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Willian M. H. Natori

Publications and source records attributed to Willian M. H. Natori.

6 recordsLinked to original sources

The spin-orbital Kitaev model: from kagome spin ice to classical fractons

We study an exactly solvable spin-orbital model that can be regarded as a classical analogue of the celebrated Kitaev honeycomb model and describes interactions between Rydberg atoms on the ruby lattice. We leverage its local and nonlocal symmetries to determine the exact partition function and the static structure factor. A mapping between $S=3/2$ models on the honeycomb lattice and kagome spin Hamiltonians allows us to interpret the thermodynamic properties in terms of a classical kagome spin ice. Partially lifting the symmetries associated with line operators, we obtain a model characterized by immobile excitations, called classical fractons, and a ground state degeneracy that increases exponentially with the length of the system. We formulate a continuum theory that reveals the underlying gauge structure and conserved charges. Extensions of our theory to other lattices and higher-spin systems are suggested.

cond-mat.str-el↗

An Exact Chiral Amorphous Spin Liquid

Topological insulator phases of non-interacting particles have been generalized from periodic crystals to amorphous lattices, which raises the question whether topologically ordered quantum many-body phases may similarly exist in amorphous systems? Here we construct a soluble chiral amorphous quantum spin liquid by extending the Kitaev honeycomb model to random lattices with fixed coordination number three. The model retains its exact solubility but the presence of plaquettes with an odd number of sides leads to a spontaneous breaking of time reversal symmetry. We unearth a rich phase diagram displaying Abelian as well as a non-Abelian quantum spin liquid phases with a remarkably simple ground state flux pattern. Furthermore, we show that the system undergoes a finite-temperature phase transition to a conducting thermal metal state and discuss possible experimental realisations.

cond-mat.str-el↗

Quantum liquids of the S=3/2 Kitaev honeycomb and related Kugel-Khomskii models

The $S=3/2$ Kitaev honeycomb model (KHM) is unique among the spin-$S$ Kitaev models due to a massive ground state quasi-degeneracy that hampered previous numerical and analytical studies. In a recent work~\cite{jin2022unveiling}, we showed how an SO(6) Majorana parton mean-field theory of the $S=3/2$ isotropic KHM explains the anomalous features of this Kitaev spin liquid (KSL) in terms of an emergent low-energy Majorana flat band. Away from the isotropic limit, the $S=3/2$ KSL generally displays a quadrupolar order with gapped or gapless Majorana excitations, features that were quantitatively confirmed by DMRG simulations. In this paper, we explore the connection between the $S = 3/2$ KHM with Kugel-Khomskii models and discover new exactly soluble examples for the latter. We perform a symmetry analysis for the variational parton mean-field \emph{Ans{ä}tze} in the spin and orbital basis for different quantum liquid phases of the $S=3/2$ KHM. Finally, we investigate a proposed time-reversal symmetry breaking spin liquid induced by a {[}111{]} single ion anisotropy and elucidate its topological properties as well as experimental signatures, e.g. an unquantized thermal Hall response.

cond-mat.str-el↗

Dynamics of a two-dimensional quantum spin-orbital liquid: spectroscopic signatures of fermionic magnons

We provide an exact study of dynamical correlations for the quantum spin-orbital liquid phases of an SU(2)-symmetric Kitaev honeycomb lattice model. We show that the spin dynamics in this Kugel-Khomskii type model is exactly the density-density correlation function of S=1 fermionic magnons, which could be probed in resonant inelastic x-ray scattering experiments. We predict the characteristic signatures of spin-orbital fractionalization in inelastic scattering experiments and compare them to the ones of the spin-anisotropic Kitaev honeycomb spin liquid. In particular, the resonant inelastic x-ray scattering response shows a characteristic momentum dependence directly related to the dispersion of fermionic excitations. The neutron scattering cross section displays a mixed response of fermionic magnons as well as spin-orbital excitations. The latter has a bandwidth of broad excitations and a vison gap that is three times larger than that of the spin-1/2 Kitaev model.

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Orbital Magnetic Field Effects in Mott Insulators with Strong Spin-Orbit Coupling

We study the effect of a magnetic field on the low energy description of Mott insulators with strong spin-orbit (SO) coupling. In contrast to the standard case of the Hubbard model without SO coupling, we show that Peierls phases can modulate the magnetic exchange at leading order in the interaction. Our mechanism crucially depends on the existence of distinct exchange paths between neighboring magnetic ions enclosing a well-defined area. Thus it will generically be present in any solid state realisation of the Kitaev model and its extensions. We explicitly calculate the variation of the exchange constants of the so-called $JKΓ$ model as a function of the magnetic flux. We discuss experimental implications of our findings for various settings of candidate Kitaev spin liquids.

cond-mat.str-el↗

SU(4)-symmetric spin-orbital liquids on the hyperhoneycomb lattice

We study the effective spin-orbital model that describes the magnetism of 4$d^1$ or 5$d^1$ Mott insulators in ideal tricoordinated lattices. In the limit of vanishing Hund's coupling, the model has an emergent SU(4) symmetry which is made explicit by means of a Klein transformation on pseudospin degrees of freedom. Taking the hyperhoneycomb lattice as an example, we employ parton constructions with fermionic representations of the pseudospin operators to investigate possible quantum spin-orbital liquid states. We then use variational Monte Carlo (VMC) methods to compute the energies of the projected wave functions. Our numerical results show that the lowest-energy quantum liquid corresponds to a zero-flux state with a Fermi surface of four-color fermionic partons. In spite of the Fermi surface, we demonstrate that this state is stable against tetramerization. A combination of linear flavor wave theory and VMC applied to the complete microscopic model also shows that this liquid state is stable against the formation of collinear long-range order.

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