arXiv subjects

Wei-Chao Jiang

Publications and source records attributed to Wei-Chao Jiang.

5 recordsLinked to original sources

arXiv2026

Observation of Strong Electron Correlation in Planetary Atomic Structure

Unravelling two-electron correlation is a long-standing challenge at the heart of few-body quantum physics, underlying correlated phenomena across atomic, molecular and condensed-matter science. In prototypical three-body Coulomb systems, such strong correlation in doubly excited states (DESs) of planetary atomic systems leaves distinct signatures in nonsequential above-threshold double ionization (NS-ATDI) driven by coherent laser fields, yet such targeted study has long remained elusive. Here we present kinematically complete measurements of multi-photon double ionization in cold strontium atoms. Our results reveal a dominant NS-ATDI channel exhibiting well-defined band structures that encode pronounced energy and angular correlations between the two emitted electrons. Autoionization spectra confirm the presence of DESs as transition states that effectively promote the NS-ATDI process. These observations provide direct evidence that both electrons are synchronously excited and ionized via resonant high-lying DES transitions, meaning the structure-linked two-electron correlation of DES is preserved and propagated in the laser-driven time-dependent three-body system. Our work transcends the traditional paradigm of multi-photon double ionization, and fundamentally reshapes the core understanding of intrinsic electron correlation governing many-body systems in nature.

physics.atom-ph↗

arXiv2023

Spin-orientation-resolved attosecond chronoscopy in strong field ionization

Attosecond chronoscopy represents a major breakthrough in the study of ultrafast phenomena and has the potential to revolutionize our understanding of the fundamental physics of matter. We theoretically investigate the spin-orientation-resolved attosecond chronoscopy for the first time by the circular RABBIT technique for Kr atoms. Due to the spin-orbit interaction and the sensitivity of ionization in circularly polarized fields to the sense of electron rotation in the initial state, the spin-resolved ionization rates of photoelectrons emitted from $^2P_{1/2}$ and $^2P_{3/2}$ channels can be expressed via $m$-resolved ionization rates of initial state, where $m$ is the orbital magnetic quantum number. We demonstrate that the yields difference between spin-up and spin-down photoelectrons from each channel are closely associated with the different behaviors of corresponding Wigner time delay. We find that the Wigner time delay between spin-up and spin-down photoelectrons in the polarization plane can reach several tens of attoseconds in the co-rotating geometry, but a few attoseconds in the counter-rotating geometry. Our approach opens up a new avenue for probing the spin-dependent behavior of Wigner time delay, and lays the foundation for spin-orientation-resolved attosecond chronoscopy, which can be verified by the current experimental techniques.

physics.atom-ph↗

arXiv2022

Magnetic-Field effect in Laser-assisted XUV ionization

The magnetic-field effect of the laser pulse is investigated in laser-assisted XUV ionization. By numerically solving the three-dimensional time-dependent Schrödinger equation, we find that the photoelectron momentum distribution is distorted by the magnetic-field effect of the IR streaking field. It results in a transverse-momentum- and time-delay-dependent longitudinal photoelectron momentum shift, which is further analytically confirmed by employing the nondipole corrected strong field approximation. We also demonstrate that the magnetic field does not affect the time shift retrieved from the streaking spectrum, although the streaking spectrum is apparently altered by the momentum shift induced by the magnetic-field effect. Our work reveals the time-resolved nondipole effect of the laser pulse by the attosecond streaking technique.

physics.atom-ph↗

arXiv2018

Nondipole effects in atomic dynamic interference

Nondipole effects in the atomic dynamic interference are investigated by numerically solving the time-dependent Schrödinger equation~(TDSE) of hydrogen. It is found that the inclusion of nondipole corrections in the TDSE can induce momentum shifts of photoelectrons in the opposite direction of the laser propagation. The magnitude of the momentum shift is roughly proportional to the laser peak intensity and to the momentum component of the photoelectron along the laser propagation. By including the nondipole corrections of the Volkov phase into a semi-analytical model previously developed under the dipole approximation, all the main features of the momentum shifts can be nicely reproduced. Through an analytic expression, the origin of such momentum shifts is attributed to the nondipole phase difference between the two electron wave packets ejected in the rising edge and the falling edge, which will interfere with each other and result in the final fringe pattern. One important consequence of such momentum shifts is that they can smooth out the peak splitting induced by the dynamic interference in the photoelectron energy spectrum. Nevertheless, it should be emphasized that the dynamic interference persists in the photoelectron momentum distributions and is not suppressed at all for the laser parameters considered in this work.

physics.atom-ph↗

arXiv2014

Attosecond streaking of Cohen-Fano interferences in the photoionization of H$_2^+$

We present the first numerical simulation of the time delay in the photoionization of the simplest diatomic molecule H$_2^+$ as observed by attosecond streaking. We show that the strong variation of the Eisenbud-Wigner-Smith time delay as a function of energy and emission angle becomes observable in the streaking time shift provided laser field-induced components are accounted for. The strongly enhanced photoemission time shifts are traced to destructive Cohen-Fano (or two-center) interferences. Signatures of these interferences in the streaking trace are shown to be enhanced when the ionic fragments are detected in coincidence.

physics.atom-ph↗