arXiv subjects

X. Du

Publications and source records attributed to X. Du.

At least 37 records · Page 2Linked to original sources

arXiv2023

Orbital-selective charge-density wave in TaTe$_4$

TaTe$_4$, a metallic charge-density wave (CDW) material discovered decades ago, has attracted renewed attention due to its rich interesting properties such as pressure-induced superconductivity and candidate non-trivial topological phase. Here, using high-resolution angle-resolved photoemission spectroscopy and ab-initio calculation, we systematically investigate the electronic structure of TaTe$_4$. At 26 K, we observe a CDW gap as large as 290 meV, which persists up to 500 K. The CDW-modulated band structure shows a complex reconstruction that closely correlates with the lattice distortion. Inside the CDW gap, there exist highly dispersive energy bands contributing to the remnant Fermi surface and metallic behavior in the CDW state. Interestingly, our ab-initio calculation reveals that the large CDW gap mainly opens in the electronic states with out-of-plane orbital components, while the in-gap metallic states originate from in-plane orbitals, suggesting an orbital texture that couples with the CDW order. Our results shed light on the interplay between electron, lattice, and orbital in quasi-one-dimensional CDW materials.

cond-mat.str-el↗

arXiv2023

Evidence for Band Renormalizations in Strong-coupling Superconducting Alkali-fulleride Films

There has been a long-standing debate about the mechanism of the unusual superconductivity in alkali-intercalated fulleride superconductors. In this work, using high-resolution angle-resolved photoemission spectroscopy, we systematically investigate the electronic structures of superconducting K3C60 thin films. We observe a dispersive energy band crossing the Fermi level with an occupied bandwidth of about 130 meV. The measured band structure shows prominent quasiparticle kinks and a replica band involving high-energy Jahn-Teller active Hg(8) phonon mode, reflecting strong electron-phonon coupling in the system. The electron-phonon coupling constant is estimated to be about 1.2, which dominates the quasiparticle mass renormalization. Moreover, we observe an isotropic nodeless superconducting gap beyond the mean-field estimation. Both the large electron-phonon coupling constant and large reduced superconducting gap suggest a strong-coupling superconductivity in K3C60, while the electronic correlation effect is indicated by the observation of a waterfall-like band dispersion and the small bandwidth compared with the effective Coulomb interaction. Our results not only directly visualize the crucial band structure of superconducting fulleride but also provide important insights into the mechanism of the unusual superconductivity.

cond-mat.supr-con↗

arXiv2023

Thermal hysteretic behavior and negative magnetoresistance in an unusual charge-density-wave material EuTe4

EuTe4 is a newly-discovered van der Waals material exhibiting a novel charge-density wave (CDW) with a large thermal hysteresis in the resistivity and CDW gap. In this work, we systematically study the electronic structure and transport properties of EuTe4 using high-resolution angle-resolved photoemission spectroscopy (ARPES), magnetoresistance measurements, and scanning tunneling microscopy (STM). We observe a CDW gap of about 200 meV at low temperatures that persists up to 400 K, suggesting that the CDW transition occurs at a much higher temperature. We observe a large thermal hysteretic behavior of the ARPES intensity near the Fermi level, consistent with the resistivity measurement. The hysteresis in the resistivity measurement does not change under a magnetic field up to 7 T, excluding the thermal magnetic hysteresis mechanism. Instead, the surface topography measured with STM shows surface domains with different CDW trimerization directions, which may be important for the thermal hysteretic behavior of EuTe4. Interestingly, we observe a large negative magnetoresistance at low temperatures that can be associated with the canting of magnetically ordered Eu spins. Our work shed light on the understanding of magnetic, transport, and electronic properties of EuTe4.

cond-mat.str-el↗

arXiv2023

Development of a Laser-based angle-resolved-photoemission spectrometer with sub-micrometer spatial resolution and high-efficiency spin detection

Angle-resolved photoemission spectroscopy with sub-micrometer spatial resolution (μ-ARPES), has become a powerful tool for studying quantum materials. To achieve sub-micrometer or even nanometer-scale spatial resolution, it is important to focus the incident light beam (usually from the synchrotron radiation) using X-ray optics such as the zone plate or ellipsoidal capillary mirrors. Recently, we developed a laser-based μ-ARPES with spin-resolution (LMS-ARPES). The 177 nm laser beam is achieved by frequency doubling a 355 nm beam using a KBBF crystal and subsequently focused using an optical lens with a focal length of about 16 mm. By characterizing the focused spot size using different methods and performing spatial-scanning photoemission measurement, we confirm the sub-micron spatial resolution of the system. Compared with the μ-ARPES facilities based on synchrotron radiation, our LMS-ARPES system is not only more economical and convenient but also with higher photon flux (> 5E13 photons/s), thus enabling the high-resolution and high-statistics measurements. Moreover, the system is equipped with a two-dimensional spin detector based on exchange scattering at a surface-passivated iron film grown on a W(100) substrate. We investigate the spin structure of the prototype topological insulator Bi2Se3 and reveal a high spin-polarization rate, confirming its spin-momentum locking property. This lab-based LMS-ARPES will be a powerful research tool for studying the local fine electronic structures of different condensed matter systems, including topological quantum materials, mesoscopic materials and structures, and phase-separated materials.

cond-mat.mtrl-sci↗

arXiv2022

Crossed Luttinger Liquid Hidden in a Quasi-two-dimensional Material η-Mo4O11

Although the concept of Luttinger liquid (LL) that describes a one-dimensional (1D) interacting fermion system collapses in higher dimensions, it has been proposed to be closely related to many mysteries including the normal state of cuprate superconductor, unconventional metal, and quantum criticality. Therefore, the generalization of LL model to higher dimensions has attracted substantial research attention. Here we systematically investigate the electronic structure of a quasi-2D compound η-Mo4O11 using high-resolution angle-resolved photoemission spectroscopy and ab-initio calculation. Remarkably, we reveal a prototypical LL behavior originating from the crossing quasi-1D chain arrays hidden in the quasi-2D crystal structure. Our results suggest that η-Mo4O11 materializes the long sought-after crossed LL phase, where the orthogonal orbital components significantly reduce the coupling between intersecting quasi-1D chains and therefore maintain the essential properties of LL. Our finding not only presents a realization of 2D LL, but also provides a new angle to understand non-Fermi liquid behaviors in other 2D and 3D quantum materials.

cond-mat.str-el↗

arXiv2022

Hybridization and Correlation between f- and d-orbital electrons in a valence fluctuating compound EuNi2P2

The interaction between localized f and itinerant conduction electrons is crucial in the electronic properties of heavy fermion and valence fluctuating compounds. Using high-resolution angle-resolved photoemission spectroscopy, we systematically investigate the electronic structure of the archetypical valence fluctuating compound EuNi2P2 that hosts multiple f electrons. At low temperatures, we reveal the hybridization between Eu 4f and Ni 3d states, which contributes to the electron mass enhancement, consistent with the periodic Anderson model. With increasing temperature, interestingly, we observe opposite temperature evolution of electron spectral function above and below the Kondo coherence temperature near 110 K, which is in contrast to the monotonic valence change and beyond the expectation of the periodic Anderson model. We argue that both f-d hybridization and correlation are imperative in the electronic properties of EuNi2P2. Our results shed light on the understanding of novel properties, such as heavy fermion behaviors and valence fluctuation, of rare-earth transition-metal intermetallic compounds with multiple f electrons.

cond-mat.str-el↗

arXiv2022

Design and simulation of an Imaging Neutral Particle Analyzer for the ASDEX Upgrade tokamak

An Imaging Neutral Particle Analyser (INPA) diagnostic has been designed for the ASDEX Upgrade (AUG) tokamak. The AUG INPA diagnostic will measure fast neutrals escaping the plasma after CX reactions. The neutrals will be ionised by a 20 nm carbon foil and deflected towards a scintillator by the local magnetic field. The use of a neutral beam injector (NBI) as active source of neutrals will provide radially resolved measurements while the use of a scintillator as active component will allow us to cover the whole plasma along the NBI line with unprecedented phase-space resolution ($ < $ 12 keV and 8 cm) and fast temporal response (up to 1 kHz with the high resolution acquisition system and above 100 kHz with the low resolution one); making it suitable to study localised fast-ions redistributions in phase-space.

physics.plasm-ph↗

arXiv2022

Robust Kagome Electronic Structure in Topological Quantum Magnets XMn6Sn6 (X = Dy, Tb, Gd, Y)

Crystal geometry can greatly influence the emergent properties of quantum materials. As an example, the kagome lattice is an ideal platform to study the rich interplay between topology, magnetism, and electronic correlation. In this work, combining high-resolution angle-resolved photoemission spectroscopy and ab-initio calculation, we systematically investigate the electronic structure of XMn6Sn6 (X = Dy, Tb, Gd, Y) family compounds. We observe the Dirac fermion and the flat band arising from the magnetic kagome lattice of Mn atoms. Interestingly, the flat band locates in the same energy region in all compounds studied, regardless of their different magnetic ground states and 4f electronic configurations. These observations suggest a robust Mn magnetic kagome lattice across the XMn6Sn6 family, thus providing an ideal platform for the search and investigation on new emergent phenomena in magnetic topological materials.

cond-mat.str-el↗

arXiv2022

Nitrogen Plasma Passivated Niobium Resonators for Superconducting Quantum Circuits

Microwave loss in niobium metallic structures used for superconducting quantum circuits is limited by a native surface oxide layer formed over a timescale of minutes when exposed to an ambient environment. In this work, we show that nitrogen plasma treatment forms a niobium nitride layer at the metal-air interface which prevents such oxidation. X-ray photoelectron spectroscopy confirms the doping of nitrogen more than 5 nm into the surface and a suppressed oxygen presence. This passivation remains stable after aging for 15 days in an ambient environment. Cryogenic microwave characterization shows an average filling factor adjusted two-level-system loss tangent $\rm{Fδ_{TLS}}$ of $(2.9\pm0.5)\cdot10^{-7}$ for resonators with 3 $\rmμ$m center strip and $(1.0\pm0.3)\cdot10^{-7}$ for 20 $\rmμ$m center strip, exceeding the performance of unpassivated samples by a factor of four.

physics.app-ph↗

arXiv2021

Fabrication and surface treatment of electron-beam evaporated niobium for low-loss coplanar waveguide resonators

We characterize low-loss electron-beam evaporated niobium thin films deposited under ultra-high vacuum conditions. Slow deposition yields films with a high superconducting transition temperature ($9.20 \pm 0.06 \rm ~K$) as well as a residual resistivity ratio of $4.8$. We fabricate the films into coplanar waveguide resonators to extract the intrinsic loss due to the presence of two-level-system fluctuators using microwave measurements. For a coplanar waveguide resonator gap of $2~μ\rm m$, the films exhibit filling-factor-adjusted two-level-system loss tangents as low as $1.5 \times 10^{-7}$ with single-photon regime internal quality factors in excess of one million after removing native surface oxides of the niobium.

cond-mat.supr-con↗

arXiv2021

Band-selective Holstein polaron in Luttinger liquid material A0.3MoO3 (A = K, Rb)

(Quasi-)one-dimensional systems exhibit various fascinating properties such as Luttinger liquid behavior, Peierls transition, novel topological phases, and the accommodation of unique quasiparticles (e.g., spinon, holon, and soliton, etc.). Here we study molybdenum blue bronze A0.3MoO3 (A = K, Rb), a canonical quasi-one-dimensional charge-density-wave material, using laser-based angle-resolved photoemission spectroscopy. Our experiment suggests that the normal phase of A0.3MoO3 is a prototypical Luttinger liquid, from which the charge-density-wave emerges with decreasing temperature. Prominently, we observe strong renormalizations of band dispersions, which is recognized as the spectral function of Holstein polaron derived from band-selective electron-phonon coupling in the system. We argue that the strong electron-phonon coupling plays a dominant role in electronic properties and the charge-density-wave transition in blue bronzes. Our results not only reconcile the long-standing heavy debates on the electronic properties of blue bronzes but also provide a rare platform to study novel composite quasiparticles in Luttinger liquid materials.

cond-mat.str-el↗

arXiv2020

Runaway Electron Seed Formation at Reactor-Relevant Temperature

Systematic variation of the pre-disruption core electron temperature (Te) from 1 to 12 keV using an internal transport barrier scenario reveals a dramatic increase in the production of seed runaway electrons (REs), ultimately accessing near-complete conversion of the pre-disruption current into sub-MeV RE current. Injected Ar pellets are observed to ablate more intensely and promptly as Te rises. At high Te, the observed ablation exceeds predictions from published thermal ablation models. Simultaneously, the thermal quench (TQ) is observed to significantly shorten with increasing Te -- a surprising result. While the reason for the shorter TQ is not yet understood, candidate mechanisms include: insufficiently accurate thermal ablation models, enhanced ablation driven by the seed RE population, or significant parallel heat transport along stochastic fields. Kinetic modeling that self-consistently treats the plasma cooling via radiation, the induced electric field, and the formation of the seed RE is performed. Including the combined effect of the inherent dependence of hot-tail RE seeding on Te together with the shortened TQ, modeling recovers the progression towards near-complete conversion of the pre-disruption current to RE current as Te rises. Measurement of the HXR spectrum during the early current quench (CQ) reveals a trend of decreasing energy with pre-disruption Te. At the very highest Te ($\approx$ 12 keV), $\approx$ 100% conversion of the thermal current to runaway current is found. The energy of this peculiar RE beam is inferred to be sub-MeV as it emits vanishingly few MeV hard X-rays (HXRs). These measurements demonstrate novel TQ dynamics as Te is varied and illustrate the limitations of treating the RE seed formation problem without considering the inter-related dependencies of the pellet ablation, radiative energy loss, and resultant variations of the TQ duration.

physics.plasm-ph↗

arXiv2019

The DRAO Synthesis Telescope

The DRAO Synthesis Telescope (ST) is a forefront telescope for imaging large-scale neutral hydrogen and polarized radio continuum emission at arcminute resolution. Equipped for observations at 1420 and 408 MHz, the ST completed the Canadian Galactic Plane Survey, providing pioneering measurements of arcminute-scale structure in HI emission and self-absorption and of the diffuse polarized emission, using a fine grid of Rotation Measures to chart the large-scale Galactic magnetic field, and advancing the knowledge of the Galactic rotation curve. In this paper we describe a plan for renewal of the Synthesis Telescope that will create a forefront scientific instrument, a testbed for new radio astronomy technologies, and a training ground for the next generation of Canadian radio astronomers and radio telescope engineers. The renewed telescope will operate across the entire range 400 to 1800 MHz. Collaborations between DRAO and university partners have already demonstrated a novel feed antenna to cover this range, low-noise amplifiers, and a new GPU-based correlator of bandwidth 400 MHz. The renewed ST will provide excellent sensitivity to extended HI, covering the Galactic disk and halo, spectro-polarimetry with unprecedented resolution in angle and in Faraday depth, the ability to search for OH masers in all four 18-cm lines simultaneously, and sensitive recombination-line observations stacked over as many as forty transitions. As a testbed the renewed ST will evaluate low-cost digital clocking and sampling techniques of wide significance for the ngVLA, SKA, and other future telescopes, and a prototype of the digital correlator developed at DRAO for SKA-mid.

astro-ph.IM↗

arXiv2019

Hyperons and quarks in proto-neutron stars

In this work, we study matter in the cores of proto-neutron stars, focusing on the impact of their composition on the stellar structure. We begin by examining the effects of finite temperature (through a fixed entropy per baryon) and lepton fraction on purely nucleonic matter by making use of the DSH model . We then turn our attention to a relativistic mean-field model containing exotic degrees of freedom, the Chiral Mean Field (CMF) model, again, under the conditions of finite temperature and trapped neutrinos. In the latter, since both hyperons and quarks are found in the cores of large-mass stars, their interplay and the possibility of mixtures of phases is taken into account and analyzed. Finally, we discuss how stellar rotation can affect our results.

astro-ph.HE↗

arXiv2019

From the microscopic to the macroscopic world: from nucleons to neutron stars

Recent observations of neutron-star properties, in particular the recent detection of gravitational waves emitted from binary neutron stars, GW 170817, open the way to put strong constraints on nuclear interactions. In this paper, we review the state of the art in calculating the equation of state of strongly interacting matter from first principle calculations starting from microscopic interactions among nucleons. We then review selected properties of neutron stars that can be directly compared with present and future observations.

nucl-th↗

arXiv2019

Future physics opportunities for high-density QCD at the LHC with heavy-ion and proton beams

The future opportunities for high-density QCD studies with ion and proton beams at the LHC are presented. Four major scientific goals are identified: the characterisation of the macroscopic long wavelength Quark-Gluon Plasma (QGP) properties with unprecedented precision, the investigation of the microscopic parton dynamics underlying QGP properties, the development of a unified picture of particle production and QCD dynamics from small (pp) to large (nucleus--nucleus) systems, the exploration of parton densities in nuclei in a broad ($x$, $Q^2$) kinematic range and the search for the possible onset of parton saturation. In order to address these scientific goals, high-luminosity Pb-Pb and p-Pb programmes are considered as priorities for Runs 3 and 4, complemented by high-multiplicity studies in pp collisions and a short run with oxygen ions. High-luminosity runs with intermediate-mass nuclei, for example Ar or Kr, are considered as an appealing case for extending the heavy-ion programme at the LHC beyond Run 4. The potential of the High-Energy LHC to probe QCD matter with newly-available observables, at twice larger center-of-mass energies than the LHC, is investigated.

hep-ph↗

arXiv2016

Soft phonon driven orbital order in CaMn7O12

We use variable-temperature x-ray thermal diffuse scattering and inelastic scattering to investigate the lattice dynamics in single crystals of multiferroic CaMn7O12 which undergo a series of orbital and magnetic transitions at low temperatures. Upon approaching the charge and orbital ordering temperature To=250 K from above, we observe intense diffuse scattering features and a pronounced optical phonon softening centered around the superstructure reflections of the incommensurately modulated structure. The phonon anomaly appears well above To and continuously increases upon cooling, following a canonical power-law temperature dependence that confirms the transition at To to be of second order and related to a soft-phonon lattice instability. Microscopic mechanisms for the incommensurate charge and orbital ordering based on competing interactions and on momentum dependent electron-phonon coupling could both account for the observed extended momentum width of the phonon softening. Our results highlight the importance of the lattice interactions in the physics of this magnetically induced ferroelectric system.

cond-mat.str-el↗

arXiv2014

The strong running coupling at $τ$ and $Z_0$ mass scales from lattice QCD

This letter reports on the first computation, from data obtained in lattice QCD with $u,d,s$ and $c$ quarks in the sea, of the running strong coupling via the ghost-gluon coupling renormalized in the MOM Taylor scheme. We provide with estimates of $\ams(m_τ^2)$ and $\ams(m_Z^2)$ in very good agreement with experimental results. Including a dynamical c quark makes safer the needed running of $\ams$.

hep-ph↗