arXiv subjects

X. Ke

Publications and source records attributed to X. Ke.

At least 19 recordsLinked to original sources

arXiv2025

Interplay between trimer structure and magnetic ground state in Ba5Ru3O12 probed by Neutron and muSR techniques

We report a detailed inelastic neutron scattering (INS) and muon spin relaxation (muSR) investigation of a trimer Ruthenate Ba5Ru3O12 system, which undergoes long-range antiferromagnetic ordering at TN = 60 K. The INS reveals two distinct spin wave excitations below TN: one at 5.6 meV and the other at 10-15 meV. By accompanying the INS spectra based on a linear spin wave theory using SpinW software and machine learning force fields (MLFFs), we show that Ba5Ru3O12 exhibits spin frustration due to competing exchange interactions between neighboring and next-neighboring Ru-moments, exchange anisotropy, and strong spin-orbit coupling, which yields a non-collinear spin structure, in contrast to other ruthenate trimers in this series. Interestingly, these magnetic excitations do not completely vanish even at high temperatures above TN, evidencing short-range magnetic correlations in this trimer system. This is further supported by muSR spectroscopy, which exhibits a gradual drop in the initial asymmetry around the magnetic phase transition and is further verified through maximum entropy analysis. The results of muSR spectroscopy indicate a dynamic nature of magnetic order, attributed to local magnetic anisotropy within the trimer as a result of local structural distortion and different hybridization, consistent with canted spin-structure. We predict the ground state of Ru3O12-isolated trimer through theoretical calculations, which agree with the experimentally observed spin excitation

cond-mat.str-el↗

arXiv2025

Anisotropic superconductivity in the quasi-one-dimensional superconductor V$_2$Ga$_5$

The intermetallic quasi-one-dimensional binary superconductor V$_2$Ga$_5$ was recently found to exhibit a topologically nontrivial normal state, making it a natural candidate for a topological superconductor (TSC). By combining dc-magnetization, nuclear magnetic resonance (NMR), and muon-spin rotation ({$\mu$SR) measurements on high-quality V$_2$Ga$_5$ single crystals, we investigate the electronic properties of its normal- and superconducting (SC) ground states. NMR measurements in the normal state indicate a strong anisotropy in both the line shifts and the relaxation rates. Such anisotropy persists also in the superconducting state, as shown by the magnetization- and $\mu$SR-spectroscopy results. In the latter case, data collected at different temperatures, pressures, and directions of the magnetic field evidence a fully-gapped, strongly anisotropic superconductivity. At the same time, hydrostatic pressure is shown to only lower the $T_c$ value, but not to change the superfluid density nor its temperature dependence. Lastly, we discuss the search for topological signatures in the normal state of V$_2$Ga$_5$, as well as a peak splitting in the FFT of the $\mu$SR spectrum, possibly related to an unconventional vortex lattice. Our results suggest that V$_2$Ga$_5$ is a novel system, whose anisotropy plays a key role in determining its unusual electronic properties.

cond-mat.supr-con↗

arXiv2023

CATS: The Hubble Constant from Standardized TRGB and Type Ia Supernova Measurements

The Tip of the Red Giant Branch (TRGB) provides a luminous standard candle for constructing distance ladders to measure the Hubble constant. In practice its measurements via edge-detection response (EDR) are complicated by the apparent fuzziness of the tip and the multi-peak landscape of the EDR. As a result, it can be difficult to replicate due to a case-by-case measurement process. Previously we optimized an unsupervised algorithm, Comparative Analysis of TRGBs (CATs), to minimize the variance among multiple halo fields per host without reliance on individualized choices, achieving state-of-the-art $\sim$ $<$ 0.05 mag distance measures for optimal data. Further, we found an empirical correlation at 5$\sigma$ confidence in the GHOSTS halo survey between our measurements of the tip and their contrast ratios (ratio of stars 0.5 mag just below and above the tip), useful for standardizing the apparent tips at different host locations. Here, we apply this algorithm to an expanded sample of SN Ia hosts to standardize these to multiple fields in the geometric anchor, NGC 4258. In concert with the Pantheon$+$ SN Ia sample, this analysis produces a (baseline) result of $H_0= 73.22 \pm 2.06$ km/s/Mpc. The largest difference in $H_0$ between this and similar studies employing the TRGB derives from corrections for SN survey differences and local flows used in most recent SN Ia compilations but which were absent in earlier studies. SN-related differences total $\sim$ 2.0 km/s/Mpc. A smaller share, $\sim$ 1.4 km/s/Mpc, results from the inhomogeneity of the TRGB calibration across the distance ladder. We employ a grid of 108 variants around the optimal TRGB algorithm and find the median of variants is $72.94\pm1.98$ km/s/Mpc with an additional uncertainty due to algorithm choices of 0.83 km/s/Mpc. None of these TRGB variants result in $H_0$ less than 71.6 km/s/Mpc.

astro-ph.CO↗

arXiv2022

Comparative Analysis of TRGBs (CATs) from Unsupervised, Multi-Halo-Field Measurements: Contrast is Key

The Tip of the Red Giant Branch (TRGB) is an apparent discontinuity in the color-magnitude diagram (CMD) along the giant branch due to the end of the red giant evolutionary phase and is used to measure distances in the local universe. In practice, the tip is often fuzzy and its localization via edge detection response (EDR) relies on several methods applied on a case-by-case basis. It is hard to evaluate how individual choices affect a distance estimation using only a single host field while also avoiding confirmation bias. To devise a standardized approach, we compare unsupervised, algorithmic analyses of the TRGB in multiple halo fields per galaxy, up to 11 fields for a single host and 50 fields across 10 galaxies, using high signal-to-noise stellar photometry obtained by the GHOSTS survey with the Hubble Space Telescope. We first optimize methods for the lowest field-to-field dispersion including spatial filtering to remove star forming regions, smoothing and weighting of the luminosity function, selection of the RGB by color, and tip selection based on the number of likely RGB stars and the ratio of stars above versus below the tip ($R$). We find $R$, which we call the tip `contrast', to be the most important indicator of the quality of EDR measurements; we find that field-to-field EDR repeatability varies from 0.3 mag to $\leq$ 0.05 mag for $R=4$ to 7, respectively, though less than half the fields reach the higher quality. Further, we find that $R$, which varies with the age/metallicity of the stellar population based on models, correlates with the magnitude of the tip (and after accounting for low internal extinction), i.e., a tip-contrast relation with slope of $-0.023\pm0.0046$ mag/ratio, a $\sim 5\sigma$ result that improves standardization of the TRGB. We discuss the value of consistent TRGB standardization across rungs for robust distance ladder measurements.

astro-ph.CO↗

arXiv2022

Thermal and thermoelectric properties of an antiferromagnetic topological insulator MnBi$_2$Te$_4$

The discovery of an intrinsic antiferromagnetic topological insulator (AFM-TI) in MnBi$_2$Te$_4$ has attracted intense attention, most of which lies on its electrical properties. In this paper, we report electronic, thermal, and thermoelectric transport studies of this newly found AFM-TI. The temperature and magnetic field dependence of its resistivity, thermal conductivity, and Seebeck coefficient indicate strong coupling between charge, lattice, and spin degrees of freedom in this system. Furthermore, MnBi$_2$Te$_4$ exhibits a large anomalous Nernst signal, which is associated with non-zero Berry curvature of the field-induced canted antiferromagnetic state.

cond-mat.mtrl-sci↗

arXiv2021

Coupling between Antiferromagnetic and Spin Glass Orders in the Quasi-One-Dimensional Iron Telluride TaFe$_{1+x}$Te$_3$ ($x$=0.25)

Understanding the interplay among different magnetic exchange interactions and its physical consequences, especially in the presence of itinerant electrons and disorders, remains one of the central themes in condensed matter physics. In this vein, the coupling between antiferromagnetic and spin glass orders may lead to large exchange bias, a property of potential broad technological applications. In this article, we report the coexistence of antiferromagnetic order and spin glass behaviors in a quasi-one-dimensional iron telluride TaFe$_{1+x}$Te$_3$ ($x$=0.25). Its antiferromagnetism is believed to arise from the antiferromagnetic interchain coupling between the ferromagnetically aligned FeTe chains along the $b$-axis, while the spin glassy state stems from the disordered Fe interstitials. This dichotomic role of chain and interstitial sublattices is responsible for the large exchange bias observed at low temperatures, with the interstitial Fe acting as the uncompensated moment and its neighboring Fe chain providing the source for its pinning. This iron-based telluride may thereby represent a new paradigm to study the large family of transition metal chalcogenides whose magnetic order or even the dimensionality can be tuned to a large extent, forming a fertile playground to manipulate or switch the spin degrees of freedom thereof.

cond-mat.mtrl-sci↗

arXiv2021

Superconductivity in PtPb$_{4}$ with Possible Nontrivial Band Topology

Superconductivity in topological quantum materials is much sought after as it represents the key avenue to searching for topological superconductors, which host a full pairing gap in the bulk but Majorana bound states at the surface. To date, however, the simultaneous realization of nontrivial band topology and superconductivity in the same material under ambient conditions remains rare. In this paper, we study both superconducting and topological properties of a binary compound PtPb$_{4}$ ($T_c$ $\sim$ 2.7 K) that was recently reported to exhibit large Rashba splitting, inherent to the heavy 5$d$ Pt and 6$p$ Pb. We show that in PtPb$_{4}$, the specific heat jump at $T_c$ reaches $\Delta C/\gamma T_{c}$$\sim$1.70$\pm0.04$, larger than 1.43 expected for the weak-coupling BCS superconductors. Moreover, the measurement of quantum oscillation suggests the possibility for a topological band structure, which is further studied by density functional theory calculations. Our study may stimulate future experimental and theoretical investigations in this intriguing material.

cond-mat.supr-con↗

arXiv2021

Anisotropic transport and de Haas$-$van Alphen oscillations in quasi-one-dimensional TaPtTe$_5$

Because of the unique physical properties and potential applications, the exploration of quantum materials with diverse symmetry-protected topological states has attracted considerable interest in the condensed-matter community in recent years. Most of the topologically nontirvial materials identified thus far have two-dimensional or three-dimensional structural characteristics, while the quasi-one-dimensional (quasi-1D) analogs are rare. Here we report on anisotropic magnetoresistance, Hall effect, and quantum de Haas$-$van Alphen (dHvA) oscillations in TaPtTe$_5$ single crystals, which possess a layered crystal structure with quasi-1D PtTe$_2$ chains. TaPtTe$_5$ manifests an anisotropic magnetoresistance and a nonlinear Hall effect at low temperatures. The analysis of the dHvA oscillations reveals two major oscillation frequencies (63.5 T and 95.2 T). The corresponding light effective masses and the nonzero Berry phases suggest the nontrivial band topology in TaPtTe$_5$, which is further corroborated by the first-principles calculations. Our results suggest that TaPtTe$_5$, in analogy with its sister compounds TaPdTe$_5$ and TaNiTe$_5$, is another quasi-1D material hosting topological Dirac fermions.

cond-mat.str-el↗

arXiv2020

Complex magnetic structure in Ba5Ru3O12 with isolated Ru3O12-trimer

We report detailed magnetic, transport, heat-capacity, and neutron diffraction measurements of Ba5Ru3O12, a compound consisting of isolated Ru3O12 trimers. We show that this system develops long-range antiferromagnetic ordering at 60 K (TN) without structural distortion and metal-insulator-type transition, which is in sharp contrast to other Barium Ruthenate trimer systems such as 9R-BaRuO3 and Ba4Ru3O10. A complex magnetic structure is revealed which is attributable to the magnetic frustration due to competing exchange interactions between Ru ions on different crystallographic sites within the Ru3O12 trimer.

cond-mat.str-el↗

arXiv2020

Magnetic Field Induced Phase Transition in Spinel GeNi2O4

Cubic spinel GeNi2O4 exhibits intriguing magnetic properties with two successive antiferromagnetic phase transitions (TN1 12.1 and TN2 11.4 K) with the absence of any structural transition. We have performed detailed heat capacity and magnetic measurements in different crystallographic orientations. A new magnetic phase in presence of magnetic field (H > 4 T) along the [111] direction is revealed, which is not observed when the magnetic field is applied along the [100] and [110] directions. High field neutron powder diffraction measurements confirm such a change in magnetic phase, which could be ascribed to a spin reorientation in the presence of magnetic field. A strong magnetic anisotropy and competing magnetic interactions play a crucial role on the complex magnetic behavior in this cubic system.

cond-mat.str-el↗

arXiv2020

Field-induced magnetic phase transitions and the resultant giant anomalous Hall effect in antiferromagnetic half-Heusler DyPtBi

We report field-induced magnetic phase transitions and transport properties of antiferromagnetic DyPtBi. We show that DyPtBi hosts a delicate balance between two different magnetic ground states, which can be controlled by a moderate magnetic field. Furthermore, it exhibits giant anomalous Hall effect (σ_A=1540 (ohm cm)^{-1},θ_{AHE} = 24%) in a field-induced Type-I spin structure, presumably attributed to the enhanced Berry curvature associated with avoided band-crossings near the Fermi energy and / or non-zero spin chirality. The latter mechanism points DyPtBi towards a rare potential realization of anomalous Hall effect in an antiferromagnet with face-center-cubic lattice that was proposed in [Physical Review Letters 87, 116801 (2001)].

cond-mat.str-el↗

arXiv2020

Coexistence and interaction of spinons and magnons in an antiferromagnet with alternating antiferromagnetic and ferromagnetic quantum spin chains

In conventional quasi-one-dimensional antiferromagnets with quantum spins, magnetic excitations are carried by either magnons or spinons in different energy regimes: they do not coexist independently, nor could they interact with each other. In this Letter, by combining inelastic neutron scattering, quantum Monte Carlo simulations and Random Phase Approximation calculations, we report the discovery and discuss the physics of the coexistence of magnons and spinons and their interactions in Botallackite-Cu2(OH)3Br. This is a unique quantum antiferromagnet consisting of alternating ferromagnetic and antiferromagnetic Spin-1/2 chains with weak inter-chain couplings. Our study presents a new paradigm where one can study the interaction between two different types of magnetic quasiparticles, magnons and spinons.

cond-mat.str-el↗

arXiv2020

Cooperative Ru(4d)-Ho(4f) magnetic orderings and phase coexistence in the 6H-perovskite multiferroic Ba3HoRu2O9

We report cooperative magnetic orderings in a 6H-perovskite multiferroic system, Ba3HoRu2O9, via comprehensive neutron powder diffraction measurements. This system undergoes long-range antiferromagnetic ordering at TN1 ~ 50 K with a propagation wave vector of K1 = (0.5 0 0), a transition temperature much higher than the previously reported one at ~10 K (TN2). Both Ru and Ho-moments order simultaneously below TN1, followed by spin-reorientations at lower temperatures, demonstrating strong Ru(4d)-Ho(4f) magnetic correlation. Below TN1 another magnetic phase with a propagation wave vector K2 = (0.25 0.25 0) emerges and coexists with the one associated with K1, which is rarely observed and suggests complex magnetism due to phase competition in the magnetic ground state. We argue that the exchange-striction arising from the up-up-down-down spin structure associated with K2-wave vector below TN2 may be responsible for the small ferroelectric polarization reported previously in this compound.

cond-mat.str-el↗

arXiv2020

Anisotropic transport and quantum oscillations in the quasi-one-dimensional TaNiTe5: Evidence for the nontrivial band topology

The past decade has witnessed the burgeoning discovery of a variety of topological states of matter with distinct nontrivial band topologies. Thus far, most of materials studied possess two-dimensional or three-dimensional electronic structures, with only a few exceptions that host quasi-one-dimensional (quasi-1D) topological electronic properties. Here we present the clear-cut evidence for Dirac fermions in the quasi-1D telluride TaNiTe5. We show that its transport behaviors are highly anisotropic and we observe nontrivial Berry phases via the quantum oscillation measurements. The nontrivial band topology is further corroborated by first-principles calculations. Our results may help to guide the future quest for topological states in this new family of quasi-1D ternary chalcogenides.

cond-mat.str-el↗

arXiv2020

Magnetic-field-induced nontrivial electronic state in the Kondo-lattice semimetal CeSb

Synergic effect of electronic correlation and spin-orbit coupling is an emerging topic in topological materials. Central to this rapidly developing area are the prototypes of strongly correlated heavy-fermion systems. Recently, some Ce-based compounds are proposed to host intriguing topological nature, among which the electronic properties of CeSb are still under debate. In this paper, we report a comprehensive study combining magnetic and electronic transport measurements, and electronic band structure calculations of this compound to identify its topological nature. Quantum oscillations are clearly observed in both magnetization and magnetoresistance at high fields, from which one pocket with a nontrivial Berry phase is recognized. Angular-dependent magnetoresistance shows that this pocket is elongated in nature and corresponds to the electron pocket as observed in LaBi. Nontrivial electronic structure of CeSb is further confirmed by first-principle calculations, which arises from spin splitting in the fully polarized ferromagnetic state. These features indicate that magnetic-field can induce nontrivial topological electronic states in this prototypical Kondo semimetal.

cond-mat.mtrl-sci↗

arXiv2020

Topological magnon bands in a room temperature Kagome magnet

Topological magnon is a vibrant research field gaining more and more attention in the past few years. Among many theoretical proposals and limited experimental studies, ferromagnetic Kagome lattice emerges as one of the most elucidating systems. Here we report neutron scattering studies of YMn6Sn6, a metallic system consisting of ferromagnetic Kagome planes. This system undergoes a commensurate-to-incommensurate antiferromagnetic phase transition upon cooling with the incommensurability along the out-of-plane direction. We observe magnon band gap opening at the symmetry-protected K points and ascribe this feature to the antisymmetric Dzyaloshinskii-Moriya (DM) interactions. Our observation supports the existence of topological Dirac magnons in both the commensurate collinear and incommensurate coplanar magnetic orders, which is further corroborated by symmetry analysis. This finding places YMn6Sn6 as a promising candidate for room-temperature magnon spintronics applications.

cond-mat.str-el↗

arXiv2018

Temperature- and field-driven spin reorientations in triple-layer ruthenate Sr$_4$Ru$_3$O$_{10}$

Sr$_4$Ru$_3$O$_{10}$, the $n$ = 3 member of the Ruddlesden-Popper type ruthenate Sr$_{n+1}$Ru$_n$O$_{3n+1}$, is known to exhibit a peculiar metamagnetic transition in an in-plane magnetic field. However, the nature of both the temperature- and field-dependent phase transitions remains as a topic of debate. Here, we have investigated the magnetic transitions of Sr$_4$Ru$_3$O$_{10}$ via single-crystal neutron diffraction measurements. At zero field, we find that the system undergoes a ferromagnetic transition with both in-plane and out-of-plane magnetic components at $T_{c}$ ~ 100 K. Below $T^{*}$ ~ 50 K, the magnetic moments incline continuously toward the out-of-plane direction. At $T$ ~ 1.5 K, where the spins are nearly aligned along the $c$ axis, a spin reorientation occurs above a critical field $B_c$, giving rise to a spin component perpendicular to the plane defined by the field direction and the $c$ axis. We suggest that both the temperature- and field-driven spin reorientations are associated with a change in the magnetocrystalline anisotropy, which is strongly coupled to the lattice degrees of freedom. This study elucidates the long-standing puzzles on the zero-field magnetic orders of Sr$_4$Ru$_3$O$_{10}$ and provides new insights into the nature of the field-induced metamagnetic transition.

cond-mat.str-el↗

arXiv2018

Tipping the magnetic instability in paramagnetic Sr$_3$Ru$_2$O$_7$ by Fe impurities

We report the magnetic and electronic properties of the bilayer ruthenate Sr$_3$Ru$_2$O$_7$ upon Fe substitution for Ru. We find that Sr$_3$(Ru$_{1-x}$Fe$_x$)$_2$O$_7$ shows a spin-glass-like phase below 4 K for $x$ = 0.01 and commensurate E-type antiferromagnetically ordered insulating ground state characterized by the propagation vector $q_c$ = (0.25 0.25 0) for $x$ $\geq$ 0.03, respectively, in contrast to the paramagnetic metallic state in the parent compound with strong spin fluctuations occurring at wave vectors $q$ = (0.09 0 0) and (0.25 0 0). The observed antiferromagnetic ordering is quasi-two-dimensional with very short correlation length along the $c$ axis, a feature similar to the Mn-doped Sr$_3$Ru$_2$O$_7$. Our results suggest that this ordered ground state is associated with the intrinsic magnetic instability in the pristine compound, which can be readily tipped by the local magnetic coupling between the 3$d$ orbitals of the magnetic dopants and Ru 4$d$ orbitals.

cond-mat.str-el↗