arXiv subjects

Wanyu Chen

Publications and source records attributed to Wanyu Chen.

13 recordsLinked to original sources

arXiv2025

Extreme Strain Controlled Correlated Metal-Insulator Transition in the Altermagnet CrSb

Correlated flat bands and altermagnetism are two important directions in quantum materials, centred respectively on interaction-dominated phases and symmetry-enforced spin-textured states, yet both derive from lattice symmetry and orbital hybridization. This common origin implies that extreme crystal distortion, by narrowing bandwidths, enhancing correlations and reshaping the symmetries of altermagnetic spin splittings, could unify flat-band and altermagnetic physics in a single material; in practice, however, achieving such large distortions in a crystalline altermagnet is a formidable challenge. Here we combine a dedicated strain device with a tailored single-crystal mounting scheme to impose a highly tensile strain gradient in bulk CrSb, a prototypical altermagnet, creating a near-surface layer in which the in-plane lattice is strongly distorted relative to the weakly strained bulk, while the average bulk distortion remains small. Angle-resolved photoemission reveals a reversible regime at moderate strain, where a deeper flat-band feature, attributed to a strain-gradient-driven suppression of Cr-Sb hybridization, coexists with a correlation-enhanced Cr 3d flat band, and an irreversible regime at larger strain where partial bond decoupling drives a predominantly insulating spectral response. Density-functional calculations show that an orbital-selective altermagnetic spin texture persists across this correlated regime despite strong bandwidth renormalisation. These results define a strain-symmetry-correlation map for CrSb and establish extreme tensile strain as a route to co-engineer flat-band tendencies and spin-textured, zero-net-moment correlated states in altermagnets, pointing toward strain-adaptive, spin-selective Mott filtering and related device concepts.

cond-mat.str-el↗

arXiv2025

MLLMRec: A Preference Reasoning Paradigm with Graph Refinement for Multimodal Recommendation

Multimodal recommendation combines the user historical behaviors with the modal features of items to capture the tangible user preferences, presenting superior performance compared to the conventional ID-based recommender systems. However, existing methods still encounter two key problems in the representation learning of users and items, respectively: (1) the initialization of multimodal user representations is either agnostic to historical behaviors or contaminated by irrelevant modal noise, and (2) the widely used KNN-based item-item graph contains noisy edges with low similarities and lacks audience co-occurrence relationships. To address such issues, we propose MLLMRec, a novel preference reasoning paradigm with graph refinement for multimodal recommendation. Specifically, on the one hand, the item images are first converted into high-quality semantic descriptions using a multimodal large language model (MLLM), thereby bridging the semantic gap between visual and textual modalities. Then, we construct a behavioral description list for each user and feed it into the MLLM to reason about the purified user preference profiles that contain the latent interaction intents. The reasoned profiles and the multimodal descriptions of items, together with their ID embeddings, are propagated over the user-item interaction graph to absorb the high-order collaborative signals. On the other hand, we develop the threshold-controlled denoising and topology-aware enhancement strategies to refine the suboptimal item-item graph, which are applied to both the multimodal and ID item representations to improve the accuracy of item representation learning. Extensive experiments on three publicly available datasets demonstrate that MLLMRec achieves the state-of-the-art performance. The source code is provided at https://github.com/Yuzhuo-Dang/MLLMRec.git.

cs.IR↗

arXiv2024

Set-CLIP: Exploring Aligned Semantic From Low-Alignment Multimodal Data Through A Distribution View

Multimodal fusion breaks through the boundaries between diverse modalities and has already achieved notable performances. However, in many specialized fields, it is struggling to obtain sufficient alignment data for training, which seriously limits the use of previously effective models. Therefore, semi-supervised learning approaches are attempted to facilitate multimodal alignment by learning from low-alignment data with fewer matched pairs, but traditional techniques like pseudo-labeling may run into troubles in the label-deficient scenarios. To tackle these challenges, we reframe semi-supervised multimodal alignment as a manifold matching issue and propose a new methodology based on CLIP, termed Set-CLIP. Specifically, by designing a novel semantic density distribution loss, we constrain the latent representation distribution with fine granularity and extract implicit semantic alignment from unpaired multimodal data, thereby reducing the reliance on numerous strictly matched pairs. Furthermore, we apply coarse-grained modality adaptation and unimodal self-supervised guidance to narrow the gaps between modality spaces and improve the stability of representation distributions. Extensive experiments conducted on a range of tasks in various fields, including protein analysis, remote sensing, and the general vision-language field, validate the efficacy of our proposed Set-CLIP method. Especially with no paired data for supervised training, Set-CLIP is still outstanding, which brings an improvement of 144.83% over CLIP.

cs.LG↗

arXiv2024

Non-Hermitian Boundary in a Surface Selective Reconstructed Magnetic Weyl Semimetal

Non-Hermitian physics, studying systems described by non-Hermitian Hamiltonians, reveals unique phenomena not present in Hermitian systems. Unlike Hermitian systems, non-Hermitian systems have complex eigenvalues, making their effects less directly observable. Recently, significant efforts have been devoted to incorporating the non-Hermitian effects into condensed matter physics. However, progress has been hindered by the absence of a viable experimental approach. Here, the discovery of surface-selectively spontaneous reconstructed Weyl semimetal NdAlSi provides a feasible experimental platform for studying non-Hermitian physics. Utilizing angle-resolved photoemission spectroscopy measurements, surface-projected density functional theory calculations, and scanning tunneling microscopy measurements, we demonstrate that surface reconstruction in NdAlSi alters surface Fermi arc connectivity and generates new isolated non-topological surface Fermi arcs. In the presence of a magnetic field, the surface-selective spontaneous reconstructed Weyl semimetal NdAlSi can be viewed as a Hermitian bulk--non-Hermitian boundary system. The isolated non-topological surface Fermi arcs on the reconstructed surface act as a loss mechanism and open boundary condition for the topological electrons and bulk states, serving as non-Hermitian boundary states. This discovery provides a good experimental platform for exploring new physical phenomena and potential applications based on boundary non-Hermitian effects, extending beyond purely mathematical concepts.

cond-mat.mtrl-sci↗

arXiv2024

Disorder Driven Non-Anderson Transition in a Weyl Semimetal

For several decades, it was widely believed that a non-interacting disordered electronic system could only undergo an Anderson metal-insulator transition due to Anderson localization. However, numerous recent theoretical works have predicted the existence of a disorder-driven non-Anderson phase transition that differ from Anderson localization. The frustration lies in the fact that this non-Anderson disorder-driven transition has not yet been experimentally demonstrated in any system. Here, using angle-resolved photoemission spectroscopy, we present a case study of observing the non-Anderson disorder-driven transition by visualizing the electronic structure of the Weyl semimetal NdAlSi on surfaces with varying amounts of disorder. Our observations reveal that strong disorder can effectively suppress all surface states in the Weyl semimetal NdAlSi, including the topological surface Fermi arcs. This disappearance of surface Fermi arcs is associated with the vanishing of the bulk topological invariant, indicating a quantum phase transition from a Weyl semimetal to a diffusive metal. By analyzing the changes in the electronic structure of NdAlSi, as the surface degrades, we provide a physical picture of this non-Anderson transition from a Weyl semimetal to a diffuse metal. These observations provide the first direct experimental evidence of the non-Anderson disorder-driven transition, a discovery long anticipated by theoretical physicists. The finding dispels longstanding suspicions among researchers that non-Anderson transitions exist in real quantum systems.

cond-mat.mtrl-sci↗

arXiv2024

Topological Weyl Altermagnetism in CrSb

Altermagnets constitute a novel, third fundamental class of collinear magnetic ordered materials, alongside with ferro- and antiferromagnets. They share with conventional antiferromagnets the feature of a vanishing net magnetization. At the same time they show a spin-splitting of electronic bands, just as in ferromagnets, caused by the atomic exchange interaction. On the other hand, topology has recently revolutionized our understanding of condensed matter physics, introducing new phases of matter classified by intrinsic topological order. Here we connect the worlds of altermagnetism and topology, showing that the electronic structure of the altermagnet CrSb is topological and hosts a novel Weyl semimetallic state. Using high-resolution and spin angleresolved photoemission spectroscopy, we observe a large momentum-dependent spin-splitting in CrSb, reaching up to 1 eV, that induces altermagnetic Weyl nodes with an associated magnetic quantum number. At the surface we observe their spin-polarized topological Fermi-arcs. This establishes that in altermagnets the large energy scale intrinsic to the spin-splitting - orders of magnitude larger than the relativistic spin-orbit coupling - creates its own realm of robust electronic topology.

cond-mat.mtrl-sci↗

arXiv2023

Ferrimagnetic Regulation of Weyl Fermions in a Noncentrosymmetric Magnetic Weyl Semimetal

The study of interaction between electromagnetism and elementary particles is a long-standing topic in physics. Likewise, the connection between particle physics and emergent phenomena in condensed matter physics is a recurring theme and condensed matter physics has often provided a platform for investigating the interplay between particles and fields in cases that have not been observed in high-energy physics, so far. Here, using angle-resolved photoemission spectroscopy, we provide a new example of this by visualizing the electronic structure of a noncentrosymmetric magnetic Weyl semimetal candidate NdAlSi in both the paramagnetic and ferrimagnetic states. We observe surface Fermi arcs and bulk Weyl fermion dispersion as well as the regulation of Weyl fermions by ferrimagnetism. Our results establish NdAlSi as a magnetic Weyl semimetal and provide the first experimental observation of ferrimagnetic regulation of Weyl fermions in condensed matter.

cond-mat.str-el↗

arXiv2022

An efficient low-density grating setup for monochromatization of XUV ultrafast light sources

Ultrafast light sources have become an indispensable tool to access and understand transient phenomenon in material science. However, a simple and easy-to-implement method for harmonic selection, with high transmission efficiency and pulse duration conservation, is still a challenge. Here we showcase and compare two approaches for selecting the desired harmonic from a high harmonic generation source while achieving the above goals. The first approach is the combination of extreme ultraviolet spherical mirrors with transmission filters and the second approach uses a normal-incidence spherical grating. Both solutions target time- and angle-resolved photoemission spectroscopy with photon energies in the 10-20 eV range but are relevant for other experimental techniques as well. The two approaches for harmonic selection are characterized in terms of focusing quality, efficiency, and temporal broadening. It is demonstrated that a focusing grating is able to provide much higher transmission as compared to the mirror+filter approach (3.3 times higher for 10.8 eV and 12.9 times higher for 18.1 eV), with only a slight temporal broadening (6.8% increase) and a somewhat larger spot size (~30% increase). Overall, our study establishes an experimental perspective on the trade-off between a single grating normal incidence monochromator design and the use of filters. As such, it provides a basis for selecting the most appropriate approach in various fields where an easy-to-implement harmonic selection from high harmonic generation is needed.

physics.optics↗

arXiv2022

A narrow bandwidth extreme ultra-violet light source for time- and angle-resolved photoemission spectroscopy

Here we present a high repetition rate, narrow band-width, extreme ultraviolet (XUV) photon source for time- and angle-resolved photoemission spectroscopy (tr-ARPES). The narrow band width pulses $ΔE=9, 14, 18$ meV for photon energies $hν=10.8, 18.1, 25.3$ eV are generated through High Harmonic Generation (HHG) using ultra-violet (UV) drive pulses with relatively long pulse lengths (461 fs). The HHG setup employs an annuluar drive beam in a tight focusing geometry at a repetition rate of 250 kHz. Photon energy selection is provided by a series of selectable multilayer bandpass mirrors and thin film filters, thus avoiding any time broadening introduced by single grating monochromators. A two stage optical-parametric amplifier provides $< 100$ fs tunable pump pulses from 0.65 $μ$m to 9 $μ$m. The narrow bandwidth performance of the light source is demonstrated through ARPES measurements on a series of quantum materials including the high-temperature superconductor Bi-2212, WSe$_2$ and graphene.

cond-mat.str-el↗

arXiv2020

Attribute-aware Diversification for Sequential Recommendations

Users prefer diverse recommendations over homogeneous ones. However, most previous work on Sequential Recommenders does not consider diversity, and strives for maximum accuracy, resulting in homogeneous recommendations. In this paper, we consider both accuracy and diversity by presenting an Attribute-aware Diversifying Sequential Recommender (ADSR). Specifically, ADSR utilizes available attribute information when modeling a user's sequential behavior to simultaneously learn the user's most likely item to interact with, and their preference of attributes. Then, ADSR diversifies the recommended items based on the predicted preference for certain attributes. Experiments on two benchmark datasets demonstrate that ADSR can effectively provide diverse recommendations while maintaining accuracy.

cs.IR↗

arXiv2019

Improving End-to-End Sequential Recommendations with Intent-aware Diversification

Sequential Recommendation (SRs) that capture users' dynamic intents by modeling user sequential behaviors can recommend closely accurate products to users. Previous work on SRs is mostly focused on optimizing the recommendation accuracy, often ignoring the recommendation diversity, even though it is an important criterion for evaluating the recommendation performance. Most existing methods for improving the diversity of recommendations are not ideally applicable for SRs because they assume that user intents are static and rely on post-processing the list of recommendations to promote diversity. We consider both recommendation accuracy and diversity for SRs by proposing an end-to-end neural model, called Intent-aware Diversified Sequential Recommendation (IDSR). Specifically, we introduce an Implicit Intent Mining module (IIM) into SRs to capture different user intents reflected in user behavior sequences. Then, we design an Intent-aware Diversity Promoting (IDP) loss to supervise the learning of the IIM module and force the model to take recommendation diversity into consideration during training. Extensive experiments on two benchmark datasets show that IDSR significantly outperforms state-of-the-art methods in terms of recommendation diversity while yielding comparable or superior recommendation accuracy.

cs.IR↗

arXiv2019

Joint Neural Collaborative Filtering for Recommender Systems

We propose a J-NCF method for recommender systems. The J-NCF model applies a joint neural network that couples deep feature learning and deep interaction modeling with a rating matrix. Deep feature learning extracts feature representations of users and items with a deep learning architecture based on a user-item rating matrix. Deep interaction modeling captures non-linear user-item interactions with a deep neural network using the feature representations generated by the deep feature learning process as input. J-NCF enables the deep feature learning and deep interaction modeling processes to optimize each other through joint training, which leads to improved recommendation performance. In addition, we design a new loss function for optimization, which takes both implicit and explicit feedback, point-wise and pair-wise loss into account. Experiments on several real-word datasets show significant improvements of J-NCF over state-of-the-art methods, with improvements of up to 8.24% on the MovieLens 100K dataset, 10.81% on the MovieLens 1M dataset, and 10.21% on the Amazon Movies dataset in terms of HR@10. NDCG@10 improvements are 12.42%, 14.24% and 15.06%, respectively. We also conduct experiments to evaluate the scalability and sensitivity of J-NCF. Our experiments show that the J-NCF model has a competitive recommendation performance with inactive users and different degrees of data sparsity when compared to state-of-the-art baselines.

cs.IR↗

arXiv2018

Attention-based Hierarchical Neural Query Suggestion

Query suggestions help users of a search engine to refine their queries. Previous work on query suggestion has mainly focused on incorporating directly observable features such as query co-occurrence and semantic similarity. The structure of such features is often set manually, as a result of which hidden dependencies between queries and users may be ignored. We propose an AHNQS model that combines a hierarchical structure with a session-level neural network and a user-level neural network to model the short- and long-term search history of a user. An attention mechanism is used to capture user preferences. We quantify the improvements of AHNQS over state-of-the-art RNN-based query suggestion baselines on the AOL query log dataset, with improvements of up to 21.86% and 22.99% in terms of MRR@10 and Recall@10, respectively, over the state-of-the-art; improvements are especially large for short sessions.

cs.IR↗