arXiv subjects

X. H. Chen

Publications and source records attributed to X. H. Chen.

At least 73 records · Page 4Linked to original sources

arXiv2014

Structure determination and coexistence of superconductivity and antiferromagnetic order in (Li0.8Fe0.2)OHFeSe

FeSe-derived superconductors show some unique behaviors relative to iron-pnictide superconductors, which are very helpful to understand the mechanism of superconductivity in high-Tc iron-based superconductors. The low-energy electronic structure of the heavily electron-doped AxFe2Se2 (A=K, Rb, Cs) demonstrates that interband scattering or Fermi surface nesting is not a necessary ingredient for the unconventional superconductivity in iron-based superconductors. The superconducting transition temperature (Tc) in the one-unit-cell FeSe on SrTiO3 substrate can reach as high as ~65 K, largely transcending the bulk Tc of all known iron-based superconductors. However, in the case of AxFe2Se2, the inter-grown antiferromagnetic insulating phase makes it difficult to study the underlying physics. Superconductors of alkali metal ions and NH3 molecules or organic-molecules intercalated FeSe and single layer or thin film FeSe on SrTiO3 substrate are extremely air-sensitive, which prevents the further investigation of their physical properties. Therefore, it is urgent to find a stable and accessible FeSe-derived superconductor for physical property measurements so as to study the underlying mechanism of superconductivity. Here, we report the air-stable superconductor (Li0.8Fe0.2)OHFeSe with high temperature superconductivity at ~40 K synthesized by a novel hydrothermal method. The crystal structure is unambiguously determined by the combination of X-ray and neutron powder diffraction and nuclear magnetic resonance. It is also found that an antiferromagnetic order coexists with superconductivity in such new FeSe-derived superconductor. This novel synthetic route opens a new avenue for exploring other superconductors in the related systems. The combination of different structure characterization techniques helps to complementarily determine and understand the details of the complicated structures.

cond-mat.supr-con↗

arXiv2014

Evolution of Anisotropic In-plane Resistivity with doping level in Ca$_{1-x}$Na$_x$Fe$_2$As$_2$ Single Crystals

We measured the in-plane resistivity anisotropy in the underdoped Ca$_{1-x}$Na$_x$Fe$_2$As$_2$ single crystals. The anisotropy (indicated by $ρ_{\rm b} - ρ_{\rm a}$) appears below a temperature well above magnetic transition temperature $T_{\rm N}$, being positive ($ρ_{\rm b} - ρ_{\rm a} > 0$) as $x\leq$ 0.14. With increasing the doping level to $x$ = 0.19, an intersection between $ρ_{\rm b}$ and $ρ_{\rm a}$ is observed upon cooling, with $ρ_{\rm b} - ρ_{\rm a} < 0$ at low-temperature deep inside a magnetically ordered state, while $ρ_{\rm b} - ρ_{\rm a}> 0$ at high temperature. Subsequently, further increase of hole concentration leads to a negative anisotropy $ρ_{\rm b} - ρ_{\rm a} < 0$ in the whole temperature range. These results manifest that the anisotropic behavior of resistivity in the magnetically ordered state depends strongly on the competition of the contributions from different mechanisms, and the competition between the two contributions results in a complicated evolution of the anisotropy of in-plane resistivity with doping level.

cond-mat.supr-con↗

arXiv2014

Angle-resolved Photoemission Spectroscopy Study on the Surface States of the Correlated Topological Insulator YbB6

We report the electronic structure of YbB6, a recently predicted moderately correlated topological insulator, measured by angle-resolved photoemission spectroscopy. We directly observed linearly dispersive bands around the time-reversal invariant momenta Γ and X with negligible kz dependence, consistent with odd number of surface states crossing the Fermi level in a Z2 topological insulator. Circular dichroism photoemission spectra suggest that these in-gap states possess chirality of orbital angular momentum, which is related to the chiral spin texture, further indicative of their topological nature. The observed insulating gap of YbB6 is about 100 meV, larger than that reported by theoretical calculations. Our results present strong evidence that YbB6 is a correlated topological insulator and provide a foundation for further studies of this promising material.

cond-mat.str-el↗

arXiv2014

Sudden reversal in the pressure dependence of Tc in the iron-based superconductor CsFe2As2: A possible link between inelastic scattering and pairing symmetry

We report a sudden reversal in the pressure dependence of Tc in the iron-based superconductor CsFe2As2, similar to that discovered recently in KFe2As2 [Tafti et al., Nat. Phys. 9, 349 (2013)]. As in KFe2As2, we observe no change in the Hall coefficient at the zero temperature limit, again ruling out a Lifshitz transition across the critical pressure Pc. We interpret the Tc reversal in the two materials as a phase transition from one pairing state to another, tuned by pressure, and investigate what parameters control this transition. Comparing samples of different residual resistivity, we find that a 6-fold increase in impurity scattering does not shift Pc. From a study of X-ray diffraction on KFe2As2 under pressure, we report the pressure dependence of lattice constants and As-Fe-As bond angle. The pressure dependence of these lattice parameters suggests that Pc should be significantly higher in CsFe2As2 than in KFe2As2, but we find on the contrary that Pc is lower in CsFe2As2. Resistivity measurements under pressure reveal a change of regime across Pc, suggesting a possible link between inelastic scattering and pairing symmetry.

cond-mat.supr-con↗

arXiv2014

Electronic structure of the BaTi$_2$As$_2$O parent compound of the titanium based oxypnictide superconductor

The electronic structure of BaTi2As2O, a parent compound of the newly discovered titanium-based oxypnictide superconductors, is studied by angle-resolved photoemission spectroscopy. The electronic structure shows multi-orbital nature and possible three-dimensional character. An anomalous temperature-dependent spectral weight redistribution and broad lineshape indicate the incoherent nature of the spectral function. At the density-wave-like transition temperature around 200 K, a partial gap opens at the Fermi patches. These findings suggest that BaTi2As2O is likely a charge density wave material in the strong interaction regime.

cond-mat.supr-con↗

arXiv2014

Anomalous impurity effects in the iron-based superconductor KFe$_2$As$_2$

High-quality K(Fe$_{1-x}$Co$_x$)$_2$As$_2$ single crystals have been grown by using KAs flux method. Instead of increasing the superconducting transition temperature $T_{\rm c}$ through electron doping, we find that Co impurities rapidly suppress $T_{\rm c}$ down to zero at only $x \approx$ 0.04. Such an effective suppression of $T_{\rm c}$ by impurities is quite different from that observed in Ba$_{0.5}$K$_{0.5}$Fe$_2$As$_2$ with multiple nodeless superconducting gaps. Thermal conductivity measurements in zero field show that the residual linear term $κ_0/T$ only change slightly with $3.4\%$ Co doping, despite the sharp increase of scattering rate. The implications of these anomalous impurity effects are discussed.

cond-mat.supr-con↗

arXiv2014

Spectral measurement of electron antineutrino oscillation amplitude and frequency at Daya Bay

A measurement of the energy dependence of antineutrino disappearance at the Daya Bay Reactor Neutrino Experiment is reported. Electron antineutrinos ($\overlineν_{e}$) from six $2.9$ GW$_{\rm th}$ reactors were detected with six detectors deployed in two near (effective baselines 512 m and 561 m) and one far (1579 m) underground experimental halls. Using 217 days of data, 41589 (203809 and 92912) antineutrino candidates were detected in the far hall (near halls). An improved measurement of the oscillation amplitude $\sin^{2}2θ_{13} = 0.090^{+0.008}_{-0.009} $ and the first direct measurement of the $\overlineν_{e}$ mass-squared difference $|Δm^{2}_{ee}|= (2.59_{-0.20}^{+0.19}) \times 10^{-3}\ {\rm eV}^2 $ is obtained using the observed $\overlineν_{e}$ rates and energy spectra in a three-neutrino framework. This value of $|Δm^{2}_{ee}|$ is consistent with $|Δm^{2}_{μμ}|$ measured by muon neutrino disappearance, supporting the three-flavor oscillation model.

hep-ex↗

arXiv2013

Electronic Structure Reconstruction across the Antiferromagnetic Transition in TaFe$_{1.23}$Te$_3$ Spin Ladder

With angle-resolved photoemission spectroscopy, we studied the electronic structure of TaFe$_{1.23}$Te$_3$, which is a two-leg spin ladder compound with a novel antiferromagnetic ground state. Quasi-two-dimensional Fermi surface is observed, indicating sizable inter-ladder hopping, which would facilitate the in-plane ferromagnetic ordering through double exchange interactions. Moreover, an energy gap is not observed at the Fermi surface in the antiferromagnetic state. Instead, the shifts of various bands have been observed. Combining these observations with density-functional-theory calculations, we propose that the large scale reconstruction of the electronic structure, caused by the interactions between the coexisting itinerant electrons and local moments, is most likely the driving force behind the magnetic transition. TaFe$_{1.23}$Te$_3$ thus provides a simpler system that contains similar ingredients as the parent compounds of iron-based superconductors, which yet could be readily modeled and understood.

cond-mat.str-el↗

arXiv2013

Superconductivity in LiFeO2Fe2Se2 with anti-PbO-type Spacer Layers

Superconductivity has been found in the iron-arsenides with different structures by alternative stacking of the conducting Fe2As2 layers and spacer layers including alkali- or alkali-earth metal ions and PbO- or perovskite-type oxides blocks. So far, no spacer layer could be intercalated in between the neutral Fe2Se2 layers similar in structure to Fe2As2 layers except for alkali-metal ions in AxFe2-ySe2. The superconducting phase in AxFe2-ySe2 with transition temperature of 32 K is always inter-grown with the insulating phase which exhibits an antiferromagnetic order with extremely high Neel temperature of ~560 K and the order of Fe vacancies. Such inhomogeneity makes the investigation on the underlying physics in AxFe2-ySe2 complicated. Here we report the synthesis of a novel superconductor LiFeO2Fe2Se2 by hydrothermal method, exhibiting superconductivity at ~43 K, in which anti-PbO-type spacer layers of LiFeO2 have been successfully intercalated between anti-PbO-type Fe2Se2 layers. This finding demonstrates that superconductivity can be realized in the iron selenide with a novel spacer layer of anti-PbO-type, which is not found in the iron arsenides, and expands the category of the iron-based superconductors. Such a new synthetic method paves a new way to search for possible novel superconductors with different spacer layers, which is helpful to further study the underlying physics in iron-based high-Tc superconductors.

cond-mat.supr-con↗

arXiv2013

Low-energy interband transitions in the infrared response of Ba(Fe1-xCox)2As2

We studied the doping and temperature (T) dependence of the infrared (IR) response of Ba(Fe1-xCox)2As2 single crystals. We show that a weak band around 1000 cm-1, that was previously interpreted in terms of interaction of the charge carriers with magnetic excitations or of a pseudogap, is rather related to low-energy interband transitions. Specifically, we show that this band exhibits a similar doping and T-dependence as the hole pockets seen by angle resolved photoemission spectroscopy (ARPES). Notably, we find that it vanishes as a function of doping near the critical point where superconductivity is suppressed in the overdoped regime. Our IR data thus provide bulk specific information (complementary to the surface sensitive ARPES) for a Lifshitz transition. Our IR data also reveal a second low-energy band around 2300 cm-1 which further emphasizes the necessity to consider the multiband nature of these iron arsenides in the analysis of the optical response.

cond-mat.supr-con↗

arXiv2013

Assembly and Installation of the Daya Bay Antineutrino Detectors

The Daya Bay reactor antineutrino experiment is designed to make a precision measurement of the neutrino mixing angle theta13, and recently made the definitive discovery of its nonzero value. It utilizes a set of eight, functionally identical antineutrino detectors to measure the reactor flux and spectrum at baselines of 300 - 2000m from the Daya Bay and Ling Ao Nuclear Power Plants. The Daya Bay antineutrino detectors were built in an above-ground facility and deployed side-by-side at three underground experimental sites near and far from the nuclear reactors. This configuration allows the experiment to make a precision measurement of reactor antineutrino disappearance over km-long baselines and reduces relative systematic uncertainties between detectors and nuclear reactors. This paper describes the assembly and installation of the Daya Bay antineutrino detectors.

physics.ins-det↗

arXiv2013

Phase diagram and physical properties of NaFe$_{1-x}$Cu$_x$As single crystals

A series of high quality NaFe$_{1-x}$Cu$_x$As single crystals has been grown by a self-flux technique, which were systematically characterized via structural, transport, thermodynamic, and high pressure measurements. Both the structural and magnetic transitions are suppressed by Cu doping, and bulk superconductivity is induced by Cu doping. Superconducting transition temperature ($T_c$) is initially enhanced from 9.6 to 11.5 K by Cu doping, and then suppressed with further doping. A phase diagram similar to NaFe$_{1-x}$Co$_x$As is obtained except that insulating instead of metallic behavior is observed in extremely overdoped samples. $T_c$'s of underdoped, optimally doped, and overdoped samples are all notably enhanced by applying pressure. Although a universal maximum transition temperature ($T_c^{max}$) of about 31 K under external pressure is observed in underdoped and optimally doped NaFe$_{1-x}$Co$_x$As, $T_c^{max}$ of NaFe$_{1-x}$Cu$_x$As is monotonously suppressed by Cu doping, suggesting that impurity potential of Cu is stronger than Co in NaFeAs. The comparison between Cu and Co doping effect in NaFeAs indicates that Cu serves as an effective electron dopant with strong impurity potential, but part of the doped electrons are localized and do not fill the energy bands as predicted by the rigid-band model.

cond-mat.supr-con↗

arXiv2013

Change of pairing symmetry in the iron-based superconductor KFe2As2

The pairing mechanism in iron-based superconductors is the subject of ongoing debate. Proximity to an antiferromagnetic phase suggests that pairing is mediated by spin fluctuations, but orbital fluctuations have also been invoked. The former typically favour a pairing state of extended s-wave symmetry with a gap that changes sign between electron and hole Fermi surfaces (s+-), while the latter yield a standard s-wave state without sign change (s++). Here we show that applying pressure to KFe2As2 induces a change of pairing state. The critical temperature Tc decreases with pressure initially, and then suddenly increases, above a critical pressure Pc. The constancy of the Hall coefficient through Pc rules out a change in the Fermi surface. There is compelling evidence that the pairing state below Pc is d-wave, from bulk measurements at ambient pressure. Above Pc, the high sensitivity to disorder argues for a particular kind of s+- state. The change from d-wave to s-wave is likely to proceed via an unusual s + id state that breaks time-reversal symmetry. The proximity of two distinct pairing states found here experimentally is natural given the near degeneracy of d-wave and s+- states found theoretically. These findings make a compelling case for spin-fluctuation-mediated superconductivity in this key iron-arsenide material.

cond-mat.supr-con↗

arXiv2013

Observation of in-gap surface states in the Kondo insulator SmB6 by photoemission

Kondo insulators (KIs) are strongly correlated materials in which the interactions between 4f and conduction electrons lead to a hybridization gap opening at low temperature 1-2. SmB6 is a typical KI, but its resistivity does not diverge at low temperatures, which was attributed to some in-gap states 3-10. However after several decades of research, the nature and origin of the in-gap states remain unclear. Recent band calculation and transport measurements suggest that the in-gap states could actually be ascribed to topological surface states. SmB6 thus might be the first realization of topological Kondo insulator (TKI) 13, the strongly correlated version of topological insulator (TI) 11,12. Here by performing angle-resolved photoemission spectroscopy (ARPES), we directly observed several dispersive states within the hybridization gap of SmB6, which cross the Fermi level and show negligible kz dependence, indicative of their surface origin. Furthermore, the circular dichroism (CD) ARPES results of the in-gap states suggest the chirality of orbital momentum, and temperature dependent measurements have shown that the in-gap states vanish simultaneously with the hybridization gap around 150 K. These strongly suggest their possible topological origin.

cond-mat.str-el↗

arXiv2013

Quantum oscillations in Kondo Insulator SmB$_6$

In Kondo insulator samarium hexaboride SmB$_6$, strong correlation and band hybridization lead to an insulating gap and a diverging resistance at low temperature. The resistance divergence ends at about 5 Kelvin, a behavior recently demonstrated to arise from the surface conductance. However, questions remain whether and where a topological surface state exists. Quantum oscillations have not been observed to map the Fermi surface. We solve the problem by resolving the Landau Level quantization and Fermi surface topology using torque magnetometry. The observed Fermi surface suggests a two dimensional surface state on the (101) plane. Furthermore, the tracking of the Landau Levels in the infinite magnetic field limit points to -1/2, which indicates a 2D Dirac electronic state.

cond-mat.str-el↗

arXiv2013

Nodal gap in iron-based superconductor CsFe$_2$As$_2$ probed by quasiparticle heat transport

The thermal conductivity of iron-based superconductor CsFe$_2$As$_2$ single crystal ($T_c =$ 1.81 K) was measured down to 50 mK. A significant residual linear term $κ_0/T$ = 1.27 mW K$^{-2}$ cm$^{-1}$ is observed in zero magnetic field, which is about 1/10 of the normal-state value in upper critical field $H_{c2}$. In low magnetic field, $κ_0/T$ increases rapidly with field. The overall field dependence of $κ_0/T$ for our CsFe$_2$As$_2$ (with residual resistivity $ρ_0$ = 1.80 $μΩ$ cm) lies between the dirty KFe$_2$As$_2$ (with $ρ_0$ = 3.32 $μΩ$ cm) and the clean KFe$_2$As$_2$ (with $ρ_0$ = 0.21 $μΩ$ cm). These results strongly suggest nodal superconducting gap in CsFe$_2$As$_2$, similar to its sister compound KFe$_2$As$_2$.

cond-mat.supr-con↗

arXiv2013

Upper critical magnetic field in K0.83Fe1.83Se2 and Eu0.5K0.5Fe2As2 single crystals

The H-T phase diagrams of single crystalline electron-doped K0.83Fe1.83Se2 (KFS1), K0.8Fe2Se2 (KFS2) and hole-doped Eu0.5K0.5Fe2As2 (EKFA) have been deduced from tunnel diode oscillator-based contactless measurements in pulsed magnetic fields up to 57 T for the inter-plane (H//c) and in-plane (H//ab) directions. The temperature dependence of the upper critical magnetic field Hc2(T) relevant to EFKA is accounted for by the Pauli model including an anisotropic Pauli paramagnetic contribution (μ_BHp=114 T for H//ab and 86 T for H//c). This is also the case of KFS1 and KFS2 for H//ab whereas a significant upward curvature, accounted for by a two-gap model, is observed for H//c. Despite the presence of antiferromagnetic lattice order within the superconducting state of the studied compounds, no influence of magnetic ordering on the temperature dependence of Hc2(T) is observed.

cond-mat.supr-con↗

arXiv2013

Calorimetric study in single crystal of CsFe$_2$As$_2$

We measured resistivity and specific heat of high-quality CsFe$_2$As$_2$ single crystals, which were grown by using a self-flux method. The CsFe$_2$As$_2$ crystal shows sharp superconducting transition at 1.8 K with the transition width of 0.1 K. The sharp superconducting transition and pronounced jump in specific heat indicate high quality of the crystals. Analysis on the superconducting-state specific heat supports unconventional pairing symmetry in CsFe$_2$As$_2$.

cond-mat.supr-con↗