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Wai-Kwong Kwok

Publications and source records attributed to Wai-Kwong Kwok.

At least 37 records · Page 2Linked to original sources

Non-Ohmic negative longitudinal magnetoresistance in two-dimensional electron gas

Negative longitudinal magnetoresistance (NLMR) has been reported in a variety of materials and has attracted extensive attention as an electrotransport hallmark of topological Weyl semimetals. However, its origin is still under debate. Here, we demonstrate that the NLMR in a two dimensional electron gas can be influenced by the measurement current. While the NLMR persists up to 130 K, its magnitude and magnetic field response become dependent on the applied current below 60 K. The tunable NLMR at low and high currents can be best attributed to quantum interference and disorder scattering effects, respectively. This work uncovers non-Ohmic NLMR in a non-Weyl material and highlights potential effects of the measurement current in elucidating electrotransport phenomena. We also demonstrate that NLMRs can be a valuable phenomenon in revealing the origins of other properties, such as negative MRs in perpendicular magnetic fields.

cond-mat.mtrl-sci↗

Reconfigurable pinwheel artificial-spin-ice and superconductor hybrid device

The ability to control the potential landscape in a medium of interacting particles could lead to intriguing collective behavior and innovative functionalities. Here, we utilize spatially reconfigurable magnetic potentials of a pinwheel artificial spin ice structure to tailor the motion of superconducting vortices. The reconstituted chain structures of the magnetic charges in the artificial pinwheel spin ice and the strong interaction between magnetic charges and superconducting vortices allow significant modification of the transport properties of the underlying superconducting thin film, resulting in a reprogrammable resistance state that enables a reversible and switchable vortex Hall effect. Our results highlight an effective and simple method of using artificial spin ice as an in-situ reconfigurable nanoscale energy landscape to design reprogrammable superconducting electronics, which could also be applied to the in-situ control of properties and functionalities in other magnetic particle systems, such as magnetic skyrmions.

cond-mat.supr-con↗

Switchable X-ray Orbital Angular Momentum from an Artificial Spin Ice

Artificial spin ices (ASI) have been widely investigated as magnetic metamaterials with exotic properties governed by their geometries. In parallel, interest in X-ray photon orbital angular momentum (OAM) has been rapidly growing. Here we show that a square ASI with a programmed topological defect, a double edge dislocation, imparts OAM to scattered X-rays. Unlike single dislocations, a double dislocation does not introduce magnetic frustration, and the ASI equilibrates to its antiferromagnetic (AF) ground state. The topological charge of the defect differs with respect to the structural and magnetic order; thus, X-ray diffraction from the ASI produces photons with even and odd OAM quantum numbers at the structural and AF Bragg conditions, respectively. The magnetic transitions of the ASI allow the AF OAM beams to be switched on and off by modest variations of temperature and applied magnetic field. These results demonstrate ASIs can serve as metasurfaces for reconfigurable X-ray optics that could enable selective probes of electronic and magnetic properties.

cond-mat.mes-hall↗

Charge density wave and superconductivity competition in Lu$_5$Ir$_4$Si$_{10}$ : a proton irradiation study

Real-space modulated Charge Density Waves (CDW) are an ubiquituous feature in many families of superconductors. In particular, how CDW relates to superconductivity is an active and open question that has recently gathered much interest since CDWs have been discovered in many cuprates superconductors. Here we show that disorder induced by proton irradiation is a full-fledged tuning parameter that can bring essential information to answer this question as it affects CDW and superconductivity with different and unequivocal mechanisms. Specifically, in the model CDW superconductor Lu$_5$Ir$_4$Si$_{10}$ that develops a 1D CDW below 77\,K and s-wave superconductivity below 4\,K, we show that disorder enhances the superconducting critical temperature $T_\mathrm{c}$ and $H_\mathrm{c2}$ while it suppresses the CDW. Discussing how disorder affects both superconductivity and the CDW, we make a compelling case that superconductivity and CDW are competing for electronic density of states at the Fermi level in Lu$_5$Ir$_4$Si$_{10}$, and we reconcile the results obtained via the more common tuning parameters of pressure and doping. Owing to its prototypical, 1D, Peierls type CDW and the s-wave, weak-coupling nature of its superconductivity, this irradiation study of Lu$_5$Ir$_4$Si$_{10}$ provides the basis to understand and extend such studies to the more complex cases of density waves and superconductivity coexistence in heavy fermions, Fe-based or cuprates superconductors.

cond-mat.supr-con↗

Hybrid magnonics: physics, circuits and applications for coherent information processing

Hybrid dynamic systems have recently gained interests with respect to both fundamental physics and device applications, particularly with their potential for coherent information processing. In this perspective, we will focus on the recent rapid developments of magnon-based hybrid systems, which seek to combine magnonic excitations with diverse excitations for transformative applications in devices, circuits and information processing. Key to their promising potentials is that magnons are highly tunable excitations and can be easily engineered to couple with various dynamic media and platforms. The capability of reaching strong coupling with many different excitations has positioned magnons well for studying solid-state coherent dynamics and exploiting unique functionality. In addition, with their gigahertz frequency bandwidth and the ease of fabrication and miniaturization, magnonic devices and systems can be conveniently integrated into microwave circuits for mimicking a broad range of device concepts that have been applied in microwave electronics, photonics and quantum information. We will discuss a few potential directions for advancing magnon hybrid systems, including on-chip geometry, novel coherent magnonic functionality, and coherent transduction between different platforms. As future outlook, we will discuss the opportunities and challenges of magnonic hybrid systems for their applications in quantum information and magnonic logic.

cond-mat.mes-hall↗

The quest for high critical current in applied high-temperature superconductors

We present a perspective on a new critical-current-by-design paradigm to tailor and enhance the current-carrying capacity of applied superconductors. Critical current by design is based on large-scale simulations of vortex matter pinning in high-temperature superconductors and has qualitative and quantitative predictive powers to elucidate vortex dynamics under realistic conditions and to propose vortex pinning defects that could enhance the critical current, particularly at high magnetic fields. The simulations are validated with controlled experiments and demonstrate a powerful tool for designing high-performance superconductors for targeted applications.

cond-mat.supr-con↗

Magnetization governed magnetoresistance anisotropy in topological semimetal CeBi

Magnetic topological semimetals, the latest member of topological quantum materials, are attracting extensive attention as they may lead to topologically-driven spintronics. Currently, magnetotransport investigations on these materials are focused on anomalous Hall effect. Here, we report on the magnetoresistance anisotropy of topological semimetal CeBi, which has tunable magnetic structures arising from localized Ce 4f electrons and exhibits both negative and positive magnetoresistances, depending on the temperature. We found that the angle dependence of the negative magnetoresistance, regardless of its large variation with the magnitude of the magnetic field and with temperature, is solely dictated by the field-induced magnetization that is orientated along a primary crystalline axis and flops under the influence of a rotating magnetic field. The results reveal the strong interaction between conduction electrons and magnetization in CeBi. They also indicate that magnetoresistance anisotropy can be used to uncover the magnetic behavior and the correlation between transport phenomena and magnetism in magnetic topological semimetals.

cond-mat.mtrl-sci↗

Nanocalorimetric Evidence for Nematic Superconductivity in the Doped Topological Insulator Sr$_{0.1}$Bi$_{2}$Se$_{3}$

Spontaneous rotational-symmetry breaking in the superconducting state of doped $\mathrm{Bi}_2\mathrm{Se}_3$ has attracted significant attention as an indicator for topological superconductivity. In this paper, high-resolution calorimetry of the single-crystal $\mathrm{Sr}_{0.1}\mathrm{Bi}_2\mathrm{Se}_3$ provides unequivocal evidence of a two-fold rotational symmetry in the superconducting gap by a \emph{bulk thermodynamic} probe, a fingerprint of nematic superconductivity. The extremely small specific heat anomaly resolved with our high-sensitivity technique is consistent with the material's low carrier concentration proving bulk superconductivity. The large basal-plane anisotropy of $H_{c2}$ is attributed to a nematic phase of a two-component topological gap structure $\vecη = (η_{1}, η_{2})$ and caused by a symmetry-breaking energy term $δ(|η_{1}|^{2} - |η_{2}|^{2}) T_{c}$. A quantitative analysis of our data excludes more conventional sources of this two-fold anisotropy and provides the first estimate for the symmetry-breaking strength $δ\approx 0.1$, a value that points to an onset transition of the second order parameter component below 2K.

cond-mat.supr-con↗

Phase transition preceding magnetic long-range order in the double perovskite Ba2NaOsO6

Recent theoretical studies [Chen et al., Phys. Rev. B 82, 174440 (2010), Ishizuka et al., Phys. Rev. B 90, 184422 (2014)] for the magnetic Mott insulator Ba2NaOsO6 have proposed a low-temperature order parameter that breaks lattice rotational symmetry without breaking time reversal symmetry leading to a nematic phase just above magnetic ordering temperature. We present high-resolution calorimetric and magnetization data of the same Ba2NaOsO6 single crystal and show evidence for a weakly field-dependent phase transition occurring at a temperature of Ts ~ 9.5K, above the magnetic ordering temperature of Tc ~ 7.5K. This transition appears as a broadened step in the low-field temperature dependence of the specific heat. The evolution of the phase boundary with applied magnetic field suggests that this phase coincides with the phase of broken local point symmetry seen in high field NMR experiments [Lu et al., Nat.\ Comm. 8 14407 (2017)]. Furthermore, the magnetic field dependence of the specific heat provides clear indications for magnetic correlations persisting at temperatures between Tc and Ts where long-range magnetic order is absent giving support for the existence of the proposed nematic phase.

cond-mat.str-el↗

Orbital-flop Induced Magnetoresistance Anisotropy in Rare Earth Monopnictide CeSb

The charge and spin of the electrons in solids have been extensively exploited in electronic devices and in the development of spintronics. Another attribute of electrons - their orbital nature - is attracting growing interest for understanding exotic phenomena and in creating the next-generation of quantum devices such as orbital qubits. Here, we report on orbital-flop induced magnetoresistance anisotropy in CeSb. In the low temperature high magnetic-field driven ferromagnetic state, a series of additional minima appear in the angle-dependent magnetoresistance. These minima arise from the anisotropic magnetization originating from orbital-flops and from the enhanced electron scattering from magnetic multidomains formed around the first-order orbital-flop transition. The measured magnetization anisotropy can be accounted for with a phenomenological model involving orbital-flops and a spin-valve-like structure is used to demonstrate the viable utilization of orbital-flop phenomenon. Our results showcase a contribution of orbital behavior in the emergence of intriguing phenomena.

cond-mat.mtrl-sci↗

Disorder raises the critical temperature of a cuprate superconductor

With the discovery of charge density waves (CDW) in most members of the cuprate high temperature superconductors, the interplay between superconductivity and CDW has become a key point in the debate on the origin of high temperature superconductivity. Some experiments in cuprates point toward a CDW state competing with superconductivity, but others raise the possibility of a CDW-superconductivity intertwined order, or more elusive pair-density wave (PDW). Here we have used proton irradiation to induce disorder in crystals of La$_{1.875}$Ba$_{0.125}$CuO$_4$ and observed a striking 50% increase of $T_\mathrm{c}$ accompanied by a suppression of the CDW. This is in clear contradiction with the behaviour expected of a d-wave superconductor for which both magnetic and non-magnetic defects should suppress $T_\mathrm{c}$. Our results thus make an unambiguous case for the strong detrimental effect of the CDW on bulk superconductivity in La$_{1.875}$Ba$_{0.125}$CuO$_4$. Using tunnel diode oscillator (TDO) measurements, we find evidence for dynamic layer decoupling in PDW phase. Our results establish irradiation-induced disorder as a particularly relevant tuning parameter for the many families of superconductors with coexisting density waves, which we demonstrate on superconductors such as the dichalcogenides and Lu$_5$Ir$_4$Si$_{10}$.

cond-mat.supr-con↗

Targeted evolution of pinning landscapes for large superconducting critical currents

The ability of type-II superconductors to carry large amounts of current at high magnetic fields is a key requirement for future design innovations in high-field magnets for accelerators and compact fusion reactors and largely depends on the vortex pinning landscape comprised of material defects. The complex interaction of vortices with defects that can be grown chemically, e.g., self-assembled nanoparticles and nanorods, or introduced by post-synthesis particle irradiation precludes a priori prediction of the critical current and can result in highly non-trivial effects on the critical current. Here, we borrow concepts from biological evolution to create a genetic algorithm evolving pinning landscapes to accommodate vortex pinning and determine the best possible configuration of inclusions for two different scenarios: an evolution process starting from a pristine system and one with pre-existing defects to demonstrate the potential for a post-processing approach to enhance critical currents. Furthermore, the presented approach is even more general and can be adapted to address various other targeted material optimization problems.

cond-mat.supr-con↗

Strong magnon-photon coupling in ferromagnet-superconducting resonator thin-film devices

We demonstrate strong magnon-photon coupling of a thin-film permalloy device fabricated on a coplanar superconducting resonator. A coupling strength of 0.152 GHz and a cooperativity of 68 are found for a 30-nm-thick permalloy stripe. The coupling strength is tunable by rotating the biasing magnetic field or changing the volume of permalloy. We also observe an enhancement of magnon-photon coupling in the nonlinear regime of the superconducting resonator, which is mediated by the nucleation of dynamic flux vortices. Our results demonstrate a critical step towards future integrated hybrid systems for quantum magnonics and on-chip coherent information transfer.

cond-mat.mes-hall↗

Negative longitudinal magnetoresistance in GaAs quantum wells

Negative longitudinal magnetoresistances (NLMRs) have been recently observed in a variety of topological materials and often considered to be associated with Weyl fermions that have a defined chirality. Here we report NLMRs in non-Weyl GaAs quantum wells. In the absence of a magnetic field the quantum wells show a transition from semiconducting-like to metallic behaviour with decreasing temperature. We observed pronounced NLMRs up to 9 Tesla at temperatures above the transition and weak NLMRs in low magnetic fields at temperatures close to the transition and below 5 K. The observed NLMRs show various types of magnetic field behaviour resembling those reported in topological materials. We attribute them to microscopic disorder and use a phenomenological three-resistor model to account for their various features. Our results showcase a new contribution of microscopic disorder in the occurrence of novel phenomena. They may stimulate further work on tuning electronic properties via disorder/defect nano-engineering.

cond-mat.mes-hall↗

Chemical stability and superconductivity in Ag-sheathed CaKFe4As4 superconducting tapes

Ag-sheathed CaKFe4As4 superconducting tapes have been fabricated via the ex-situ powder-in-tube method. Thermal and X-ray diffraction analyses suggest that the CaKFe4As4 phase is unstable at high temperatures. It decomposes into the CaAgAs phase which reacts strongly with the silver sheath. We therefore sintered the tape at 500C and obtain a transport critical current density Jc(4.2 K, 0 T)~ 2.7x10^4 A/cm2. The pinning potential derived from magnetoresistance measurements is one order of magnitude lower than that of the (Ba/Sr)1-xKxFe2As2 tapes. Combining with the scanning electron microscopy and magneto-optical imaging results, we suggest that bad connectivity between superconducting grains caused by the low sintering temperature is the main factor responsible for the low Jc. However, this system is still a promising candidate for superconducting wires and tapes if we further optimize the post-annealing process to achieve better grain connectivity.

cond-mat.supr-con↗

Switchable geometric frustration in an artificial-spin-ice-superconductor hetero-system

Geometric frustration emerges when local interaction energies in an ordered lattice structure cannot be simultaneously minimized, resulting in a large number of degenerate states. The numerous degenerate configurations may lead to practical applications in microelectronics, such as data storage, memory and logic. However, it is difficult to achieve extensive degeneracy, especially in a two-dimensional system. Here, we showcase in-situ controllable geometric frustration with massive degeneracy in a two-dimensional flux quantum system. We create this in a superconducting thin film placed underneath a reconfigurable artificial-spin-ice structure. The tunable magnetic charges in the artificial-spin-ice strongly interact with the flux quanta in the superconductor, enabling the switching between frustrated and crystallized flux quanta states. The different states have measurable effects on the superconducting critical current profile, which can be reconfigured by precise selection of the spin ice magnetic state through application of an external magnetic field. We demonstrate the applicability of these effects by realizing a reprogrammable flux quanta diode. The tailoring of the energy landscape of interacting 'particles' using artificial-spin-ices provides a new paradigm for the design of geometric frustration, which allows us to control new functionalities in other material systems, such as magnetic skyrmions, electrons/holes in two-dimensional materials and topological insulators, as well as colloids in soft materials.

cond-mat.mes-hall↗

Glassy Dynamics in a heavy ion irradiated NbSe2 crystal

Fascination with glassy states has persisted since Fisher introduced the vortex-glass as a new thermodynamic phase that is a true superconductor that lacks conventional long-range order. Though Fisher's original model considered point disorder, it was later predicted that columnar defects (CDs) could also induce glassiness -- specifically, a Bose-glass phase. In YBa$_2$Cu$_3$O$_{7-x}$ (YBCO), glassy states can cause distinct behavior in the temperature ($T$) dependent rate of thermally activated vortex motion ($S$). The vortex-glass state produces a plateau in $S(T)$ whereas a Bose-glass can transition into a state hosting vortex excitations called double-kinks that can expand, creating a large peak in $S(T)$. Although glass phases have been well-studied in YBCO, few studies exist of other materials containing CDs that could contribute to distinguishing universal behavior. Here, we report on the effectiveness of CDs tilted ~30$°$ from the c-axis in reducing $S$ in a NbSe$_2$ crystal. The magnetization is 5 times higher and $S$ is minimized when the field is parallel to the defects versus aligned with the c-axis. We see signatures of glassiness in both field orientations, but do not observe a peak in $S(T)$ nor a plateau at values observed in YBCO. We discuss the possibility that competing disorder induces a field-orientation-driven transition from a Bose-glass to an anisotropic glass involving both point and columnar disorder.

cond-mat.supr-con↗

Parallel magnetic field suppresses dissipation in superconducting nanostrips

The motion of Abrikosov vortices in type-II superconductors results in a finite resistance in the presence of an applied electric current. Elimination or reduction of the resistance via immobilization of vortices is the "holy grail" of superconductivity research. Common wisdom dictates that an increase in the magnetic field escalates the loss of energy since the number of vortices increases. Here we show that this is no longer true if the magnetic field and the current are applied parallel to each other.Our experimental studies on the resistive behavior of a superconducting Mo$_{0.79}$Ge$_{0.21}$ nanostrip reveal the emergence of a dissipative state with increasing magnetic field, followed by a pronounced resistance drop, signifying a reentrance to the superconducting state. Large-scale simulations of the 3D time-dependent Ginzburg-Landau model indicate that the intermediate resistive state is due to an unwinding of twisted vortices. When the magnetic field increases, this instability is suppressed due to a better accommodation of the vortex lattice to the pinning configuration. Our findings show that magnetic field and geometrical confinement can suppress the dissipation induced by vortex motion and thus radically improve the performance of superconducting materials.

cond-mat.mes-hall↗