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Wenxiang Wang

Publications and source records attributed to Wenxiang Wang.

3 recordsLinked to original sources

Weyl points enabling significant enhancement of thermoelectric performance in an antiferromagnetic van der Waals metal GdTe3

Magneto-thermoelectric (MTE) effect has demonstrated significant ad-vantages in achieving optimal thermoelectric (TE) properties compared to conventional methods. Topological materials pro-vide a unique platform for investigating the MTE effect, leveraging their exotic electronic structure topology. In this study, we report that the topological material GdTe3 exhibits an unsaturated power factor of up to 18846 μW m-1 K-1 under a magnetic field of 13.5 T at 20 K, which represents the highest value observed in metallic systems and surpasses most state-of-the-art TE materials. The relative enhancement under magnetic field in thermopower and power factor reaches 873% and 1075%, respectively, attributed to the Weyl points contribution resulting from the field-induced topological transition, as confirmed by our theoretical calculations. Our findings demonstrate a promising candidate for solid-state cooling and reveal the substantial contribution of Weyl points to TE enhancement, thereby offering a novel approach to optimizing TE properties in topological materials.

cond-mat.mtrl-sci

Suppressed Rupture of Thin Metal Films via van der Waals Epitaxy

Ultrathin metal films exhibit liquid-like instabilities, rupturing via surface diffusion far below their melting points. This behavior constrains thermal budgets for advanced integrated circuits and emerging 2D-crystal devices. Here, we demonstrate that these instabilities can be fundamentally suppressed using graphene as a van der Waals (vdW) template. While conventional 20-nm-thick gold films break up into islands below 300 {\textdegree}C, templated films not only remain stable but also become structurally refined after annealing above 600 {\textdegree}C. This exceptional stability stems from a vdW-mediated crystallographic texture that reorganizes grain boundaries into a mechanically robust network. This mechanism significantly widens the processing window for nanoscale interconnects and enables high-temperature integration of metals with 2D-crystal technologies.

cond-mat.soft

Superconductivity at 40 K in lithiation-processed [(Fe,Al)(OH)2][FeSe]1.2 with a layered structure

Exploration of new superconductors has always been one of the research directions in condensed matter physics. We report here a new layered heterostructure of [(Fe,Al)(OH)2][FeSe]1.2, which is synthesized by the hydrothermal ion-exchange technique. The structure is suggested by a combination of X-ray powder diffraction and the electron diffraction (ED). [(Fe,Al)(OH)2][FeSe]1.2 is composed of the alternating stacking of tetragonal FeSe layer and hexagonal (Fe,Al)(OH)2 layer. In [(Fe,Al)(OH)2][FeSe]1.2, there exists mismatch between the FeSe sub-layer and (Fe,Al)(OH)2 sub-layer, and the lattice of the layered heterostructure is quasi-commensurate. The as-synthesized [(Fe,Al)(OH)2][FeSe]1.2 is non-superconducting due to the Fe vacancies in the FeSe layer. The superconductivity with a Tc of 40 K can be achieved after a lithiation process, which is due to the elimination of the Fe vacancies in the FeSe layer. The Tc is nearly the same as that of (Li,Fe)OHFeSe although the structure of [(Fe,Al)(OH)2][FeSe]1.2 is quite different from that of (Li,Fe)OHFeSe. The new layered heterostructure of [(Fe,Al)(OH)2][FeSe]1.2 contains an iron selenium tetragonal lattice interleaved with a hexagonal metal hydroxide lattice. These results indicate that the superconductivity is very robust for FeSe-based superconductors. It opens a path for exploring super-conductivity in iron-base superconductors.

cond-mat.supr-con