arXiv subjects

Wenjun Kuang

Publications and source records attributed to Wenjun Kuang.

5 recordsLinked to original sources

arXiv2025

Unconventional magnetization in the multiphase superconductor PdBi$_2$

Unconventional superconductors have specific signatures in their magnetic properties, such as intrinsic magnetization at interfaces and around defects and fractional and multiquanta vortices, with much attention focused on heavy fermion and high-$T_c$ superconductors. Here, we report the observation of highly anomalous magnetization in $\beta$-PdBi$_2$, a layered superconductor previously shown to exhibit a magnetic field-induced transition from s-wave to nodal p-wave superconductivity at a transition field $H^*\sim$0.1 T ($H_{C1}<H^*<H_{C2}$). This transition is driven by the coupling between spin-polarized electronic bands and the in-plane magnetic field. In the unconventional phase (above $H^*$) we observe three striking features: strictly linear and non-hysteretic dc magnetization, a sharp drop in the ac susceptibility when the field is applied parallel to the ab-plane, and a pronounced anisotropy in the magnetic response between parallel and perpendicular field orientations. We show that these features are directly correlated with the expected transition to the nodal p-wave state and propose that the unusual magnetization behavior can be explained by a transition from a conventional vortex lattice in the low-field s-wave phase to a domain structure corresponding to spatial phase separation into superconducting (p-wave) and normal domains above $H^*$. Our work identifies new experimental signatures of unconventional multiphase superconductivity, offering an insight into the magnetic-field response of nodal states.

cond-mat.supr-con↗

arXiv2024

Multiphase superconductivity in PdBi2

Unconventional superconductivity, where electron pairing does not involve electron-phonon interactions, is often attributed to magnetic correlations in a material. Well known examples include high-T_c cuprates and uranium-based heavy fermion superconductors. Less explored are unconventional superconductors with strong spin-orbit coupling, where interactions between spin-polarised electrons and external magnetic field can result in multiple superconducting phases and field-induced transitions between them, a rare phenomenon in the superconducting state. Here we report a magnetic-field driven phase transition in \beta-PdBi2, a layered non-magnetic superconductor. Our tunnelling spectroscopy on thin PdBi2 monocrystals incorporated in planar superconductor-insulator-normal metal junctions reveals a marked discontinuity in the superconducting properties with increasing in-plane field, which is consistent with a transition from conventional (s-wave) to nodal pairing. Our theoretical analysis suggests that this phase transition may arise from spin polarisation and spin-momentum locking caused by locally broken inversion symmetry, with p-wave pairing becoming energetically favourable in high fields. Our findings also reconcile earlier predictions of unconventional multigap superconductivity in \beta-PdBi2 with previous experiments where only a single s-wave gap could be detected.

cond-mat.supr-con↗

arXiv2021

Magnetization signature of topological surface states in a non-symmorphic superconductor

Superconductors with nontrivial band structure topology represent a class of materials with unconventional and potentially useful properties. Recent years have seen much success in creating artificial hybrid structures exhibiting main characteristics of two-dimensional (2D) topological superconductors. Yet, bulk materials known to combine inherent superconductivity with nontrivial topology remain scarce, largely because distinguishing their central characteristic -- topological surface states -- proved challenging due to a dominant contribution from the superconducting bulk. Reported here is a highly anomalous behaviour of surface superconductivity in topologically nontrivial 3D superconductor In2Bi where the surface states result from its nontrivial band structure, which itself is a consequence of the non-symmorphic crystal symmetry and strong spin-orbit coupling. In contrast to smoothly decreasing diamagnetic susceptibility above the bulk critical field Hc2, associated with surface superconductivity in conventional superconductors, we observe near-perfect, Meissner-like screening of low-frequency magnetic fields well above Hc2. The enhanced diamagnetism disappears at a new phase transition close to the critical field of surface superconductivity Hc3. Using theoretical modelling, we show that the anomalous screening is consistent with modification of surface superconductivity due to the presence of topological surface states. The demonstrated possibility to detect signatures of the surface states using macroscopic magnetization measurements provides an important new tool for discovery and identification of topological superconductors.

cond-mat.supr-con↗

arXiv2020

Quantum rescaling, domain metastability and hybrid domain-walls in two-dimensional CrI3 magnets

Higher-order exchange interactions and quantum effects are widely known to play an important role in describing the properties of low-dimensional magnetic compounds. Here we identify the recently discovered two-dimensional (2D) van der Waals (vdW) CrI3 as a quantum non-Heisenberg material with properties far beyond an Ising magnet as initially assumed. We find that biquadratic exchange interactions are essential to quantitatively describe the magnetism of CrI3 but requiring quantum rescaling corrections to reproduce its thermal properties. The quantum nature of the heat bath represented by discrete electron-spin and phonon-spin scattering processes induced the formation of spin fluctuations in the low temperature regime. These fluctuations induce the formation of metastable magnetic domains evolving into a single macroscopic magnetization or even a monodomain over surface areas of a few micrometers. Such domains display hybrid characteristics of Neel and Bloch types with a narrow domain wall width in the range of 3-5 nm. Similar behaviour is expected for the majority of 2D vdW magnets where higher-order exchange interactions are appreciable.

cond-mat.mes-hall↗

arXiv2020

Giant magneto-birefringence effect and tuneable colouration of 2D crystals' suspensions

One of the long sought-after goals in manipulation of light through light-matter interactions is the realization of magnetic-field-tuneable colouration, so-called magneto-chromatic effect, which holds great promise for optical, biochemical and medical applications due to its contactless and non-invasive nature. This goal can be achieved by magnetic-field controlled birefringence, where colours are produced by the interference between phase-retarded components of transmitted polarised light. Thus far birefringence-tuneable coloration has been demonstrated using electric field, material chirality and mechanical strain but magnetic field control remained elusive due to either weak magneto-optical response of transparent media or low transmittance to visible light of magnetically responsive media, such as ferrofluids. Here we demonstrate magnetically tuneable colouration of aqueous suspensions of two-dimensional cobalt-doped titanium oxide which exhibit an anomalously large magneto-birefringence effect. The colour of the suspensions can be tuned over more than two wavelength cycles in the visible range by moderate magnetic fields below 0.8 T. We show that such giant magneto-chromatic response is due to particularly large phase retardation (>3 pi) of the polarised light, which in its turn is a combined result of a large Cotton-Mouton coefficient (three orders of magnitude larger than for known liquid crystals), relatively high saturation birefringence (delta n = 2 x 10^-4) and high transparency of our suspensions to visible light. The work opens a new avenue to achieve tuneable colouration through engineered magnetic birefringence and can readily be extended to other magnetic 2D nanocrystals. The demonstrated effect can be used in a variety of magneto-optical applications, including magnetic field sensors, wavelength-tuneable optical filters and see-through printing.

physics.app-ph↗