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Weihang Lu

Publications and source records attributed to Weihang Lu.

7 recordsLinked to original sources

Giant spontaneous Kerr effect and its self-doping dependence in altermagnetic MnTe

Altermagnetism, a third class of collinear magnetism with spin-split bands and vanishing net magnetization, has emerged in hexagonal {\alpha}-MnTe, a promising platform for ultrafast, stray-field-free spintronics. Whether MnTe's macroscopic symmetry-breaking signatures reflect ideal altermagnetic order or are activated by defects remains open. Here we report giant spontaneous Kerr rotations of up to 1500 rad in {\alpha}-MnTe single crystals at the telecommunication wavelength of 1550 nm, onsetting precisely at the N\'eel temperature TN = 307 K. The signal appears in disjoint macroscopic patches whose amplitude tracks the sample conductivity, and a hole-conducting {\alpha}-MnTe film reproduces this response together with an anomalous Hall effect. Within a single crystal, Kerr-active regions are optically distinct from their Kerr-silent surroundings in co-registered reflection maps. These observations indicate that carrier self-doping, rather than ideal altermagnetic order alone, governs the giant magneto-optical response, and establish telecom-wavelength Kerr imaging as a practical readout for altermagnetic spintronics.

cond-mat.str-el

Direct imaging of a Berry curvature nematic state in a spin-compensated magnet

Density waves conventionally describe the periodic modulation of charge or spin, yet the spatial modulation of electronic geometry has remained elusive. Here, we report subtle micrometer-scale spatial modulations of the magneto-optical Kerr signal in the noncollinear antiferromagnet Mn3NiN with compensated spins, consistent with a magnetic-field-induced Berry curvature density wave . These Berry curvature modulations exhibit orientations unpinned from the crystal lattice, forming a nematic state that spontaneously breaks rotational symmetry. We attribute this spatial instability to field-induced spatial variations of the spin texture driven by competing magnetic interactions. This discovery unveils a new class of collective order in spin-compensated magnets mediated by the geometric phase of the wavefunction itself. Its wavelength is controlled by chemical doping and its amplitude by magnetic field, providing concrete tuning knobs for antiferromagnetic and altermagnetic spintronics.

cond-mat.str-el

Temperature-invariant magneto-optical Kerr effect in a noncollinear antiferromagnet

Noncollinear antiferromagnets exhibit anomalous Hall and magneto-optical Kerr effects driven by Berry curvature despite negligible net magnetization, promising ultrafast spintronic applications. While both effects are theoretically expected to reveal the intrinsic Berry curvature that serves as a spintronic memory bit, their quantitative interpretation is complicated by additional temperature-dependent contributions superimposed on the magnetic order parameter: extrinsic skew scattering in dc Hall transport, and optical-resonance effects in visible-wavelength Kerr measurements. Here we perform polar Kerr measurements at the infrared telecommunication wavelength (1550 nm) on epitaxial, stoichiometric Mn3NiN single crystal films, revealing for the first time a spontaneous Kerr signal that remains stable within a few percent over a 200 K range below the N\'eel temperature. This temperature-invariant intrinsic Kerr response contrasts with the strongly temperature-dependent anomalous Hall effect in the same sample dominated by extrinsic skew scattering. Our findings establish infrared Kerr effect as a robust, local probe of Berry curvature in noncollinear antiferromagnets, enabling quantitative characterization and advancing antiferromagnetic spintronic technologies.

cond-mat.str-el

Topological Magneto-optical Kerr Effect without Spin-orbit Coupling in Spin-compensated Antiferromagnet

The magneto-optical Kerr effect (MOKE), the differential reflection of oppositely circularly polarized light, has traditionally been associated with relativistic spin-orbit coupling (SOC), which links a particle's spin with its orbital motion. In ferromagnets, large MOKE signals arise from the combination of magnetization and SOC, while in certain coplanar antiferromagnets, SOC-induced Berry curvature enables MOKE despite zero net magnetization. Theoretically, large MOKE can also arise in a broader class of magnetic materials with compensated spins, without relying on SOC - for example, in systems exhibiting real-space scalar spin chirality. The experimental verification has remained elusive. Here, we demonstrate such a SOC- and magnetization-free MOKE in the noncoplanar antiferromagnet Co1/3TaS2. Using a Sagnac interferometer microscope, we image domains of scalar spin chirality and their reversal. Our findings establish experimentally a new mechanism for generating large MOKE signals and position chiral spin textures in compensated magnets as a compelling platform for ultrafast, stray-field-immune opto-spintronic applications.

physics.optics

Nonvolatile Nematic Order Manipulated by Strain and Magnetic Field in a Layered Antiferromagnet

The operation mechanism of nematic liquid crystals lies in the control of their optical properties by the orientation of underlying nematic directors. In analogy, electronic nematicity refers to a state whose electronic properties spontaneously break rotation symmetries of the host crystalline lattice, leading to anisotropic electronic properties. In this work, we demonstrate that the layered antiferromagnet CoTa$_3$S$_6$ exhibits a switchable nematic order, evidenced by the emergence of both resistivity anisotropy and optical birefringence. This nematic state sets in at a temperature $T^*$ distinct from that of the antiferromagnetic transitions in the system, indicating a separate symmetry-breaking mechanism. The nematic order can be manipulated either by an in-plane rotation symmetry-breaking strain or in-plane magnetic field, with the latter exhibiting a pronounced non-volatile memory effect. Remarkably, we find that the broken three-fold rotation symmetry in electronic transport is restored with a moderate out-of-plane field. We hypothesize that the nematicity is of electronic origin and emerges from instabilities associated with van Hove singularities. The resulting phase diagram points to an intertwined interplay between the electronic nematicity and the proposed underlying collinear and non-coplanar spin orders. Our findings establish CoTa$_3$S$_6$ as a versatile antiferromagnetic platform with highly tunable functionalities arising from the breaking of rotational, time-reversal, and inversion symmetries.

cond-mat.str-el

Discovery of an Intermediate Nematic State in a Bilayer Kagome Metal ScV6Sn6

Nematicity, where rotational symmetry of the crystal lattice is spontaneously broken, is a ubiquitous phenomenon in correlated quantum matter, often intertwining with other orders to produce a richer spectrum of phases. Here we report a new phase transition in high-quality ScV6Sn6 bilayer kagome metal at a temperature T^*, occurring seven Kelvins below the charge density wave (CDW) transition at T_CDW, as indicated by thermodynamic, transport, and optical measurements. This emerging intermediate phase does not exhibit spontaneous time-reversal-symmetry breaking, as evidenced by zero-field Sagnac interferometer experiments. However, it displays a strong, spontaneous (strain- and field-free) anisotropy in the kagome plane between T^* and T_CDW, as revealed by transport and optical polarization rotation measurements. Additionally, a pronounced depolarization effect detected by the Sagnac interferometer further confirms its nematic nature. This intermediate nematic phase, alongside the recently discovered intra-unit cell nematic order at much lower temperatures, presents a diverse landscape of nematicities at multiple length and temperature scales, distinguishing it from those observed in kagome metals AV3Sb5. Our findings highlight ScV6Sn6 and the broader RM6X6 intermetallic family as fertile platforms for realizing symmetry-breaking phases driven by a unique interplay of competing CDW instabilities, kagome physics, and Van Hove singularities.

cond-mat.str-el

Direct imaging and control of Berry curvature in noncollinear antiferromagnetic single-crystal thin films

The discovery of the intrinsic anomalous Hall effect (AHE) in noncollinear antiferromagnets where transverse Hall voltage emerges without magnetic field, has opened a plethora of promising opportunities in antiferromagnetic devices. The key challenges limiting their full potential are (1) high-quality epitaxial thin-film growth and (2) the understanding of Berry curvature domain physics. Here, we focus on a noncollinear antiperovskite antiferromagnet Mn3NiN as a model system, successfully grown as a single-crystal epitaxial thin film. Combining multiple experiments supported by theoretical calculations, we probe the Berry curvature associated with antiferromagnetic {\Gamma}4g domains in Mn3NiN and its strong connection to an AHE. We directly image the intrinsic Berry curvature with high-resolution Sagnac microscopy, controlling spatial distribution and dynamics by varying temperature and applied magnetic fields. We discover that the {\Gamma}4g domains are switchable near the N\'eel transition, but become frozen and unresponsive to external stimuli at low temperature. This behavior enables the tuning of Berry-curvature driven AHE and magneto-optic Kerr effect responses through controlled experimental conditions. Our findings provide critical advancement of the fundamental understanding and wide tunability of Berry curvature in noncollinear antiferromagnets important for realization in potential spintronic applications.

cond-mat.mtrl-sci