arXiv subjects

Wen-Hao Zhang

Publications and source records attributed to Wen-Hao Zhang.

34 records · Page 2Linked to original sources

arXiv2021

Mott insulator tuning via structural distortion in monolayer 1T-NbSe2

Mott state in 1T-TaS2 is predicted to host quantum spin liquids (QSL). However, its insulating mechanism is controversial due to complications from interlayer coupling. Here, we study the Mott state in monolayer 1T-NbSe2, an electronic analogy to TaS2 exempt from interlayer coupling, using spectroscopic imaging scanning tunneling microscopy and first principles calculations. Monolayer NbSe2 surprisingly displays two types of Star-of-David (SD) motifs with different Mott gap sizes, that are interconvertible via temperature variation. And, bilayer 1T-NbSe2 shows Mott collapse by interlayer coupling. Our calculation unveils the two types of SDs possess distinct structural distortions, altering the effective Coulomb energies of the central Nb orbital. Our calculation suggests the Mott gap, the same parameter for determining the QSL regime, is tunable with strain. This finding offers a general strategy for manipulating the Mott state in 1T-NbSe2 and related systems via structural distortions, which may be tuned into the potential QSL regime.

cond-mat.mes-hall↗

arXiv2021

Improving the Precision of Optical Metrology by Detecting Fewer Photons

In optical metrological protocols to measure physical quantities, it is, in principle, always beneficial to increase photon number to improve measurement precision. However, practical constraints prevent arbitrary increase of n due to the imperfections of a practical detector, especially when the detector response is dominated by saturation effect. In this work, we show that a modified weak measurement protocol, namely, biased weak measurement significantly improves the precision of optical metrology in the presence of saturation effect. This method detects an ultra-small fraction of photons while maintains considerable amount of metrological information. The biased pre-coupling leads to an additional reduction of photons in the post-selection and generates an extinction point in the spectrum distribution, which is extremely sensitive to the estimated parameter and difficult to be saturated. Therefore, the Fisher information can be persistently enhanced by increasing the photon number. In our magnetic-sensing experiment, biased weak measurement achieves precision approximately one order of magnitude better than those of previously used methods. The proposed method can be applied in various optical measurement schemes to circumvent detector saturation effect with low-cost apparatuses.

quant-ph↗

arXiv2021

Realization of AlSb in the double layer honeycomb structure: a robust new class of two-dimensional material

Exploring new two-dimensional (2D) van der Waals (vdW) systems is at the forefront of materials physics. Here, through molecular beam epitaxy on graphene-covered SiC(0001), we report successful growth of AlSb in the double-layer honeycomb (DLHC) structure, a 2D vdW material which has no direct analogue to its 3D bulk and is predicted kinetically stable when freestanding. The structural morphology and electronic structure of the experimental 2D AlSb are characterized with spectroscopic imaging scanning tunneling microscopy and cross-sectional imaging scanning transmission electron microscopy, which compare well to the proposed DLHC structure. The 2D AlSb exhibits a bandgap of 0.93 eV versus the predicted 1.06 eV, which is substantially smaller than the 1.6 eV of bulk. We also attempt the less-stable InSb DLHC structure; however, it grows into bulk islands instead. The successful growth of a DLHC material here opens the door for the realization of a large family of novel 2D DLHC traditional semiconductors with unique excitonic, topological, and electronic properties.

cond-mat.mtrl-sci↗

arXiv2020

Classical Communication Enhanced Quantum State Verification

Quantum state verification provides an efficient approach to characterize the reliability of quantum devices for generating certain target states. The figure of merit of a specific strategy is the estimated infidelity $ε$ of the tested state to the target state, given a certain number of performed measurements n. Entangled measurements constitute the globally optimal strategy and achieve the scaling that εis inversely proportional to n. Recent advances show that it is possible to achieve the same scaling simply with non-adaptive local measurements, however, the performance is still worse than the globally optimal bound up to a constant factor. In this work, by introducing classical communication, we experimentally implement an adaptive quantum state verification. The constant-factor is minimized from ~2.5 to 1.5 in this experiment, which means that only 60% measurements are required to achieve a certain value of εcompared to optimal non-adaptive local strategy. Our results indicate that classical communication significantly enhances the performance of quantum state verification, and leads to an efficiency that further approaches the globally optimal bound.

quant-ph↗

arXiv2020

Experimental observation of coherent-information superadditivity in a dephrasure channel

We present an experimental approach to construct a dephrasure channel, which contains both dephasing and erasure noises, and can be used as an efficient tool to study the superadditivity of coherent information. By using a three-fold dephrasure channel, the superadditivity of coherent information is observed, and a substantial gap is found between the zero single-letter coherent information and zero quantum capacity. Particularly, we find that when the coherent information of n channel uses is zero, in the case of larger number of channel uses, it will become positive. These phenomena exhibit a more obvious superadditivity of coherent information than previous works, and demonstrate a higher threshold for non-zero quantum capacity. Such novel channels built in our experiment also can provide a useful platform to study the non-additive properties of coherent information and quantum channel capacity.

quant-ph↗

arXiv2020

Possible phason-polaron effect on purely one dimensional charge order of Mo6Se6 nanowires

In one-dimensional (1D) metallic systems, the diverging electron susceptibility and electron-phonon coupling collaboratively drive the electrons into a charge density wave (CDW) state. However, strictly 1D system is unstable against perturbations, whose effect on CDW order requires clarification ideally with altered coupling to surroundings. Here, we fabricate such a system with nanowires of Mo6Se6 bundles, which are either attached to edges of monolayer MoSe2 or isolated freely, by post-annealing the preformed MoSe2. Using scanning tunneling microscopy (STM), we visualized charge modulations and CDW gaps with prominent coherent peaks in the edge-attached nanowires. Astonishingly, the CDW order becomes suppressed in the isolated nanowires, showing CDW correlation gaps without coherent peaks. The contrasting behavior, as revealed with theoretical modeling, is interpreted as the effect of phason-polarons on the 1D CDW state. Our work elucidates a possibly unprecedented many body effect that may be generic to strictly 1D system but undermined in quasi-1D system.

cond-mat.mes-hall↗

arXiv2019

Mott phase in a van der Waals transition-metal halide at single layer limit

Two-dimensional materials offer opportunities for unravelling unprecedented ordered states at single layer limit. Among such ordered states, Mott phase is rarely explored. Here, we report the Mott phase in van der Waals chromium (II) iodide (CrI2) films. High quality CrI2 films with atomically flat surface and macro size are grown on graphitized 6H-SiC(0001) substrate by molecular beam epitaxy. By in situ low temperature scanning tunneling microscopy and spectroscopy (STM/STS), we reveal that the film has a band gap as large as ~3.2 eV, which is nearly thickness independent. Density functional plus dynamic mean field theory calculations suggest that CrI2 films may be a strong Mott insulator with a ferromagnetically ordered ground state. The Mott phase is corroborated by the spectral band splitting, that is consistent with the extended Hubbard model, and gap reduction at charge dopants. Our study provides a platform for studying correlated electron states at single layer limit.

cond-mat.mes-hall↗

arXiv2019

Experimental demonstration of secure quantum remote sensing

Quantum metrology aims to enhance the precision of various measurement tasks by taking advantages of quantum properties. In many scenarios, precision is not the sole target; the acquired information must be protected once it is generated in the sensing process. Considering a remote sensing scenario where a local site performs cooperative sensing with a remote site to collect private information at the remote site, the loss of sensing data inevitably causes private information to be revealed. Quantum key distribution is known to be a reliable solution for secure data transmission, however, it fails if an eavesdropper accesses the sensing data generated at a remote site. In this study, we demonstrate that by sharing entanglement between local and remote sites, secure quantum remote sensing can be realized, and the secure level is characterized by asymmetric Fisher information gain. Concretely, only the local site can acquire the estimated parameter accurately with Fisher information approaching 1. In contrast, the accessible Fisher information for an eavesdropper is nearly zero even if he/she obtains the raw sensing data at the remote site. This achievement is primarily due to the nonlocal calibration and steering of the probe state at the remote site. Our results explore one significant advantage of ``quantumness'' and extend the notion of quantum metrology to the security realm.

quant-ph↗

arXiv2019

Experimental Optimal Verification of Entangled States using Local Measurements

The initialization of a quantum system into a certain state is a crucial aspect of quantum information science. While a variety of measurement strategies have been developed to characterize how well the system is initialized, for a given one, there is in general a trade-off between its efficiency and the accessible information of the quantum state. Conventional quantum state tomography can characterize unknown states by reconstructing the density matrix; however, its exponentially expensive postprocessing is likely to produce a deviate result. Alternatively, quantum state verification provides a technique to quantify the prepared state with significantly fewer measurements, especially for quantum entangled states. Here, we experimentally implement an optimal verification of entangled states with local measurements, where the estimated infidelity is inversely proportional to the number of measurements. The utilized strategy is tolerant of the impurity of realistic states, hence being highly robust in a practical sense. Even more valuable, our method only requires local measurements, which incurs only a small constant-factor (<2.5) penalty compared to the globally optimal strategy requiring nonlocal measurements.

quant-ph↗

arXiv2018

Achieving Heisenberg-scaling precision with projective measurement on single photons

It has been suggested that both quantum superpositions and nonlinear interactions are important resources for quantum metrology. However, to date the different roles that these two resources play in the precision enhancement are not well understood. Here, we experimentally demonstrate a Heisenberg-scaling metrology to measure the parameter governing the nonlinear coupling between two different optical modes. The intense mode with n (more than 10^6 in our work) photons manifests its effect through the nonlinear interaction strength which is proportional to its average photon-number. The superposition state of the weak mode, which contains only a single photon, is responsible for both the linear Hamiltonian and the scaling of the measurement precision. By properly preparing the initial state of single photon and making projective photon-counting measurement, the extracted classical Fisher information (FI) can saturate the quantum FI embedded in the combined state after coupling, which is ~ n^2 and leads to a practical precision ~ 1.2/n. Free from the utilization of entanglement, our work paves a way to realize Heisenberg-scaling precision when only a linear Hamiltonian is involved.

quant-ph↗

arXiv2018

Heisenberg-scaling measurement of the single-photon Kerr non-linearity using mixed states

Improving the precision of measurements is a significant scientific challenge. The challenge is twofold: first, overcoming noise that limits the precision given a fixed amount of a resource, N, and second, improving the scaling of precision over the standard quantum limit (SQL), 1/\sqrt{N}, and ultimately reaching a Heisenberg scaling (HS), 1/N. Here we present and experimentally implement a new scheme for precision measurements. Our scheme is based on a probe in a mixed state with a large uncertainty, combined with a post-selection of an additional pure system, such that the precision of the estimated coupling strength between the probe and the system is enhanced. We performed a measurement of a single photon's Kerr non-linearity with an HS, where an ultra-small Kerr phase of around 6 *10^{-8} rad was observed with an unprecedented precision of around 3.6* 10^{-10} rad. Moreover, our scheme utilizes an imaginary weak-value, the Kerr non-linearity results in a shift of the mean photon number of the probe, and hence, the scheme is robust to noise originating from the self-phase modulation.

quant-ph↗

arXiv2018

Experimentally Robust Self-testing for Bipartite and Tripartite Entangled States

Self-testing refers to a method with which a classical user can certify the state and measurements of quantum systems in a device-independent way. Especially, the self-testing of entangled states is of great importance in quantum information process. A comprehensible example is that violating the CHSH inequality maximally necessarily implies the bipartite shares a singlet. One essential question in self-testing is that, when one observes a non-maximum violation, how close is the tested state to the target state (which maximally violates certain Bell inequality)? The answer to this question describes the robustness of the used self-testing criterion, which is highly important in a practical sense. Recently, J. Kaniewski predicts two analytic self-testing bounds for bipartite and tripartite systems. In this work, we experimentally investigate these two bounds with high quality two-qubit and three-qubit entanglement sources. The results show that these bounds are valid for various of entangled states we prepared, and thus, we implement robust self-testing processes which improve the previous results significantly.

quant-ph↗

arXiv2018

Experimental self-testing of entangled states

Quantum entanglement is the key resource for quantum information processing. Device-independent certification of entangled states is a long standing open question, which arouses the concept of self-testing. The central aim of self-testing is to certify the state and measurements of quantum systems without any knowledge of their inner workings, even when the used devices cannot be trusted. Specifically, utilizing Bell's theorem, it is possible to place a boundary on the singlet fidelity of entangled qubits. Here, beyond this rough estimation, we experimentally demonstrate a complete self-testing process for various pure bipartite entangled states up to four dimensions, by simply inspecting the correlations of the measurement outcomes. We show that this self-testing process can certify the exact form of entangled states with fidelities higher than 99.9% for all the investigated scenarios, which indicates the superior completeness and robustness of this method. Our work promotes self-testing as a practical tool for developing quantum techniques.

quant-ph↗

arXiv2017

A self-guide method to search maximal Bell violation for unknown quantum states

In recent decades, a great variety of researches and applications concerning Bell nonlocality have been developed with the advent of quantum information science. Providing that Bell nonlocality can be revealed by the violation of a family of Bell inequalities, finding maximal Bell violation (MBV) for unknown quantum states becomes an important and inevitable task during Bell experiments. In this paper we introduce a self-guide method to find MBVs for unknown states using a stochastic gradient ascent algorithm (SGA), by parameterizing the corresponding Bell operators. For all the investigated systems (2-qubit, 3-qubit and 2-qutrit), this method can ascertain the MBV accurately within 100 iterations. Moreover, SGA exhibits significant superiority in efficiency, robustness and versatility compared to other possible methods.

quant-ph↗

arXiv2016

Strengthen Weak Measurement with Conjugated Destructive Interference

Standard weak measurement (SWM) has been proved to be a useful ingredient for measuring small longitudinal phase shifts. [Phys. Rev. Lett. 111, 033604 (2013)]. In this letter, we show that with specfic pre-coupling and postselection, destructive interference can be observed for the two conjugated variables, i.e. time and frequency, of the meter state. Using a broad band source, this conjugated destructive interference (CDI) can be observed in a regime approximately 1 attosecond, while the related spectral shift reaches hundreds of THz. This extreme sensitivity can be used to detect tiny longitudinal phase perturbation. Combined with a frequency-domain analysis, conjugated destructive interference weak measurement (CDIWM) is proved to outperform SWM by two orders of magnitude.

quant-ph↗

arXiv2012

Interface induced high temperature superconductivity in single unit-cell FeSe films on SrTiO3

Searching for superconducting materials with high transition temperature (TC) is one of the most exciting and challenging fields in physics and materials science. Although superconductivity has been discovered for more than 100 years, the copper oxides are so far the only materials with TC above 77 K, the liquid nitrogen boiling point. Here we report an interface engineering method for dramatically raising the TC of superconducting films. We find that one unit-cell (UC) thick films of FeSe grown on SrTiO3 (STO) substrates by molecular beam epitaxy (MBE) show signatures of superconducting transition above 50 K by transport measurement. A superconducting gap as large as 20 meV of the 1 UC films observed by scanning tunneling microcopy (STM) suggests that the superconductivity could occur above 77 K. The occurrence of superconductivity is further supported by the presence of superconducting vortices under magnetic field. Our work not only demonstrates a powerful way for finding new superconductors and for raising TC, but also provides a well-defined platform for systematic study of the mechanism of unconventional superconductivity by using different superconducting materials and substrates.

cond-mat.supr-con↗