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X. C. Hong

Publications and source records attributed to X. C. Hong.

At least 19 recordsLinked to original sources

Nematicity in LaFeAsO single crystals studied by elastoresistance, high-resolution thermal expansion and shear-modulus measurements

Nematicity in LaFeAsO single crystals is studied by means of high-resolution thermal expansion, shear modulus, and elastoresistivity measurements. A softening of the shear modulus $C_{\rm 66}$ towards the structural phase transition at $T_{\rm S}$ is observed. In addition, a similar Curie-Weiss-like divergence of the nematic susceptibilities is found in the temperature dependence of both $\chi^{sh}$ and $\chi^{er}$, which are deduced from the shear modulus (sh) and the elastoresistivity (er) studies, respectively. These observations provide evidence for an electronic origin of nematicity in LaFeAsO. The characteristic energy of the coupling between the lattice and the electronic degrees of freedom is deduced to $\sim$30~K. The comparison to corresponding measurements on BaFe$_2$As$_2$ single crystals reveals a very similar temperature dependence of the shear modulus but yields contrasting results for $\chi^{er}$ : In BaFe$_2$As$_2$, $\chi^{er}$ diverges similarly as the uncoupled nematicity deduced from the shear modulus data as it is expected from the underlying Landau theory. In contrast, the Weiss temperatures of $\chi^{er}$ and $\chi^{sh}$ are significantly different in LaFeAsO. This difference is at odds with the commonly anticipated theories of resistivity anisotropy and electronic nematicity in iron pnictides.

cond-mat.supr-con

Quantum Critical Magnetic Excitations in Spin-1/2 and Spin-1 Chain Systems

The study of CoNb$_2$O$_6$ sits at the confluence of simplicity and complexity: on one hand, the model for Ising chains -- the building blocks of CoNb$_2$O$_6$ -- in a transverse field, can be exactly solved and, thus, serves as an archetype of quantum criticality; on the other hand, the weak but nonzero interchain coupling adds geometric frustration to the stage, substantially complicating the phase diagram. Here we utilize low-temperature specific heat and thermal conductivity measurements to study the low-lying magnetic excitations in CoNb$_2$O$_6$ and its spin-1 analogue NiNb$_2$O$_6$. The thermal conductivity is found to be suppressed around the quantum critical point, where the specific heat is enhanced due to gapless magnetic excitations, pointing to the localized nature of the latter. These results highlight the predominant role of frustration in determining the quantum critical magnetic excitations of spin chains, which may furthermore underlie the remarkable similarities between the phenomenology of these spin-1/2 and spin-1 systems.

cond-mat.str-el

The incommensurate magnet iron monophosphide FeP: Crystal growth and characterization

We report an optimized chemical vapor transport method, which allows growing FeP single crystals up to 500 mg in mass and 80 $mm^{3}$ in volume. The high quality of the crystals obtained by this method was confirmed by means of EDX, high-resolution TEM, low-temperature single crystal XRD and neutron diffraction experiments. We investigated the transport and magnetic properties of the single crystals and calculated the electronic band structure of FeP. We show both theoretically and experimentally, that the ground state of FeP is metallic. The examination of the magnetic data reveals antiferromagnetic order below T$_{N}$ =119 K while transport remains metallic in both the paramagnetic and the antiferromagnetic phase. The analysis of the neutron diffraction data shows an incommensurate magnetic structure with the propagation vector Q=(0, 0, $\pmδ$), where $δ$ $\sim$ 0.2. For the full understanding of the magnetic state, further experiments are needed. The successful growth of large high-quality single crystals opens the opportunity for further investigations of itinerant magnets with incommensurate spin structures using a wide range of experimental tools.

cond-mat.mtrl-sci

Absence of magnetic thermal conductivity in the quantum spin liquid candidate YbMgGaO4

We present the ultra-low-temperature specific heat and thermal conductivity measurements on the single crystals of YbMgGaO$_4$, which was recently argued to be a promising candidate for quantum spin liquid (QSL). In the zero magnetic field, a large magnetic contribution of specific heat is observed, and exhibits a power-law temperature dependence ($C_m \sim T^{0.74}$). On the contrary, we do not observed any significant contribution of thermal conductivity from magnetic excitations. In magnetic fields $H \ge$ 6 T, the exponential $T$-dependence of $C_m$ and the enhanced thermal conductivity indicate a magnon gap of the fully-polarized state. The absence of magnetic thermal conductivity at the zero field in this QSL candidate puts a strong constraint on the theories of its ground state.

cond-mat.str-el

Multiband nodeless superconductivity near the charge-density-wave quantum critical point in ZrTe3-xSex

Recently it was found that selenium doping can suppress the charge-density-wave (CDW) order and induce bulk superconductivity in ZrTe$_3$. The observed superconducting dome suggests the existence of a CDW quantum critical point (QCP) in ZrTe$_{3-x}$Se$_x$ near $x \approx$ 0.04. To elucidate its superconducting state near the CDW QCP, we measure the thermal conductivity of two ZrTe$_{3-x}$Se$_x$ single crystals ($x$ = 0.044 and 0.051) down to 80 mK. For both samples, the residual linear term $κ_0/T$ at zero field is negligible, which is a clear evidence for nodeless superconducting gap. Furthermore, the field dependence of $κ_0/T$ manifests multigap behavior. These results demonstrate multiple nodeless superconducting gaps in ZrTe$_{3-x}$Se$_x$, which indicates conventional superconductivity despite of the existence of a CDW QCP.

cond-mat.supr-con

Fully gapped superconducting state in Au2Pb: a natural candidate for topological superconductor

We measured the ultra-low-temperature specific heat and thermal conductivity of Au$_2$Pb single crystal, a possible three-dimensional Dirac semimetal with a superconducting transition temperature $T_c \approx$ 1.05 K. The electronic specific heat can be fitted by a two-band s-wave model, which gives the gap amplitudes $Δ_1$(0)/$k_BT_c$ = 1.38 and $Δ_2$(0)/$k_BT_c$ = 5.25. From the thermal conductivity measurements, a negligible residual linear term $κ_0/T$ in zero field and a slow field dependence of $κ_0/T$ at low field are obtained. These results suggest that Au$_2$Pb has a fully gapped superconducting state in the bulk, which is a necessary condition for topological superconductor if Au$_2$Pb is indeed one.

cond-mat.supr-con

Nodal superconductivity in FeS: Evidence from quasiparticle heat transport

We report low-temperature heat transport measurements on superconducting iron sulfide FeS with $T_c \approx$ 5 K, which has the same crystal structure and similar electronic band structure to the superconducting iron selenide FeSe. In zero magnetic field, a significant residual linear term $κ_0/T$ is observed. At low field, $κ_0/T$ increases rapidly with the increase of field. These results provide strong evidence for nodal superconducting gap in FeS. We compare it with the sister compound FeSe, and other iron-based superconductors with nodal gap.

cond-mat.supr-con

Observation of two distinct superconducting domes under pressure in tetragonal FeS

As the simplest iron-based superconductor, FeSe forms a tetragonal structure with transition temperature Tc ~ 8 K. With assistance of pressure, or other techniques, Tc can be greatly enhanced, even to above liquid nitrogen temperature. The newly discovered superconducting tetragonal FeS (Tc ~ 4.5 K), a sulfide counterpart of FeSe, promotes us on its high pressure investigation. The transport and structure evolution of FeS with pressure have been studied. A rapid suppression of Tc and vanishing of superconductivity at 4.0 GPa are observed, followed by a second superconducting dome with a 30% enhancement in maximum Tc. An onsite tetragonal to hexagonal phase transition occurs around 7.0 GPa, followed by a broad pressure range of phase coexistence. The residual deformed tetragonal phase is considered as the source of second superconducting dome. The observation of two superconducting domes in iron-based superconductors poses great challenges for understanding their pairing mechanism.

cond-mat.supr-con

Pressure-induced superconductivity in the three-dimensional Dirac semimetal Cd3As2

The recently discovered Dirac and Weyl semimetals are new members of topological materials. Starting from them, topological superconductivity may be achieved, e.g. by carrier doping or applying pressure. Here we report high-pressure resistance and X-ray diffraction study of the three-dimensional topological Dirac semimetal Cd3As2. Superconductivity with Tc ~ 2.0 K is observed at 8.5 GPa. The Tc keeps increasing to about 4.0 K at 21.3 GPa, then shows a nearly constant pressure dependence up to the highest pressure 50.9 GPa. The X-ray diffraction measurements reveal a structure phase transition around 3.5 GPa. Our observation of superconductivity in pressurized topological Dirac semimetal Cd3As2 provides a new candidate for topological superconductor, as argued in a recent point contact study and a theoretical work.

cond-mat.supr-con

Multiple nodeless superconducting gaps in noncentrosymmetric superconductor PbTaSe2 with topological bulk nodal lines

Low-temperature thermal conductivity measurements were performed on single crystal of PbTaSe$_2$, a noncentrosymmetric superconductor with topological bulk nodal lines in the electronic band structure. It is found that the residual linear term $κ_0/T$ is negligible in zero magnetic field. Furthermore, the field dependence of $κ_0/T$ exhibits a clear "$S$"-shape curve. These results suggest that PbTaSe$_2$ has multiple nodeless superconducting gaps. Therefore, the spin-triplet state with gap nodes does not play an important role in this noncentrosymmetric superconductor with strong spin-orbital coupling. The fully gapped superconducting state also meets the requirement of a topological superconductor, if PbTaSe$_2$ is indeed the case.

cond-mat.supr-con

Universal Heat Conduction in Ce1-xYbxCoIn5: Evidence for Robust Nodal d-wave Superconducting Gap

In heavy-fermion superconductor Ce$_{1-x}$Yb$_x$CoIn$_5$ system, Yb doping was reported to cause a possible change from nodal $d$-wave superconductivity to a fully gapped $d$-wave molecular superfluid of composite pairs near $x \approx$ 0.07 (nominal value $x_{nom}$ = 0.2). Here we present systematic thermal conductivity measurements on Ce$_{1-x}$Yb$_x$CoIn$_5$ ($x$ = 0.013, 0.084, and 0.163) single crystals. The observed finite residual linear term $κ_0/T$ is insensitive to Yb doping, verifying the universal heat conduction of nodal $d$-wave superconducting gap in Ce$_{1-x}$Yb$_x$CoIn$_5$. Similar universal heat conduction is also observed in CeCo(In$_{1-y}$Cd$_y$)$_5$ system. These results reveal robust nodal $d$-wave gap in CeCoIn$_5$ upon Yb or Cd doping.

cond-mat.supr-con

Doping evolution of the superconducting gap structure in heavily hole-doped Ba$_{1-x}$K$_x$Fe$_2$As$_2$: heat transport study

We performed systematic thermal conductivity measurements on heavily hole-doped Ba$_{1-x}$K$_x$Fe$_2$As$_2$ single crystals with 0.747 $\leq x \leq$ 0.974. At $x$ = 0.747, the $κ_0/T$ is negligible, indicating nodeless superconducting gap. A small residual linear term $κ_0/T$ ($\approx$ 0.035 mW/K$^2$ cm) appears at $x$ = 0.826, and it increases slowly up to $x$ = 0.974, followed by a drastic increase of more than 20 times to the pure KFe$_2$As$_2$ ($x$ = 1.0). This doping dependence of $κ_0/T$ clearly shows that the nodal gap appears near $x = 0.8$, likely associated with the change of Fermi surface topology. The small values of $κ_0/T$ from $x$ = 0.826 to 0.974 support a "$\curlyvee$"-shaped nodal $s$-wave gap recently revealed by angle-resolved photoemission spectroscopy experiments at $x$ = 0.9. Furthermore, the drastic increase of $κ_0/T$ from $x$ = 0.974 to 1.0 is inconsistent with a symmetry-imposed $d$-wave gap in KFe$_2$As$_2$, and the possible nodal gap structure in KFe$_2$As$_2$ is discussed.

cond-mat.supr-con

Drastic pressure effect on the extremely large magnetoresistance in WTe2: quantum oscillation study

The quantum oscillations of the magnetoresistance under ambient and high pressure have been studied for WTe$_2$ single crystals, in which extremely large magnetoresistance was discovered recently. By analyzing the Shubnikov-de Haas oscillations, four Fermi surfaces are identified, and two of them are found to persist to high pressure. The sizes of these two pockets are comparable, but show increasing difference with pressure. At 0.3 K and in 14.5 T, the magnetoresistance decreases drastically from 1.25 $\times$ $10^5$\% under ambient pressure to 7.47 $\times$ $10^3$\% under 23.6 kbar, which is likely caused by the relative change of Fermi surfaces. These results support the scenario that the perfect balance between the electron and hole populations is the origin of the extremely large magnetoresistance in WTe$_2$.

cond-mat.mtrl-sci

Nodal superconductivity and superconducting dome in new layered superconductor Ta4Pd3Te16

We measured the low-temperature thermal conductivity of a new layered superconductor with quasi-one-dimensional characteristics, the ternary telluride Ta$_4$Pd$_3$Te$_{16}$ with transition temperature $T_c \approx$ 4.3 K. The significant residual linear term of thermal conductivity in zero magnetic field and its rapid field dependence provide evidences for nodes in the superconducting gap. By measuring resistivity under pressures, we reveal a superconducting dome in the temperature-pressure phase diagram. The existence of gap nodes and superconducting dome suggests unconventional superconductivity in Ta$_4$Pd$_3$Te$_{16}$, which may relate to a charge-density wave instability in this low-dimensional compound.

cond-mat.supr-con

Heat transport in RbFe2As2 single crystal: evidence for nodal superconducting gap

The in-plane thermal conductivity of iron-based superconductor RbFe$_2$As$_2$ single crystal ($T_c \approx$ 2.1 K) was measured down to 100 mK. In zero field, the observation of a significant residual linear term $κ_0/T$ = 0.65 mW K$^{-2}$ cm$^{-1}$ provides clear evidence for nodal superdonducting gap. The field dependence of $κ_0/T$ is similar to that of its sister compound CsFe$_2$As$_2$ with comparable residual resistivity $ρ_0$, and lies between the dirty and clean KFe$_2$As$_2$. These results suggest that the (K,Rb,Cs)Fe$_2$As$_2$ serial superconductors have a common nodal gap structure.

cond-mat.supr-con

Multi-gap nodeless superconductivity in nickel chalcogenide TlNi2Se2

Low-temperature thermal conductivity measurements were performed on single crystals of TlNi$_2$Se$_2$, a nickel-chalcogenide heavy-electron superconductor with $T_c$ $\simeq$ 3.7 K. In zero field, the residual electronic contribution at $T$ $\rightarrow$ 0 K ($κ_0/T$) was well separated from the total thermal conductivity, which is less than 0.45\% of its normal-state value. Such a tiny residual $κ_0/T$ is unlikely contributed by the nodal quasiparticles. Nodeless gap structure is supported by the very weak field dependence of $κ_0(H)/T$ in low magnetic fields. In the whole field range, $κ_0(H)/T$ exhibits an "$S$"-shape curve, as in the case of nickel pnictides BaNi$_2$As$_2$ and SrNi$_2$P$_2$. This common feature of nickel-based superconductors can be explained by multiple nodeless superconducting gaps.

cond-mat.supr-con

Quantum transport evidence for a three-dimensional Dirac semimetal phase in Cd3As2

The material termed three-dimensional (3D) Dirac semimetal has attracted great interests recently, since it is an electronic analogue to two-dimensional graphene. Starting from this novel phase, various topologically distinct phases may be obtained, such as topological insulator, Weyl semimetal, quantum spin Hall insulator, and topological superconductor. Soon after the theoretical predictions, the angle-resolve photoemission spectroscopy and scanning tunnelling microscopy experiments gave evidences for 3D Dirac points in Na3Bi and Cd3As2. Here we report quantum transport properties of Cd3As2 single crystal in magnetic field. A sizable linear quantum magnetoresistance is observed at high temperature. With decreasing temperature, the Shubnikov-de Haas oscillations appear in both longitudinal resistance Rxx and transverse Hall resistance Rxy. From the strong oscillatory component ΔRxx, the linear dependence of Landau index n on 1/B gives an n-axis intercept 0.58. Our quantum transport result clearly reveals a nontrivial π Berry's phase, thus provides strong bulk evidence for a 3D Dirac semimetal phase in Cd3As2. This may open new perspectives for its use in electronic devices.

cond-mat.str-el

Nodeless superconducting gaps in Ca$_{10}$(Pt$_{4-δ}$As$_8$)((Fe$_{1-x}$Pt$_{x}$)$_2$As$_2$)$_5$ probed by quasiparticle heat transport

The in-plane thermal conductivity of iron-based superconductor Ca$_{10}$(Pt$_{4-δ}$As$_8$)((Fe$_{1-x}$Pt$_{x}$)$_2$As$_2$)$_5$ single crystal (``10-4-8", $T_c$ = 22 K) was measured down to 80 mK. In zero field, the residual linear term $κ_0/T$ is negligible, suggesting nodeless superconducting gaps in this multiband compound. In magnetic fields, $κ_0/T$ increases rapidly, which mimics those of multiband superconductor NbSe$_2$ and LuNi$_2$B$_2$C with highly anisotropic gap. Such a field dependence of $κ_0/T$ is an evidence for multiple superconducting gaps with quite different magnitudes or highly anisotropic gap. Comparing with the London penetration depth results of Ca$_{10}$(Pt$_3$As$_8$)((Fe$_{1-x}$Pt$_{x}$)$_2$As$_2$)$_5$ (``10-3-8") compound, the 10-4-8 and 10-3-8 compounds may have similar superconducting gap structure.

cond-mat.supr-con