SearcharxivSearch

arXiv subjects

Wencheng Huang

Publications and source records attributed to Wencheng Huang.

2 recordsLinked to original sources

Pressure-Induced Superconducting-like Transition in the $\it d$-wave Altermagnet Candidate CsV$_2$Se$_2$O

Altermagnetism generates exchange-type spin splitting without net magnetization and, in its $\it d$-wave form, resembles the angular symmetry of unconventional $\it d$-wave superconductivity. Whether this correspondence bears directly on superconducting instabilities in real correlated materials remains open. Here we study the quasi-two-dimensional vanadium oxychalcogenide CsV$_2$Se$_2$O (CVSO), a square-net $\it d$-wave altermagnet candidate, through combined experimental and theoretical investigation of its lattice structure, electronic structure and transport properties. At ambient pressure, CVSO is a weakly insulating parent state with a density-wave-like anomaly near 100 K, and its bulk properties are most consistent with a G-type compensated antiferromagnetic background. Under compression, the density-wave-like feature is suppressed, the magnetoresistance evolves from predominantly negative to positive, and a superconducting-like resistive downturn emerges below about 3 K. This low-temperature anomaly is reproducible across samples and pressure media, and is suppressed by magnetic field. Room-temperature X-ray diffraction reveals no symmetry lowering, whereas does show a pronounced compressibility anomaly over the same pressure range. CVSO thus reveals a pressure-tuned phase diagram in which a reconstructed weakly insulating parent state gives way to strange-metal-like transport and superconducting-like behavior, echoing broader phenomenology associated with unconventional superconductors, including cuprates and nickelates.

cond-mat.supr-con

Pressure-Induced Metal-Insulator and Paramagnet-Altermagnet Transitions in Rutile OsO2 Single Crystals

Altermagnets with compensated spin structures and nonrelativistic spin splitting have emerged as a new class of magnetic materials. Rutile OsO2 has been theoretically predicted to be altermagnetic, but experimental studies have been limited by synthesis challenges. We have succeeded in synthesizing high-quality single crystals of rutile OsO2. Electrical transport studies reveal that OsO2 is highly conductive and exhibits clear Fermi liquid behavior, indicating strong electron-electron scattering. Magnetic measurements show that the crystals are isotropically paramagnetic. Density-functional theory calculations indicate that bulk OsO2 is semimetallic with coexisting electron and hole pockets, with its magnetic ground state strongly dependent on the on-site Coulomb correlation U. Angle-resolved photoemission spectroscopy studies unveil that the bulk bands do not yet show altermagnetic spin splitting. Interestingly, resistivity is rather pressure sensitive: at 44 GPa, a clear metal-insulator transition occurs. Hybrid functional calculations reveal that applying pressure significantly increases the Hubbard U value, driving a phase transition from a paramagnetic metal to an altermagnetic metal, and eventually to an altermagnetic insulator. These findings suggest that tuning external pressure effectively modulates the magnetic ground state of OsO2, providing a pathway to realize altermagnetism in this material.

cond-mat.mes-hall