerator facility. We review the fundamental physics motivations for antihydrogen studies, and their potential physics reach. We argue that initial spectroscopy measurements, once antihydrogen is trapped, could provide competitive tests of CPT, possibly probing physics at the Planck Scale. We discuss some of the particle detection techniques used in ALPHA. Preliminary results from commissioning studies of a partial system of the ALPHA Si vertex detector are presented, the results of which highlight the power of annihilation vertex detection capability in antihydrogen studies.

hep-ex↗

arXiv2008

de Haas-van Alphen oscillations in the underdoped cuprate YBa$_2$Cu$_3$O$_{6.5}$

The de Haas-van Alphen effect was observed in the underdoped cuprate YBa$_2$Cu$_3$O$_{6.5}$ via a torque technique in pulsed magnetic fields up to 59 T. Above an irreversibility field of $\sim$30 T, the magnetization exhibits clear quantum oscillations with a single frequency of 540 T and a cyclotron mass of 1.76 times the free electron mass, in excellent agreement with previously observed Shubnikov-de Haas oscillations. The oscillations obey the standard Lifshitz-Kosevich formula of Fermi-liquid theory. This thermodynamic observation of quantum oscillations confirms the existence of a well-defined, close and coherent, Fermi surface in the pseudogap phase of cuprates.

cond-mat.supr-con↗

arXiv2008

Polar Kerr Effect Measurements of YBa2Cu3O6+x: Evidence for Broken Symmetry Near the Pseudogap Temperature

Polar Kerr effect in the high-Tc superconductor \YBCO was measured at zero magnetic field with high precision using a cyogenic Sagnac fiber interferometer. We observed non-zero Kerr rotations of order $\sim 1 μ$rad appearing near the pseudogap temperature $T^*$, and marking what appears to be a true phase transition. Anomalous magnetic behavior in magnetic-field training of the effect suggests that time reversal symmetry is already broken above room temperature.

cond-mat.supr-con↗

arXiv2008

Raman study of Twin Free YBa$_2$Cu$_3$O$_{6.5}$ (Ortho-II) Single Crystals

The polarized Raman scattering spectra from freshly cleaved $ab$, $ac$, and $bc$ surfaces of high quality twin free YBa$_2$Cu$_3$O$_{6.5}$ (Ortho-II) single crystals ($T_c$=57.5 K and $ΔT = 0.6$ K) were studied between 80 and 300 K. All eleven $A_g$ Raman modes expected for the Ortho-II structure as well some modes of $B_{2g}$ and $B_{3g}$ symmetry were identified in close comparison with predictions of lattice dynamical calculations. The electronic scattering from the $ab$ planes is strongly anisotropic and decreases between 200 and 100 K within the temperature range of previously reported pseudogap opening. The coupling of phonons to Raman active electronic excitations manifested by asymmetric (Fano) profiles of several modes also decreases in the same range. Among the new findings that distinguish the Raman scattering of Ortho-II from that of Ortho-I phase is the unusual relationship ($α_{xx} \approx -α_{yy}$) between the elements of the Raman tensor of the apex oxygen $A_g$ mode.

cond-mat.supr-con↗

arXiv2008

Two-dimensional vortex behavior in highly underdoped YBa_2Cu_3O_{6+x} observed by scanning Hall probe microscopy

We report scanning Hall probe microscopy of highly underdoped superconducting YBa_2Cu_3O_{6+x} with T_c ranging from 5 to 15 K which showed distinct flux bundles with less than one superconducting flux quantum (Phi_0) through the sample surface. The sub-Phi_0 features occurred more frequently for lower T_c, were more mobile than conventional vortices, and occurred more readily when the sample was cooled with an in-plane field component. We show that these features are consistent with kinked stacks of pancake vortices.

cond-mat.supr-con↗

arXiv2008

Spin dynamics near the critical doping in weakly-superconducting underdoped YBa2Cu3O6.35 (Tc=18K)

Using neutron scattering we have determined the magnetic structure and fluctuations in the YBa2Cu3O6.35 superconductor (Tc=18 K). The long-range ordered collinear spins of the insulating antiferromagnet are replaced by a commensurate central mode arising from slow, isotropically polarized, short-range spin correlations. The inelastic spectrum up to 30 meV is broad in wave vector and commensurate. In contrast to the the resonance peak of higher Tc superconductors, the spins exhibit a single overdamped spectrum whose rate of relaxation decreases on cooling and saturates at 5 meV below 50 K. As the relaxation rate saturates the quasi-static spin correlations grow and become resolution limited in energy. The spin susceptibility at high temperatures illustrates that the dominant energy scale is set by the temperature. At low temperatures, the scale length is geometric and not linked by velocity to dynamic widths. There is no observable suppression of the spin fluctuations or central mode upon the onset of superconductivity. The spins respond not to coherent charge pairs but to hole doping allowing coexistence of glassy short range spin order with superconductivity. Since the physics of the weakly superconducting system YBCO6.35 must connect continuously with that in more strongly superconducting YBCO6.5, we find that neither incommensurate stripe-like spin modulations nor a well-defined neutron spin resonance are essential for the onset with doping of pairing in a high temperature cuprate superconductor.

cond-mat.supr-con↗

arXiv2008

Controlling the self-doping of YBa2C3O7-d polar surfaces: From Fermi surface to nodal Fermi arcs by ARPES

The discovery of quantum oscillations in the normal-state electrical resistivity of YBa2Cu3O6.5 provides the first evidence for the existence of Fermi surface (FS) pockets in an underdoped cuprate. However, the pockets' electron vs. hole character, and the very interpretation in terms of closed FS contours, are the subject of considerable debate. Angle-resolved photoemission spectroscopy (ARPES), with its ability to probe electronic dispersion as well as the FS, is ideally suited to address this issue. Unfortunately, the ARPES study of YBa2C3O7-d (YBCO) has been hampered by the technique's surface sensitivity. Here we show that this stems from the polarity and corresponding self-doping of the YBCO surface. By in-situ deposition of potassium atoms on the cleaved surface, we are able to continuously tune the doping of a single sample from the heavily overdoped to the underdoped regime. This reveals the progressive collapse of the normal-metal-like FS into four disconnected nodal FS arcs, or perhaps into hole but not electron pockets, in underdoped YBCO6.5.

cond-mat.supr-con↗

arXiv2008

Quantum oscillations and the Fermi surface in an underdoped high-Tc superconductor

Despite twenty years of research, the phase diagram of high transition- temperature superconductors remains enigmatic. A central issue is the origin of the differences in the physical properties of these copper oxides doped to opposite sides of the superconducting region. In the overdoped regime, the material behaves as a reasonably conventional metal, with a large Fermi surface. The underdoped regime, however, is highly anomalous and appears to have no coherent Fermi surface, but only disconnected "Fermi arcs". The fundamental question, then, is whether underdoped copper oxides have a Fermi surface, and if so, whether it is topologically different from that seen in the overdoped regime. Here we report the observation of quantum oscillations in the electrical resistance of the oxygen-ordered copper oxide YBa2Cu3O6.5, establishing the existence of a well-defined Fermi surface in the ground state of underdoped copper oxides, once superconductivity is suppressed by a magnetic field. The low oscillation frequency reveals a Fermi surface made of small pockets, in contrast to the large cylinder characteristic of the overdoped regime. Two possible interpretations are discussed: either a small pocket is part of the band structure specific to YBa2Cu3O6.5 or small pockets arise from a topological change at a critical point in the phase diagram. Our understanding of high-transition temperature (high-Tc) superconductors will depend critically on which of these two interpretations proves to be correct.

cond-mat.supr-con↗

arXiv2007

Superfluid Density in a Highly Underdoped YBCO Superconductor

The superfluid density rho_s(T) = 1/lambda^2(T) has been measured at 2.64 GHz in highly underdoped YBCO, at 37 dopings with T_c between 3 K and 17 K. Within limits set by the transition width Delta T_c ~ 0.4 K, rho_s(T) shows no evidence of critical fluctuations as T goes to T_c, with a mean-field-like transition and no indication of vortex unbinding. Instead, we propose that rho_s displays the behaviour expected for a quantum phase transition in the (3 + 1)-dimensional XY universality class, with rho_s0 ~ (p - p_c), T_c ~ (p - p_c)^1/2 and rho_s(T) ~ (T_c - T)^1 as T goes to T_c.

cond-mat.supr-con↗

arXiv2007

Spin-glass state of vortices in YBa2Cu3Oy and La2-xSrxCuO4 below the metal-to-insulator crossover

Highly disordered magnetism confined to individual weakly interacting vortices is detected by muon spin rotation in two different families of high-transition-temperature superconductors, but only in samples on the low-doping side of the low-temperature normal state metal-to-insulator crossover (MIC). The results support an extended quantum phase transition (QPT) theory of competing magnetic and superconducting orders that incorporates the coupling between CuO2 planes. Contrary to what has been inferred from previous experiments, the static magnetism that coexists with superconductivity near the field-induced QPT is not ordered. Our findings unravel the mystery of the MIC and establish that the normal state of high-temperature superconductors is ubiquitously governed by a magnetic quantum critical point in the superconducting phase.

cond-mat.supr-con↗

arXiv2007

Hole doping dependences of the magnetic penetration depth and vortex core size in YBa2Cu3Oy: Evidence for stripe correlations near 1/8 hole doping

We report on muon spin rotation measurements of the internal magnetic field distribution n(B) in the vortex solid phase of YBa2Cu3Oy (YBCO) single crystals, from which we have simultaneously determined the hole doping dependences of the in-plane Ginzburg-Landau (GL) length scales in the underdoped regime. We find that Tc has a sublinear dependence on 1/lambda_{ab}^2, where lambda_{ab} is the in-plane magnetic penetration depth in the extrapolated limits T -> 0 and H -> 0. The power coefficient of the sublinear dependence is close to that determined in severely underdoped YBCO thin films, indicating that the same relationship between Tc and the superfluid density is maintained throughout the underdoped regime. The in-plane GL coherence length (vortex core size) is found to increase with decreasing hole doping concentration, and exhibit a field dependence that is explained by proximity-induced superconductivity on the CuO chains. Both the magnetic penetration depth and the vortex core size are enhanced near 1/8 hole doping, supporting the belief by some that stripe correlations are a universal property of high-Tc cuprates.

cond-mat.supr-con↗

arXiv2007

Antiferromagnetic correlations near the lower edge of superconducting dome in YBCO6+x

Neutron scattering from high-quality YBCO6.334 single crystals with a T$_c$ of 8.4 K shows that there is no coexistence with long-range antiferromagnetic order at this very low, near-critical doping of $\sim$0.055, in contrast to claims based on local probe techniques. We find that the neutron resonance seen in optimally doped YBCO7 and underdoped YBCO6.5, has undergone large softening and damping. It appears that the overdamped resonance, with a relaxation rate of 2 meV, is coupled to a zero-energy central mode that grows with cooling and eventually saturates with no change at or below T$_c$. Although a similar qualitative behaviour is found for YBCO6.35, our study shows that the central mode is stronger in YBCO6.334 than YBCO6.35. The system remains subcritical with short-ranged three dimensional correlations.

cond-mat.supr-con↗