arXiv subjects

Willem L. Vos

Publications and source records attributed to Willem L. Vos.

At least 37 records · Page 2Linked to original sources

arXiv2022

Controlled light scattering of a single nanoparticle by wavefront shaping

Controlling light scattering by nanoparticles is fundamentally important for the understanding and the control of light with photonic nanostructures, as well as for nanoparticle scattering itself, including Mie scattering. Here, we theoretically and numerically investigate the possibility to manipulate nanoparticle scattering by wavefront shaping that was initially developed to control light scattered by large numbers of nanoparticles in nanophotonic media. By employing a scattering matrix analysis, we find that even a single nanoparticle supports multiple strongly scattering eigenchannels, suggesting wavefront shaping as a promising tool to manipulate scattered light of a single nanoparticle. By sending in shaped wavefronts, we selectively excite eigenchannels, as is apparent from the distinct field distributions. These scattering eigenchannels are related to different resonant leaky modes of the scatterer, that reveal remarkable localized "hot spots" where the field is substantially enhanced. Moreover, we investigate the backscattered spectra; to this send in wavefronts relevant for a particular eigenchannel, and observe that the backscattered spectrum reveals not only the excited channel but also several others. This result points to the existence of short and long-range spectral correlations for an eigenchannel. Our work offers a flexible tool to manipulate light scattering of a single nanoparticle, and thus opens new possibilities to control field patterns and light-matter interactions in a nanoparticle, as well as to explore new features of nanoparticle scattering such as the spectral correlation and temporal response of light scattered by nano scatterers, including Mie spheres.

physics.optics↗

arXiv2022

Optical Properties of Chiral Three-Dimensional Photonic Crystals made from Semiconductors

We perform a theoretical and numerical study of the optical properties of both direct and inverse three-dimensional (3D) chiral woodpile structures, and a corresponding chiral Bragg stack. We compute transmission spectra in the helical direction for finite crystals, and photonic band structures, where we ensure the effective index of all structures to be the same. We find that both 3D structures show dual-band circular dichroism, where light with a particular circular polarization state - either left- or right-handed - reveals a broad stop band with major attenuation, whereas the other polarization state is transmitted nearly unimpeded. We observe such gaps in different frequency ranges, with alternating handedness. The appearance of the circular-polarized gaps is successfully interpreted with a physical model wherein the circular polarization either co-rotates or counter-rotates with the chiral structure, thereby effectively leading to a spatially-dependent or a constant refractive index, and thus to the presence or absence of a gap. We find that the presence or absence of circularly polarized gaps is tuned by the transverse periods perpendicular to the chiral axis in both the 3D direct and inverse chiral woodpile crystal structures. The tunability of circular dichroism may find applications as on-chip sensors for circularly polarized light and in the on-chip detection of chiral molecules.

physics.optics↗

arXiv2022

Scaling theory of wave confinement in classical and quantum periodic systems

Functional defects in periodic media confine waves - acoustic, electromagnetic, electronic, spin, etc. - in various dimensions, depending on the structure of the defect. While defects are usually modelled by a superlattice with a typical band-structure representation of energy levels, determining the confinement associated with a given band is highly non-trivial and no analytical method is known to date. Therefore, we propose a rigorous method to classify the dimensionality of the confinement. Starting from the confinement energy and the mode volume, we use finite-size scaling to find that ratios of these quantities to certain powers yield the confinement dimensionality of each band. This classification has negligible additional computational costs compared to a band structure calculation and is valid for any type of wave in both quantum and classical regimes, and any dimension. In the quantum case, we illustrate our method on electronic confinement in 2D hexagonal BN with a nitrogen vacancy, which confirms the previous results. In the classical case, we study a three-dimensional photonic band gap cavity superlattice, where we identify novel acceptor-like behavior.

cond-mat.dis-nn↗

arXiv2022

Breakdown of light transport models in photonic scattering slabs with strong absorption and anisotropy

The radiative transfer equation (RTE) models the transport of light inside photonic scattering samples such as paint, foam and tissue. Analytic approximations to solve the RTE fail for samples with strong absorption and dominant anisotropic scattering and predict unphysical negative energy densities and the diffuse flux in the wrong direction. Here we fully characterize the unphysical regions of three popular approximations to the RTE for a slab, namely the $P_1$ approximation (or diffusion approximation), the $P_3$ approximation, and a popular modification to $P_3$ that corrects the forward scattering in the approximation. We find that the delta function correction to $P_3$ eliminates the unphysical range in the forward scattering. In addition, we compare the predictions of these analytical methods to exact Monte Carlo simulations for the physical and unphysical regions. We present maps of relative errors for the albedo and the anisotropy of the scatterers for a realistic index contrast typical of a polymer slab in air and optical thickness. The relative error maps provide a guideline for the accuracy of the analytical methods to interpret experiments on light transport in photonic scattering slabs. Our results show that the $P_1$ approximation is significantly inaccurate to extract transport parameters unless the sample scatters purely isotropic and elastic. The $P_3$ approximation exceeds $P_1$ in terms of accuracy in its physical range for moderate absorption, and the $P_3$ with the delta function correction is the most accurate approximation considered here for the forward direction.

physics.optics↗

arXiv2021

Enhanced Absorption in thin and ultrathin silicon films by 3D photonic band gap back reflectors

Since thin-film silicon solar cells have limited optical absorption, we explore the effect of a nanostructured back reflector to recycle the unabsorbed light. As a back reflector we investigate a 3D photonic band gap crystal made from silicon that is readily integrated with the thin films. We numerically obtain the optical properties by solving the 3D time-harmonic Maxwell equations using the finite-element method, and model silicon with experimentally determined optical constants. The absorption enhancement relevant for photovoltaics is obtained by weighting the absorption spectra with the AM 1.5 standard solar spectrum. We study thin films either thicker ($L_{Si} = 2400$ nm) or much thinner ($L_{Si} = 80$ nm) than the wavelength of light. At $L_{Si} = 2400$ nm, the 3D photonic band gap crystal enhances the spectrally averaged ($λ= 680$ nm to $880$ nm) silicon absorption by $2.22$x (s-pol.) to $2.45$x (p-pol.), which exceeds the enhancement of a perfect metal back reflector ($1.47$ to $1.56$x). The absorption is enhanced by the (i) broadband angle and polarization-independent reflectivity in the 3D photonic band gap, and (ii) the excitation of many guided modes in the film by the crystal's surface diffraction leading to enhanced path lengths. At $L_{Si} = 80$ nm, the photonic crystal back reflector yields a striking average absorption enhancement of $9.15$x, much more than $0.83$x for a perfect metal, which is due to a remarkable guided mode confined within the combined thickness of the thin film and the photonic crystal's Bragg attenuation length. The broad bandwidth of the 3D photonic band gap leads to the back reflector's Bragg attenuation length being much shorter than the silicon absorption length. Consequently, light is confined inside the thin film and the absorption enhancements are not due to the additional thickness of the photonic crystal back reflector.

physics.optics↗

arXiv2021

Observation of mutual extinction and transparency in light scattering

Interference of scattered waves is fundamental for modern light-scattering techniques, such as optical wavefront shaping. Recently, a new type of wavefront shaping was introduced where the extinction is manipulated instead of the scattered intensity. The underlying idea is that upon changing the phases or the amplitudes of incident beams, the total extinction will change due to interference described by the cross terms between different incident beams. Here, we experimentally demonstrate the mutual extinction and transparency effects in scattering media, in particular, a human hair and a silicon bar. To this end, we send two light beams with a variable mutual angle on the sample. Depending on the relative phase of the incident beams we observe either nearly zero extinction, mutual transparency, or almost twice the single-beam extinction, mutual extinction, in agreement with theory. We use an analytical approximation for the scattering amplitude, starting from a completely opaque object and we discuss the limitations of our approximation. We discuss the applications of the mutual extinction and transparency effects in various fields such as non-line-of-sight communications, microscopy, and biomedical imaging.

physics.optics↗

arXiv2020

Spatially shaping waves to penetrate deep inside a forbidden gap

It is well known that waves incident upon a crystal are transported only over a limited distance - the Bragg length - before being reflected by Bragg interference. Here, we demonstrate how to send waves much deeper into crystals, by studying light in exemplary two-dimensional silicon photonic crystals. By spatially shaping the optical wavefronts, we observe that the intensity of laterally scattered light, that probes the internal energy density, is enhanced at a tunable distance away from the front surface. The intensity is up to $100 \times$ enhanced compared to random wavefronts and extends as far as $8 \times$ the Bragg length. Our novel steering of waves inside a forbidden gap exploits the transport channels induced by unavoidable deviations from perfect periodicity, here unavoidable fabrication deviations.

physics.optics↗

arXiv2020

The local density of optical states in the 3D band gap of a finite photonic crystal

A three-dimensional (3D) photonic band gap crystal is an ideal tool to completely inhibit the local density of optical states (LDOS) at every position in the crystal throughout the band gap. This notion, however, pertains to ideal infinite crystals, whereas any real crystal device is necessarily finite. This raises the question as to how the LDOS in the gap depends on the position and orientation inside a finite-size crystal. Therefore, we employ rigorous numerical calculations using finite-difference time-domain (FDTD) simulations of 3D silicon inverse woodpile crystals filled with air or with toluene, as previously studied in experiments. We find that the LDOS versus position decreases exponentially into the bulk of the crystal. From the dependence on dipole orientation, we infer that the characteristic LDOS decay length $\ell_ρ$ is mostly related to far-field dipolar radiation effects, whereas the prefactor is mostly related to near-field dipolar effects. The LDOS decay length has a remarkably similar magnitude as the Bragg length for directional transport, which suggests that the LDOS in the crystal is dominated by vacuum states that tunnel from the closest interface towards the position of interest. Our work leads to design rules for applications of 3D photonic band gaps in emission control and lighting, quantum information processing, and in photovoltaics.

physics.optics↗

arXiv2020

Reflectivity of Finite 3D GaAs Photonic Band Gap Crystals

We study the optical reflectivity of three-dimensional (3D) photonic band gap crystals with increasing thickness. The crystals consist of GaAs plates with nanorod arrays that are assembled by an advanced stacking method into high-quality 3D woodpile structures. We observe intense and broad reflectivity peak with stop bands that correspond to a broad gap in the photonic band structures. The maximum reflectivity quickly reaches high values even for a few crystal layers. Remarkably, the bandwidth of the stop bands hardly decreases with increasing crystal thickness, in good agreement with FDTD simulations. This behavior differs remarkably from the large changes observed earlier in weakly interacting 3D photonic crystals. The nearly constant bandwidth and high reflectivity are rationalized by multiple Bragg interference that occurs in strongly interacting photonic band gap crystals, whereby the incident light scatters from multiple reciprocal lattice vectors simultaneously, in particular from oblique ones that are parallel to a longer crystal dimension and thus experience hardly any finite size effects. Our new insights have favorable consequences for the application of 3D photonic band gap crystals, notably since even thin structures reveal the full band gap functionality, including devices that shield quantum bits from vacuum fluctuations.

physics.optics↗

arXiv2019

Generation of ultrashort (~10ps) spontaneous emission pulses by quantum dots in a switched optical microcavity

We report on the generation of few-ps long spontaneous emission pulses by quantum dots (QDs) in a switched optical microcavity. We use a pulsed optical injection of free charge carriers to induce a large frequency shift of the fundamental mode of a GaAs/AlAs micropillar. We track in real time by time-resolved photoluminescence its fundamental mode during its relaxation, using the emission of the QD ensemble as a broadband internal light source. Sub-ensembles of QDs emitting at a given frequency, interact transiently with the mode and emit an ultrashort spontaneous emission pulse into it. By playing with switching parameters and with the emission frequency of the QDs, selected by spectral filtering, pulse durations ranging from 300 ps down to 6 ps have been obtained. These pulses display a very small coherence length, which opens potential applications in the field of ultrafast imaging. The control of QD-mode coupling on ps-time scales establishes also cavity switching as a key resource for quantum photonics.

cond-mat.mes-hall↗

arXiv2019

Experimental probe of a complete 3D photonic band gap

The identification of a complete three-dimensional (3D) photonic band gap in real crystals always employs theoretical or numerical models that invoke idealized crystal structures. Thus, this approach is prone to false positives (gap wrongly assigned) or false negatives (gap missed). Therefore, we propose a purely experimental probe of the 3D photonic band gap that pertains to many different classes of photonic materials. We study position and polarization-resolved reflectivity spectra of 3D inverse woodpile structures that consist of two perpendicular nanopore arrays etched in silicon. We observe intense reflectivity peaks $(R > 90\%)$ typical of high-quality crystals with broad stopbands. We track the stopband width versus pore radius, which agrees much better with the predicted 3D photonic band gap than with a directional stop gap on account of the large numerical aperture used. A parametric plot of s-polarized versus p-polarized stopband width agrees very well with the 3D band gap and is model-free. This practical probe provides fast feedback on the advanced nanofabrication needed for 3D photonic crystals and stimulates practical applications of band gaps in 3D silicon nanophotonics and photonic integrated circuits, photovoltaics, cavity QED, and quantum information processing.

physics.optics↗

arXiv2019

Nonlinear frequency conversion is controlled by vacuum fluctuations

Ever since the advent of nonlinear optics, the generation of light by frequency-conversion is drawing continued attention, and leading to emerging applications such as supercontinuum sources for ultra stable clocks and advanced microscopy. A modern approach to frequency-conversion is to switch light confined in micro- and nanocavity resonances to enable on-chip operation. Supposedly, nonlinear frequency conversion in such confined media differs from traditional non-linear optics in three key features regarding output spectrum, frequency shift, and critical time scale. Therefore, we switch GaAs-AlAs microcavities by the electronic Kerr effect, and study a range of quality factors to bridge the confined and the traditional non-linear regimes. We uncover the key role of the density of vacuum fluctuations, i.e., the local density of optical states (LDOS) for newly generated frequencies, a concept inspired by cavity quantum electrodynamics (cQED). As a result, we succeed to establish a framework, which not only describes nonlinear optics both in traditional bulk and in confined media but also opens a new control dimension in changing the color of light.

physics.optics↗

arXiv2019

Universal Validity Ranges of Diffusion Theory for Light and Other Electromagnetic Waves

The well-known diffusion theory describes propagation of light and electromagnetic waves in complex media. While diffusion theory is known to fail both for predominant forward scattering or strong absorption, its precise range of validity has never been established. Therefore we present precise, universal limits on the scattering properties, beyond which diffusion theory yields unphysical negative energy density and negative incident flux. When applying diffusion theory to samples outside validity ranges to {\it infer} scattering properties from transmission and reflection, the resulting transport parameters deviate by up to an order of magnitude compared to the true ones. These discrepancies are relevant to atmospheric and climate sciences, biophysics and health sciences, white LEDs and lighting, and Anderson localization of waves.

physics.optics↗

arXiv2019

Systematic design of the color point of a white LED

Lighting is a crucial technology that is used every day. The introduction of the white light emitting diode (LED) that consists of a blue LED combined with a phosphor layer, greatly reduces the energy consumption for lighting. Despite the fast-growing market white LED's are still designed using slow, numerical, trial-and-error algorithms. Here we introduce a radically new design principle that is based on an analytical model instead of a numerical approach. Our design model predicts the color point for any combination of design parameters. In addition the model provides the reflection and transmission coefficients - as well as the energy density distribution inside the LED - of the scattered and re-emitted light intensities. To validate our model we performed extensive experiments on an emblematic white LED and found excellent agreement. Our model provides for a fast and efficient design, resulting in reduction of both design and production costs.

physics.optics↗

arXiv2018

"Cartesian light": unconventional propagation of light in a 3D superlattice of coupled cavities within a 3D photonic band gap

We explore the unconventional propagation of light in a three-dimensional (3D) superlattice of coupled resonant cavities in a 3D photonic band gap crystal. Such a 3D cavity superlattice is the photonic analogue of the Anderson model for spins and electrons in the limit of zero disorder. Using the plane-wave expansion method, we calculate the dispersion relations of the 3D cavity superlattice with the cubic inverse woodpile structure that reveal five coupled-cavity bands, typical of quadrupole-like resonances. For three out of five bands, we observe that the dispersion bandwidth is significantly larger in the $(k_x, k_z)$-diagonal directions than in other directions. To explain the directionality of the dispersion bandwidth, we employ the tight-binding method from which we derive coupling coefficients in 3D. For all converged coupled-cavity bands, we find that light hops predominantly in a few high-symmetry directions including the Cartesian $(x, y, z)$ directions, therefore we propose the name "Cartesian light". Such 3D Cartesian hopping of light in a band gap yields propagation as superlattice Bloch modes that differ fundamentally from the conventional 3D spatially-extended Bloch wave propagation in crystals, from light tunneling through a band gap, from coupled-resonator optical waveguiding, and also from light diffusing at the edge of a gap.

physics.optics↗

arXiv2018

Three-dimensional photonic band gap cavity with finite support: enhanced energy density and optical absorption

We study numerically the transport and storage of light in a 3D photonic band gap crystal doped by a single embedded resonant cavity. The crystal has finite support since it is surrounded by vacuum, as in experiments. Therefore, we employ the finite element method to model the diamond-like inverse woodpile crystal that consists of two orthogonal arrays of pores in a high-index dielectric such as silicon and that has experimentally been realized by CMOS-compatible methods. A point defect that functions as the resonant cavity is formed in the proximal region of two selected orthogonal pores with a radius smaller than the ones in the bulk of the crystal. We present a field-field cross-correlation method to identify resonances in the finite-support crystal with defect states that appear in the 3D photonic band gap of the infinite crystal. Out of 5 observed angle-independent cavity resonances, one is s-polarized and 4 are p-polarized for light incident in the X or Z directions. It is remarkable that quality factors up to Q = 1000 appear in such thin structures (3 unit cells). We find that the optical energy density is remarkably enhanced at the cavity resonances by up to 2400x the incident energy density in vacuum or up to 1200x the energy density of the equivalent effective medium. We find that an inverse woodpile photonic band gap cavity with a suitably adapted lattice parameter reveals substantial absorption in the visible range. Below the 3D photonic band gap, Fano resonances arise due to interference between the discrete fundamental cavity mode and the continuum light scattered by the photonic crystal. We argue that the five eigenstates of our 3D photonic band gap cavity have quadrupolar symmetry, in analogy to d-like orbitals of transition metals. We conclude that inverse woodpile cavities offer interesting perspectives for applications in optical sensing and photovoltaics.

physics.optics↗

arXiv2018

Finite size scaling of density of states in photonic bandgap crystals

The famous vanishing of the density of states (DOS) in a band gap, be it photonic or electronic, pertains to the infinite-crystal limit. In contrast, all experiments and device applications refer to finite crystals, which raises the question: Upon increasing the linear size $L$ of a crystal, how fast does the DOS approach the infinite-crystal limit? We present a theory for finite crystals that includes Bloch-mode broadening due to the presence of crystal boundaries. Our results demonstrate that the DOS for frequencies inside a band gap has a $1/L$ scale dependence for crystals in one, two and three dimensions.

physics.optics↗

arXiv2017

3D spatially-resolved optical energy density enhanced by wavefront shaping

We study the three-dimensional (3D) spatially-resolved distribution of the energy density of light in a 3D scattering medium upon the excitation of open transmission channels. The open transmission channels are excited by spatially shaping the incident optical wavefronts. To probe the local energy density, we excite isolated fluorescent nanospheres distributed inside the medium. From the spatial fluorescent intensity pattern we obtain the position of each nanosphere, while the total fluorescent intensity gauges the energy density. Our 3D spatially-resolved measurements reveal that the local energy density versus depth (z) is enhanced up to 26X at the back surface of the medium, while it strongly depends on the transverse (x; y) position. We successfully interpret our results with a newly developed 3D model that considers the time-reversed diffusion starting from a point source at the back surface. Our results are relevant for white LEDs, random lasers, solar cells, and biomedical optics.

physics.optics↗