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Xianjing Zhou

Publications and source records attributed to Xianjing Zhou.

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Fast coherent control of a charge qubit on solid neon with a spin-qubit-compatible resonator

Electrons floating in vacuum provide a clean platform for quantum information processing owing to their isolation from material defects. In particular, electrons on solid neon have emerged as a promising qubit platform because of their potentially long coherence times. Here, toward spin-qubit realization, we couple a single electron on solid neon to a magnetic-field-compatible superconducting NbTiN nanowire resonator. We realize a charge qubit and demonstrate microwave readout and coherent control, with Rabi frequencies up to 76 MHz, an order of magnitude larger than in previous studies. Under strong driving, we observe a qubit frequency shift from nonlinear interactions with the intense microwave field. Deterministic electron trapping at an intended position remains challenging due to solid neon surface roughness; we characterize the electron's position from its differential coupling to distinct electrodes. Although not trapped at an intended position, our estimates indicate that spin-qubit demonstrations remain feasible.

cond-mat.mes-hall

Solid neon as a noise-resilient host for electron qubits above 100 mK

Solid neon can be used as a solid host for single-electron qubits, and at temperatures of around 10 mK, electron-on-solid-neon charge qubits exhibit long coherence times and high operation fidelities. However, systematic characterization of the noise features of such systems is needed for the development of scalable quantum information architectures. Here, we show that solid neon can be used as a noise-resilient host for electron qubits above 100 mK. We examine the resilience of solid neon against charge and thermal noise when electron-on-solid-neon charge qubits are operated away from the charge-insensitive sweet spot and at elevated temperatures. We show that the extracted high-frequency charge noise density of electron-on-solid-neon qubits, projected as voltage fluctuations on nearby electrodes, is between $10^{-4}$ and $10^{-6}~\mathrm{μV^2/Hz}$ at 0.01 to 1 MHz, which is comparable with common semiconductor hosts. We also show that the electron-on-solid-neon charge qubits operating around 5 GHz frequencies can maintain echo coherence times of over 1 $μ$s at temperatures up to 400 mK.

quant-ph

Coherent manipulation of interacting electron qubitson solid neon

Electrons trapped on solid neon surfaces serve as low-noise charge qubits with long coherence times and high operational fidelities. Such charge qubits offer full electrical control and compact device footprints, convenient for scaling up with quantum circuits. Realizing two-qubit gates on this platform is a critical step towards practical quantum information processing. In this work, we report the first experimental demonstration of coherent manipulation of multiple interacting electron-on-solid-neon (eNe) charge qubits. By exploiting the electrons naturally confined in close proximity by the surface structures of solid neon, we have achieved a direct qubit-qubit coupling strength of up to 62.5 MHz, as well as implemented cross-resonance (CR) and bSWAP two-qubit gates using global microwave drives. The natural electron confinement by solid neon mitigates the high-density-wiring challenge, simplifies the multi-qubit control, and establishes a unique path to scale up the eNe qubit platform.

quant-ph

Uniaxial spin texture in a superconducting electron gas revealed by exchange interactions

Two-dimensional superconductors with spin-textured Fermi surfaces can be a platform for realizing unconventional pairing states and are of substantial interest in the context of quantum information science, and superconducting spintronics/orbitronics. We observed an unusual in-plane uniaxial anisotropy in the superconducting 2D electron gas (2DEG) formed at EuOx/KTaO3 (110) interfaces, where the EuOx is magnetic. This anisotropy is not evident in AlOx/KTaO3 (110) where the overlayer is non-magnetic. Our results are consistent with a highly anisotropic 'half-Rashba' spin-textured Fermi surface in 2DEGs formed at the KTaO3 (110) interface that is hidden from external magnetic fields due to a near cancellation between orbital and spin moments but revealed by exchange interactions of the electrons in the 2DEG with Eu moments near the EuOx/KTaO3 (110) interface. The interactions between the uniaxial spin texture and the magnetic overlayer offer new ways to explore the interplay between magnetism and 2D superconductivity.

cond-mat.supr-con

Quantum computing using floating electrons on cryogenic substrates: Potential And Challenges

In this review, we introduce a developing qubit platform: floating-electron-based qubits. Electrons floating in a vacuum above the surface of liquid helium or solid neon emerge as promising candidates for qubits, especially due to their expected long coherence times. Despite being in the early stages, a variety of recent experiments from different groups have shown substantial potential in this role. We survey a range of theoretical proposals and recent experiments, primarily focusing on the use of the spin state as the qubit state, wherein the spin and charge states are hybridized. Throughout these proposals and experiments, the charge state is coupled to an LC resonator, which facilitates both the control and readout mechanisms for the spin state via an artificially introduced spin-charge coupling.

quant-ph

Electron charge qubits with 0.1 millisecond coherence time

Electron charge qubits are compelling candidates for solid-state quantum computing because of their inherent simplicity in qubit design, fabrication, control, and readout. However, all existing electron charge qubits, built upon conventional semiconductors and superconductors, suffer from severe charge noise that limits the coherence time to the order of 1 microsecond. Here, we report our experimental realization of ultralong-coherence electron charge qubits, based upon isolated single electrons trapped on an ultraclean solid neon surface in vacuum. Quantum information is encoded in the motional states of an electron that is strongly coupled with microwave photons in an on-chip superconducting resonator. The measured relaxation time $T_1$ and coherence time $T_2$ are both on the order of 0.1 milliseconds. The single-shot readout fidelity without using a quantum-limited amplifier is 98.1%. The average single-qubit gate fidelity using Clifford-based randomized benchmarking is 99.97%. Simultaneous strong coupling of two qubits with the same resonator is demonstrated, as a first step toward two-qubit entangling gates for universal quantum computing. These results manifest that the electron-on-solid-neon (eNe) charge qubits outperform all existing charge qubits to date and rival state-of-the-art superconducting transmon qubits, offering an appealing platform for quantum computing.

quant-ph

Tunable superconductivity at the oxide-insulator/KTaO$_3$ interface and its origin

Superconductivity forms out of the condensation of Cooper pairs of electrons. The mechanism by which Cooper pairs are created in non-conventional superconductors is often elusive because experimental signatures that connect a specific pairing mechanism to the properties of superconducting state are rare. The recently discovered superconducting oxide-insulator/KTaO$_3$ interface may offer clues about its origins. Here we observe distinct dependences of the superconducting transition temperature Tc on carrier density n$_{2D}$ for electron gases formed at KTaO$_3$ (111), (001) and (110) interfaces. For the KTaO$_3$ (111) interface, a remarkable linear dependence of Tc on n$_{2D}$ is observed over a range of nearly one order of magnitude. Further, our study of the dependence of superconductivity on gate electric fields reveals the role of the interface in mediating superconductivity, which also allows for a reversible electric switching of superconductivity at T = 2 K. We found that the extreme sensitivity of superconductivity to crystallographic orientation can be explained by Cooper pairing via inter-orbital interactions induced by the inversion-breaking transverse optical (TO1) phonons and quantum confinement. This mechanism is also consistent with the dependence of Tc on n$_{2D}$ at the KTaO$_3$ (111) interface. Our study may shed light on the pairing mechanism in other superconducting quantum-paraelectrics.

cond-mat.supr-con

Single electrons on solid neon as a solid-state qubit platform

Progress toward the realization of quantum computers requires persistent advances in their constituent building blocks - qubits. Novel qubit platforms that simultaneously embody long coherence, fast operation, and large scalability offer compelling advantages in the construction of quantum computers and many other quantum information systems. Electrons, ubiquitous elementary particles of nonzero charge, spin, and mass, have commonly been perceived as paradigmatic local quantum information carriers. Despite superior controllability and configurability, their practical performance as qubits via either motional or spin states depends critically on their material environment. Here we report our experimental realization of a new qubit platform based upon isolated single electrons trapped on an ultraclean solid neon surface in vacuum. By integrating an electron trap in a circuit quantum electrodynamics architecture, we achieve strong coupling between the motional states of a single electron and a single microwave photon in an on-chip superconducting resonator. Qubit gate operations and dispersive readout are implemented to measure the energy relaxation time $T_1$ of $15~μ$s and phase coherence time $T_2$ over $200~$ns. These results indicate that the electron-on-solid-neon qubit already performs near the state of the art as a charge qubit.

quant-ph

Space-time crystalline order of a high-critical-temperature superconductor with intrinsic Josephson junctions

We theoretically demonstrate that the high-critical-temperature superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ (BSCCO) is a natural candidate for the recently envisioned classical space-time crystal. BSCCO intrinsically forms a stack of Josephson junctions. Under a periodic parametric modulation of the Josephson critical current density, the Josephson currents develop coupled space-time crystalline order, breaking the continuous translational symmetry in both space and time. The modulation frequency and amplitude span a (nonequilibrium) phase diagram for a so-defined spatiotemporal order parameter, which displays rigid pattern formation within a particular region of the phase diagram. Based on our calculations using representative material properties, we propose a laser-modulation experiment to realize the predicted space-time crystalline behavior. Our findings bring new insight into the nature of space-time crystals and, more generally, into nonequilibrium driven condensed matter systems.

cond-mat.mes-hall

Discovery of two-dimensional anisotropic superconductivity at KTaO$_3$ (111) interfaces

The unique electronic structure found at interfaces between materials can allow unconventional quantum states to emerge. Here we observe superconductivity in electron gases formed at interfaces between (111) oriented KTaO$_3$ and insulating overlayers of either EuO or LaAlO$_3$. The superconducting transition temperature, approaching 2.2 K, is about one order of magnitude higher than that of the LaAlO$_3$/SrTiO$_3$ system. Strikingly, similar electron gases at (001) KTaO$_3$ interfaces remain normal down to 25 mK. The critical field and current-voltage measurements indicate that the superconductivity is two dimensional. Higher mobility EuO/KTaO$_3$ (111) samples show a large in-plane anisotropy in transport properties at low temperatures prior to onset of superconductivity, suggesting the emergence of a stripe like phase where the superconductivity is nearly homogeneous in one direction, but strongly modulated in the other.

cond-mat.supr-con

On-chip sensing of hotspots in superconducting terahertz emitters

Intrinsic Josephson junctions in high-temperature superconductor Bi2Sr2CaCu2O8 are known for their capability to emit high-power terahertz photons with widely tunable frequencies. Hotspots, as inhomogeneous temperature distributions across the junctions, are believed to play a critical role in synchronizing the gauge-invariant phase difference among the junctions, so as to achieve coherent strong emission. Previous optical imaging techniques have indirectly suggested that the hotspot temperature can go higher than the superconductor critical temperature. However, such optical approaches often disturb the local temperature profile and are too slow for device applications. In this paper, we demonstrate an on-chip in situ sensing technique that can precisely quantify the local temperature profile. This is achieved by fabricating a series of micro "sensor" junctions on top of an "emitter" junction and measuring the critical current on the sensors versus the bias current applied to the emitter. This fully electronic on-chip design could enable efficient close-loop control of hotspots in BSCCO junctions and significantly enhance the functionality of superconducting terahertz emitters.

cond-mat.supr-con

Quantum optics of single electrons in quantum liquid and solid helium-4

Single electrons can be conceived as the simplest quantum nodes in a quantum network. Between electrons, single photons can act as quantum channels to exchange quantum information. Despite this appealing picture, in conventional materials, it is extremely difficult to make individual electrons and photons coherently interact with each other at the visible-infrared wavelengths suitable for long-distance communication. Here we theoretically demonstrate that the self-confined single-electron structure in condensed helium-4 can be a fascinating candidate for single-electron quantum nodes. Each electron in helium forms a bubble of 1 to 2 nm radius and coherently interacts with mid-infrared photons. A parametrically amplified femtosecond laser can drive the electrons into any superposition between the ground and excited states. An electron inside a slot-waveguide cavity can strongly couple with cavity photons and exhibits vacuum Rabi oscillations. Two electrons in the cavity naturally generate entanglement through their respective coupling to the lossy cavity. The electron-in-helium system offers unique insight in understanding nonequilibrium quantum dynamics.

quant-ph

Experimental observation of exceptional surface in synthetic dimensions with magnon polaritons

Exceptional points (EPs) are singularities of energy levels in non-Hermitian systems. In this Letter, we demonstrate the surface of EPs on a magnon polariton platform composed of coupled magnons and microwave photons. Our experiments show that EPs form a three-dimensional exceptional surface (ES) when the system is tuned in a four-dimensional synthetic space. We demonstrated that there exists an exceptional saddle point (ESP) in the ES which originates from the unique couplings between magnons and microwave photons. Such an ESP exhibits unique anisotropic behaviors in both the real and imaginary part of the eigenfrequencies. To the best of our knowledge, this is the first experimental observation of ES, opening up new opportunities for high-dimensional control of non-Hermitian systems.

cond-mat.mes-hall

Poly(ionic liquid)s: platform for CO2 capture and catalysis

Capture and conversion of CO2 are of great importance for environment-friendly and sustainable development of human society. Poly(ionic liquid)s (PILs) combine some unique properties of ILs with that of polymers and are versatile materials for CO2 utilization. In this contribution, we briefly outline innovative poly(ionic liquid)s emerged over the past few years, such as polytriazoliums, deep eutectic monomer (DEM) based PILs, and polyurethane PILs. Additionally, we discuss their advantages and challenges as materials for Carbon Capture and Storage (CCS), and the fixation of CO2 into useful materials.

physics.chem-ph

3D simulations of the electrothermal and THz emission properties of Bi$_2$Sr$_2$CaCu$_2$O$_8$ intrinsic Josephson junction stacks

We used 2D coupled sine-Gordon equations combined with 3D heat diffusion equations to numerically investigate the thermal and electromagnetic properties of a $250 \times 70\,μ\mathrm{m}^2$ intrinsic Josephson junction stack. The 700 junctions are grouped to 20 segments; we assume that in a segment all junctions behave identically. At large input power a hot spot forms in the stack. Resonant electromagnetic modes, oscillating either along the length ((0, $n$) modes) or the width (($m$, 0) modes) of the stack or having a more complex structure, can be excited both with and without a hot spot. At fixed bath temperature and bias current several cavity modes can coexist in the absence of a magnetic field. The (1, 0) mode, considered to be the most favorable mode for THz emission, can be stabilized by applying a small magnetic field along the length of the stack. A strong field-induced enhancement of the emission power is also found in experiment, for an applied field around 5.9 mT.

cond-mat.supr-con