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Xavier Mougeot

Publications and source records attributed to Xavier Mougeot.

11 recordsLinked to original sources

Aluminum-Based Superconducting Tunnel Junction Sensors for Nuclear Recoil Spectroscopy

The BeEST experiment is searching for sub-MeV sterile neutrinos by measuring nuclear recoil energies from the decay of $^7$Be implanted into superconducting tunnel junction (STJ) sensors. The recoil spectra are affected by interactions between the radioactive implants and the sensor materials. We are therefore developing aluminum-based STJs (Al-STJs) as an alternative to existing tantalum devices (Ta-STJs) to investigate how to separate material effects in the recoil spectrum from potential signatures of physics beyond the Standard Model. Three iterations of Al-STJs were fabricated. The first had electrode thicknesses similar to existing Ta-STJs. They had low responsivity and reduced resolution, but were used successfully to measure $^7$Be nuclear recoil spectra. The second iteration had STJs suspended on thin SiN membranes by backside etching. These devices had low leakage current, but also low yield. The final iteration was not backside etched, and the Al-STJs had thinner electrodes and thinner tunnel barriers to increase signal amplitudes. These devices achieved 2.96 eV FWHM energy resolution at 50 eV using a pulsed 355 nm (~3.5 eV) laser. These results establish Al-STJs as viable detectors for systematic material studies in the BeEST experiment.

physics.ins-det

Shake-up and shake-off spectra in the electron capture decay of atomic $^7$Be

The most stringent laboratory-based experimental limits on the existence of sub-MeV sterile neutrinos are currently set by decay spectroscopy of radioactive $^7$Be embedded into superconducting sensors. The systematic uncertainties are dominated by the modeling of the electron shake-up and shake-off spectra that are not based on state-of-the-art atomic theory and do not include electron correlations or relativistic effects. We have used the multiconfiguration Dirac-Fock formalism to obtain correlated wavefunctions ab initio and compute all single and double shake processes in the electron capture decay of atomic $^7$Be. The simulations can explain some but not all of the observed spectral features, likely because the wave functions are modified by the Ta sensor material that the $^7$Be is embedded into. The new models also show that the L/K electron capture ratio of $^7$Be in Ta has previously been slightly underestimated revising the previous value of 0.070(7) to a new value of 0.0756(20).

physics.atom-ph

Precision measurement and modelling of the threshold-free 210Pb β spectrum

Beta decay is a fundamental process that governs nuclear stability and serves as a sensitive probe of the weak interaction and possible physics beyond the Standard Model of particle physics. However, precise measurements of complete $β$ decay spectra, particularly at low energies, remain experimentally and theoretically challenging. Here we report a high-precision, threshold-free measurement of the full $β$ decay spectrum of 210Pb to excited states of 210Bi, using a transition-edge sensor (TES)-based micro-calorimeter. This approach enables the detection of $β$ particle energies from 0 keV up to their endpoint by coincidence summing with subsequent de-excitation energy, thereby eliminating reconstruction artifacts near zero energy that have traditionally limited low-energy spectral accuracy. To our knowledge, this is the first complete, high-precision $β$ decay spectrum from 0 keV. The data resolve theoretical uncertainties associated with the atomic quantum exchange (AQE) effect. An accompanying ab initio theoretical framework, incorporating atomic, leptonic, and nuclear components, predicts a statistically significant (7.2 {$σ$}) enhancement in $β$ emission probability near zero energy, in agreement with the measurement and in contrast to models that omit AQE corrections. These results provide a new benchmark for $β$ decay theory at low energies, deepen our understanding of the weak interaction, and establish a critical foundation for searches for new physics, including dark matter interactions and precision studies of neutrinos.

nucl-ex

Signal processing and spectral modeling for the BeEST experiment

The Beryllium Electron capture in Superconducting Tunnel junctions (BeEST) experiment searches for evidence of heavy neutrino mass eigenstates in the nuclear electron capture decay of $^7$Be by precisely measuring the recoil energy of the $^7$Li daughter. In Phase-III, the BeEST experiment has been scaled from a single superconducting tunnel junction (STJ) sensor to a 36-pixel array to increase sensitivity and mitigate gamma-induced backgrounds. Phase-III also uses a new continuous data acquisition system that greatly increases the flexibility for signal processing and data cleaning. We have developed procedures for signal processing and spectral fitting that are sufficiently robust to be automated for large data sets. This article presents the optimized procedures before unblinding the majority of the Phase-III data set to search for physics beyond the standard model.

physics.ins-det

Direct Experimental Constraints on the Spatial Extent of a Neutrino Wavepacket

Despite their high relative abundance in our Universe, neutrinos are the least understood fundamental particles of nature. They also provide a unique system to study quantum coherence and the wavelike nature of particles in fundamental systems due to their extremely weak interaction probabilities. In fact, the quantum properties of neutrinos emitted in experimentally relevant sources are virtually unknown and the spatial extent of the neutrino wavepacket is only loosely constrained by reactor neutrino oscillation data with a spread of 13 orders of magnitude. Here, we present the first direct limits of this quantity through a new experimental concept to extract the energy width, $σ_{\textrm{N},E}$, of the recoil daughter nucleus emitted in the nuclear electron capture (EC) decay of $^7$Be. The final state in the EC decay process contains a recoiling $^7$Li nucleus and an electron neutrino ($ν_e$) which are entangled at their creation. The $^7$Li energy spectrum is measured to high precision by directly embedding $^7$Be radioisotopes into a high resolution superconducting tunnel junction that is operated as a cryogenic sensor. The lower limit on the spatial uncertainty of the recoil daughter was found to be $σ_{\textrm{N}, x} \geq 6.2$\,pm, which implies the final-state system is localized at a scale more than a thousand times larger than the nucleus itself. From this measurement, the first direct lower limits on the spatial extent of the neutrino wavepacket were extracted using two different theoretical methods. These results have wide-reaching implications in several areas including the nature of spatial localization at sub-atomic scales, interpretation of neutrino physics data, and the potential reach of future large-scale experiments.

nucl-ex

High precision measurement of the $^{99}$Tc $β$ spectrum

Highly precise measurements of the $^{99}$Tc beta spectrum were performed in two laboratories using metallic magnetic calorimeters. Independent sample preparations, evaluation methods and analyses yield consistent results and the spectrum could be measured down to less than 1 keV. Consistent beta spectra were also obtained via cross-evaluations of the experimental data sets. An additional independent measurement with silicon detectors in a $4π$ configuration confirms the spectrum shape above 25 keV. Detailed theoretical calculations were performed including nuclear structure and atomic effects. The spectrum shape was found to be sensitive to the effective value of the axial-vector coupling constant. Combining measurements and predictions, we extracted $Q_β=$295.82(16) keV and $g_A^{\text{eff}} = 1.530 (83)$. Furthermore, we derived the mean energy of the beta spectrum $\overline{E}_β$=98.45(20) keV, $\log f = -0.47660 (22)$ and $\log ft = 12.3478 (23)$.

nucl-ex

Precise determination of $^{210}$Pb $β$ Decay Spectrum at 0 keV and its Implication to Theoretical Calculations

The atomic exchange effect will lead to a significant increase in the probability density of $β$ decays below a few keV. This effect is very important for scientific experiments that performed by low-energy electron spectroscopy measurements. However, the atomic exchange effect involves multi-electron interactions, especially for a system with 82 electrons such as lead. Different parameters will lead to different trends in the energy spectrum predicted by the theory, so it is urgent to carry out experimental measurements to provide parameter limits for the theory. The probability increase brought about by the atomic exchange effect is most obvious near 0keV, and the $β$ energy spectrum is accurately measured near this energy point, so as to provide constraints for the physical model of atomic exchange. However, it is extremely difficult to measure the $β$ energy spectrum at 0keV due to the limitations of electronic noise and internal conversion effects. The excited decay path of $^{210}$Pb was taken as the observation object,by measuring the total energy spectrum of $β$ rays and cascaded gamma rays, the precise measurement of the $β$ energy spectrum near 0keV has been completed. The analysis of the $β$ energy spectrum of $^{210}$Pb gives the following conclusions. The experimental results first verified the theory that the exchange effect causes the probability increase at the low energy end near 0keV. At the same time, the experimental results are higher than the existing predictions of the atomic exchange effect. At least for Pb element, all the electron shells have played a role in improving the probability density of the low end of the $β$ energy spectrum. This discovery will promote the theoretical calculation of the $β$ energy spectrum of $^{214}$Pb, at the same time, it also indicates that the reactor neutrinos have a higher probability density at the omnipotent end.

nucl-ex

A comprehensive revision of the summation method for the prediction of reactor antineutrino fluxes and spectra

The summation method for the calculation of reactor $\barν_e$ fluxes and spectra is methodically revised and improved. For the first time, a complete uncertainty budget accounting for all known effects likely to impact these calculations is proposed. Uncertainties of a few percents at low energies and ranging up to 20% at high energies are obtained on the calculation of a typical reactor $\barν_e$ spectrum. Although huge improvements have been achieved over the past decade, the quality and incompleteness of the present day evaluated nuclear decay data still limit the accuracy of the calculations and therefore dominate by far these uncertainties. Pushing the $β$-decay modeling of the thousands of branches making a reactor $\barν_e$ spectrum to a high level of details comparatively brings modest changes. In particular, including nuclear structure calculations in the evaluation of the non-unique forbidden transitions gives a smaller impact than anticipated in past studies. Finally, this new modeling is challenged against state-of-the-art predictions and measurements. While a good agreement is observed with the most recent Inverse Beta Decay measurements of reactor $\barν_e$ fluxes and spectra, it is unable to properly describe the reference aggregate $β$ spectra measured at the Institut Laue-Langevin High-Flux reactor in the 80s. This result adds to recent suspicions $β$ the reliability of these data and preferentially points toward a misprediction of the $^{235}$U $\barν_e$ spectrum.

nucl-ex

Proposal for Measurement of the Two-body Neutron Decay using Microcalorimeter

The bound beta-decay (BoB) of neutron is also known as the two-body neutron decay, which is a rare decay mode into a hydrogen atom and an anti-neutrino. The state of neutrino can be exactly inferred by measuring the state of hydrogen atom, providing a possible pathway to explore new physics. However, this rare decay mode has not yet been observed so far since it was predicted in 1947. The challenge in observing this decay is not only that its cross section is extremely low, equivalent to about branching ratio of the order of $10^{-6}$ of the three-body decay, but also that the final-state hydrogen atom is neutral and has extremely low kinetic energy, which cannot be effectively detected. In this study, we propose a microcalorimeter-based scheme for measuring the kinetic energies of hydrogen atoms produced from BoB of ultracold neutrons, which has a great advantage in terms of accuracy of the energy measurement. In this study, first, several important issues that require rigorous considerations for the decay measurements and possible solutions are discussed. Then, the requirements of the neutron flux and the appropriate structure design of the microcalorimeter are present by theoretical calculations. In short, this paper outlines our proposed novel experimental scheme for observing the BoB mode, addressing the possible solutions to all the necessary problems.

hep-ex

Improved calculations of beta decay backgrounds to new physics in liquid xenon detectors

We present high-precision theoretical predictions for the electron energy spectra for the ground-state to ground-state $β$ decays of $^{214}$Pb, $^{212}$Pb, and $^{85}$Kr most relevant to the background of liquid xenon dark matter detectors. The effects of nuclear structure on the spectral shapes are taken into account using large-scale shell model calculations. Final spectra also include atomic screening and exchange effects. The impact of nuclear structure effects on the $^{214}$Pb and $^{212}$Pb spectra below $\approx100$ keV, pertinent for several searches for new physics, are found to be comparatively larger than those from the atomic effects alone. We find that the full calculation for $^{214}$Pb ($^{212}$Pb) predicts 15.0-23.2% (12.1-19.0%) less event rate in a 1-15 keV energy region of interest compared to the spectrum calculated as an allowed transition when using values of the weak axial vector coupling in the range $g_{\rm A}=0.7-1.0$. The discrepancy highlights the importance of both a proper theoretical treatment and the need for direct measurements of these spectra for a thorough understanding of $β$ decay backgrounds in future experiments.

hep-ex

High precision analytical description of the allowed $β$ spectrum shape

A fully analytical description of the allowed $β$ spectrum shape is given in view of ongoing and planned measurements. Its study forms an invaluable tool in the search for physics beyond the standard electroweak model and the weak magnetism recoil term. Contributions stemming from finite size corrections, mass effects, and radiative corrections are reviewed. A particular focus is placed on atomic and chemical effects, where the existing description is extended and analytically provided. The effects of QCD-induced recoil terms are discussed, and cross-checks were performed for different theoretical formalisms. Special attention was given to a comparison of the treatment of nuclear structure effects in different formalisms. Corrections were derived for both Fermi and Gamow-Teller transitions, and methods of analytical evaluation thoroughly discussed. In its integrated form, calculated $f$ values were in agreement with the most precise numerical results within the aimed for precision. We stress the need for an accurate evaluation of weak magnetism contributions, and note the possible significance of the oft-neglected induced pseudoscalar interaction. Together with improved atomic corrections, we then present an analytical description of the allowed $β$ spectrum shape accurate to a few parts in $10^{-4}$ down to 1\,keV for low to medium $Z$ nuclei, thereby extending the work by previous authors by nearly an order of magnitude.

nucl-th