arXiv subjects

Wojciech Brzezicki

Publications and source records attributed to Wojciech Brzezicki.

At least 19 recordsLinked to original sources

arXiv2026

Far-field terahertz spectroscopy across the charge-density-wave transition in 2H-NbSe$_2$

Charge-density-wave (CDW) formation in 2H-NbSe$_2$ modifies the low-energy electronic structure and gives rise to collective excitations coupled to the lattice. Here, we investigate bulk 2H-NbSe$_2$ single crystals using far-field terahertz time-domain spectroscopy (THz-TDS) in reflection geometry across the CDW transition at $T_{\mathrm{CDW}} \approx 33$~K. Below $T_{\mathrm{CDW}}$, the THz response shows a pronounced high-frequency feature near 1.5~THz together with longer-lived sub-THz oscillations. Both responses progressively weaken upon warming and are strongly suppressed across the CDW transition, supporting their association with the CDW state. Using time-dependent Ginzburg--Landau simulations, we reproduce the main features of the experimental THz response, associating the high-frequency response mainly with CDW amplitude dynamics and the sub-THz response with defect-pinned phase dynamics. The $\sim1.5$~THz feature lies close to the frequency range reported for the Raman CDW amplitude mode, while coupling to lattice degrees of freedom may also influence its spectral position. We also performed complementary angle-resolved photoemission spectroscopy measurements, which reveal momentum-selective redistribution of near-Fermi-level spectral weight across the transition. Together, these results show that far-field THz spectroscopy provides a sensitive probe of collective CDW dynamics in bulk 2H-NbSe$_2$.

cond-mat.mtrl-sci↗

arXiv2026

Tuning Dirac-Rashba and Double Dirac Cone Surface States of Topological Crystalline Insulator Pb$_{1-x}$Sn$_{x}$Se by Transition Metal Adsorbate

The electronic structure of topological insulator/magnetic metal (TI/MM) interfaces is of great importance for understanding of exotic spin-dependent phenomena and realization of advanced spin-orbitronic devices. Here, we employ a model system of submonolayer transition metal (TM) deposited on the surface of a topological crystalline insulator (TCI) of Pb$_{1-x}$Sn$_{x}$Se to systematically map out the modification of the surface electronic structure by angle-resolved photoemission spectroscopy (ARPES) as a function of coverage. For the polar (111) Pb$_{1-x}$Sn$_{x}$Se surface, we observe the coexistence of the Dirac topological surface states (TSS) and Rashba-split surface states (RSS) induced by the combined effects of inversion-symmetry breaking, surface band bending and orbital angular momentum effects. In particular, we demonstrate very large Rashba splittings can be obtained and the Rashba parameter ($α_R$) can be tuned over a remarkably wide range from 0 to 3.5 eV ${\cdot}$ $\mathring{\mathrm{A}}$, depending on the type and coverage of the TM adatoms. Model-Hamiltonian calculations corroborate the experimental findings and reveal that this coexistence results from the filling of the TSS by the surface doping caused by the TM. In contrast, for the nonpolar (001) surface exhibiting a double Dirac cone topological surface state, the inversion symmetry is preserved and hence no Rashba-split surface states emerge. Instead, surface charge imbalance induces dephasing of the wave functions of the double Dirac cones that diminishes the momentum-space separation between them. These findings shed light on novel phenomena occurring at the topological insulator / transition metal interface, offering a versatile platform for future spintronic and quantum devices.

cond-mat.mtrl-sci↗

arXiv2026

Band topology and symmetry-driven magneto-optical response in two-dimensional d-wave altermagnets with staggered spin-orbit coupling

Altermagnets combine compensated collinear magnetic order with momentum-dependent spin splitting, providing a route to transverse electronic and optical responses without a net ferromagnetic moment. We develop a strictly periodic four-band tight-binding model for a two-dimensional d-wave altermagnet and distinguish the roles of three spin orbit coupling (SOC) channels: uniform Rashba SOC, a sublattice-staggered Rashba interaction, and bond-staggered SOC. In the absence of SOC, the d-wave kinetic anisotropy produces spin-polarized Dirac points on orthogonal Brillouin-zone boundaries, related by the altermagnetic fourfold spin-group symmetry. Uniform Rashba SOC mixes the spin sectors and shifts these nodes but preserves the antiunitary symmetry that forbids an integrated Hall response. The sublattice-staggered Rashba term breaks this symmetry and activates transverse optical response, whereas the bond-staggered SOC provides the mass that gaps the boundary nodes. Their combined action generates strong Berry-curvature hot spots and, within a narrow parameter window, an isolated lower two-band manifold with Chern number C=-2. For the representative parameters considered here it is possible to stabilize a Chern insulator phase. Using covariant-velocity Kubo calculations, we show that large optical Hall conductivity and circular dichroism extend well beyond the nonzero-Chern region and are controlled by SOC-induced avoided crossings and symmetry breaking. We further find that carrier doping strongly modifies the resonant and dc Hall responses through Pauli blocking and the occupation of Berry-curvature hot spots, enabling gate-controlled sign reversals. These results identify the complementary roles of distinct interfacial SOC mechanisms in producing topology and tunable magneto-optical activity in compensated two-dimensional magnets.

cond-mat.mes-hall↗

arXiv2026

Unveiling Hidden Magnons with Anomalous Rotational Symmetry

Correlated materials with competing spin-orbit and crystal-field interactions can host composite spin-orbital magnons that are highly susceptible to structural and electronic perturbations, enabling the control of magnetic dynamics beyond spin-only physics. Using Raman spectroscopy on Ca$_2$RuO$_4$, we show that the partial substitution of Ru with Mn reconstructs the magnon spectrum and reveals one-magnon modes that are hidden in the undoped state. We demonstrate that the transition-metal substitution activates otherwise symmetry-forbidden magnon modes through mirror-symmetry breaking of the underlying spin-orbital configuration. This effect can be theoretically explained by the local structural distortions induced in the RuO$_6$ octahedra near the dopant, that enable the observation of mixed-parity one-magnon modes. These excitations display a distinctive polarization dependence, with a lowering from fourfold to twofold rotational symmetry arising from the mixed-parity character of the coupled magnons and interference between resonant and nonresonant scattering channels. Our results show that spin-orbit-lattice entanglement provides a route to tailoring collective magnetic excitations and their polarization response in spin-orbit-coupled correlated systems.

cond-mat.str-el↗

arXiv2025

Electronic and magnetic properties of the NdNiO$_2$/SrTiO$_3$ thin films

The hole-doped NdNiO$_2$ layer deposited on the SrTiO$_{3}$ surface exhibits unconventional superconductivity. Here, we present a systematic study of the electronic and magnetic properties of the NdNiO$_2$ superconductor using the density functional theory (DFT). The strong local Coulomb interactions in the Ni($3d)$ and Nd($4f$) states are included within the DFT+$U$ method. The effect of Sr doping on the electronic band structure and density of states was studied for the NdNiO$_2$ thin films deposited on the SrTiO$_3$ (001) surface. The results obtained for the uncapped thin films were compared with the calculations for the NdNiO$_2$ films capped by the SrTiO$_3$ layer. We have found significant changes in the electronic structure and magnetic properties of the thin films compared to the bulk crystal.

cond-mat.mtrl-sci↗

arXiv2025

Dual topology and edge-reconstruction in $α$-Sn

We formulate the tight-binding model for cubic $α$-Sn based on the DFT calculations. In the model, we incorporate a variable bond angle, which allows us to simulate the effect of the in-plane strain. In the bulk, we demonstrate the presence of the $\mathbb{Z}_2$ topological invariant and a non-zero mirror Chern number, making $α$-Sn one of the rare cases where dual topology can be observed. We calculate the topological phase diagram of multi-layer $α$-Sn as a function of strain and number of layers. We find that a non-trivial quantum spin Hall state appears only for compressive strain above five layers of thickness. Quite surprisingly, both in the trivial and non-trivial phases, we find a plethora of edge-states with energies inside the bulk gap of the system. Some of these states are localized at the side surfaces of the slab, some of them prefer top/bottom surfaces and some are localized in the hinges. We trace the microscopic origin of these states back to a minimal model that supports chiral symmetry and multiple one-dimensional winding numbers that take different values in different directions in the Brillouin zone.

cond-mat.mes-hall↗

arXiv2025

Neodymium ions as charge reservoir in NdNiO$_2$: from lack of long range order to electron-doping-induced antiferromagnetism

We study magnetism in the electron-doped infinite-layer nickelate NdNiO$_2$. We perform an unrestricted Hartree-Fock calculation for a tight-binding model which contains both nickel and neodymium orbitals. We reproduce the self-doping effect, which is the escape of charge onto the neodymium bands. By fixing all free parameters to realistic values we find that undoped NdNiO$_2$ lies right {\it outside} the antiferromagnetic (AFM) region of the phase diagram. This is consistent with experiments, which find no long-range order in the ground state of NdNiO$_2$, yet see short-range AFM correlations and broad magnetic excitations. We also find that the self-doping effect leads to a dramatic increase in the stability of the AFM solution upon electron doping -- a behavior that is strikingly different from what is, for instance, observed in the cuprates. Finally, for smaller charge transfer energies than suggested for NdNiO$_2$, the self-doping effect may be quite strong and stabilise various stripe configurations already on the mean-field level.

cond-mat.str-el↗

arXiv2025

Sign competing sources of Berry curvature and anomalous Hall conductance humps in topological ferromagnets

The use of Berry-phase concepts has established a strong link between the anomalous Hall effect (AHE) and the topological character of the Hall currents. However, the occurrence of sign competition in the Berry curvature often hinders the topological origin of the observed anomalous Hall effects. Here, we study a two-dimensional topological ferromagnet with coupled spin and orbital degrees of freedom to assess the anomalous Hall effects in the presence of sign-competing sources of Berry curvature. We show that 2D itinerant topological ferromagnets described by t2g electronic states can generally lead to topological metallic bands marked by a non-zero Chern number. We find that the resulting Berry curvature at the Fermi level exhibits a characteristic anisotropic profile with a non-monotonous angular dependence when the magnetization is reversed. The sign change of the intrinsic contribution to the anomalous Hall conductance can occur together with topological transitions or be driven by the population imbalance of the topological bands. The breaking of the inversion symmetry introduces the orbital Rashba coupling in the system. The interplay between the orbital Rashba and sign competing sources of Berry curvature leads to anomalies in the anomalous Hall conductance at values of magnetic fields for which the magnetization switches its orientation. The humps in topological ferromagnets arise when the anomalous Hall conductivity is small in absolute value and they can be detected only close to the sign-change of the AHE and far from half-filling. This study could be relevant for the family of the topological 2D ferromagnets as well as Weyl ferromagnets, and can particularly account for the variety of unconventional behaviors observed in ultrathin films of SrRuO$_3$.

cond-mat.str-el↗

arXiv2025

Filtering Spin and Orbital Moment in Centrosymmetric Systems

The control of spin and orbital angular momentum without relying on magnetic materials is commonly accomplished by breaking of inversion symmetry, which enables charge-to-spin conversion and spin selectivity in electron transfer processes occurring in chiral media. In contrast to this perspective, we show that orbital moment filtering can be accomplished in centrosymmetric systems: the electron states can be selectively manipulated allowing for the preferential transfer of electrons with a particular orbital momentum orientation. We find that orbital moment filtering is indeed efficiently controlled through orbital couplings that break both mirror and rotational symmetries. We provide the symmetry conditions required for the electron transmission to achieve orbital filtering and relate them to the orientation of the orbital moment. The presence of atomic spin-orbit interaction in the centrosymmetric transmission medium leads to the selective filtering of spin and orbital moments. Our findings allow to identify optimal regimes for having highly efficient simultaneous spin and orbital moment filtering.

cond-mat.other↗

arXiv2025

Anomalous spin-optical helical effect in Ti-based kagome metal

The kagome lattice stands as a rich platform for hosting a wide array of correlated quantum phenomena, ranging from charge density waves and superconductivity to electron nematicity and loop current states. Direct detection of loop currents in kagome systems has remained a formidable challenge due to their intricate spatial arrangements and the weak magnetic field signatures they produce. This has left their existence and underlying mechanisms a topic of intense debate. In this work, we uncover a hallmark reconcilable with loop currents: spin handedness-selective signals that surpass conventional dichroic, spin, and spin-dichroic responses. We observe this phenomenon in the kagome metal CsTi$_3$Bi$_5$ and we call it the anomalous spin-optical helical effect. This effect arises from the coupling of light' s helicity with spin-orbital electron correlations, providing a groundbreaking method to visualize loop currents in quantum materials. Our discovery not only enriches the debate surrounding loop currents but also paves the way for new strategies to exploit the electronic phases of quantum materials via light-matter interaction.

cond-mat.str-el↗

arXiv2025

Fate of gapless edge states in two-dimensional topological insulators with Hatsugai-Kohmoto interaction

Topologically protected edge states are the highlight feature of an interface between non-equivalent insulators. The robustness/sensitivity of these states to local single-particle perturbations is well understood, while their stability in the presence of various types of two-particle interactions remains unclear. To add to previous discussions of the Hubbard and unscreened Coulomb interactions, we address this problem from the point of view of infinite-range Hatsugai-Kohmoto interaction. Based on our numerical results for two models of Chern insulators, the Kane-Mele and spinful Haldane model, on a ribbon geometry with zig-zag edges, we argue that any finite interaction strength $U$ is sufficient to open a charge gap in the spectrum of either Chern insulator. We explain the differences between the two cases and present how their edge states phase out as the system enters the strongly correlated phase. We show that the closing of the many-body gap in periodic variants of these models can be connected to the onset of hybridization between the edge and bulk modes in finite geometries. Providing an example of the bulk-boundary correspondence in systems where there is a topological phase transition without closing of the spectral gap.

cond-mat.str-el↗

arXiv2024

Topology of chalcogen chains

We investigate the topological properties of the helical atomic chains occurring in elemental selenium and tellurium. We postulate a realistic model that includes spin-orbit interaction and show this to be topologically non-trivial, with a topological invariant protected by a crystalline symmetry. We describe the end-states, which are orbitally polarized, with an orbital density modulation strongly peaked at the edge. Furthermore, we propose a simplified model that decomposes into three orbital chains, allowing us to define a topological invariant protected by a crystalline symmetry. We contrast this result with recent observations made for the orbital Su-Schrieffer-Heeger model containing a $p$-orbital zigzag chain.

cond-mat.mtrl-sci↗

arXiv2024

Topological properties of the [110] SnTe nanowires

SnTe materials are know to be a platform for realization of various strong and symmetry protected topological phases in one, two and three spatial dimensions. We study symmetry-protected topological states in $[110]$ SnTe nanowires in the presence of various combinations of Zeeman field, $s-$wave superconductivity, inversion-symmetry-breaking field and the thickness of the wire. In the normal state we find a Weyl semimetal phase protected by a twofold screw axis symmetry and a topological insulating phase characterized by a $\mathbb{Z}$ invariant protected by a mirror symmetry. In the presence of superconductivity, we find inversion-symmetry-protected gapless phase which becomes fully gapped and topologically non-trivial by introducing an inversion-symmetry-breaking field. Consequently, we find topologically protected localized Majorana zero modes appear at the ends of the wire. We find that this Majorana phase is much easier to achieve in a $[110]$ SnTe nanowire than in a $[001]$ one.

cond-mat.mes-hall↗

arXiv2024

Non-hermitian topology and entanglement in an optomechanical superlattice

The interplay between topology, dissipation and nonlinearities can give rise to a wealth of new phenomena and pave the way for novel topological lasers, sensors and other quantum devices. Along these lines, we propose here an optomechanical setup in which the concomitant presence of a spatially modulated external drive and dissipation gives rise to a topologically nontrivial state for mechanical and optical excitations. We are able to show that the one-dimensional system considered here exhibits topologically protected end states for which mechanical and optical degrees of freedom are entangled. We show such entanglement to be robust with respect to the presence of nonzero-temperature baths and we propose a protocol for experimental observation of the entanglement.

quant-ph↗

arXiv2024

Pentagonal nanowires from topological crystalline insulators: a platform for intrinsic core-shell nanowires and higher-order topology

We report on the experimental realization of Pb1-xSnxTe pentagonal nanowires (NWs) with [110] orientation using molecular beam epitaxy techniques. Using first-principles calculations, we investigate the structural stability in NWs of SnTe and PbTe in three different structural phases: cubic, pentagonal with [001] orientation and pentagonal with [110] orientation. Within a semiclassical approach, we show that the interplay between ionic and covalent bonds favors the formation of pentagonal NWs. Additionally, we find that this pentagonal structure is more likely to occur in tellurides than in selenides. The disclination and twin boundary cause the electronic states originating from the NW core region to generate a conducting band connecting the valence and conduction bands, creating a symmetry-enforced metallic phase. The metallic core band has opposite slopes in the cases of Sn and Te twin boundary, while the bands from the shell are insulating. We finally study the electronic and topological properties of pentagonal NWs unveiling their potential as a new platform for higher-order topology and fractional charge. These pentagonal NWs represent a unique case of intrinsic core-shell one-dimensional nanostructures with distinct structural, electronic and topological properties between the core and the shell region.

cond-mat.mtrl-sci↗

arXiv2024

Signatures of a surface spin-orbital chiral metal

The relation between crystal symmetries, electron correlations, and electronic structure steers the formation of a large array of unconventional phases of matter, including magneto-electric loop currents and chiral magnetism. Detection of such hidden orders is a major goal in condensed matter physics. However, to date, nonstandard forms of magnetism with chiral electronic ordering have been experimentally elusive. Here, we develop a theory for symmetry-broken chiral ground states and propose a methodology based on circularly polarized spin-selective angular-resolved photoelectron spectroscopy to probe them. We exploit the archetypal quantum material Sr2RuO4 and reveal spectroscopic signatures which, even though subtle, may be reconciled with the formation of spin-orbital chiral currents at the material surface. As we shed light on these chiral regimes, our findings pave the way for a deeper understanding of ordering phenomena and unconventional magnetism.

cond-mat.str-el↗

arXiv2024

Impact of correlations on topology in Kane-Mele model decorated with impurities

We propose an effective model for the study of the interplay between correlation and topology by decorating the Kane-Mele model with a set of localized interacting orbitals hybridized to just one sublattice, breaking the inversion symmetry. We show that in the time-reversal symmetric case, the interplay between interactions and hybridization extends the stability of the topological phase and depending on the driving mechanism very different behaviors are observed after the topological phase transition (TPT). We discuss the fate of the TPT in presence of weak ferromagnetic order, by introducing a weak local magnetic field at the localized orbitals, which splits the two band inversion points. One of the platforms to apply this model to are ferrovalley compounds, which are characterized by two independent band inversion points. Understanding this family of materials is crucial for the development of the valleytronics. An alternative to spintronics, which uses valley polarization as opposed to spin degrees of freedom as the building block, promises great opportunities for the development of information storage.

cond-mat.str-el↗

arXiv2023

Topological Mott insulator in the odd-integer filled Anderson lattice model with Hatsugai-Kohmoto interactions

Recently, a quantum anomalous Hall state at odd integer filling in moiré stacked MoTe$_2$/WSe$_2$ was convincingly interpreted as a topological Mott insulator state appearing due to strong interactions in {\it band} basis [P. Mai, J. Zhao, B. E. Feldman, and P. W. Phillips, Nat. Commun. {\bf 14}, 5999 (2023)]. In this work, we aim to analyze the formation of a topological Mott insulator due to interactions in {\it orbital} basis instead, being more natural for systems where interactions originate from the character of $f$ or $d$ orbitals rather than band flatness. For that reason, we study an odd-integer filled Anderson lattice model incorporating odd-parity hybridization between orbitals with different degrees of correlations introduced in the Hatsugai-Kohmoto spirit. We demonstrate that a topological Mott insulating state can be realized in a considered model only when weak intra- and inter-orbital correlations involving dispersive states are taken into account. Interestingly, we find that all topological transitions between trivial and topological Mott insulating phases are not accompanied by a spectral gap closing, consistent with a phenomenon called {\it first-order topological transition}. Instead, they are signaled by a kink developed in spectral function at one of the time reversal invariant momenta. We believe that our approach can provide insightful phenomenology of topological Mott insulators in spin-orbit coupled $f$ or $d$ electron systems.

cond-mat.str-el↗