arXiv subjects

Xiao-Long Zhou

Publications and source records attributed to Xiao-Long Zhou.

7 recordsLinked to original sources

arXiv2026

Observation of multiphoton entanglement in resonance fluoresce

Resonance fluorescence, the process in which a single two-level quantum emitter interacts with a near-resonant coherent light, is a cornerstone of quantum optics as a paradigmatic light-matter interaction. Quantum phenomena in resonance fluorescence have been accounted for in terms of one- and two-photon processes; however, the physical processes arising from the interaction of a single two-level atom with higher photon numbers remain unexplored experimentally. Here we experimentally reveal the multiphoton scattering nature of resonance fluorescence, which intrinsically gives rise to multiphoton entanglement. By accessing quantum fluctuations in the field emitted from a cavity-quantum electrodynamics system, we resolve third- and fourth-order photon scattering events from a single two-level atom. In the three-photon component, the scattered photons are shown to be genuinely energy-time entangled, as verified by a violation of Svetlichny's inequality. As a demonstration of an application, a quantum secret sharing protocol (QSS) is implemented using this entangled photon source. Our study refines the descriptive framework of resonance fluorescence and broadens the scope of its investigation. It also establishes a fundamentally simple route for generating multiphoton entangled states for quantum information processing and quantum metrology.

physics.atom-ph↗

arXiv2026

Bell nonlocality with directly generated telecom-band spin-photon entanglement

Quantum nonlocality, typically revealed through entanglement distribution across quantum networks, is a cornerstone of quantum information science. Long-distance distribution of entanglement requires the information carrier, i.e. flying photons, to operate in the minimum-loss telecom band of optical fiber. While extensive efforts have been devoted to the direct generation of entanglement between C-band telecom photons and various stationary spins, the verification of quantum nonlocality remains an outstanding challenge. Here, utilizing a dipole transition in rubidium atoms with a wavelength of 1530 nm and a cavity-assisted protocol, we achieve resonant excitation and direct emission of C-band telecom photons from a single atom, generating spin-photon entanglement with a measured Bell state fidelity exceeding 91.4%. We then verify Bell nonlocality by observing a Bell inequality violation of 2.455(77) > 2 using this high-quality entangled pair. These results extend the wavelength of a single-atom quantum emitter to the telecom C-band, achieving sufficiently high-fidelity spin-photon entanglement to finally verify Bell nonlocality. This work thereby provides a promising building block for a large-scale atom-based quantum network capable of distributed quantum metrology and long-distance quantum communication.

quant-ph↗

arXiv2024

Ultrafast high-fidelity state readout of single neutral atom

The capability to measure the state of a quantum system is vital to a practical quantum network, for applications including distributed quantum computing and long-distance quantum communication. As a thriving platform for quantum information technology, single neutral atoms suffer from low achievable photon scattering rate and shallow trapping potential, which limits the fidelity and speed of state readout process. Here, by coupling an single neutral atom with a high-finesse fiber-based Fabry-Pérot microcavity (FFPC) in Purcell regime, we realize strong enhancement of the atomic photoemission rate, which enables ultrafast and high-fidelity discrimination of bright and dark hyperfine states of the atom. The readout fidelity can reach 99.1(2)% within 200 ns and 99.985(8)% within 9 $μ$s. Furthermore, we demonstrate that state preparation via optical pumping can be efficiently accelerated by real-time decision protocol based on ultrafast state readout. This work paves the way to the implementation of quantum networking protocols with high communication rate and high fidelity.

quant-ph↗

arXiv2024

Purcell-Enhanced Generation of Photonic Bell States via the Inelastic Scattering of Single Atoms

Single atoms trapped in optical cavities exhibit immense potential as key nodes in future quantum information processing. They have already demonstrated significant advancement in various quantum technologies, particularly regarding the generation of nonclassical light. Here, we efficiently produce genuine photonic Bell states through the inelastic scattering process of single two-level intracavity atoms. An experimental violation of the Bell inequality, arising from the interference between the probability amplitudes of two photons, validates the intrinsic nature of energy-time entanglement. Coupling atoms with an optical cavity in the Purcell regime substantially enhances the two-photon scattering. This Bell state generation process does not require atomic spin control, thereby rendering it inherently immune to decoherence effects. This work advances the comprehension of resonance fluorescence and has the potential to broaden the landscape of quantum technologies and facilitate the application of photonic Bell states.

quant-ph↗

arXiv2024

Continuously and widely tunable frequency-stabilized laser based on an optical frequency comb

Continuously and widely tunable lasers actively stabilized on a frequency reference are broadly employed in atomic, molecular and optical (AMO) physics. The frequency-stabilized optical frequency comb (OFC) provides a novel optical frequency reference with a broadband spectrum that meets the requirement of laser frequency stabilization. Therefore, we demonstrate a frequency-stabilized and precisely tunable laser system based on it. In this scheme, the laser frequency locked to the OFC is driven to jump over the ambiguity zones, which blocks the wide tuning of the locked laser, and tuned until the mode hopping happens with the always-activated feedback loop. Meanwhile, we compensate the gap of the frequency jump with a synchronized acoustic optical modulator to ensure the continuity. This scheme is applied to an external cavity diode laser (ECDL) and we achieve tuning at a rate of about 7 GHz/s with some readily available commercial electronics. Furthermore, we tune the frequency-stabilized laser only with the feedback of diode current and its average tuning speed can exceed 100 GHz/s. Due to the resource-efficient configuration and the simplicity of completion, this scheme can be referenced and find wide applications in AMO experiments.

physics.atom-ph↗

arXiv2024

Photoassociation of multiple cold molecules in a dipole trap

The generation of cold molecules is a core topic in the field of cold atoms and molecules, which has advanced relevant research like ultracold chemistry, quantum computation, and quantum metrology. With high atomic phase space density, optical dipole trap has been widely performed to prepare and trap cold molecules, and can also be further developed for multiple cold molecule formation and dynamics study. In this work, Rb2 molecules are photoassociated in the magneto-optical trap to obtain precise rovibrational spectroscopy, which provides accurate numerical references for multiple photoassociations. By achieving the harsh requirements of photoassociation in the optical dipole trap, the cold molecule photoassociation process is well explored, and different rovibrational cold molecules are formed in the optical dipole trap for the first time. This method can be universally extended to simultaneously photoassociate various molecules with different internal states or atomic species in just one optical dipole trap, and then advance generous cold molecule research such as cold molecule collision dynamics.

physics.atom-ph↗

arXiv2020

The Gravitational Wave Emission of Double White Dwarf Coalescences

Type Ia Supernovae (SNe Ia) are widely used as standard candles to probe the Universe. However, how these fierce explosions are produced itself is still a highly debated issue. There are mainly two popular models for SNe Ia, i.e. the double-degenerate scenario and the single-degenerate scenario. The double-degenerate scenario suggests that SNe Ia are produced by the coalescence of two degenerate white dwarfs, while the single-degenerate scenario suggests that the continuous accretion of a single degenerate white dwarf from its normal stellar companion will finally lead to a disastrous explosion when it is over-massive, resulting in an SN Ia. The rapid development of the gravitational wave astronomy sheds new light on the nature of SNe Ia. In this study, we calculate the gravitational wave emissions of double white dwarf coalescences and compare them with the sensitivities of several upcoming detectors. It is found that the gravitational wave emissions from double white dwarf mergers in the locale universe are strong enough to be detected by LISA. We argue that LISA-like gravitational wave detectors sensitive in the frequency range of 0.01 - 0.1 Hz will be a powerful tool to test the double-degenerate model of SNe Ia, and also to probe the Universe.

astro-ph.HE↗