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Wai Ting Tai

Publications and source records attributed to Wai Ting Tai.

4 recordsLinked to original sources

Quantum-Geometric Raman Response in Multiorbital Flat-Band Systems

Flat-band materials host rich collective phenomena, yet a complete theory of their signatures in inelastic light scattering remains lacking. While naive theories of interacting flat bands would predict that Raman scattering vertices vanish identically in the limit of vanishing dispersion, we show that this picture is incomplete upon including the multiorbital character of such systems. We show that virtual interband processes generate a finite subgap Raman vertex controlled by the quantum geometric tensor even in the strict flat-band limit. We develop a systematic perturbative theory for Raman scattering from flat bands in the limit where the photon energy is far from resonance with interband transitions. Treating interband Coulomb scattering and light-matter coupling on equal footing, we decompose the Raman scattering vertices into an interaction-independent geometric term expressible directly in terms of the quantum geometric tensor, together with effective resonant and non-resonant pieces generated by virtual interband Coulomb scattering. We then study the polarization-resolved Raman response from collective excitations of an interacting flat band with nontrivial quantum geometry, and demonstrate quantitative agreement of our framework with a full multi-orbital calculation at large photon detuning from interband transitions. These results establish quantum geometry as an intrinsic contribution to inelastic light scattering in flat-band systems, and suggest polarization-resolved Raman spectroscopy as a quantum geometry-sensitive probe of the collective excitations of correlated flat-band platforms.

cond-mat.str-el

Quantum-Geometric Light-Matter Coupling in Correlated Quantum Materials

Irradiation with light provides a powerful tool to interrogate, control or induce new quantum states of matter out of equilibrium, however a microscopic understanding of light-matter coupling in interacting electron systems remains a profound challenge. Here, we show that light grants a new quantum-geometric handle to steer and probe correlated quantum materials, whereby photons can couple directly to the shape and center of the maximally-localized Wannier functions that comprise the material's interacting bands, dressing both electronic motion and electronic interactions with light. Notably, this effect is generic to any material and purely geometric in origin, but dominates emergent optical responses in correlated electron systems with poorly localized or obstructed Wannier functions. Spectroscopic consequences are first illustrated for a paradigmatic strongly interacting model with a tunable Wannier obstruction. We then present ramifications for non-equilibrium control of moiré heterostructures and find that subjecting magic-angle twisted bilayer graphene to weak THz radiation can conspire with a fragile topological obstruction to profoundly alter the material's competing interactions and tune across boundaries to competing phases.

cond-mat.str-el

Proximity-induced quasi-one-dimensional superconducting quantum anomalous Hall state: a promising scalable top-down approach towards localized Majorana modes

In this work, ~100 nm wide quantum anomalous Hall insulator (QAHI) nanoribbons are etched from a two-dimensional QAHI film. One part of the nanoribbon is covered with superconducting Nb, while the other part is connected to an Au lead via two-dimensional QAHI regions. Andreev reflection spectroscopy measurements were performed, and multiple in-gap conductance peaks were observed in three different devices. In the presence of an increasing magnetic field perpendicular to the QAHI film, the multiple in-gap peak structure evolves into a single zero-bias conductance peak (ZBCP). Theoretical simulations suggest that the measurements are consistent with the scenario that the increasing magnetic field drives the nanoribbons from a multi-channel occupied regime to a single channel occupied regime, and that the ZBCP may be induced by zero energy Majorana modes as previously predicted [24]. Although further experiments are needed to clarify the nature of the ZBCP, we provide initial evidence that quasi-1D QAHI nanoribbon/superconductor heterostructures are new and promising platforms for realizing zero-energy Majorana modes.

cond-mat.supr-con

Interfacial superconductivity and zero bias peak in quasi-one-dimensional Bi2Te3/Fe1+yTe heterostructure nanostructures

Bi2Te3/Fe1+yTe heterostructures are known to exhibit interfacial superconductivity between two non-superconducting materials: Fe1+yTe as the parent compound of Fe-based superconducting materials and the topological insulator Bi2Te3. Here, we present a top-down approach starting from two-dimensional (2D) heterostructures to fabricate one-dimensional (1D) Bi2Te3/Fe1+yTe nanowires or narrow nanoribbons. We demonstrate that the Bi2Te3/Fe1+yTe heterostructure remains intact in nanostructures of widths on the order of 100 nm and the interfacial superconductivity is preserved, as evidenced by electrical transport and Andreev reflection point contact spectroscopy experiments measured at the end of the nanowire. The differential conductance shows a similar superconducting twin-gap structure as in two-dimensional heterostructures, but with enhanced fluctuation effects due to the lower dimensionality. A zero-bias conductance peak indicates the presence of an Andreev bound state and given the involvement of the topological Bi2Te3 surface state, we discuss a possible topological nature of superconductivity with strong interplay with an emerging ferromagnetism due to the interstitial excess iron in the Fe1+yTe layer, developing in parallel with superconductivity at low temperatures.

cond-mat.supr-con