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Wenzheng Wei

Publications and source records attributed to Wenzheng Wei.

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Stripe-Like Superconducting Enhancement and Coexisting Magnetic Texture in an Infinite Layer Nickelate

Despite their promise as structural and electronic analogs to cuprates, nickelate thin films consistently exhibit broadened superconducting transitions in many experiments that remain poorly understood. Local measurements are ideal for revealing the presence of defects or competing phases, which may cause this transition broadening through a phase-separation. Here, we use scanning SQUID microscopy to investigate local superfluid density and magnetic texture of optimally doped $\mathrm{Nd}_{1-x}\mathrm{Eu}_{x}\mathrm{NiO}_{2}$ (NENO) (x=0.25) grown via molecular beam epitaxy. We observed a weakly-magnetic texture coexisting with superconductivity. Spatially resolved susceptibility imaging reveals a highly non-uniform superconducting state, characterized by a robust stripe-like enhancement pattern appearing near the phase transition. By resolving the mesoscopic landscape of electronic and magnetic inhomogeneities, these findings suggest that a competing magnetic phase is a primary contributor to the unusually broad superconducting transitions of these optimally doped NENO samples. Understanding the uncovered superconducting enhancement may provide a path to raising superconducting temperatures in these materials.

cond-mat.supr-con

Re-entrant unconventional superconductivity induced by rare-earth substitution in Nd1-xEuxNiO2 thin films

High temperature superconductivity is typically associated with strong coupling and a large superconducting gap, yet these characteristics have not been demonstrated in the nickelates. Here, we provide experimental evidence that Eu substitution in the spacer layer of Nd1-xEuxNiO2 (NENO) thin films enhances the superconducting gap, driving the system toward a strong-coupling regime. This is accompanied by a magnetic-exchange-driven magnetic-field-enhanced superconductivity. We investigate the upper critical magnetic field, Hc2, and superconducting gap of superconducting NENO thin films with x=0.2 to 0.35. Magnetoresistance measurements reveal magnetic-field-enhanced superconductivity in NENO films. We interpret this phenomenon as a result of interaction between magnetic Eu ions and superconducting states in the Ni dx2-y2 orbital. The upper critical magnetic field strongly violates the weak-coupling Pauli limit. Infrared spectroscopy confirms a large gap-to-Tc ratio $2 Δk_B T_c \approx 5 - 6$, indicating a stronger coupling pairing mechanism in NENO relative to the Sr-doped NdNiO2. The substitution of Eu in the rare-earth layer provides a method to modify the superconducting gap in Nd-based nickelates, an essential factor in engineering high-Tc superconductivity in infinite-layer nickelates.

cond-mat.supr-con

Layer controlled orbital selective Mott transition in monolayer nickelate

Dimensionality and electronic correlations are crucial elements of many quantum material properties. An example is the change of the electronic structure accompanied by the loss of quasiparticles when a metal is reduced from three dimensions to a lower dimension, where the Coulomb interaction between carriers becomes poorly screened. Here, using angle-resolved photoemission spectroscopy (ARPES), we report an orbital-selective decoherence of spectral density in the perovskite nickelate LaNiO3 towards the monolayer limit. The spectral weight of the dz2 band vanishes much faster than that of the dx2-y2 band as the thickness of the LaNiO3 layer is decreased to a single unit cell, indicating a stronger correlation effect for the former upon dimensional confinement. Dynamical mean-field theory (DMFT) calculations show an orbital-selective Mott transition largely due to the localization of dz2 electrons along the c axis in the monolayer limit. This orbital-selective correlation effect underpins many macroscopic properties of nickelates, such as metal-to-insulator transition and superconductivity, where most theories are built upon a dx2-y2-dz2 two-band model.

cond-mat.str-el