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W. Tong

Publications and source records attributed to W. Tong.

21 records · Page 2Linked to original sources

Superconductivity at 44 K in K intercalated FeSe system with excess Fe

We report here that a new superconducting phase with much higher Tc has been found in K intercalated FeSe compound with excess Fe. We successfully grew crystals by precisely controlling the starting amount of Fe. Besides the superconducting (SC) transition at ~30 K, we observed a sharp drop in resistivity and a kink in susceptibility at 44 K. By combining thermodynamic measurements with electron spin resonance (ESR), we demonstrate that this is a new SC transition. Structural analysis unambiguously reveals two phases coexisting in the crystals, which are responsible respectively for the SC transitions at 30 and 44 K. The structural experiments and first-principles calculations consistently indicate that the 44 K SC phase is close to a 122 structure, but with an unexpectedly large c-axis of 18.10 Å. We further find a novel monotonic dependence of the maximum Tc on the separation of neighbouring FeSe layers.

cond-mat.supr-con↗

Coexistence of superconductivity and magnetism in K0.8Fe2Se1.4S0.4

High-quality single crystals of K0.8Fe2Se1.4S0.4 are successfully synthesized by self-flux method with the superconducting transition temperatures Tconset = 32.8 K and Tczero = 31.2 K. In contrast to external pressure effect on superconductivity, the substitution of S for Se does not suppress Tc, which suggests that chemical doping may mainly modulate the anion height from Fe-layer rather than compressing interlayer distance. The investigation of the micromagnetism by electron spin resonance shows clear evidence for strong spin fluctuation at temperatures above Tc. Accompanied by the superconducting feature spectra, a novel resonance signal develops gradually upon cooling below Tc, indicating the coexistence of superconductivity and magnetism in K0.8Fe2Se1.4S0.4 crystal.

cond-mat.supr-con↗

Optical Metamaterials at Near and Mid IR Range Fabricated by Nanoimprint Lithography

Two types of optical metamaterials operating at near-IR and mid-IR frequencies, respectively, have been designed, fabricated by nanoimprint lithography (NIL), and characterized by laser spectroscopic ellipsometry. The structure for the near-IR range was a metal/dielectric/metal stack "fishnet" structure that demonstrated negative permittivity and permeability in the same frequency region and hence exhibited a negative refractive index at a wavelength near 1.7 um. In the mid-IR range, the metamaterial was an ordered array of four-fold symmetric L-shaped resonators (LSRs) that showed both a dipole plasmon resonance resulting in negative permittivity and a magnetic resonance with negative permeability near wavelengths of 3.7 um and 5.25 um, respectively. The optical properties of both metamaterials are in agreement with theoretical predictions. This work demonstrates the feasibility of designing various optical negative-index metamaterials and fabricating them using the nanoimprint lithography as a low-cost, high-throughput fabrication approach.

cond-mat.mtrl-sci↗