arXiv subjects

Wu Shi

Publications and source records attributed to Wu Shi.

At least 19 recordsLinked to original sources

arXiv2026

Giant bulk photovoltaic effect driven by interfacial symmetry breaking in MoS2/Ta2NiSe5 heterostructures

Van der Waals (vdW) heterostructures offer a versatile platform for engineering unconventional bulk photovoltaic (BPV) effect through interfacial symmetry breaking. However, the coexistence of multiple photophysical mechanisms, driven by structural complexity, spontaneous charge transfer, and strong interlayer coupling, often obscures the microscopic origin of the BPV response and hinders its rational optimization. Here, we demonstrate a pronounced BPV effect localized at the overlap region of a cross-bar MoS2/Ta2NiSe5 vdW heterostructure, where symmetry breaking induced by vertical stacking lifts the inversion center of MoS2. The orthogonal device geometry enables the independent probing of intralayer and interfacial photoresponse pathways, facilitating clear separation of competing mechanisms. Spontaneous interfacial charge transfer between MoS2 and Ta2NiSe5 further establishes a strong interlayer electronic coupling. By modulating the interlayer potential landscape through gate voltage and vertical electric fields, we achieve an optimized zero-bias photocurrent density of 247 A/cm2 and a BPV coefficient of 0.99 V-1. Supported by theoretical modelling, our results illustrate how minimalist device geometry can transform complex heterostructures into experimentally tractable platforms. This strategy paves the way for analyzing and optimizing interface-driven BPV effect, with implications for self-powered optoelectronics, broadband photodetection, and energy-harvesting nanodevices.

cond-mat.mes-hall↗

arXiv2026

Electric field switching of altermagnetic spin-splitting in multiferroic skyrmions

Magnetic skyrmions are localized magnetic structures that retain their shape and stability over time, thanks to their topological nature. Recent theoretical and experimental progress has laid the groundwork for understanding magnetic skyrmions characterized by negligible net magnetization and ultrafast dynamics. Notably, skyrmions emerging in materials with altermagnetism, a novel magnetic phase featuring lifted Kramers degeneracy-have remained unreported until now. In this study, we demonstrate that BiFeO3, a multiferroic renowned for its strong coupling between ferroelectricity and magnetism, can transit from a spin cycloid to a Neel-type skyrmion under antidamping spin-orbit torque at room temperature. Strikingly, the altermagnetic spin splitting within BiFeO3 skyrmion can be reversed through the application of an electric field, revealed via the Circular photogalvanic effect. This quasiparticle, which possesses a neutral topological charge, holds substantial promise for diverse applications-most notably, enabling the development of unconventional computing systems with low power consumption and magnetoelectric controllability.

cond-mat.mtrl-sci↗

arXiv2025

Rewritable Complementary Nanoelectronics Enabled by Electron-Beam Programmable Ambipolar Doping

The ability to reversibly and site-selectively tune ambipolar doping in a single semiconductor is crucial for reconfigurable electronics beyond silicon, but remains highly challenging. Here, we present a rewritable architecture based on electron-beam programmable field-effect transistors (FETs). Using WSe$_2$ as a model system, we demonstrate electron-beam-induced doping that enables reversible, precisely controlled carrier modulation exceeding $10^{13}$ cm$^{-2}$. The in-situ writing, erasing, and rewriting of ambipolar doping of nanoscale patterns was directly visualized by scanning microwave impedance microscopy. This mask-free, lithography-compatible approach can achieve precise band engineering within individual channels, yielding near-ideal subthreshold swings (~ 60 mV/dec) and finely tunable threshold voltages for both carrier types without specialized contact engineering. These capabilities allow on-demand realization of high performance logic, including CMOS inverters with high voltage gains and low power consumption, as well as NAND-to-NOR transitions on the same device via direct polarity rewriting. Our platform offers a scalable and versatile route for rapid prototyping of complementary electronics.

cond-mat.mtrl-sci↗

arXiv2025

Acoustoelectric Probing of Fractal Energy Spectra in Graphene/hBN Moir\'e Superlattices

Moir\'e superlattices with long-range periodicity exhibit Hofstadter energy spectra under accessible magnetic fields, enabling the exploration of emergent quantum phenomena through a hierarchy of fractal states. However, higher-order features, located at elevated energies with narrow bandwidths, typically require high carrier densities and remain difficult to resolve using conventional electrical transport due to limited sensitivity and strong background conductivity. Here, we utilize acoustoelectric (AE) transport to probe high-order fractal states and the Hofstadter spectrum in graphene/hBN moir\'e superlattices. Surface acoustic waves on a ferroelectric LiNbO$_3$ substrate generate an AE voltage proportional to the derivative of electrical conductivity, significantly enhancing sensitivity to weak spectral features. Combined with substrate-induced high electron doping, this technique resolves fractal Brown-Zak oscillations up to the fifth-order and provides the first AE observation of the Hofstadter butterfly, revealing high-order fractal magnetic Bloch states and symmetry-broken Landau levels over a wide carrier density range. Our results establish AE transport as a powerful derivative-sensitive probe for emergent fractal quantum states in moir\'e-engineered 2D systems.

cond-mat.mes-hall↗

arXiv2025

Harnessing Diffusion-Yielded Score Priors for Image Restoration

Deep image restoration models aim to learn a mapping from degraded image space to natural image space. However, they face several critical challenges: removing degradation, generating realistic details, and ensuring pixel-level consistency. Over time, three major classes of methods have emerged, including MSE-based, GAN-based, and diffusion-based methods. However, they fail to achieve a good balance between restoration quality, fidelity, and speed. We propose a novel method, HYPIR, to address these challenges. Our solution pipeline is straightforward: it involves initializing the image restoration model with a pre-trained diffusion model and then fine-tuning it with adversarial training. This approach does not rely on diffusion loss, iterative sampling, or additional adapters. We theoretically demonstrate that initializing adversarial training from a pre-trained diffusion model positions the initial restoration model very close to the natural image distribution. Consequently, this initialization improves numerical stability, avoids mode collapse, and substantially accelerates the convergence of adversarial training. Moreover, HYPIR inherits the capabilities of diffusion models with rich user control, enabling text-guided restoration and adjustable texture richness. Requiring only a single forward pass, it achieves faster convergence and inference speed than diffusion-based methods. Extensive experiments show that HYPIR outperforms previous state-of-the-art methods, achieving efficient and high-quality image restoration.

cs.CV↗

arXiv2025

Observation of ferron transport in ferroelectrics

Ferroelectrics feature spontaneous electric dipolar order reconfigurable via electric fields. Recent theoretical studies of the collective excitations of this electric dipolar order give rise to the hope that "ferron" quasiparticles may complement the magnons of magnetic materials in information and heat management technologies. Yet direct experimental evidence of ferron transport remains elusive. Here we demonstrate efficient ferron injection and detection enabled by ferromagnetic metal contacts, achieving nonlocal signal transmission over micrometer distances in a prototypical ferroelectric PMN-PT. The transmission efficiency can be switched by external magnetic fields that couple to the contacts and gate electric fields that control the ferron excitations. Ferron-based devices open new power saving strategies that employ ferroelectric materials in a future sustainable information society.

physics.app-ph↗

arXiv2025

Unexpected large electrostatic gating by pyroelectric charge accumulation

Pyroelectricity refers to the accumulation of charges due to changes in the spontaneous polarization of ferroelectric materials when subjected to temperature variations. Typically, these pyroelectric charges are considered unstable and dissipate quickly through interactions with the external environment. Consequently, the pyroelectric effect has been largely overlooked in ferroelectric field-effect transistors. In this work, we leverage the van der Waals interface of hBN to achieve a substantial and long-term electrostatic gating effect in graphene devices via the pyroelectric properties of a ferroelectric LiNbO3 substrate. Upon cooling, the polarization change in LiNbO3 induces high doping concentrations up to 1013 cm-2 in the adjacent graphene. Through a combination of transport measurements and non-contact techniques, we demonstrate that the pyroelectric charge accumulation, as well as its enhancement in electric fields, are responsible for this unexpectedly high doping level. Our findings introduce a novel mechanism for voltage-free electrostatic gating control with long retention.

cond-mat.mtrl-sci↗

arXiv2025

Broadband photoresponse enhancement by band engineering in Sb-doped MnBi2Te4

Topological materials have attracted considerable attention for their potential in broadband and fast photoresponse, particularly in the infrared regime. However, the high carrier concentration in these systems often leads to rapid recombination of photogenerated carriers, limiting the photoresponsivity. Here, we demonstrate that Sb doping in MnBi2Te4 effectively reduces carrier concentration and suppresses electron-hole recombination, thereby significantly improving the optoelectronic performance across the visible to mid-infrared spectra. The optimally doped Mn(Bi0.82Sb0.18)2Te4 photodetector achieves a responsivity of 3.02 mA W-1 with a response time of 18.5 {\mu}s at 1550 nm, and 0.795 mA W-1 with a response time of 9.0 {\mu}s at 4 {\mu}m. These values represent nearly two orders of magnitude improvement compared to undoped MnBi2Te4. Our results highlight band engineering as an effective strategy to enhance the infrared performance of topological material-based photodetectors, opening new avenues for high-sensitivity infrared detection.

cond-mat.mtrl-sci↗

arXiv2025

Coherent detection of the oscillating acoustoelectric effect in graphene

In recent years, surface acoustic waves (SAWs) have emerged as a novel technique for generating quasiparticle transport and band modulation in condensed matter systems. SAWs interact with adjacent materials through piezoelectric and strain fields, dragging carriers in the direction of wave propagation. Most studies on the acoustoelectric effect have focused on the collective directional motion of carriers, which generates a steady electric potential difference, while the oscillating component from dynamic spatial charge modulation has remained challenging to probe. In this work, we report the coherent detection of oscillating acoustoelectric effect in graphene. This is achieved through the coherent rectification of spatial-temporal charge oscillation with electromagnetic waves emitted by interdigital transducers. We systematically investigate the frequency and gate dependence of rectified signals and quantitatively probe the carrier redistribution dynamics driven by SAWs. The observation of oscillating acoustoelectric effect provides direct access to the dynamic spatial charge modulation induced by SAWs through transport experiments.

cond-mat.mes-hall↗

arXiv2024

Magnetoresistance oscillations in vertical junctions of 2D antiferromagnetic semiconductor CrPS$_4$

Magnetoresistance (MR) oscillations serve as a hallmark of intrinsic quantum behavior, traditionally observed only in conducting systems. Here we report the discovery of MR oscillations in an insulating system, the vertical junctions of CrPS$_4$ which is a two dimensional (2D) A-type antiferromagnetic semiconductor. Systematic investigations of MR peaks under varying conditions, including electrode materials, magnetic field direction, temperature, voltage bias and layer number, elucidate a correlation between MR oscillations and spin-canted states in CrPS$_4$. Experimental data and analysis point out the important role of the in-gap electronic states in generating MR oscillations, and we proposed that spin selected interlayer hopping of localized defect states may be responsible for it. Our findings not only illuminate the unusual electronic transport in CrPS$_4$ but also underscore the potential of van der Waals magnets for exploring interesting phenomena.

cond-mat.mes-hall↗

arXiv2024

Memristive switching in the surface of a charge-density-wave topological semimetal

Owing to the outstanding properties provided by nontrivial band topology, topological phases of matter are considered as a promising platform towards low-dissipation electronics, efficient spin-charge conversion, and topological quantum computation. Achieving ferroelectricity in topological materials enables the non-volatile control of the quantum states, which could greatly facilitate topological electronic research. However, ferroelectricity is generally incompatible with systems featuring metallicity due to the screening effect of free carriers. In this study, we report the observation of memristive switching based on the ferroelectric surface state of a topological semimetal (TaSe4)2I. We find that the surface state of (TaSe4)2I presents out-of-plane ferroelectric polarization due to surface reconstruction. With the combination of ferroelectric surface and charge-density-wave-gapped bulk states, an electric switchable barrier height can be achieved in (TaSe4)2I-metal contact. By employing a multi-terminal grounding design, we manage to construct a prototype ferroelectric memristor based on (TaSe4)2I with on/off ratio up to 10^3, endurance over 10^3 cycles, and good retention characteristics. The origin of the ferroelectric surface state is further investigated by first-principles calculations, which reveals an interplay between ferroelectricity and band topology. The emergence of ferroelectricity in (TaSe4)2I not only demonstrates it as a rare but essential case of ferroelectric topological materials, but also opens new routes towards the implementation of topological materials in functional electronic devices.

cond-mat.mtrl-sci↗

arXiv2024

Gate-tunable quantum acoustoelectric transport in graphene

Transport probes the motion of quasiparticles in response to external excitations. Apart from the well-known electric and thermoelectric transport, acoustoelectric transport induced by traveling acoustic waves has been rarely explored. Here, by adopting a hybrid nanodevices integrated with piezoelectric substrates, we establish a simple design of acoustoelectric transport with gate tunability. We fabricate dual-gated acoustoelectric devices based on BN-encapsuled graphene on LiNbO3. Longitudinal and transverse acoustoelectric voltages are generated by launching pulsed surface acoustic wave. The gate dependence of zero-field longitudinal acoustoelectric signal presents strikingly similar profiles as that of Hall resistivity, providing a valid approach for extracting carrier density without magnetic field. In magnetic fields, acoustoelectric quantum oscillations appear due to Landau quantization, which are more robust and pronounced than Shubnikov-de Haas oscillations. Our work demonstrates a feasible acoustoelectric setup with gate tunability, which can be extended to the broad scope of various Van der Waals materials.

cond-mat.mes-hall↗

arXiv2024

Unveiling the origin of unconventional moire ferroelectricity

Interfacial ferroelectricity emerges in heterostructures consisting of nonpolar van der Waals (vdW) layers, greatly expanding the scope of two dimensional ferroelectrics. In particular, the unconventional moire ferroelectricity observed in bilayer graphene/boron nitride (BN) heterostructures, exhibits promising functionalities with topological current, superconductivity and synaptic responses. However, the debate about its mechanism - correlation driven charge transfer between two graphene layers - limits device reproducibility and hence large-scale production. Here by designing a single-layer graphene encapsulated by lattice-mismatched WSe2, we identify the ferroelectricity as stemming from - instead of graphene moire bands - the particular BN, where interfacial sliding ferroelectricity must play a role. With similar structures, multilayer twisted MoS2 is found to reproduce the ferroelectricity. The key is a conductive moire ferroelectric, where the screened gate and the pinned domain wall together result in unchanged electronic states, i.e. anomalous screening. The intimate connection to interfacial sliding ferroelectricity thus provides advantages of diverse choices of constituent materials and robust polarization switching while preserving the unique anomalous screening, paving the way to reproducible and reliable memory-based devices in artificial intelligence.

cond-mat.mtrl-sci↗

arXiv2023

Acousto-drag photovoltaic effect by piezoelectric integration of two-dimensional semiconductors

Light-to-electricity conversion is crucial for energy harvesting and photodetection, requesting efficient electron-hole pair separation to prevent recombination. Traditional junction-based mechanisms using built-in electric fields fail in non-barrier regions. Homogeneous material harvesting under photovoltaic effect is appealing but only realized in non-centrosymmetric systems via bulk photovoltaic effect. Here we report the realization of photovoltaic effect by employing surface acoustic waves (SAW) to generate zero-bias photocurrent in a conventional layered semiconductor MoSe2. SAW induces periodic modulation to electronic bands and drags the photoexcited pairs toward the travelling direction. The photocurrent is extracted by a local barrier. The separation of generation and extraction processes suppresses recombination and yields large nonlocal photoresponse. We distinguish acousto-electric drag and electron-hole pair separation effect by fabricating devices of different configurations. The acousto-drag photovoltaic effect, enabled by piezoelectric integration, offers an efficient light-to-electricity conversion method, independent of semiconductor crystal symmetry.

cond-mat.mes-hall↗

arXiv2023

Absence of metallicity and bias-dependent resistivity in low-carrier-density EuCd2As2

EuCd2As2 was theoretically predicted to be a minimal model of Weyl semimetals with a single pair of Weyl points in the ferromagnet state. However, the heavily p-doped EuCd2As2 crystals in previous experiments prevent direct identification of the semimetal hypothesis. Here we present a comprehensive magneto-transport study of high-quality EuCd2As2 crystals with ultralow bulk carrier density (10^13 cm-3). In contrast to the general expectation of a Weyl semimetal phase, EuCd2As2 shows insulating behavior in both antiferromagnetic and ferromagnetic states as well as surface-dominated conduction from band bending. Moreover, the application of a dc bias current can dramatically modulate the resistance by over one order of magnitude, and induce a periodic resistance oscillation due to the geometric resonance. Such nonlinear transport results from the highly nonequilibrium state induced by electrical field near the band edge. Our results suggest an insulating phase in EuCd2As2 and put a strong constraint on the underlying mechanism of anomalous transport properties in this system.

cond-mat.mes-hall↗

arXiv2022

Improving Training and Inference of Face Recognition Models via Random Temperature Scaling

Data uncertainty is commonly observed in the images for face recognition (FR). However, deep learning algorithms often make predictions with high confidence even for uncertain or irrelevant inputs. Intuitively, FR algorithms can benefit from both the estimation of uncertainty and the detection of out-of-distribution (OOD) samples. Taking a probabilistic view of the current classification model, the temperature scalar is exactly the scale of uncertainty noise implicitly added in the softmax function. Meanwhile, the uncertainty of images in a dataset should follow a prior distribution. Based on the observation, a unified framework for uncertainty modeling and FR, Random Temperature Scaling (RTS), is proposed to learn a reliable FR algorithm. The benefits of RTS are two-fold. (1) In the training phase, it can adjust the learning strength of clean and noisy samples for stability and accuracy. (2) In the test phase, it can provide a score of confidence to detect uncertain, low-quality and even OOD samples, without training on extra labels. Extensive experiments on FR benchmarks demonstrate that the magnitude of variance in RTS, which serves as an OOD detection metric, is closely related to the uncertainty of the input image. RTS can achieve top performance on both the FR and OOD detection tasks. Moreover, the model trained with RTS can perform robustly on datasets with noise. The proposed module is light-weight and only adds negligible computation cost to the model.

cs.CV↗

arXiv2022

GCFSR: a Generative and Controllable Face Super Resolution Method Without Facial and GAN Priors

Face image super resolution (face hallucination) usually relies on facial priors to restore realistic details and preserve identity information. Recent advances can achieve impressive results with the help of GAN prior. They either design complicated modules to modify the fixed GAN prior or adopt complex training strategies to finetune the generator. In this work, we propose a generative and controllable face SR framework, called GCFSR, which can reconstruct images with faithful identity information without any additional priors. Generally, GCFSR has an encoder-generator architecture. Two modules called style modulation and feature modulation are designed for the multi-factor SR task. The style modulation aims to generate realistic face details and the feature modulation dynamically fuses the multi-level encoded features and the generated ones conditioned on the upscaling factor. The simple and elegant architecture can be trained from scratch in an end-to-end manner. For small upscaling factors (<=8), GCFSR can produce surprisingly good results with only adversarial loss. After adding L1 and perceptual losses, GCFSR can outperform state-of-the-art methods for large upscaling factors (16, 32, 64). During the test phase, we can modulate the generative strength via feature modulation by changing the conditional upscaling factor continuously to achieve various generative effects.

cs.CV↗

arXiv2019

Learning to Synthesize Fashion Textures

Existing unconditional generative models mainly focus on modeling general objects, such as faces and indoor scenes. Fashion textures, another important type of visual elements around us, have not been extensively studied. In this work, we propose an effective generative model for fashion textures and also comprehensively investigate the key components involved: internal representation, latent space sampling and the generator architecture. We use Gram matrix as a suitable internal representation for modeling realistic fashion textures, and further design two dedicated modules for modulating Gram matrix into a low-dimension vector. Since fashion textures are scale-dependent, we propose a recursive auto-encoder to capture the dependency between multiple granularity levels of texture feature. Another important observation is that fashion textures are multi-modal. We fit and sample from a Gaussian mixture model in the latent space to improve the diversity of the generated textures. Extensive experiments demonstrate that our approach is capable of synthesizing more realistic and diverse fashion textures over other state-of-the-art methods.

cs.CV↗