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Xiangping Li

Publications and source records attributed to Xiangping Li.

At least 19 recordsLinked to original sources

Defects encode high-dimensional topological information

In polarization fields, Stokes skyrmions are continuous vectorial textures that encode integer-valued topological invariants across real space, enabling robust optical information encoding under complex perturbations. This topological resilience, however, fails when singular points occur where the Stokes vector has no unique limiting value, placing a fundamental constraint on skyrmion-based information manipulation. Here, we show, paradoxically, that the very defects that destroy conventional resilience can become the carriers of topological information. We introduce the resulting structures as Stokes defect skyrmions, in which singular Stokes responses constitute measurable topological degrees of freedom with theoretically minimal size. We design and realize one class of them using all-dielectric metasurfaces that combine arbitrarily controlled distinguished fast-axis singularities with customized retardance profiles. The resulting fields are then described by high-dimensional integer-valued topological tuples, providing theoretically unbounded information capacity at the nanoscale. As a proof-of-concept demonstration, selected tuple components are mapped to represent predefined alphabetic symbols, realizing controlled high-dimensional information representation within a single optical field. Our results establish Stokes defects as functional units for higher-dimensional topological encoding, expanding the role of defects from failure points to engineerable carriers of optical information.

physics.optics

Correlation invariance unlocks robust calibration-free orbital-angular-momentum multiplexing transmission under dynamic scattering scenarios

Orbital angular momentum (OAM) multiplexing offers a promising approach to high-capacity optical communication by harnessing the orthogonality of vortex beams. However, its practical deployment is severely limited in real-world settings where dynamic scattering media, such as turbulent atmosphere, distort multiplexed fields into random speckles and disrupt OAM demultiplexing. Although existing wavefront shaping and deep learning methods can mitigate static distortions, they fail under time-varying scattering conditions, leading to significant crosstalk and unreliable recovery. Here, we introduce a new concept, correlation invariance, which enables scattering-immune, robust OAM multiplexed transmission through dynamic media. By capturing orthogonally polarized speckle holograms in a compact common-path geometry and computing their intensity cross-correlation, dynamically imposed scattering phases are cancelled out while deterministic object information is preserved. This allows single-shot reconstruction of both amplitude and phase of the input OAM-multiplexed fields, without any pre-calibration or training. As a proof of principle, we demonstrate high-fidelity transmission of 24-bit RGB data with 99.61% accuracy under static scattering and 98.97% accuracy under dynamic scattering. This approach addresses a long-standing barrier in OAM-based systems and opens avenues for robust high-capacity optical communications, encryption, and imaging in dynamic scattering environments.

physics.optics

A 160 {\deg} x 160 {\deg} Dynamic Holographic Meta-Projector

Holography can reconstruct immersive light fields for virtual and augmented reality by modulating optical wavefront. Due to huge pixel sizes, current spatial light modulators (SLMs) have small field-of-view (FOV) for holographic displays. Despite various methods for etendue expansion, the largest full-screen FOV for dynamic holography is only 70 {\deg} X 70 {\deg}, which remains insufficient for large-scale, high-resolution, three-dimensional displays. Here, we report a pixel-interpolation-assisted holographic meta-projector that substantially expands the FOV by integrating multiple subwavelength metasurface pixels within each microscale pixel of a traditional SLM. Leveraging large-angle diffraction of the metasurface and implementing k-space distortion correction for ultra-wide angles, we experimentally demonstrate dynamic holographic image reconstruction with a FOV of 160 {\deg} X 160 {\deg} -equivalent to a system numerical aperture of 0.985-at a high framerate of 60 Hz, surpassing the temporal resolution threshold of human vision. This system represents the state-of-the-art near-full-screen holographic dynamic display, thereby opening the door to high-dynamic-range and large-FOV holographic displays.

physics.optics

Observation of polaronic state assisted sub-bandgap saturable absorption

Polaronic effects involving stabilization of localized charge character by structural deformations and polarizations have attracted considerable investigations in soft lattice lead halide perovskites. However, the concept of polaron assisted nonlinear photonics remains largely unexplored, which has a wide range of applications from optoelectronics to telecommunications and quantum technologies. Here, we report the first observation of the polaronic state assisted saturable absorption through subbandgap excitation with a redshift exceeding 60 meV. By combining photoluminescence, transient absorption measurements and density functional theory calculations, we explicate that the anomalous nonlinear saturable absorption is caused by the transient picosecond timescale polaronic state formed by strong carrier exciton phonon coupling effect. The bandgap fluctuation can be further tuned through exciton phonon coupling of perovskites with different Young's modulus. This suggests that we can design targeted soft lattice lead halide perovskite with a specific structure to effectively manipulate exciton phonon coupling and exciton polaron formation. These findings profoundly expand our understanding of exciton polaronic nonlinear optics physics and provide an ideal platform for developing actively tunable nonlinear photonics applications.

physics.optics

Nanophotonic inspection of deep-subwavelength integrated optoelectronic chips

Artificial nanostructures with ultrafine and deep-subwavelength feature sizes have emerged as a paradigm-shifting platform to advanced light field management, becoming a key building block for high-performance integrated optoelectronics and flat optics. However, direct optical inspection of such integrated chips with densely packed complex and small features remains a missing metrology gap that hinders quick feedback between design and fabrications. Here, we demonstrate that photothermal nonlinear scattering microscopy can be utilized for direct imaging and resolving of integrated optoelectronic chips beyond the diffraction limit. We reveal that the inherent coupling among deep-subwavelength nanostructures supporting leaky resonances allows for the pronounced heating effect to access reversible nonlinear modulations of the confocal reflection intensity, leading to optical resolving power down to 80 nm (~lambda/7). The versatility of this approach has been exemplified by direct imaging of silicon grating couplers and metalens with a minimum critical dimension of 100 nm, as well as central processing unit (CPU) chip with 45 nm technology, unfolding the long-sought possibility of in-situ, non-destructive, high-throughput optical inspection of integrated optoelectronic chips and nanophotonic chips.

physics.optics

Topological structures of energy flow: Poynting vector skyrmions

Topological properties of energy flow of light are fundamentally interesting and have rich practical applications in optical manipulations. Here, skyrmion-like structures formed by Poynting vectors are unveiled in the focal region of a pair of counter-propagating cylindrical vector vortex beams in free space. A N\'eel-Bloch-N\'eel skyrmion type transformation of Poynting vectors is observed along the light propagating direction within a volume with subwavelength feature sizes. The corresponding skyrmion type can be determined by the phase singularities of the individual components of the coherently superposed electromagnetic field in the focal region. This work reveals a new family member of optical skyrmions and may introduce novel physical phenomena associated with light scattering and optical force.

physics.optics

Dual-band polarized upconversion photoluminescence enhanced by resonant dielectric metasurfaces

Lanthanide-doped upconversion nanoparticles emerged recently as an attractive material platform underpinning a broad range of innovative applications such as optical cryptography, luminescent probes, and lasing. However, the intricate 4f-associated electronic transition in upconversion nanoparticles leads only to a weak photoluminescence intensity and unpolarized emission, hindering many applications that demand ultrabright and polarized light sources. Here, we uncover a new strategy for achieving ultrabright and dual-band polarized upconversion photoluminescence. We employ resonant dielectric metasurfaces supporting high-quality resonant modes at dual upconversion bands enabling two-order-of-magnitude amplification of upconversion emissions. We demonstrate that dual-band resonances can be selectively switched on polarization, endowing cross-polarization controlled upconversion luminescence with ultra-high degrees of polarization, reaching approximately 0.86 and 0.91 at dual emission wavelengths of 540 nm and 660 nm, respectively. Our strategy offers an effective approach for enhancing photon upconversion processes paving the way toward efficient low-threshold polarization upconversion lasers.

physics.optics

Planar chiral metasurfaces with maximal tunable chiroptical response driven by bound states in the continuum

Optical metasurfaces with high-Q chiral resonances can boost light-matter interaction for various applications of chiral response for ultrathin, active, and nonlinear metadevices. Usually, such metasurfaces require sophisticated depth-resolved nanofabrication to realize subwavelength stereo-nanostructures, posing overwhelming challenges, especially in the short-wavelength range. Here, we suggest a novel planar design for chiral metasurfaces supporting bound states in the continuum (BICs) and demonstrate experimentally chiroptical responses with record-high Q-factors (Q=390) and near-perfect circular dichroism (CD=0.93) at optical frequencies. The symmetry-reduced meta-atoms are highly birefringent and support winding elliptical eigen-polarizations with opposite helicity surrounding the BIC polarization singularity, providing a convenient way for achieving maximal planar chirality tuned by either breaking in-plane symmetry or changing illumination direction. Such sharply resonant chirality realized in planar metasurfaces promises various practical applications in classical and quantum optics including chiral sensing, enantiomer selection, and chiral quantum emitters.

physics.optics

Generating tightly focused perfect optical vortex for ultra-secure optical encryption

Light's orbital angular momentum (OAM) with inherent mode orthogonality has been suggested as a new way to the optical encryption. However, the dependence of annular intensity profiles on the topological charge complicates nanoscale light-matter interactions and hampers the ultra-secure encryption application. In this paper, we demonstrate ultra-secure image encryption by tightly focusing perfect optical vortex (POV) beams with controllable annular intensity profiles and OAM states. A simple scheme composed of single spatial light modulator is proposed to generate radius-controllable POV in tightly focused beams. Such focused POV beams with identical intensity profiles but varied OAM states are applied to disorder-coupled gold nanorod aggregates to selectively excite electromagnetic hot spots for encoding information through photothermal deformation. As such, ultra-secure image encryption in OAM states of POV beams in combination with different polarizations can be achieved. Our results lay the ground for diverse nanophotonic applications harnessing the OAM division of POV beams.

physics.optics

Perfect diffraction metagratings supporting bound states in the continuum and exceptional points

Resonance coupling in non-Hermitian systems can lead to exotic features, such as bound states in the continuum (BICs) and exceptional points (EPs), which have been widely employed to control the propagation and scattering of light. Yet, similar tools to control diffraction and engineering spatial wavefronts have remained elusive. Here, we show that, by operating a suitably tailored metagrating around a BIC and EPs, it is possible to achieve an extreme degree of control over coupling to different diffraction orders in metasurfaces. We stack subwavelength metallic slit arrays on a metal-insulator-metal waveguide, enabling a careful control of the coupling between localized and guided modes. By periodically tuning the coupling strength from weak to strong, we largely tailor the overall spectrum and enable the emergence of singular features, like BICs and EPs. Perfect unitary diffraction efficiency with large spectrum selectivity is achieved around these singular features, with promising applications for arbitrary wavefront shaping combined with filtering and sensing.

physics.optics

Cylindrical vector beams reveal radiationless anapole condition in a resonant state

Nonscattering optical anapole condition is corresponding to the excitation of radiationless field distributions in open resonators, which offers new degrees of freedom for tailoring light-matter interaction. Conventional mechanisms for achieving such a condition relies on sophisticated manipulation of electromagnetic multipolar moments of all orders to guarantee superpositions of vanished moment strengths at the same wavelength. In contrast, here we report on the excitation of optical radiationless anapole hidden in a resonant state of a Si nanoparticle utilizing tightly focused radially polarized (RP) beam. The coexistence of magnetic resonant state and anapole condition at the same wavelength further enables the triggering of resonant state by tightly focused azimuthally polarized (AP) beam whose corresponding electric multipole coefficient could be zero. As a result, high contrast inter-transition between radiationless anapole condition and ideal magnetic resonant scattering can be achieved experimentally in visible spectrum. The proposed mechanism is general which can be realized in different types of nanostructures. Our results showcase that the unique combination of structured light and structured Mie resonances could provide new degrees of freedom for tailoring light-matter interaction, which might shed new light on functional meta-optics.

physics.optics

Near-perfect fidelity polarization-encoded multilayer optical data storage based on aligned gold nanorods

Encoding information in light polarization is of great importance in facilitating optical data storage (ODS) for information security and data storage capacity escalation. However, despite recent advances in nanophotonic techniques vastly enhancing the feasibility of applying polarization channels, the data fidelity in reconstructed bits has been constrained by severe crosstalks occurring between varied polarization angles during data recording and reading process, which gravely hindered the utilization of this technique in practice. In this paper, we demonstrate an ultra-low crosstalk polarization-encoding multilayer optical data storage technique for high-fidelity data recording and retrieving by utilizing a nanofibre-based nanocomposite film involving highly aligned gold nanorods (GNRs). With parallelizing the gold nanorods in the recording medium, the information carrier configuration minimizes miswriting and misreading possibilities for information input and output, respectively, compared with its randomly self-assembled counterparts. The enhanced data accuracy has significantly improved the bit recall fidelity that is quantified by a correlation coefficient higher than 0.99. It is anticipated that the demonstrated technique can facilitate the development of multiplexing ODS for a greener future.

physics.optics

Observation of Topologically Robust Localized Magnetic Plasmon Skyrmions

Optical skyrmions have recently been constructed by tailoring electric or spin field distributions through the interference of multiple surface plasmon polaritons, offering promising features for advanced information processing, transport and storage. Here, we construct topologically robust plasmonic skyrmions in a wisely tailored space-coiling meta-structure supporting magnetic localized spoof plasmons (LSPs), which are strongly squeezed down to {\lambda}3/106 and do not require stringent external interference conditions. By directly measuring the spatial profile of all three vectorial magnetic fields, we reveal multiple {\pi}-twist target skyrmion configurations mapped to multi-resonant near-equidistant LSP eigen-modes. The real-space topological robustness of these skyrmion configurations is confirmed by arbitrary deformations of the meta-structure, demonstrating flexible skyrmionic textures with arbitrary shapes. The observed magnetic LSP skyrmions pave the way to ultra-compact and topologically robust plasmonic devices, such as flexible sensors, wearable electronics and ultra-compact antennas.

physics.optics

Topological-darkness-assisted phase regulation for atomically thin meta-optics

Two-dimensional (2D) noble-metal dichalcogenides have emerged as a new platform for the realization of versatile flat optics with a considerable degree of miniaturization. However, light field manipulation at the atomic scale is widely considered unattainable since the vanishing thickness and intrinsic losses of 2D materials completely suppress both resonances and phase accumulation effects. Empowered by conventionally perceived adverse effects of intrinsic losses, we show that the structured PtSe2 films integrated with a uniform substrate can regulate nontrivial singular phase and realize atomic-thick meta-optics in the presence of topological darkness. We experimentally demonstrate a series of atomic-thick binary meta-optics that allows angle-robust and high unit-thickness diffraction efficiency of 0.96%/nm in visible frequencies, given its thickness of merely 4.3 nm. Our results unlock the potential of a new class of 2D flat optics for light field manipulation at an atomic thickness.

physics.optics

Great Chiral Fluorescence from Optical Duality Silver Nanostructures Enabled by 3D Laser Printing

Featured by prominent flexibility and fidelity in producing sophisticated stereoscopic structures transdimensionally, three-dimensional (3D) laser printing technique has vastly extended the toolkit for delivering diverse functional devices. Yet chiral nanoemitters heavily resorting to artificial structures that manifest efficient emission and tightly confined light-mater interactions simultaneously remains alluring but dauntingly challenging for this technique at this moment. In this work, we assert the chiral photoluminescence is implemented from silver nanostructures of optical duality in one go via a twofold three-dimensional laser printing scheme. Such laser printing protocol allows the highly desired duality by simultaneously producing uniformly distributed fluorescent silver nanoclusters and aggregated plasmonic silver nanoparticles to tightly confine chiral interactions at the nanoscale. A helical emitter of 550 nm-helix-diameter as fabricated has seen a record-high luminescence anisotropic factor with the absolute value up to 0.58, which is two orders of magnitude greater than fluorescent chiral silver clusters. This method holds great promise for future versatile applications in chiroptical nanodevices.

physics.optics

Anapole mediated giant photothermal nonlinearity in nanostructured silicon

Featured with a plethora of electric and magnetic Mie resonances, high index dielectric nanostructures offer a versatile platform to concentrate light-matter interactions at the nanoscale. By integrating unique features of far-field scattering control and near-field concentration from radiationless anapole states, here, we demonstrate a giant photothermal nonlinearity in single subwavelength-sized silicon nanodisks. The nanoscale energy concentration and consequent near-field enhancements mediated by the anapole mode yield a reversible nonlinear scattering with a large modulation depth and a broad dynamic range, unveiling a record-high nonlinear index change up to 0.5 at mild incident light intensities on the order of MW/cm2. The observed photothermal nonlinearity showcases three orders of magnitude enhancement compared with that of unstructured bulk silicon, as well as nearly one order of magnitude higher than that through the radiative electric dipolar mode. Such nonlinear scattering can empower distinctive point spread functions in confocal reflectance imaging, offering the potential for far-field localization of nanostructured Si with an accuracy approaching 40 nm. Our findings shed new light on active silicon photonics based on optical anapoles.

physics.optics

Arbitrary Polarization Conversion Dichroism Metasurfaces for All-in-One Full Poincar\'e Sphere Polarizers

The control of polarization, an essential property of light, is of wide scientific and technological interest. Polarizer is an indispensable optical element for direct polarization generations. Except common linear and circular polarizations, however, arbitrary polarization generation heavily resorts to bulky optical components by cascading linear polarizers and waveplates. Here, we present a general strategy for designing all-in-one full Poincar\'e sphere polarizers based on perfect arbitrary polarization conversion dichroism, and realize it in a monolayer all-dielectric metasurface. It allows preferential transmission and conversion of one polarization state locating at an arbitrary position of the Poincar\'e sphere to its handedness-flipped state, while completely blocking its orthogonal state. In contrast to previous work with limited flexibility to only linear or circular polarizations, our method manifests perfect dichroism close to 100% in theory and exceeding 90% in experiments for arbitrary polarization states. Leveraging this tantalizing dichroism, our demonstration of monolithic full Poincar\'e sphere polarization generators directly from unpolarized light can enormously extend the scope of meta-optics and dramatically push the state-of-the-art nanophotonic devices.

physics.optics

Transmissive Metagrating for Arbitrary Wavefront Shaping Over the Full Visible Spectrum

Metagratings have been shown to form an agile and efficient platform for extreme wavefront manipulation, going beyond the limitations of gradient metasurfaces. Previous approaches for transmissive metagratings have resorted on compound asymmetric inclusions to achieve single-channel near-perfect diffraction. However, such complex inclusions are sensitive to geometric parameters and lack the flexibility for arbitrary phase modulation, restricting applications to beam deflection. Here, we show perfect unitary diffraction in all-dielectric transmissive metagratings using rectangular inclusions by tailoring their multipole interferences. Using this principle, we experimentally demonstrate analog phase profile encoding of a hologram through displacement modulation of CMOS-compatible silicon nitride nanobars, manifesting broadband and wide-angle high diffraction efficiencies for both polarizations and across the entire visible range. Featured with extreme angle/wavelength/polarization tolerance and alleviated structural complexity for both design and fabrication, our demonstration unlocks the full potential of metagrating-based wavefront manipulation for a variety of practical applications.

physics.optics