SearcharxivSearch

arXiv subjects

Walter Zimmermann

Publications and source records attributed to Walter Zimmermann.

At least 19 recordsLinked to original sources

Impact of the history force on the motion of droplets in shaken liquids

Droplets, solid particles, and gas bubbles in unsteady flows experience the Basset-Boussinesq history force (BBH) in addition to steady viscous drag, added mass, and buoyancy. Although physically relevant, the BBH term is often neglected because its inclusion is analytically and numerically demanding. To assess when this approximation fails, we revisit unsteady Stokes flows around spherical droplets of finite viscosity and derive, from first principles, the velocity fields and hydrodynamic forces, including both the classical rigid-particle limit and the free-slip (zero-viscosity) bubble limit. The resulting expressions also encompass cases with time-dependent bubble radii. We further illustrate how the BBH force arises from transient, diffusion-driven vortex structures around accelerating particles. Applying these results to droplets or particles in horizontally shaken liquids (periodically accelerated flows), we find that in the transition regime between the quasi-steady Stokes limit and the inertia-dominated regime, BBH can lead to a reduction of the droplet deflection amplitude by more than 60\% compared to predictions that neglect memory effects. We also derive a characteristic scaling of the displacement amplitude in the low-frequency limit, providing an unambiguous, experimentally verifiable signature of the BBH. For light particles and gas bubbles, the BBH contribution becomes more significant (relative to the other hydrodynamic forces) compared to that o heavy particles, such as droplets in air.

physics.flu-dyn

Myosin-independent amoeboid cell motility

Mammalian cell polarization and motility are important processes involved in many physiological and pathological phenomena, such as embryonic development, wound healing, and cancer metastasis. The traditional view of mammalian cell motility suggests that molecular motors, adhesion, and cell deformation are all necessary components for mammalian cell movement. However, experiments on immune system cells have shown that the inhibition of molecular motors does not significantly affect cell motility. We present a new theory and simulations demonstrating that actin polymerization alone is sufficient to induce spontaneously cell polarity accompanied by the retrograde flow. These findings provide a new understanding of the fundamental mechanisms of cell movement and at the same time provide a simple mechanism for cell motility in diverse configurations, e.g. on an adherent substrate, in a non-adherent matrix, or in liquids.

cond-mat.soft

Suppression of bacterial rheotaxis in wavy channels

Controlling the swimming behavior of bacteria is crucial, for example, to prevent contamination of ducts and catheters. We show the bacteria modeled by deformable microswimmers can accumulate in flows through straight microchannels either in their center or on previously unknown attractors near the channel walls. We predict a novel resonance effect for semiflexible microswimmers in flows through wavy microchannels. As a result, microswimmers can be deflected in a controlled manner so that they swim in modulated channels distributed over the channel cross-section rather than localized near the wall or the channel center. Thus, depending on the flow amplitude, both upstream orientation of swimmers and their accumulation at the boundaries which can lead to surface rheotaxis are suppressed. Our results suggest new strategies for controlling the behavior of live and synthetic swimmers in microchannels.

cond-mat.soft

On the band-width of stable nonlinear stripe patterns in finite size systems

Nonlinear stripe patterns occur in many different systems, from the small scales of biological cells to geological scales as cloud patterns. They all share the universal property of being stable at different wavenumbers $q$, i.e., they are multistable. The stable wavenumber range of the stripe patterns, which is limited by the Eckhaus- and zigzag instabilities even in finite systems for several boundary conditions, increases with decreasing system size. This enlargement comes about because suppressing degrees of freedom from the two instabilities goes along with the system reduction, and the enlargement depends on the boundary conditions, as we show analytically and numerically with the generic Swift-Hohenberg (SH) model and the universal Newell-Whitehead-Segel equation. We also describe how, in very small system sizes, any periodic pattern that emerges from the basic state is simultaneously stable in certain parameter ranges, which is especially important for Turing pattern in cells. In addition, we explain why below a certain system width stripe pattern behave quasi-one-dimensional in two-dimensional systems. Furthermore, we show with numerical simulations of the SH model in medium-sized rectangular domains how unstable stripe patterns evolve via the zigzag instability differently into stable patterns for different combinations of boundary conditions.

nlin.PS

Oscillatory, non-progressing flows induce directed cell motion

We present a deformation-dependent propulsion phenomenon for soft particles such as cells in microchannels. It is based on a broken time reversal symmetry generated by a fast forward and slow backward motion of a fluid which does not progress on average. In both sections, soft particles deform differently and thus progress relatively to the liquid. We demonstrate this by using Lattice-Boltzmann simulations of ubiquitous red blood cells in microchannels, as well as simulations for capsules and minimal soft tissue models in unbounded Poiseuille flows. The propulsion of the soft particles depends besides the oscillation asymmetry on their size, deformation type and elasticity. This is also demonstrated by analytical calculations for a minimal model. Our findings may stimulate a rethinking of particle sorting methods. For example, healthy and malignant cells often differ in their elasticity. With the proposed method, several cell types with different deformability can be separated simultaneously without labeling or obstacles in a microfluidic device.

cond-mat.soft

Periodic patterns displace active phase separation

In this work we identify and investigate a novel bifurcation in conserved systems. This secondary bifurcation stops active phase separation in its nonlinear regime. It is then either replaced by an extended, system-filling, spatially periodic pattern or, in a complementary parameter region, by a novel hybrid state with spatially alternating homogeneous and periodic states. The transition from phase separation to extended spatially periodic patterns is hysteretic. We show that the resulting patterns are multistable, as they show stability beyond the bifurcation for different wavenumbers belonging to a wavenumber band. The transition from active phase separation to the hybrid states is continuous. Both transition scenarios are systems-spanning phenomena in particle conserving systems. They are predicted with a generic dissipative model introduced in this work. Candidates for specific systems, in which these generic secondary transitions are likely to occur, are, for example, generalized models for motility-induced phase separation in active Brownian particles, models for cell division or chemotactic systems with conserved particle dynamics.

nlin.PS

Deflection of phototactic microswimmers through obstacle arrays

We study the effect of inhomogeneous environments on the swimming direction of the microalgae \textit{Chlamydomonas Reinhardtii} (CR) in the presence of a light stimulus. Positive or negative phototaxis describe the ability of microorganisms to bias their swimming towards or away from a light source. Here we consider microswimmers with negative phototaxis in a microfluidic device with a microfabricated square lattice of pillars as obstacles. We measured a mean deflection of microswimmers that shows an interesting nonlinear dependence on the direction of the guiding light beam with respect to the symmetry axes of the pillar lattice. By simulating a model swimmer in a pillar lattice and analyzing its scattering behavior, we identified the width of the reorientation distribution of swimmers to be also crucial for the nonlinear behavior of the swimmer deflection. On the basis of these results we suggest in addition an analytical model for microswimmers, where the pillar lattice is replaced by an anisotropic scattering medium, that depends only on a scattering rate and the width of the reorientation distribution of swimmers. This flexible and handy model fits the experimental results as well. The presented analysis of the deflection of light guided swimmers through pillar lattice may be used for separating swimmers having different reorientation distributions.

cond-mat.soft

Focusing and splitting of particle streams in microflows via viscosity gradients

Microflows are intensively used for investigating and controlling the dynamics of particles, including soft particles such as biological cells and capsules. A classic result is the tank-treading motion of elliptically deformed soft particles in linear shear flows, which do not migrate across straight stream lines in the bulk. However, soft particles migrate across straight streamlines in Poiseuille flows. In this work we describe a new mechanism of cross-streamline migration of soft particles. If the viscosity varies perpendicular to the stream lines then particles migrate across stream lines towards regions of a lower viscosity, even in linear shear flows. An interplay with the repulsive particle-boundary interaction causes then focusing of particles in linear shear flows with the attractor stream line closer to the wall in the low viscosity region. Viscosity variations perpendicular to the stream lines in Poiseuille flows leads either to a shift of the particle attractor or even to a splitting of particle attractors, which may give rise to interesting applications for particle separation. The location of attracting streamlines depend on the particle properties, like their size and elasticity. The cross-stream migration induced by viscosity variations is explained by analytical considerations, Stokesian dynamics simulations with a generalized Oseen tensor and Lattice-Boltzmann simulations.

cond-mat.soft

Systematic extension of the Cahn-Hilliard model for motility-induced phase separation

We consider a continuum model for motility-induced phase separation (MIPS) of active Brownian particles [J. Chem. Phys. 142, 224149 (2015)]. Using a recently introduced perturbative analysis [Phys. Rev. E 98, 020604(R) (2018)], we show that this continuum model reduces to the classic Cahn-Hilliard (CH) model near the onset of MIPS. This makes MIPS another example of the so-called active phase separation. We further introduce a generalization of the perturbative analysis to the next higher order. This results in a generic higher order extension of the CH model for active phase separation. Our analysis establishes the mathematical link between the basic mean-field MIPS model on the one hand, and the leading order and extended CH models on the other hand. Comparing numerical simulations of the three models, we find that the leading order CH model agrees nearly perfectly with the full continuum model near the onset of MIPS. We also give estimates of the control parameter beyond which the higher order corrections become relevant and compare the extended CH model to recent phenomenological models.

cond-mat.soft

Effective viscosity of a suspension of flagellar beating microswimmers: Three-dimensional modeling

Micro-organisms usually can swim in their liquid environment by flagellar or ciliary beating. In this numerical work, we analyze the influence of flagellar beating on the orbits of a swimming cell in a shear flow. We also calculate the effect of the flagellar beating on the rheology of a dilute suspension of micro-swimmers. A three-dimensional model is proposed for Chlamydomonas Reinhardtii swimming with a breaststroke-like beating of two anterior flagella modeled by two counter-rotating fore beads. The active swimmer model reveals unusual angular orbits in a linear shear flow. Namely, the swimmer sustains orientations transiently across the flow. Such behavior is a result of the interplay between shear flow and swimmer's periodic beating motion of flagella which exert internal torques on the cell body. This peculiar behavior has some significant consequences on the rheological properties of the suspension. We calculate the Einstein's viscosity of the suspension composed of such isolated modeled microswimmers (dilute case) in a shear flow. We use numerical simulations based on a Rotne-Prager like approximation for hydrodynamic interaction between simplified flagella and the cell body. The results show an increased intrinsic viscosity for active swimmer suspensions in comparison to non-active ones as well as a shear thinning behavior in accordance with previous experimental measurements [Phys. Rev. Lett. 104 , 098102 (2010)].

cond-mat.soft

Migration reversal of soft particles in vertical flows

Non-neutrally buoyant soft particles in vertical microflows are investigated. We find, soft particles lighter than the liquid migrate to off-center streamlines in a downward Poiseuille flow (buoyancy-force antiparallel to flow). In contrast, heavy soft particles migrate to the center of the downward (and vanishing) Poiseuille flow. A reversal of the flow direction causes in both cases a reversal of the migration direction, i. e. heavier (lighter) particles migrate away from (to) the center of a parabolic flow profile. Non-neutrally buoyant particles migrate also in a linear shear flow across the parallel streamlines: heavy (light) particles migrate along (antiparallel to) the local shear gradient. This surprising, flow-dependent migration is characterized by simulations and analytical calculations for small particle deformations, confirming our plausible explanation of the effect. This density dependent migration reversal may be useful for separating particles.

cond-mat.soft

Cross-stream transport of asymmetric particles driven by oscillating shear

We study the dynamics of asymmetric, deformable particles in oscillatory, linear shear flow. By simulating the motion of a dumbbell, a ring polymer, and a capsule we show that cross-stream migration occurs for asymmetric elastic particles even in linear shear flow if the shear rate varies in time. The migration is generic as it does not depend on the particle dimension. Importantly, the migration velocity and migration direction are robust to variations of the initial particle orientation, making our proposed scheme suitable for sorting particles with asymmetric material properties.

cond-mat.soft

Pattern orientation in finite domains without boundaries

We investigate the orientation of nonlinear stripe patterns in finite domains. Motivated by recent experiments, we introduce a control parameter drop from supercritical inside a domain to subcritical outside without boundary conditions at the domain border. As a result, stripes align perpendicular to shallow control parameter drops. For steeper drops, non-adiabatic effects lead to a surprising orientational transition to parallel stripes with respect to the borders. We demonstrate this effect in terms of the Brusselator model and generic amplitude equations.

cond-mat.soft

Effects of a temperature dependent viscosity on thermal convection in binary mixtures

We investigate the effect of a temperature dependent viscosity on the onset of thermal convection in a horizontal layer of a binary fluid mixture that is heated from below. For an exponential temperature dependence of the viscosity, we find in binary mixtures as a function of a positive separation ratio and beyond a certain viscosity contrast a discontinuous transition between two stationary convection modes having a different wavelength. In the range of negative values of the separation ratio, a (continuous or discontinuous) transition from an oscillatory to a stationary onset of convection occurs beyond a certain viscosity contrast, and for large values of the viscosity ratio, the oscillatory onset of convection is suppressed.

physics.flu-dyn

Periodic structures in binary mixtures enforced by Janus particles

Phase separation in binary mixtures in the presence of Janus particles has been studied in terms of a Cahn-Hilliard model coupled to the Langevin equations describing the particle dynamics. We demonstrate that the phase separation process is arrested leading to unexpected regular stripe patterns in the concentration field. The underlying pattern forming mechanism has been elucidated: The twofold absorption properties on the surface of Janus particles with respect to the two components of a binary mixture trigger in their neighborhood spatial concentration variations. They result in an effective interaction between the particles mediated by the binary mixture. Our findings open a route to design composite materials with nanoscale lamellar morphologies where the pattern wavelength can be tuned by changing the wetting properties of the Janus particles.

cond-mat.soft

Dumbbells in suspension: A numerical study on their dynamics and shear viscosity

The dynamics of elastic dumbbells in linear shear flow is investigated by fluid particle dynamics simulations at small Reynolds numbers. The positive contribution of a single dumbbell to the effective shear viscosity is determined via the extra stress exerted at the boundaries of the shear cell and the difference to the contributions obtained via the Kramers-Kirkwood formula are described. For a small Weissenberg number and when the mean dumbbell length becomes larger than the mean next-neighbor distance, the contribution of interacting dumbbells to the mean shear viscosity exceeds significantly the contribution of unconnected beads occupying the same volume fraction.

cond-mat.soft

Wall attraction and repulsion of hydrodynamically interacting particles

We investigate hydrodynamic interaction effects between colloidal particles in the vicinity of a wall in the low Reynolds-number limit. Hydrodynamically interacting pairs of beads being dragged by a force parallel to a wall, as for instance during sedimentation, are repelled by the boundary. If a pair of beads is trapped by harmonic potentials parallel to the external flow and at the same distance to a wall, then the particle upstream is repelled from the boundary while its neighbor downstream is attracted. The free end of a semiflexible bead-spring polymer-model, which is fixed at one end in a flow near a wall, is bent towards the wall by the same reason. The results obtained for point-like particles are exemplarily confirmed by fluid particle dynamics simulations for beads of finite radii, where the shear induced particle rotations either weaken or enhance the the effects obtained for point-like particles.

cond-mat.soft

Stability and Orientation of Lamellae in Diblock Copolymer Films

The dynamics of microphase separation and the orientation of lamellae in diblock copolymers is investigated in terms of a mean-field model. The formation of lamellar structures and their stable states are explored and it is shown that lamellae are stable not only for the period of the structure corresponding to the minimum of the free energy. The range of wavelengths of stable lamellae is determined by a functional approach, introduced with this work, which is in agreement with the results of a linear stability analysis. The effects of the interaction of block copolymers with confining plane boundaries on the lamellae orientation are studied by an extensive analysis of the free energy. By changing the surface property at one boundary, a transition from a preferentially perpendicular to a parallel lamellar orientation with respect to the boundaries is found, which is rather independent of the distance between the boundaries. Computer simulations reveal, that the time scale of the lamellar orientational order dynamics, which is quantitatively characterized in terms of an orientational order parameter and the structure factor, depends significantly on the properties of the confining boundaries as well as on the quench depth.

cond-mat.soft