arXiv subjects

Willian Natori

Publications and source records attributed to Willian Natori.

3 recordsLinked to original sources

arXiv2025

Ferrimagnetic Kitaev spin liquids in mixed spin 1/2 spin 3/2 honeycomb magnets

We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a superexchange theory specifically for this mixed-spin system, we identify the conditions under which dominant Kitaev-like interactions emerge. Focusing on the limiting case of pure Kitaev coupling with single-ion anisotropy, we employ a combination of superexchange theory, parton mean-field theory, and density matrix renormalization group (DMRG) simulations. We establish a comprehensive ground-state phase diagram identifying four distinct quantum spin liquid phases. Our findings highlight the importance of spin-orbital couplings and quadrupolar order parameters in stabilizing exotic phases, providing a foundation for exploring mixed-spin Kitaev magnets.

cond-mat.str-el↗

arXiv2020

Local Probes for Charge-Neutral Edge States in Two-Dimensional Quantum Magnets

The bulk-boundary correspondence is a defining feature of topological states of matter. However, for quantum magnets such as spin liquids or topological magnon insulators a direct observation of topological surface states has proven challenging because of the charge-neutral character of the excitations. Here we propose spin-polarized scanning tunneling microscopy as a spin-sensitive local probe to provide direct information about charge neutral topological edge states. We show how their signatures, imprinted in the local structure factor, can be extracted by specifically employing the strengths of existing technologies. As our main example, we determine the dynamical spin correlations of the Kitaev honeycomb model with open boundaries. We show that by contrasting conductance measurements of bulk and edge locations, one can extract direct signatures of the existence of fractionalized excitations and non-trivial topology. The broad applicability of this approach is corroborated by a second example of a kagome topological magnon insulator.

cond-mat.str-el↗

arXiv2017

Dynamics of a j=3/2 quantum spin liquid

We study a spin-orbital model for 4$d^{1}$ or 5$d^{1}$ Mott insulators in ordered double perovskites with strong spin-orbit coupling. This model is conveniently written in terms of pseudospin and pseudo-orbital operators representing multipoles of the effective $j=3/2$ angular momentum. Similarities between this model and the effective theories of Kitaev materials motivate the proposal of a chiral spin-orbital liquid with Majorana fermion excitations. The thermodynamic and spectroscopic properties of this quantum spin liquid are characterized using parton mean-field theory. The heat capacity, spin-lattice relaxation rate, and dynamic structure factor for inelastic neutron scattering are calculated and compared with the experimental data for the spin liquid candidate Ba$_{2}$YMoO$_{6}$. Moreover, based on a symmetry analysis, we discuss the operators involved in resonant inelastic X-ray scattering (RIXS) amplitudes for double perovskite compounds. In general, the RIXS cross sections allow one to selectively probe pseudospin and pseudo-orbital degrees of freedom. For the chiral spin-orbital liquid in particular, these cross sections provide information about the spectrum for different flavors of Majorana fermions.

cond-mat.str-el↗