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Xiangliang Li

Publications and source records attributed to Xiangliang Li.

10 recordsLinked to original sources

A nuclear clock based on $^{229}$Th

Atomic clocks have made time and frequency the most precisely measured quantities in physics, progressing from microwave standards that realize the SI second to optical clocks that now reach unprecedented levels of precision. A nuclear clock would shift the frequency reference from an electronic transition to the uniquely low-lying, laser-accessible isomeric transition in the $^{229}$Th nucleus, offering a route to compact, robust timekeeping and sensitive tests of fundamental physics. However, turning recent advances in spectroscopy of the $^{229}$Th nuclear resonance into clock operation requires the nuclear transition to serve as a stable discriminator for steering a traceable oscillator. Here we demonstrate the operation of a $^{229}$Th nuclear clock by stabilizing a continuous-wave narrow-linewidth 148.4 nm vacuum-ultraviolet (VUV) laser to a resolved nuclear transition in a solid-state host. This clock operation is enabled by fast frequency discrimination based on phototube photocurrent readout of the transmitted VUV power. The 10 $\mu$W VUV laser, generated by four-wave mixing in cadmium vapour, provides a high-signal-to-noise absorption signal from a home-grown $^{229}$Th:CaF$_2$ crystal, allowing the laser to be locked to a weakly temperature-sensitive nuclear transition. The clock reaches a fractional frequency instability of $2\times10^{-12}/\sqrt{\tau/s} $, where $\tau$ is the averaging time. Remarkably, nuclear-clock frequencies measured with two distinct crystals agree at the $10^{-13}$ level, demonstrating the reproducibility of solid-state nuclear frequency references. By making a laser-addressed atomic nucleus an operational clock reference, this work extends quantum metrology from electronic to nuclear transitions, and opens a new platform for compact clocks, solid-state nuclear quantum sensors and precision tests of fundamental physics.

physics.atom-ph

A continuous-wave vacuum ultraviolet laser for the nuclear clock

The exceptionally low-energy isomeric transition in $^{229}$Th at around 148.4 nm offers a unique opportunity for coherent nuclear control and the realisation of a nuclear clock. Recent advances, most notably the incorporation of large ensembles of $^{229}$Th nuclei in transparent crystals and the development of pulsed vacuum-ultraviolet (VUV) lasers, have enabled initial laser spectroscopy of this transition. However, the lack of an intense, narrow-linewidth VUV laser has precluded coherent nuclear manipulation. Here we introduce and demonstrate the first continuous-wave laser at 148.4 nm, generated via four-wave mixing (FWM) in cadmium vapor. The source delivers 100 nW of power with a linewidth well below 100 Hz and supports broad wavelength tunability. This represents a five-orders-of-magnitude improvement in linewidth over all previous single-frequency lasers below 190 nm, marking a major advance in laser technology. We develop a spatially resolved homodyne technique to place a stringent upper bound on the phase noise induced by the FWM process and demonstrate sub-hertz linewidth capability. These results eliminate the final technical hurdle to a $^{229}$Th-based nuclear clock, opening new directions in quantum metrology, nuclear quantum optics and precision tests of the Standard Model. More broadly, they establish a widely tunable, ultranarrow-linewidth laser platform for applications across quantum information science, condensed matter physics, and high-resolution VUV spectroscopy.

physics.atom-ph

Stability and decay of subradiant patterns in a quantum gas with photon-mediated interactions

Metastability and its relaxation mechanisms challenge our understanding of the stability of quantum many-body systems, revealing a gap between the microscopic dynamics of the individual components and the effective descriptions used for macroscopic observables. We observe excited self-ordered subradiant patterns in a quantum gas coupled to two optical cavities and report lifetimes far beyond the system's typical timescales. These patterns eventually decay through an abrupt transition reordering the atoms into a superradiant phase. Ab-initio theory fully captures this macroscopic behavior, revealing that the subradiant patterns are stabilized by photon-mediated long-range interactions, thereby manifesting universal features of metastability characteristic of long-range interacting systems, as in astrophysics and plasma physics. Our work sheds light on the microscopic mechanisms stabilizing quantum states of matter and highlights the potential of photon-mediated forces for engineering correlations in many-body quantum systems.

cond-mat.quant-gas

Efficient generation of multiqubit entanglement states using rapid adiabatic passage

We propose the implementation of a rapid adiabatic passage (RAP) scheme to generate entanglement in Rydberg atom-array systems. This method transforms a product state in a multi-qubit system into an entangled state with high fidelity and robustness. By employing global and continuous driving laser fields, we demonstrate the generation of two-qubit Bell state and three-qubit W state, via sequential RAP pulses within the Rydberg blockade regime. As an illustrative example, applying this technique to alkali atoms, we predict fidelities exceeding 0.9995 for two-qubit Bell and three-qubit W state, along with excellent robustness. Furthermore, our scheme can be extended to generate entanglement between weakly coupled atoms and to create four-qubit Greenberger- Horne-Zeilinger states through spatial correlations. Our approach holds the potential for extension to larger atomic arrays, offering a straightforward and efficient method to generate high-fidelity entangled states in neutral atom systems.

quant-ph

High-fidelity and robust controlled-Z gates implemented with Rydberg atoms via echoing rapid adiabatic passage

High-fidelity and robust quantum gates are essential for quantum information processing, where neutral Rydberg atoms trapped in optical tweezer arrays serving as a versatile platform for the implementation. We propose a rapid adiabatic passage (RAP) scheme for achieving a high-fidelity controlled-Z (CZ) gate on a neutral atom Rydberg platform. Utilizing only global laser dressing, our scheme involves echoing two identical RAP pulses within the Rydberg blockade regime to realize a CZ gate and can be readily extended to a C$^k$Z gate with additional qubits. We predict a CZ gate with fidelity over 0.9995 using akali-atom parameters, and a CCZ gate with fidelity exceeding 0.999. Moreover, the direct utilization of echoing RAP pulses enables the implementation of a four-bit CCCZ gate at fidelity over 0.996 without further optimization. The proposed scheme, remarkably robust to variations in driving fields and realistic decoherence effects, holds promise for future quantum information processing applications.

quant-ph

Dissipative time crystal in a strongly interacting Rydberg gas

The notion of spontaneous symmetry breaking has been well established to characterize classical and quantum phase transitions of matter, such as in condensation, crystallization or quantum magnetism. Generalizations of this paradigm to the time dimension can lead to a time crystal phase, which spontaneously breaks the time translation symmetry of the system. Whereas the existence of a continuous time crystal at equilibrium has been challenged by no-go theorems, this difficulty can be circumvented by dissipation in an open system. Here, we report the experimental observation of such dissipative time crystalline order in a room-temperature atomic gas, where ground-state atoms are continuously driven to Rydberg states. The emergent time crystal is revealed by persistent oscillations of the photon transmission, and we show that the observed limit cycles arise from the coexistence and competition between distinct Rydberg components. The nondecaying autocorrelation of the oscillation, together with the robustness against temporal noises, indicate the establishment of true long-range temporal order and demonstrates the realization of a continuous time crystal.

cond-mat.quant-gas

Self-oscillating pump in a topological dissipative atom-cavity system

Pumps are transport mechanisms in which direct currents result from a cyclic evolution of the potential. As Thouless has shown, the pumping process can have topological origins, when considering the motion of quantum particles in spatially and temporally periodic potentials. However, the periodic evolution that drives these pumps has always been assumed to be imparted from outside, as was the case in the experimental systems studied so far. Here we report on an emergent mechanism for pumping in a quantum gas coupled to an optical resonator, where we observe a particle current without applying a periodic drive. The pumping potential experienced by the atoms is formed by the self-consistent cavity field interfering with the static laser field driving the atoms. Due to dissipation, the cavity field evolves between its two quadratures, each corresponding to a different centrosymmetric crystal configuration. This self-oscillation results in a time-periodic potential analogous to that describing the transport of electrons in topological tight-binding models, like the paradigmatic Rice-Mele pump. In the experiment, we directly follow the evolution by measuring the phase winding of the cavity field with respect to the driving field and observing the atomic motion in-situ. The discovered mechanism combines the dynamics of topological and open systems, and features characteristics of continuous dissipative time crystals.

cond-mat.quant-gas

Controlling atomic spin-mixing via multiphoton transitions in a cavity

We propose to control spin-mixing dynamics in a gas of spinor atoms, via the combination of two off-resonant Raman transition pathways, enabled by a common cavity mode and a bichromatic pump laser. The mixing rate, which is proportional to the synthesized spin-exchange interaction strength, and the effective atomic quadratic Zeeman shift (QZS), can both be tuned by changing the pump laser parameters. Quench and driving dynamics of the atomic collective spin are shown to be controllable on a faster time scale than in existing experiments based on inherent spin-exchange collision interactions. The results we present open a promising avenue for exploring spin-mixing physics of atomic ensembles accessible in current experiments.

cond-mat.quant-gas

Measuring the dynamics of a first order structural phase transition between two configurations of a superradiant crystal

We observe a structural phase transition between two configurations of a superradiant crystal by coupling a Bose-Einstein condensate to an optical cavity and applying imbalanced transverse pump fields. We find that this first order phase transition is accompanied by transient dynamics of the order parameter which we measure in real-time. The phase transition and the excitation spectrum can be derived from a microscopic Hamiltonian in quantitative agreement with our experimental data.

cond-mat.quant-gas

Two-mode Dicke model from non-degenerate polarization modes

We realize a non-degenerate two-mode Dicke model with competing interactions in a Bose-Einstein condensate (BEC) coupled to two orthogonal polarization modes of a single optical cavity. The BEC is coupled to the cavity modes via the scalar and vectorial part of the atomic polarizability. We can independently change these couplings and determine their effect on a self-organization phase transition. Measuring the phases of the system, we characterize a crossover from a single-mode to a two-mode Dicke model. This work provides perspectives for the realization of coupled phases of spin and density.

cond-mat.quant-gas