arXiv subjects

Wenping Hu

Publications and source records attributed to Wenping Hu.

16 recordsLinked to original sources

arXiv2026

Observation of field-odd and field-free superconducting diode effects in $\mathrm{Mo}_2\mathrm{C}$ nanoflakes

The superconducting diode effect (SDE) enables nonreciprocal supercurrent flow, holding immense potential for ultra-low-power quantum electronics. Intrinsic SDE typically requires materials with inherent symmetry breakings. Here, we report the discovery of SDE in chemical vapor deposition-grown molybdenum carbide ($\mathrm{Mo}_2\mathrm{C}$) nanoflakes, a material traditionally considered centrosymmetric. Strikingly, this system uniquely hosts both field-odd and field-free SDEs. Transport measurements reveal a field-odd SDE with tunable efficiency exceeding 40% at 4 K under a perpendicular in-plane magnetic field. In a separate sample, a robust field-free SDE persists under zero-field and field-coolings. Out-of-plane field sweeps confirm the intrinsic nature of these phenomena. We propose that domain-boundary supercurrents or charge density wave-like orders drive this unexpected combination of symmetry breakings. Our findings establish air-stable $\mathrm{Mo}_2\mathrm{C}$ as an ideal platform for nonreciprocal superconducting electronics operating at liquid-helium temperatures, expanding the search for SDE into nominally centrosymmetric superconductors.

cond-mat.supr-con↗

arXiv2026

DARL: Encouraging Diverse Answers for General Reasoning without Verifiers

Reinforcement Learning with Verifiable Rewards (RLVR) has demonstrated promising gains in enhancing the reasoning capabilities of large language models. However, its dependence on domain-specific verifiers significantly restricts its applicability to open and general domains. Recent efforts such as RLPR have extended RLVR to general domains, enabling training on broader datasets and achieving improvements over RLVR. However, a notable limitation of these methods is their tendency to overfit to reference answers, which constrains the model's ability to generate diverse outputs. This limitation is particularly pronounced in open-ended tasks such as writing, where multiple plausible answers exist. To address this, we propose DARL, a simple yet effective reinforcement learning framework that encourages the generation of diverse answers within a controlled deviation range from the reference while preserving alignment with it. Our framework is fully compatible with existing general reinforcement learning methods and can be seamlessly integrated without additional verifiers. Extensive experiments on thirteen benchmarks demonstrate consistent improvements in reasoning performance. Notably, DARL surpasses RLPR, achieving average gains of 1.3 points on six reasoning benchmarks and 9.5 points on seven general benchmarks, highlighting its effectiveness in improving both reasoning accuracy and output diversity.

cs.CL↗

arXiv2026

From Tags to Trees: Structuring Fine-Grained Knowledge for Controllable Data Selection in LLM Instruction Tuning

Effective and controllable data selection is critical for LLM instruction tuning, especially with massive open-source datasets. Existing approaches primarily rely on instance-level quality scores, or diversity metrics based on embedding clusters or semantic tags. However, constrained by the flatness of embedding spaces or the coarseness of tags, these approaches overlook fine-grained knowledge and its intrinsic hierarchical dependencies, consequently hindering precise data valuation and knowledge-aligned sampling. To address this challenge, we propose Tree-aware Aligned Global Sampling (TAGS), a unified framework that leverages a knowledge tree built from fine-grained tags, thereby enabling joint control of global quality, diversity, and target alignment. Using an LLM-based tagger, we extract atomic knowledge concepts, which are organized into a global tree through bottom-up hierarchical clustering. By grounding data instances onto this tree, a tree-aware metric then quantifies data quality and diversity, facilitating effective sampling. Our controllable sampling strategy maximizes tree-level information gain and enforces leaf-level alignment via KL-divergence for specific domains. Extensive experiments demonstrate that TAGS significantly outperforms state-of-the-art baselines. Notably, it surpasses the full-dataset model by \textbf{+5.84\%} using only \textbf{5\%} of the data, while our aligned sampling strategy further boosts average performance by \textbf{+4.24\%}.

cs.CL↗

arXiv2025

Entropy Ratio Clipping as a Soft Global Constraint for Stable Reinforcement Learning

Large language model post-training relies on reinforcement learning to improve model capability and alignment quality. However, the off-policy training paradigm introduces distribution shift, which often pushes the policy beyond the trust region, leading to training instabilities manifested as fluctuations in policy entropy and unstable gradients. Although PPO-Clip mitigates this issue through importance clipping, it still overlooks the global distributional shift of actions. To address these challenges, we propose using the entropy ratio between the current and previous policies as a new global metric that effectively quantifies the relative change in policy exploration throughout updates. Building on this metric, we introduce an \textbf{Entropy Ratio Clipping} (ERC) mechanism that imposes bidirectional constraints on the entropy ratio. This stabilizes policy updates at the global distribution level and compensates for the inability of PPO-clip to regulate probability shifts of un-sampled actions. We integrate ERC into both DAPO and GPPO reinforcement learning algorithms. Experiments across multiple benchmarks show that ERC consistently improves performance.

cs.LG↗

arXiv2025

Asymmetric quantum Hall effect and diminished $\nu=0$ longitudinal resistance in graphene/InSe heterostructures

We investigate quantum transport in graphene/InSe heterostructures and find major asymmetries in the longitudinal resistance ($R_{xx}$) and vanishing $R_{xx}$ peaks at high magnetic fields, particularly at the charge-neutrality point. Our Landauer-Buttiker analysis and numerical simulations show that a monotonically varying density gradient combined with a full equilibration mechanism can explain these phenomena. Our results also suggest the presence of trivial long-range chiral edge current and offer a broadly applicable way to engineer transport properties in quantum Hall systems.

cond-mat.mes-hall↗

arXiv2025

When Importance Sampling Misallocates Credit: Asymmetric Ratios for Outcome-Supervised RL

Reinforcement learning (RL) has shown great promise in large language models (LLMs) post-training, which typically rely on token-level clipping to maintain stability during optimization. Despite the empirical success of GRPO-style methods, we identify a fundamental and previously overlooked challenge in this popular Outcome-Supervised RL (OSRL) paradigm. We reveal that in OSRL, where advantages are shared across tokens within a response, importance sampling (IS) ratios deviate from their traditional purpose of distribution correction as in classic RL, which become token-level weights that allocate the shared advantage signal across tokens. We show that this hidden role shift induces a critical mismatch for positive-advantage tokens, leading to unbalanced token weighting between positive and negative tokens. Specifically, it suppresses the update of underrepresented tokens that are lagging behind, while over-amplifying already high-probability tokens. This mismatch results in rich-get-richer dynamics that over-reinforce confident tokens, weaken catch-up learning that drive entropy collapse, excessive repetition, and premature convergence. To address this, we propose Asymmetric Importance Sampling Policy Optimization (ASPO), a simple yet effective strategy that reverses the ratio-induced weighting of positive-advantage tokens, while stabilizing extreme updates and maintaining gradient flow. This mismatch correction aligns their update direction with the learning dynamics of negative ones. Comprehensive experiments across math reasoning and coding benchmarks demonstrate that ASPO significantly mitigates entropy collapse, improves training stability, and enhances performance over strong GRPO-based baselines. Our analysis provides new insights into the role of token-level weighting in OSRL and highlights the critical importance of correcting ratio-induced weighting in LLM RL.

cs.CL↗

arXiv2025

Attention as a Compass: Efficient Exploration for Process-Supervised RL in Reasoning Models

Reinforcement Learning (RL) has shown remarkable success in enhancing the reasoning capabilities of Large Language Models (LLMs). Process-Supervised RL (PSRL) has emerged as a more effective paradigm compared to outcome-based RL. However, existing PSRL approaches suffer from limited exploration efficiency, both in terms of branching positions and sampling. In this paper, we introduce a novel PSRL framework (AttnRL), which enables efficient exploration for reasoning models. Motivated by preliminary observations that steps exhibiting high attention scores correlate with reasoning behaviors, we propose to branch from positions with high values. Furthermore, we develop an adaptive sampling strategy that accounts for problem difficulty and historical batch size, ensuring that the whole training batch maintains non-zero advantage values. To further improve sampling efficiency, we design a one-step off-policy training pipeline for PSRL. Extensive experiments on multiple challenging mathematical reasoning benchmarks demonstrate that our method consistently outperforms prior approaches in terms of performance and sampling and training efficiency.

cs.LG↗

arXiv2025

CE-GPPO: Coordinating Entropy via Gradient-Preserving Clipping Policy Optimization in Reinforcement Learning

Reinforcement learning (RL) has become a powerful paradigm for optimizing large language models (LLMs) to handle complex reasoning tasks. A core challenge in this process lies in managing policy entropy, which reflects the balance between exploration and exploitation during training. Existing methods, such as proximal policy optimization (PPO) and its variants, discard valuable gradient signals from low-probability tokens due to the clipping mechanism. We systematically analyze the entropy dynamics and reveal that these clipped tokens play a critical yet overlooked role in regulating entropy evolution. We propose \textbf{C}oordinating \textbf{E}ntropy via \textbf{G}radient-\textbf{P}reserving \textbf{P}olicy \textbf{O}ptimization (CE-GPPO), a novel algorithm that reintroduces gradients from clipped tokens in native PPO in a gentle and bounded manner. By controlling the magnitude of gradients from tokens outside the clipping interval, CE-GPPO is able to achieve an exploration-exploitation trade-off. We provide theoretical justification and empirical evidence showing that CE-GPPO effectively mitigates entropy instability. Extensive experiments on mathematical reasoning benchmarks show that CE-GPPO consistently outperforms strong baselines across different model scales.

cs.LG↗

arXiv2025

Klear-Reasoner: Advancing Reasoning Capability via Gradient-Preserving Clipping Policy Optimization

We present Klear-Reasoner, a model with long reasoning capabilities that demonstrates careful deliberation during problem solving, achieving outstanding performance across multiple benchmarks. Although there are already many excellent works related to inference models in the current community, there are still many problems with reproducing high-performance inference models due to incomplete disclosure of training details. This report provides an in-depth analysis of the reasoning model, covering the entire post-training workflow from data preparation and long Chain-of-Thought supervised fine-tuning (long CoT SFT) to reinforcement learning (RL), along with detailed ablation studies for each experimental component. For SFT data, our experiments show that a small number of high-quality data sources are more effective than a large number of diverse data sources, and that difficult samples can achieve better results without accuracy filtering. In addition, we investigate two key issues with current clipping mechanisms in RL: Clipping suppresses critical exploration signals and ignores suboptimal trajectories. To address these challenges, we propose Gradient-Preserving clipping Policy Optimization (GPPO) that gently backpropagates gradients from clipped tokens. GPPO not only enhances the model's exploration capacity but also improves its efficiency in learning from negative samples. Klear-Reasoner exhibits exceptional reasoning abilities in mathematics and programming, scoring 90.5% on AIME 2024, 83.2% on AIME 2025, 66.0% on LiveCodeBench V5 and 58.1% on LiveCodeBench V6.

cs.LG↗

arXiv2024

Breaking the Stage Barrier: A Novel Single-Stage Approach to Long Context Extension for Large Language Models

Recently, Large language models (LLMs) have revolutionized Natural Language Processing (NLP). Pretrained LLMs, due to limited training context size, struggle with handling long token sequences, limiting their performance on various downstream tasks. Current solutions toward long context modeling often employ multi-stage continual pertaining, which progressively increases the effective context length through several continual pretraining stages. However, those approaches require extensive manual tuning and human expertise. In this paper, we introduce a novel single-stage continual pretraining method, Head-Adaptive Rotary Position Encoding (HARPE), to equip LLMs with long context modeling capabilities while simplifying the training process. Our HARPE leverages different Rotary Position Encoding (RoPE) base frequency values across different attention heads and directly trains LLMs on the target context length. Extensive experiments on 4 language modeling benchmarks, including the latest RULER benchmark, demonstrate that HARPE excels in understanding and integrating long-context tasks with single-stage training, matching and even outperforming existing multi-stage methods. Our results highlight that HARPE successfully breaks the stage barrier for training LLMs with long context modeling capabilities.

cs.CL↗

arXiv2024

Observation of Anderson localization transitions in a two-dimensional conjugated metal-organic framework

Anderson localization transitions are a universal quantum phenomenon sensitive to the disorder and dimensionality of electronic systems. Over the past decades, this intriguing topic has inspired overwhelmingly more theoretical studies than experimental verifications due to the difficulty of controlling a material's disorder or dimensionality without modifying its fundamental electronic properties. Organic crystals with their rich disorders would be terrific playgrounds to investigate such disorder-driven phase transitions except for their low conductivities which usually prohibit low-temperature measurements. Here, we conduct systematic transport experiments in mesoscopic devices made with copper benzenehexathiol thin films across a wide range of thicknesses. We find metal-insulator transitions both among three-dimensional samples with different disorder strengths and between three-dimensional and quasi-two-dimensional samples. Temperature-dependence analysis of the conductivities corroborates the dimensionality crossover. Moreover, our theoretical modeling provides a basis for understanding both types of metal-insulator transitions within the framework of Anderson localization transitions. Our findings establish for the first time that organic crystals such as conductive metal-organic frameworks can exhibit such quantum interference effects. With organic materials' versatile chemical designs and crystalline structures, our work opens new avenues to search for novel quantum phenomena in organic material platforms.

cond-mat.mes-hall↗

arXiv2024

Janus graphene nanoribbons with a single ferromagnetic zigzag edge

Topological design of pi-electrons in zigzag-edged graphene nanoribbons (ZGNRs) leads to a wealth of magnetic quantum phenomena and exotic quantum phases. Symmetric ZGNRs typically exhibit antiferromagnetically coupled spin-ordered edge states. Eliminating cross-edge magnetic coupling in ZGNRs not only enables the realization of a new class of ferromagnetic quantum spin chains, enabling the exploration of quantum spin physics and entanglement of multiple qubits in the 1D limit, but also establishes a long-sought carbon-based ferromagnetic transport channel, pivotal for ultimate scaling of GNR-based quantum electronics. However, designing such GNRs entails overcoming daunting challenges, including simultaneous breaking of structural and spin symmetries, and designing elegant precursors for asymmetric fabrication of reactive zigzag edges. Here, we report a general approach for designing and fabricating such ferromagnetic GNRs in the form of Janus GNRs with two distinct edge configurations. Guided by Lieb's theorem and topological classification theory, we devised two JGNRs by asymmetrically introduced a topological defect array of benzene motifs to one zigzag edge, while keeping the opposing zigzag edge unchanged. This breaks structural symmetry and creates a sublattice imbalance within each unit cell, initiating a spin symmetry breaking. Three Z-shape precursors are designed to fabricate one parent ZGNR and two JGNRs with an optimal lattice spacing of the defect array for a complete quench of the magnetic edge states at the defective edge. Characterization via scanning probe microscopy/spectroscopy and first-principles density functional theory confirms the successful fabrication of Janus GNRs with ferromagnetic ground state delocalised along the pristine zigzag edge.

cond-mat.mes-hall↗

arXiv2022

Relaxation Oscillations of an Exciton-polariton Condensate Driven by Parametric Scattering

We report observation of coherent oscillations in the relaxation dynamics of an exciton-polariton condensate driven by parametric scattering processes. As a result of the interbranch scattering scheme and the nonlinear polariton-polariton interactions, such parametric scatterings exhibit high scattering efficiency, which leads to fast depletion of the polariton condensate and periodic shut-off of the bosonic stimulation processes, eventually causing relaxation oscillations. Employing polariton-reservoir interactions, the oscillation dynamics in the time domain can be projected onto the energy space. In theory, our simulations using the open-dissipative Gross-Pitaevskii equation are in excellent agreement with experimental observations. Surprisingly, the oscillation patterns are clearly visible in our time-integrated images including many excitation pulses, implying the high stability of the relaxation oscillations driven by polariton parametric scatterings.

physics.optics↗

arXiv2021

Electrocatalytic reduction of nitrogen to ammonia in ionic liquids

Ammonia NH3 is an important raw material for nitrogen fertilizer production and is widely used in industry. It is also a carbon free renewable fuel and an excellent hydrogen storage material. Reaction conditions of traditional Haber Bosch process are very harsh although it supports most of todays NH3 production. Recently, electrocatalytic nitrogen reduction reaction NRR has become one of the effective alternative methods to the traditional Haber Bosch process due to the advantages of mild operation conditions and almost no environmental pollutions. Ionic liquids ILs act as one of green solvents possess a lot of unique features and have shown excellent performance in electrocatalytic NRR process. In this review, we summarize fundamentals of the electrocatalytic NRR, the role of ILs in several typical electrocatalytic processes, and the possible role of ILs in the electrocatalytic NRR process. Moreover, the selection principles and issues of the application of ILs, as well as the future development direction for the electrocatalytic NRR process are concluded.

physics.chem-ph↗

arXiv2021

Topological interface states induced by incident angle in the 1D elastic wave system

Topological interface states are currently attracting rapidly growing attention in classical wave systems. However, little work has been done on topological interface states in one-dimensional (1D) elastic wave systems, especially in the case of oblique incidence. This paper theoretically demonstrates the realization of topological interface states of elastic waves in a 1D composite plate structure composed of two phononic crystals (PCs) with different topological characteristics, which can be regulated by the incident angle. For the out-of-plane SH mode, multiple topological interface states can coexist in different common bandgaps. For the in-plane complex P-SV coupled mode, topological interface states can exist in both "partial-polarization" and "omni-polarization" bandgaps. All these interface states are in the wide frequency and incident angle regions. We also discuss the polarization and the mode conversion of the interface states. Our results provide an innovative method to excite and tune topologically protected interface states for elastic waves, which may have potential applications in obtaining strong local vibration for different polarized elastic wave modes.

physics.app-ph↗

arXiv2020

Research progress of rubrene as an excellent multifunctional organic semiconductor

Rubrene, a superstar in organic semiconductors, has achieved unprecedented achievements in the application of electronic devices, and research based on its various photoelectric properties is still in progress. In this review, we introduced the preparation of rubrene crystal, summarized the applications in organic optoelectronic devices with the latest research achievements based on rubrene semiconductors. An outlook of future research directions and challenges of rubrene semiconductor for applications is also provided.

physics.app-ph↗