arXiv subjects

X. -X. Wu

Publications and source records attributed to X. -X. Wu.

7 recordsLinked to original sources

arXiv2020

Orbital selectivity of layer resolved tunneling on iron superconductor Ba0.6K0.4Fe2As2

We use scanning tunneling microscopy/spectroscopy (STM/S) to elucidate the Cooper pairing of the iron pnictide superconductor Ba0.6K0.4Fe2As2. By a cold-cleaving technique, we obtain atomically resolved termination surfaces with different layer identities. Remarkably, we observe that the low-energy tunneling spectrum related to superconductivity has an unprecedented dependence on the layer-identity. By cross-referencing with the angle-revolved photoemission results and the tunneling data of LiFeAs, we find that tunneling on each termination surface probes superconductivity through selecting distinct Fe-3d orbitals. These findings imply the real-space orbital features of the Cooper pairing in the iron pnictide superconductors, and propose a new and general concept that, for complex multi-orbital material, tunneling on different terminating layers can feature orbital selectivity.

cond-mat.supr-con↗

arXiv2019

Observation of topological transition in high-T$_{c}$ superconductor FeTe$_{1-x}$Se$_{x}$/SrTiO$_{3}$(001) monolayers

Superconductors with topological surface or edge states have been intensively explored for the prospect of realizing Majorana bound states, which obey non-Abelian statistics and are crucial for topological quantum computation. The traditional routes for making topological insulator/superconductor and semiconductor/superconductor heterostructures suffer fabrication difficulties and can only work at low temperature. Here, we use angle-resolved photoemission spectroscopy to directly observe the evolution of a topological transition of band structure nearby the Fermi level in two-dimensional high-T$_{c}$ superconductor FeTe$_{1-x}$Se$_{x}$/SrTiO$_{3}$(001) monolayers, fully consistent with our theoretical calculations. Furthermore, evidence of edge states is revealed by scanning tunneling spectroscopy with assistance of theoretical calculations. Our study provides a simple and tunable platform for realizing and manipulating Majorana states at high temperature.

cond-mat.supr-con↗

arXiv2016

Enhanced superconductivity accompanying a Lifshitz transition in electron-doped FeSe monolayer

The origin of enhanced superconductivity over 50 K in the recently discovered FeSe monolayer films grown on SrTiO$_{3}$ (STO), as compared to 8 K in bulk FeSe, is intensely debated. As with the ferrochalcogenides A$_{x}$Fe$_{2-y}$Se$_{2}$ and potassium doped FeSe, which also have a relatively high superconducting critical temperature ($T_c$), the Fermi surface (FS) of the FeSe/STO monolayer films is free of hole-like FS, suggesting that a Lifshitz transition by which these hole FSs vanish may help increasing $T_c$. However, the fundamental reasons explaining this increase of $T_c$ remain unclear. Here we report a 15 K jump of $T_c$ accompanying a second Lifshitz transition, characterized by the emergence of an electron pocket at the Brillouin zone (BZ) centre, that is triggered by high electron doping following in-situ deposition of potassium on FeSe/STO monolayer films. Our results suggest that the pairing interactions are orbital-dependent with the $d_{xy}$ orbital playing a determining role in generating enhanced superconductivity in FeSe.

cond-mat.supr-con↗

arXiv2016

Cooper Pairing and Phase Coherence in Iron Superconductor Fe1+x(Te,Se)

The Cooper pairing and phase coherence are two fundamental aspects of superconductivity. Due to breaking time reversal symmetry, magnetic impurities are detrimental to superconductivity, yet microscopically how they affect the pairing strength and phase coherence in a real material is less understood. Recently we observed a robust zero-energy bound state at an interstitial Fe impurity (IFI) in superconducting Fe1+x(Te,Se), signifying intense impurity scattering. Here we report a comprehensive study, using scanning tunnelling microscopy/spectroscopy (STM/S) technique, of the global effects of IFIs on the ground state of Fe1+x(Te,Se) over a wide range of IFI concentration x. Our high resolution tunnelling spectroscopy and quasi-particle interference data at very low temperature demonstrate that IFIs hardly affect the electron pairing strength, while they cause significant decoherence of Cooper pairs in precedence of the Coulomb correlation, eventually driving the ground state of the system from strong-coupling-superconductor to diffusive-metal with incoherent electron pairs.

cond-mat.supr-con↗

arXiv2014

Observation of momentum-confined in-gap impurity state in Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$: evidence for anti-phase $s_{\pm}$ pairing

We report the observation by angle-resolved photoemission spectroscopy of an impurity state located inside the superconducting gap of Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ and vanishing above the superconducting critical temperature, for which the spectral weight is confined in momentum space near the Fermi wave vector positions. We demonstrate, supported by theoretical simulations, that this in-gap state originates from weak non-magnetic scattering between bands with opposite sign of the superconducting gap phase. This weak scattering, likely due to off-plane Ba/K disorders, occurs mostly among neighboring Fermi surfaces, suggesting that the superconducting gap phase changes sign within holelike (and electronlike) bands. Our results impose severe restrictions on the models promoted to explain high-temperature superconductivity in these materials.

cond-mat.supr-con↗

arXiv2014

Observation of a Robust Zero-energy Bound State in Iron-based Superconductor Fe(Te,Se)

A robust zero-energy bound state (ZBS) in a superconductor, such as a Majorana or Andreev bound state, is often a consequence of non-trivial topological or symmetry related properties, and can provide indispensable information about the superconducting state. Here we use scanning tunneling microscopy/spectroscopy to demonstrate, on the atomic scale, that an isotropic ZBS emerges at the randomly distributed interstitial excess Fe sites in the superconducting Fe(Te,Se). This ZBS is localized with a short decay length of ~ 10 Å, and surprisingly robust against a magnetic field up to 8 Tesla, as well as perturbations by neighboring impurities. We find no natural explanation for the observation of such a robust zero-energy bound state, indicating a novel mechanism of impurities or an exotic pairing symmetry of the iron-based superconductivity.

cond-mat.supr-con↗

arXiv2012

Testing quantum entanglement with local measurement

We propose to detect quantum entanglement by a condition of local measurments. We find that this condition can detect efficiently the pure entangled states for both discrete and continuous variable systems. It does not depend on interference of decoherence from noise and detection loss in some systems, which allows a loophole-free test in real experiments. In particular, it is a necessary condition for the violation of some generalized Bell inequalities.

quant-ph↗