arXiv subjects

Wolfgang Tittel

Publications and source records attributed to Wolfgang Tittel.

At least 19 recordsLinked to original sources

arXiv2026

Optical characterization of excited-state spin Hamiltonians and clock transitions at telecommunication wavelength in Tm3+:YAlO3

The zero-phonon line (ZPL) between the two excited-state manifolds 3F4 and 3H4 of the trivalent thulium ion in yttrium aluminum perovskite (Tm3+:YAlO3) lies within the telecom E-band at around 1451 nm and exhibits an optical coherence time of a few μs at cryogenic temperatures. To improve this time in view of potential applications, e.g. single-photon sources and optical quantum memory, we characterized the magnetic properties of the lowest Stark levels of these two manifolds. Varying the external magnetic field amplitude and orientation, we measured the enhanced nuclear Zeeman splitting by probing the field-dependent frequency detuning of side holes created by means of spectral hole burning, and we characterized the inhomogeneous line shift caused by the quadratic Zeeman interaction. Together, this allowed us to establish the spin Hamiltonians for the lowest Stark level of the 3F4 and 3H4 manifolds, and to predict optical clock transitions for particular orientations and magnitudes of the magnetic field

quant-ph↗

arXiv2026

A unified framework for determining transition dipole polarization in solid-state spin defects

Spin-photon interfaces based on solid-state defects are key building blocks for scalable quantum networks and hybrid quantum platforms. Optimizing light-matter coupling in these systems requires precise knowledge of the optical transition dipole polarization, yet for many promising quantum emitters this quantity is hard to determine and therefore remains poorly characterized. Here, we develop a framework for reconstructing electric transition dipole polarization in spin-1/2 solid-state defects directly from ensemble spectroscopy. The approach combines the response of photoluminescence spectra to magnetic field, optical polarization, and strain. Applied to erbium ions in silicon, a particularly challenging system containing multiple crystallographic subsites, the framework identifies strain-induced shifts as the origin of asymmetric ensemble spectra and enables simultaneous determination of the optical dipole polarization and strain-orbital coupling tensor. The resulting model predicts how cavity-ion coupling depends on crystallographic orientation and magnetic-field direction, which we verify using single erbium ions coupled to a nanophotonic cavity. Together, these results establish a broadly applicable route for extracting microscopic properties of solid-state quantum emitters from ensemble spectroscopy and for engineering optimized spin-photon and spin-phonon interfaces.

quant-ph↗

arXiv2026

Spectroscopy and Coherence of an Excited-State Transition in Tm$^{3+}$:YAlO$_3$ at Telecommunication Wavelength

We characterize spectroscopic and coherence properties of the 1451.37 nm excited-state zero-phonon line (ZPL) between the $^{3}F_{4}$ and the $^{3}H_{4}$ manifolds of a thulium-doped yttrium aluminum perovskite (Tm$^{3+}$:YAlO$_3$) crystal at temperatures around 1.5 K. We measure the absorption spectrum between the $^{3}H_{6}$ - $^{3}F_{4}$ and $^{3}F_{4}$ - $^{3}H_{4}$ manifolds, the inhomogeneous broadening of the $^{3}F_{4}$ - $^{3}H_{4}$ (excited-state) ZPL, and the lifetimes of the higher-lying and lower-lying excited states. We also investigate level shifts caused by the quadratic Zeeman interaction as well as spectral hole-burning spectra with varying magnetic fields, providing insights into hyperfine interactions. Using again spectral holes but also optical free induction decays (FIDs), we assess optical coherence times, finding a maximum of $4.75 \pm 0.07~μs$ at B=2T and low ion concentration in the $^{3}F_{4}$ level. Our results -- the first to demonstrate coherence of an excited-state transition in a rare-earth crystal -- suggest the possibility of exploiting such transitions for quantum technology.

quant-ph↗

arXiv2025

Quantum networks using rare-earth ions

We review concepts and recent work related to creating light-matter interfaces for future quantum networks based on rare-earth ion-doped crystals. More precisely, we explore their unique suitability for creating photon sources, optical quantum memories for light, and qubits that allow quantum information processing. In addition, we review the state-of-the-art of elementary quantum repeater links, and provide suggestions for future research.

quant-ph↗

arXiv2024

Optical Investigations of Coherence and Relaxation Dynamics of a Thulium-doped Yttrium Gallium Garnet Crystal at sub-Kelvin Temperatures for Optical Quantum Memory

Rare-earth ion-doped crystals are of great interest for quantum memories, a central component in future quantum repeaters. To assess the promise of 1$\%$ Tm$^{3+}$-doped yttrium gallium garnet (Tm:YGG), we report measurements of optical coherence and energy-level lifetimes of its $^3$H$_6$ $\leftrightarrow$ $^3$H$_4$ transition at a temperature of around 500 mK and various magnetic fields. Using spectral hole burning, we find hyperfine ground-level (Zeeman level) lifetimes of several minutes at magnetic fields of less than 1000 G. We also measure coherence time exceeding one millisecond using two-pulse photon echoes. Three-pulse photon echo and spectral hole burning measurements reveal that due to spectral diffusion, the effective coherence time reduces to a few $μ$s over a timescale of around two hundred seconds. Finally, temporal and frequency-multiplexed storage of optical pulses using the atomic frequency comb protocol is demonstrated. Our results suggest Tm:YGG to be promising for multiplexed photonic quantum memory for quantum repeaters.

quant-ph↗

arXiv2024

Hybrid Quantum Repeaters with Ensemble-based Quantum Memories and Single-spin Photon Transducers

Reliable quantum communication over hundreds of kilometers is a daunting yet necessary requirement for a quantum internet. To overcome photon loss, the deployment of quantum repeater stations between distant network nodes is necessary. A plethora of different quantum hardware is being developed for this purpose, each platform with its own opportunities and challenges. Here, we propose to combine two promising hardware platforms in a hybrid quantum repeater architecture to lower the cost and boost the performance of long-distance quantum communication. We outline how ensemble-based quantum memories combined with single-spin photon transducers, which can transfer quantum information between a photon and a single spin, can facilitate massive multiplexing, efficient photon generation, and quantum logic for amplifying communication rates. As a specific example, we describe how a single Rubidium (Rb) atom coupled to nanophotonic resonators can function as a high-rate, telecom-visible entangled photon source with the visible photon being compatible with storage in a Thulium-doped crystal memory (Tm-memory) and the telecom photon being compatible with low loss fiber propagation. We experimentally verify that Tm and Rb transitions are in resonance with each other. Our analysis shows that by employing up to 9 repeater stations, each equipped with two Tm-memories capable of holding up to 625 storage modes, along with four single Rb atoms, one can reach a quantum communication rate of about 10 secret bits per second across distances of up to 1000 km.

quant-ph↗

arXiv2024

Qubit teleportation between a memory-compatible photonic time-bin qubit and a solid-state quantum network node

We report on a quantum interface linking a diamond NV center quantum network node and 795nm photonic time-bin qubits compatible with Thulium and Rubidium quantum memories. The interface makes use of two-stage low-noise quantum frequency conversion and waveform shaping to match temporal and spectral photon profiles. Two-photon quantum interference shows high indistinguishability of (89.5 $\pm$ 1.9)% between converted 795nm photons and the native NV center photons. We use the interface to demonstrate quantum teleportation including real-time feedforward from an unbiased set of 795nm photonic qubit input states to the NV center spin qubit, achieving a teleportation fidelity of (75.5 $\pm$ 1.0)%. This proof-of-concept experiment shows the feasibility of interconnecting different quantum network hardware.

quant-ph↗

arXiv2023

Towards a spectrally multiplexed quantum repeater

Extended quantum networks are based on quantum repeaters that often rely on the distribution of entanglement in an efficient and heralded fashion over multiple network nodes. Many repeater architectures require multiplexed sources of entangled photon pairs, multiplexed quantum memories, and photon detection that distinguishes between the multiplexed modes. Here we demonstrate the concurrent employment of (1) spectrally multiplexed cavity-enhanced spontaneous parametric down-conversion in a nonlinear crystal; (2) a virtually-imaged phased array that enables mapping of spectral modes onto distinct spatial modes for frequency-selective detection; and (3) a cryogenically cooled Tm3+:LiNbO3 crystal that allows spectral filtering in an approach that anticipates its use as a spectrally-multiplexed quantum memory. Through coincidence measurements, we demonstrate quantum correlations between energy-correlated photon pairs and a strong reduction of the correlation strength between all other photons. This constitutes an important step towards a frequency multiplexed quantum repeater.

quant-ph↗

arXiv2023

Frequency tunable, cavity-enhanced single erbium quantum emitter in the telecom band

Single quantum emitters embedded in solid-state hosts are an ideal platform for realizing quantum information processors and quantum network nodes. Among the currently-investigated candidates, Er$^{3+}$ ions are particularly appealing due to their 1.5 $μ$m optical transition in the telecom band as well as their long spin coherence times. However, the long lifetimes of the excited state -- generally in excess of 1 ms -- along with the inhomogeneous broadening of the optical transition result in significant challenges. Photon emission rates are prohibitively small, and different emitters generally create photons with distinct spectra, thereby preventing multi-photon interference -- a requirement for building large-scale, multi-node quantum networks. Here we solve this challenge by demonstrating for the first time linear Stark tuning of the emission frequency of a single Er$^{3+}$ ion. Our ions are embedded in a lithium niobate crystal and couple evanescently to a silicon nano-photonic crystal cavity that provides an up to 143 increase of the measured decay rate. By applying an electric field along the crystal c-axis, we achieve a Stark tuning greater than the ion's linewidth without changing the single-photon emission statistics of the ion. These results are a key step towards rare earth ion-based quantum networks.

quant-ph↗

arXiv2022

Long-Range QKD without Trusted Nodes is Not Possible with Current Technology

A recently published patent (https://www.ipo.gov.uk/p-ipsum/Case/PublicationNumber/GB2590064) has claimed the development of a novel quantum key distribution protocol purporting to achieve long-range quantum security without trusted nodes and without use of quantum repeaters. Here we present a straightforward analysis of this claim, and reach the conclusion that it is largely unfounded.

quant-ph↗

arXiv2022

Quadratic Zeeman Spectral Diffusion of Thulium Ion Population in a Yttrium Gallium Garnet Crystal

The creation of well understood structures using spectral hole burning is an important task in the use of technologies based on rare earth ion doped crystals. We apply a series of different techniques to model and improve the frequency dependent population change in the atomic level structure of Thulium Yttrium Gallium Garnet (Tm:YGG). In particular we demonstrate that at zero applied magnetic field, numerical solutions to frequency dependent three-level rate equations show good agreement with spectral hole burning results. This allows predicting spectral structures given a specific hole burning sequence, the underpinning spectroscopic material properties, and the relevant laser parameters. This enables us to largely eliminate power dependent hole broadening through the use of adiabatic hole-burning pulses. Though this system of rate equations shows good agreement at zero field, the addition of a magnetic field results in unexpected spectral diffusion proportional to the induced Tm ion magnetic dipole moment and average magnetic field strength, which, through the quadratic Zeeman effect, dominates the optical spectrum over long time scales. Our results allow optimization of the preparation process for spectral structures in a large variety of rare earth ion doped materials for quantum memories and other applications.

quant-ph↗

arXiv2022

Optical Properties of Yttrium Gallium Garnet

We report measurements of the reflection and transmission spectra of 2% doped Thulium Yttrium Gallium Garnet (Tm:YGG) using variable-angle spectroscopic ellipsometry(VASE) over a wavelength range from 210 to 1680 nm (0.73-5.9 eV). The well-known Tm resonances are identified and separated from the aggregate data, allowing us to calculate the previously unknown frequency dependence of the complex refractive index of the host material. This information is important for many applications of YGG in classical and quantum photonics, including constructing optical cavities, laser-based applications, and quantum information devices. A complete database of the obtained parameters is included in the supplementary information.

physics.optics↗

arXiv2021

Deployed MDI-QKD and Bell-State Measurements Coexisting with Standard Internet Data and Networking Equipment

The forthcoming quantum Internet is poised to allow new applications not possible with the conventional Internet. The ability for both quantum and conventional networking equipment to coexist on the same fiber network would greatly facilitate the deployment and adoption of coming quantum technology. Most quantum networking tasks, like quantum repeaters and the connection of quantum processors, require nodes for multi-qubit quantum measurements (often Bell-State measurements), and their real-world coexistence with the conventional Internet has yet to be shown. Here we field deploy an MDI-QKD system, containing a Bell-State measurement Node, over the same fiber network as multiple standard IP data networks, between three nearby cities in the Netherlands. We demonstrate over 10 Gb/s data communication rates simultaneously with our next-generation QKD system, and estimate 200 GB/s of classical data transmission would be easily achievable without significantly affecting QKD performance. Moreover, as the network ran autonomously for two weeks, this shows an important step towards the coexistence and integration of quantum networking into the existing telecommunication infrastructure.

quant-ph↗

arXiv2021

Spectrally Multiplexed Hong-Ou-Mandel Interference

We explore the suitability of a Virtually-Imaged Phased Array (VIPA) as a Spectral-to-Spatial Mode-Mapper (SSMM) for applications in quantum communication such as a quantum repeater. To this end we demonstrate spectrally-resolved two-photon "Hong-Ou-Mandel" (HOM) interference. Spectral sidebands are generated on a common optical carrier and weak coherent pulses are prepared in each spectral mode. The pulses are subsequently sent to a beamsplitter followed by two SSMMs and two single-photon detectors, allowing us to measure spectrally-resolved HOM interference. We show that the so-called HOM dip can be observed in the coincidence detection pattern of matching spectral modes with visibilities as high as 45% (with the maximum being 50%). For unmatched modes, the visibility drops significantly, as expected. Due to the similarity between HOM interference and a linear-optics Bell-state measurement (BSM), this establishes this simple optical arrangement as a candidate for the implementation of a spectrally-resolved BSM. Finally, we simulate the secret key generation rate using current and state-of-the-art parameters in a Measurement-Device Independent Quantum Key Distribution scenario and explore the trade-off between rate and complexity in the context of a spectrally-multiplexed quantum communication link.

quant-ph↗

arXiv2021

Measurement of the Thulium Ion Spin Hamiltonian Within a Yttrium Gallium Garnet Host Crystal

We characterize the magnetic properties for thulium ion energy levels in the Y$_3$Ga$_5$O$_{12}$ (Tm:YGG) lattice with the goal to improve decoherence and reduce line-width broadening caused by local host spins and crystal imperfections. More precisely, we measure hyperfine tensors for the lowest level of the, $^3$H$_6$, and excited, $^3$H$_4$, states using a combination of spectral hole burning, absorption spectroscopy, and optically detected nuclear magnetic resonance. By rotating the sample through a series of angles with an applied external magnetic field, we measure and analyze the orientation dependence of the Tm$^{3+}$ ion's spin-Hamiltonian. Using this spin-Hamiltonian, we propose a set of orientations to improve material properties that are important for light-matter interaction and quantum information applications. Our results yield several important external field directions: some to extend optical coherence times, another to improve spin inhomogeneous broadening, and yet another that maximizes mixing of the spin states for specific sets of ions, which allows improving optical pumping and creation of lambda systems in this material.

quant-ph↗

arXiv2021

A long-lived solid-state optical quantum memory for high-rate quantum repeaters

We argue that long optical storage times are required to establish entanglement at high rates over large distances using memory-based quantum repeaters. Triggered by this conclusion, we investigate the $^3$H$_6$ $\leftrightarrow$ $^3$H$_4$ transition at 795.325 nm of Tm:Y$_3$Ga$_5$O$_{12}$ (Tm:YGG). Most importantly, we show that the optical coherence time can reach 1.1 ms, and, using laser pulses, we demonstrate optical storage based on the atomic frequency comb protocol up to 100 $μ$s as well as a memory decay time T$_M$ of 13.1 $μ$s. Possibilities of how to narrow the gap between the measured value of T$_m$ and its maximum of 275 $μ$s are discussed. In addition, we demonstrate quantum state storage using members of non-classical photon pairs. Our results show the potential of Tm:YGG for creating quantum memories with long optical storage times, and open the path to building extended quantum networks.

quant-ph↗

arXiv2021

Optical coherence and energy-level properties of a Tm$^{3+}$-doped LiNbO$_{3}$ waveguide at sub-Kelvin temperatures

We characterize the optical coherence and energy-level properties of the 795 nm $^3$H$_6$ to $^3$H$_4$ transition of Tm$^{3+}$ in a Ti$^{4+}$:LiNbO$_{3}$ waveguide at temperatures as low as 0.65 K. Coherence properties are measured with varied temperature, magnetic field, optical excitation power and wavelength, and measurement time-scale. We also investigate nuclear spin-induced hyperfine structure and population dynamics with varying magnetic field and laser excitation power. Except for accountable differences due to difference Ti$^{4+}$ and Tm$^{3+}$-doping concentrations, we find that the properties of Tm$^{3+}$:Ti$^{4+}$:LiNbO$_{3}$ produced by indiffusion doping are consistent with those of a bulk-doped Tm$^{3+}$:LiNbO$_{3}$ crystal measured under similar conditions. Our results, which complement previous work in a narrower parameter space, support using rare-earth-ions for integrated optical and quantum signal processing.

physics.atom-ph↗

arXiv2020

Improved Light-Matter Interaction for Storage of Quantum States of Light in a Thulium-Doped Crystal Cavity

We design and implement an atomic frequency comb quantum memory for 793 nm wavelength photons using a monolithic cavity based on a thulium-doped Y$_3$Al$_5$O$_{12}$ (Tm:YAG) crystal. Approximate impedance matching results in the absorption of approximately $90\%$ of input photons and a memory efficiency of (27.5$\pm$ 2.7)% over a 500 MHz bandwidth. The cavity enhancement leads to a significant improvement over the previous efficiency in Tm-doped crystals using a quantum memory protocol. In turn, this allows us for the first time to store and recall quantum states of light in such a memory. Our results demonstrate progress toward efficient and faithful storage of single photon qubits with large time-bandwidth product and multi-mode capacity for quantum networking.

quant-ph↗