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Walter Hahn

Publications and source records attributed to Walter Hahn.

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Dynamical aspects of steady-state subradiance: Detailed balance and its breakdown

The dynamics of dissipative many-body quantum systems sometimes admit an emergent classical description in terms of a Markov chain even though the corresponding state space contains highly entangled states. In particular, a bad-cavity laser is a paradigm system whose dynamics can be formulated as a Markov chain in a two-dimensional state space spanned by collective angular momentum states. In this article, we investigate the connection between a dissipative phase transition that occurs in the subradiant regime of this system in the large atom number limit, and the properties of the underlying Markov chain. In one of the phases, the Markov chain approaches the detailed-balance condition with increasing atom number $N$ and hence becomes effectively time-reversible. This is caused by a collective atomic emission process that effectively reduces the Markov chain to one dimension. In the other phase, we find the emergence of time-asymmetric probability currents in the two-dimensional state space that signals a breakdown of detailed balance. This is accompanied by a macroscopic internal entropy production rate in the Markov chain that scales extensively with the atom number $N$. An observable consequence of the probability currents is a self-pulsing of the cavity light output in this phase, which can be detected as an anti-correlation dip in the intensity correlation function.

quant-ph

Random layers for quantum optimal control with exponential expressivity

A long-standing problem in quantum optimal control is finding an optimal pulse structure that leads to an efficient exploration of the unitary space with a minimal number of optimization parameters. We solve this problem by constructing parametrized pulse sequences from random-amplitude pulses grouped in layers with one optimization parameter per layer. We show that, when increasing the number of pulses, the resulting random unitaries converge exponentially fast to the uniform Haar-random ensemble, thus providing for an efficient exploration of the unitary space. Grouping the pulses into layers allows for lowering the total number of optimization parameters. We focus on two random-layer (RALLY) methods: In RALLY$_\text{T}$, time durations of the layers are optimized while the pulse amplitudes are randomly chosen beforehand, possibly even from a few discrete values. RALLY$_\text{A}$ optimizes a joint scaling factor of the random pulse amplitudes in each layer. We numerically validate the two methods by applying them to problems of unitary synthesis, ground-state preparation and state transfer in different quantum systems. For all problems considered, both methods approach an information-theoretic lower bound on the number of optimization parameters and outperform other commonly used algorithms. In gradient-free optimization, the RALLY methods are orders of magnitude more accurate with fewer figure-of-merit evaluations. The RALLY methods are promising for advancing quantum machine learning and variational quantum algorithms.

quant-ph

Truncated Variational Hamiltonian Ansatz: efficient quantum circuit design for quantum chemistry and material science

Quantum computing has the potential to revolutionize quantum chemistry and material science by offering solutions to complex problems unattainable with classical computers. However, the development of efficient quantum algorithms that are efficient under noisy conditions remains a major challenge. This paper introduces the truncated Variational Hamiltonian Ansatz (tVHA), a novel circuit design for conducting quantum calculations on Noisy Intermediate-Scale Quantum (NISQ) devices. tVHA provides a promising approach for a broad range of applications by utilizing principles from the adiabatic theorem in solid state physics. Our proposed ansatz significantly reduces the parameter count and can decrease circuit size substantially, with a trade-off in accuracy. Thus, tVHA facilitates easier convergence within the variational quantum eigensolver framework compared to state-of-the-art ans\"atze such as Unitary Coupled Cluster (UCC) and Hardware-Efficient Ansatz (HEA). While this paper concentrates on the practical applications of tVHA in quantum chemistry, demonstrating its suitability for both weakly and strongly correlated systems and its compatibility with active space calculations, its underlying principles suggest a wider applicability extending to the broader field of material science computations on quantum computing platforms.

quant-ph

Variational quantum thermalizers based on weakly-symmetric nonunitary multi-qubit operations

We propose incorporating multi-qubit nonunitary operations in Variational Quantum Thermalizers (VQTs). VQTs are hybrid quantum-classical algorithms that generate the thermal (Gibbs) state of a given Hamiltonian, with applications in quantum algorithms and simulations. However, current algorithms struggle at intermediate temperatures, where the target state is nonpure but exhibits entanglement. We devise multi-qubit nonunitary operations that harness weak symmetries and thereby improve the performance of the algorithm. Utilizing dissipation engineering, we create these nonunitary multi-qubit operations without the need for measurements or additional qubits. To train the ansatz, we develop and benchmark novel methods for entropy estimation of quantum states, expanding the toolbox for quantum state characterization. We demonstrate that our approach can prepare thermal states of paradigmatic spin models at all temperatures. Our work thus creates new opportunities for simulating open quantum many-body systems.

quant-ph

Inverted-circuit zero-noise extrapolation for quantum gate error mitigation

A common approach to deal with gate errors in modern quantum-computing hardware is zero-noise extrapolation. By artificially amplifying errors and extrapolating the expectation values obtained with different error strengths towards the zero-error (zero-noise) limit, the technique aims at rectifying errors in noisy quantum computing systems. For an accurate extrapolation, it is essential to know the exact factors of the noise amplification. In this article, we propose a simple method for estimating the strength of errors occurring in a quantum circuit and demonstrate improved extrapolation results. The method determines the error strength for a circuit by appending to it the inverted circuit and measuring the probability of the initial state. The estimation of error strengths is easy to implement for arbitrary circuits and does not require a previous characterisation of noise properties. We compare this method with the conventional zero-noise extrapolation method and show that the novel method leads to a more accurate calculation of expectation values. Our method proves to be particularly effective on current hardware, showcasing its suitability for near-term quantum computing applications.

quant-ph

Spin coherence in strongly coupled spin baths in quasi-two-dimensional layers

We investigate the spin-coherence decay of NV$^-$-spins interacting with the strongly-coupled bath of nitrogen defects in diamond layers. For thin diamond layers, we demonstrate that the spin-coherence times exceed those of bulk diamond, thus allowing to surpass the limit imposed by high defect concentrations in bulk. We show that the stretched-exponential parameter for the short-time spin-coherence decay is governed by the hyperfine interaction in the bath, thereby constraining random-noise models. We introduce a novel method based on the cluster-correlation expansion applied to strongly-interacting bath partitions. Our results facilitate material development for quantum-technology devices.

quant-ph

Exploring Quantum Synchronization with a Composite Two-Qubit Oscillator

Synchronization has recently been explored deep in the quantum regime with elementary few-level quantum oscillators such as qudits and weakly pumped quantum Van der Pol oscillators. To engineer more complex quantum synchronizing systems, it is practically relevant to study composite oscillators built up from basic quantum units that are commonly available and offer high controllability. Here, we consider a minimal model for a composite oscillator consisting of two interacting qubits coupled to separate baths, and show that this system exhibits a wide variety of synchronizing behaviors. We study the phase response of the constituent qubits as well as the system as a whole, when one of the qubits is weakly driven. We consider the thermal baths to have positive as well as effective negative temperatures, and discover effects that occur only when the temperatures of the baths for the two qubits are of opposite signs. We propose and analyze a circuit quantum electrodynamics implementation of this model, which exploits recent advances in dissipation engineering to realize effective negative temperature baths. Our work demonstrates the potential for assembling complex quantum synchronizing systems from basic building units, which is of pragmatic importance for advancing the field of quantum synchronization.

quant-ph

Fluorescence calorimetry of an ion crystal

Motivated by the challenge of identifying intruder ions in a cold ion crystal, we investigate calorimetry from emitted fluorescence light. Under continuous Doppler cooling, the ion crystal reaches a temperature equilibrium with a fixed level of fluorescence intensity and any change in the motional energy of the crystal results in a modification of this intensity. We theoretically determine the fluorescence rate of an ion crystal as a function of the temperature, assuming that laser light is scattered along a two-level electronic transition, which couples to the crystal's vibrations via the mechanical effects of light. We analyze how the heat dissipated by collisions of an incoming intruder ion alters the scattering rate. We argue that an energy change by an incoming $^{229}$Th$^{10+}$ ion can be unambiguously detected within 100 $\mu$s via illuminating a fraction of a 10$^{3}$ ion crystal. This method enables applications including capture and spectroscopy of charged states of thorium isotopes and investigation of highly charged ions.

physics.atom-ph

Long-lived coherence in driven spin systems: from two to infinite spatial dimensions

Long-lived coherences, emerging under periodic pulse driving in the disordered ensembles of strongly interacting spins, offer immense advantages for future quantum technologies, but the physical origin and the key properties of this phenomenon remain poorly understood. We theoretically investigate this effect in ensembles of different dimensionality, and predict existence of the long-lived coherences in two-dimensional and infinite-dimensional (where every spin is coupled to all others) systems, which are of particular importance for quantum sensing and quantum information processing. We explore the transition from two to infinite dimensions, and show that the long-time coherence dynamics in all dimensionalities is qualitatively similar, although the short-time behavior is drastically different, exhibiting dimensionality-dependent singularity. Our study establishes the common physical origin of the long-lived coherences in different dimensionalities, and suggests that this effect is a generic feature of the strongly coupled spin systems with positional disorder. Our results lay out foundation for utilizing the long-lived coherences in a range of application, from quantum sensing with two-dimensional spin ensembles, to quantum information processing with the infinitely-dimensional spin systems in the cavity-QED settings.

quant-ph

Attraction Induced by Mutual Quantum Measurements of Velocity

We define the notion of mutual quantum measurements of two macroscopic objects and investigate the effect of these measurements on the velocities of the objects. We show that multiple mutual quantum measurements can lead to an effective force emerging as a consequence of asymmetric diffusion in the velocity space. We further show that, under a certain set of assumptions involving the measurements of mutual Doppler shifts, the above force can reproduce Newton's law of gravitation. Such a mechanism would explain the equivalence between the gravitational and the inertial masses. For a broader class of measurements, the emergent force can also lead to corrections to Newton's gravitation.

quant-ph

Thermalization in Solid-State NMR Controlled by Quantum Chaos in Spin Bath

We theoretically investigate thermalization and spin diffusion driven by a quantum spin bath for a realistic solid-state NMR experiment. We consider polycrystalline L-alanine, and investigate how the spin polarization spreads among several $^{13}$C nuclear spins, which interact via dipole-dipole coupling with the bath of strongly dipolar-coupled $^1$H nuclear (proton) spins. We do this by using direct numerical simulation of the many-spin time-dependent Schrödinger equation. We find that, although the proton spins located near the carbon sites interact most strongly with the $^{13}$C spins, this interaction alone is not enough to drive spin diffusion and thermalize the $^{13}$C nuclear spins. We demonstrate that the thermalization within the $^{13}$C subsystem is driven by the collective many-body dynamics of the proton spin bath, and specifically, that the onset of thermalization among the $^{13}$C spins is directly related to the onset of chaotic behavior in the proton spin bath. Therefore, thermalization and spin diffusion within the $^{13}$C subsystem is controlled by the proton spins located far from the C sites. In spite of their weak coupling to the $^{13}$C spins, these far-away protons help produce a network of strongly coupled proton spins with collective dynamics, that drives thermalization.

quant-ph

Quantifying Stability of Quantum Statistical Ensembles

We investigate different measures of stability of quantum statistical ensembles with respect to local measurements. We call a quantum statistical ensemble "stable" if a small number of local measurements cannot significantly modify the total-energy distribution representing the ensemble. First, we numerically calculate the evolution of the stability measure introduced in our previous work [Phys. Rev. E 94, 062106 (2016)] for an ensemble representing a mixture of two canonical ensembles with very different temperatures in a periodic chain of interacting spins-1/2. Second, we propose other possible stability measures and discuss their advantages and disadvantages. We also show that, for small system sizes available to numerical simulations of local measurements, finite-size effects are rather pronounced.

quant-ph

Improvement of the Basis for the Solution of the Dirac Equation in Cassini Coordinates

We propose an improvement of the basis for the solution of the stationary two-centre Dirac equation in Cassini coordinates using the finite-basis-set method presented in Ref. [1]. For the calculations in Ref. [1], we constructed the basis for approximating the energy eigenfunctions by using smooth piecewise defined polynomials, called B-splines. In the present article, we report that an analysis of the employed representation of the Dirac matrices shows that the above approximation is not efficient using B-splines only. Therefore, we include basis functions which are defined using functions with step-like behaviour instead of B-splines. Thereby, we achieve a significant increase of accuracy of results as compared to Ref. [1].

physics.atom-ph

Thermalization as an Invisibility Cloak for Fragile Quantum Superpositions

We propose a method for protecting fragile quantum superpositions in many-particle systems from dephasing by external classical noise. We call superpositions "fragile" if dephasing occurs particularly fast, because the noise couples very differently to the superposed states. The method consists of letting a quantum superposition evolve under the internal thermalization dynamics of the system, followed by a time reversal manipulation known as Loschmidt echo. The thermalization dynamics makes the superposed states almost indistinguishable during most of the above procedure. We validate the method by applying it to a cluster of spins-1/2.

quant-ph

Stability of Quantum Statistical Ensembles with Respect to Local Measurements

We introduce a stability criterion for quantum statistical ensembles describing macroscopic systems. An ensemble is called "stable" when a small number of local measurements cannot significantly modify the probability distribution of the total energy of the system. We apply this criterion to lattices of spins-1/2, thereby showing that the canonical ensemble is nearly stable, whereas statistical ensembles with much broader energy distributions are not stable. In the context of the foundations of quantum statistical physics, this result justifies the use of statistical ensembles with narrow energy distributions such as canonical or microcanonical ensembles.

quant-ph

Non-Entangling Channels for Multiple Collisions of Quantum Wave Packets

We consider multiple collisions of quantum wave packets in one dimension. The system under investigation consists of an impenetrable wall and of two hard-core particles with very different masses. The lighter particle bounces between the heavier one and the wall. Both particles are initially represented by narrow Gaussian wave packets. A complete analytical solution of this problem is presented on the basis of a new method. The idea of the method is to decompose the two-particle wave function into a continuous superposition of terms (channels), such that the multiple collisions within each channel do not lead to subsequent entanglement between the two particles. For each channel, the time evolution of the two-particle wave function is completely determined by the motion of the corresponding classical point-like particles; therefore the whole quantum problem is reduced to a classical calculation. The calculation based on the above method reveals the following unexpected result: The entanglement between the two particles first increases with time due to the collisions, but then it begins to decrease, disappearing completely when the light particle becomes too slow to catch up with the heavy one.

quant-ph