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Xianglin Ke

Publications and source records attributed to Xianglin Ke.

27 records · Page 2Linked to original sources

Interfacial Magnetism in Complex Oxide Heterostructures Probed by Neutrons and X-rays

Magnetic complex-oxide heterostructures are of keen interest because a wealth of phenomena at the interface of dissimilar materials can give rise to fundamentally new physics and potentially valuable functionalities. Altered magnetization, novel magnetic coupling and emergent interfacial magnetism at the epitaxial layered-oxide interfaces are under intensive investigation, which shapes our understanding on how to utilize those materials, particularly for spintronics. Neutron and x-ray based techniques have played a decisive role in characterizing interfacial magnetic structures and clarifying the underlying physics in this rapidly developing field. Here we review some recent experimental results, with an emphasis on those studied via polarized neutron reflectometery and polarized x-ray absorption spectroscopy. We conclude with some perspectives.

cond-mat.mtrl-sci↗

Lattice correlation of Hubbard excitons in a Mott insulator Sr2IrO4 and reconstruction of their hopping dynamics via time-dependent coherence analysis of the Bragg diffraction

In correlated oxides the coupling of quasiparticles to other degrees of freedom such as spin and lattice plays critical roles in the emergence of symmetry-breaking quantum ordered states such as high temperature superconductivity. We report a strong lattice coupling of photon induced Hubbard excitonic quasiparticles in spin-orbital coupling Mott insulator Sr2IrO4. Combining time-resolved optical spectroscopy techniques, we further reconstructed spatiotemporal map of the diffusion of quasiparticles via time-dependent coherence analysis of the x-ray Bragg diffraction peak. Due to the unique electronic configuration of the exciton, the strong lattice correlation is unexpected but extends the similarity between Sr2IrO4 and cuprates under highly non-equilibrium conditions. The coherence analysis method we developed may have important implications for characterizing the structure and carrier dynamics in a wider group of oxide heterostructures.

cond-mat.mtrl-sci↗

Excess-Hole Induced High Temperature Polarized State and its Correlation with the Multiferroicity in Single Crystalline DyMnO3

Controlling the ferroelectricity and magnetism in multiferroic materials has been an important research topic. We report the formation of a highly polarized state in multiferroic DyMnO3 single crystals which develops well above the magnetic transition temperatures, and we attribute it the thermally stimulated depolarization current effect of excess holes forming Mn4+ ions in the system. We also show that this high temperature polarized state intimately correlates with the lower temperature ferroelectric state that is induced by the incommensurate spiral magnetic order of Mn spins. This study demonstrate an efficient approach to tune the multiferroicity in the manganite system.

cond-mat.mtrl-sci↗

Ignoring your neighbors: Moment correlations dominated by indirect or distant interactions in an ordered nanomagnet array

We have studied the moment correlations within triangular lattice arrays of single-domain co-aligned nanoscale ferromagnetic islands. Independent variation of lattice spacing along and perpendicular to the island axis tunes the magnetostatic interactions between islands through a broad range of relative strengths. For certain lattice parameters, the sign of the correlations between near-neighbor island moments is opposite to that favored by the pair-wise interaction. This finding, supported by analysis of the total correlation in terms of direct and convoluted indirect contributions across multiple pairwise interactions, indicates that indirect interactions and/or those mediated by further neighbors can be tuned to be dominant, with implications for the wide range of systems composed of interacting nanomagnets.

cond-mat.mes-hall↗

Effective Temperature in an Interacting, Externally Driven, Vertex System: Theory and Experiment on Artificial Spin Ice

Frustrated arrays of interacting single-domain nanomagnets provide important model systems for statistical mechanics, because they map closely onto well-studied vertex models and are amenable to direct imaging and custom engineering. Although these systems are manifestly athermal, we demonstrate that the statistical properties of both hexagonal and square lattices can be described by an effective temperature based on the magnetostatic energy of the arrays. This temperature has predictive power for the moment configurations and is intimately related to how the moments are driven by an oscillating external field.

cond-mat.stat-mech↗

Tuning magnetic frustration of nanomagnets in triangular-lattice geometry

We study the configuration of magnetic moments on triangular lattices of single-domain ferromagnetic islands, examining the consequences of magnetostatic interactions in this frustrated geometry. By varying the island-island distance along one direction, we are able to tune the ratio of different interactions between neighboring islands, resulting in a corresponding variation in the local correlations between the island moments. Unlike other artificial frustrated magnets, this lattice geometry displays regions of ordered moment orientation, possibly resulting from a higher degree of anisotropy leading to a reduced level of frustration.

cond-mat.mtrl-sci↗

Epitaxial magnetic perovskite nanostructures

Precise arrays of sub-100 nm diameter nanodots are fabricated from magnetic oxide perovskites with the total coverage area up to 5 mm2. Epitaxial single crystal structure of the nanodots is demonstrated by cross-sectional TEM. Low temperature MFM study confirmed the ferromagnetism of the produced particles.

cond-mat.mtrl-sci↗

Influence of the additional second neighbor hopping on the spin response in the t-J model

The influence of the additional second neighbor hopping t' on the spin response of the t-J model in the underdoped and optimally doped regimes is studied within the fermion-spin theory. Although the additional second neighbor hopping t' is systematically accompanied with the reduction of the dynamical spin structure factor and susceptibility, the qualitative behavior of the dynamical spin structure factor and susceptibility of the t-t'-J model is the same as in the case of t-J model. The integrated dynamical spin structure factor spectrum is almost t' independent, and the integrated dynamical spin susceptibility still shows the particularly universal behavior as $I(ω,T)\propto {\rm arctan}[a_{1}ω/T+a_{3}(ω/T)^{3}]$.

cond-mat.str-el↗