arXiv subjects

Xiao-Xiao Zhang

Publications and source records attributed to Xiao-Xiao Zhang.

At least 19 recordsLinked to original sources

arXiv2026

Third-order nonlinear transport in a percolative two-dimensional superconductor

Percolative superconductivity frequently arises in two-dimensional van der Waals materials due to reduced dimensionality, enhanced quantum fluctuations, and complex electron-phonon interactions, providing a unique platform where normal electrons coexist with Cooper pairs. We report the observation of substantial third-order nonlinear transport in a trilayer $1T^\prime$-MoTe$_2$ superconductor within its percolative transition regime. The third-harmonic longitudinal voltage ($V_{\|}^{3ω}$) exhibits a clear cubic dependence on excitation current below a threshold, with both its magnitude and nonlinear coefficient strongly correlated with the superconducting state. This nonlinear response is semiquantitatively captured by the superconducting fluctuation within the time-dependent Ginzburg-Landau theory, where nonlinear transport arises due to fluctuating Cooper pairs. Our results demonstrate that third-order nonlinear transport serves as a sensitive probe of superconducting transitions in percolative systems and establish a foundation for exploring higher-order transport phenomena in strongly correlated systems.

cond-mat.mes-hall↗

arXiv2026

Surface-switchable nonreciprocity protected by Fermi arcs in Weyl semimetal TaAs

Weyl semimetals host topologically protected surface states, known as Fermi arcs, which connect bulk Weyl nodes in momentum space. Both bulk Weyl nodes and Fermi arcs are anticipated to be chiral. The chirality of bulk bands has been confirmed through observations of the chiral anomaly and Weyl orbits. In contrast, despite their discovery more than a decade ago, the chiral nature of Fermi arcs has remained unresolved. Here we report Fermi-arc-induced nonlinear transport in the archetypal Weyl semimetal TaAs. Using focused ion beam techniques, we fabricated micro-scale devices that enable simultaneous transport measurements on opposing topological surfaces. While linear transport remains dominated by bulk conduction, nonlinear transport uncovers surface-specific contributions, including an exceptionally large third-order nonreciprocal response that exceeds conventional expectations and highlights the crucial role of the singular arc endpoints. Our findings unambiguously demonstrate the chiral nature of Fermi arcs and establish nonlinear transport as a direct probe of these topological surface states. By revealing a surface-switchable, room-temperature nonlinear response that is topologically protected, this work introduces a new functionality in Weyl semimetals. Given the abundance of natural materials predicted to host topological semimetal states, these results open opportunities for exploring nonlinear transport phenomena and device concepts across a broad class of systems.

cond-mat.mes-hall↗

arXiv2026

Millimeter-Scale, Atomically Controlled 2D Topological Insulators Revealed by Multimodal Spectroscopy

Quantum spin Hall insulators, or synonymously known as 2D topological insulators, are crucial 2D systems hosting topologically protected edge states. The working temperature of this topological quantum phase is dictated by the inverted bandgap. However, the previously identified large-gap 2D topological insulators are either extremely chemically unstable, or cannot be made with atomistic precision over macroscopic scales. Here, we establish two-quintuple-layer Bi2Te3 and MnBi2Te4/Bi2Te3 heterostructures as atomically controlled, millimeter-scale 2D topological insulators, enabled by precision layer-by-layer growth that yields a carpet-like morphology extending coherently over macroscopic distances. This carpet-like growth mode renders the films amenable to mechanical exfoliation and subsequent wet or dry transfer. Multimodal spectroscopies and microscopies reveal the integer-layer tuned electronic structure of (Bi2Te3)n with excellent agreement to theory. Photon-energy-dependent photoemission and time-resolved photoemission identify band inversion and band dynamics, respectively, while scanning tunneling spectroscopy resolves topological edge states, characteristic of the 2D topological insulator phase. Thickness- and photon-energy-dependent photoemission further validates MnBi2Te4/Bi2Te3 as a robust 2D topological insulator. The large inverted gaps of ~100 meV in (Bi2Te3)2 and ~150 meV in MnBi2Te4/Bi2Te3 suggest operation near ambient temperature. These results define a scalable materials platform for next-generation, low-loss quantum and energy-efficient devices.

cond-mat.mtrl-sci↗

arXiv2025

Tri-component-pairing chiral superconductivity on the honeycomb lattice with mixed $s$- and $d$-wave symmetries

In this work, we investigate chiral topological superconductors on a two-dimensional honeycomb lattice with coexisting $d_{x^2-y^2}$, $d_{xy}$, and $s$-wave pairing symmetries. Using a Ginzburg-Landau free energy analysis, the pairing gap function is shown to exhibit a tri-component form $s+d_{x^2-y^2}e^{iϕ_1}+d_{xy}e^{iϕ_2}$, where $ϕ_1$ and $ϕ_2$ are phase differences between the $d$- and $s$-wave pairing components, which spontaneously breaks both time reversal and $C_6$ rotational symmetries. Chern numbers of the energy bands are calculated to be nonzero, demonstrating the topologically nontrivial nature of the system. The anomalous AC Hall conductivity is computed, which is not invariant under $C_6$ rotations, reflecting the anisotropic nature of the pairing gap function. Fractional magnetic vortices are also discussed, arising from the multi-component nature of the pairing gap function.

cond-mat.supr-con↗

arXiv2025

Nonreciprocal Transport with Quantum Geometric Origin in Layered Hybrid Perovskite

Quantum geometry quantifies how the electron wavefunction evolves distinctly from conventional transport theory. In noncentrosymmetric materials, nonreciprocal transport with quantum geometric origin remains prominent with localized charge independent of vanished group velocity. The discovery of such nonreciprocal and nonlinear responses was realized by recent advances in two-dimensional materials. As a promising candidate, the electronic structure and symmetry of layered hybrid perovskites can be deliberately designed and manipulated by incorporating selected organic ligands. Despite the observation of exotic photogalvanic effects and chiral optical effects, the underlying mechanism how these nonlinear responses are enabled in the multi-quantum well structures remained unclear. Here we demonstrated the quantum geometric origin for interlayer spontaneous photocurrent in (PEA)2PbI4. Contrary to assumptions that charge transport across the 2D planes is limited, we observed a spontaneous photocurrent along this crystalline orientation. Theoretical analysis using a tight-binding model identifies shift current as the microscopic origin. This quantum geometric effect is enabled by ionic displacements from centrosymmetric coordinates and enhanced by multiband transition high-density bands of the layered hybrid crystal. We anticipate that such unique low-dimensional systems with structure can provide fertile ground for discovering novel optoelectronic functionalities.

cond-mat.mtrl-sci↗

arXiv2025

In-plane anomalous features in the 3D quantum Hall regime

Studies of the 3D quantum Hall effect (QHE) have primarily emphasized transport features that mimic the well-established 2D QHE. In this work, we show that qualitatively new features arise when an in-plane magnetic field is applied to a 3D Weyl semimetal in the quantum Hall regime. An unexpected Hall quantum oscillation, distinct from the Weyl-orbit oscillation, coexists with the QHE, along with an unquantized two-terminal magnetoresistance. Moreover, unconventional antichiral transmission enables a peculiar disorder-robust negative longitudinal resistance. Quantization tunable by the lead configuration is further found in this transport geometry. A unique type of nonlocal quantum backscattering channels underlies these phenomena. Our work demonstrates a breakdown of the topological characterization of transport even with 3D Chern numbers and reveals hidden 3D QHE transport properties. It opens a new class of transport measurements and phenomena.

cond-mat.mes-hall↗

arXiv2025

Rich unconventional Hall effects in a single quasi-kagome Kondo Weyl semimetal candidate Ce$_3$TiSb$_5$

It is generally believed that electronic correlation, geometric frustration, and topology, \textit{individually}, can facilitate the emergence of various intriguing properties that have attracted a broad audience for both fundamental research and potential applications. Here, we report a series of unconventional Hall effects observed in a \textit{single} compound - quasi-kagome Kondo Weyl semimetal candidate Ce$_3$TiSb$_5$. In the paramagnetic phase, signature of dynamic $c$-$f$ hybridization is revealed by a reduction of anomalous Hall effect and is connected to frustration-promoted incoherent Kondo scattering. A large topological Hall effect exceeding 0.2 $μΩ\cdot$cm is found at low temperatures, which should be ascribed to the non-collinear magnetic texture. In addition, a peculiar loop-shaped Hall effect with switching chirality is also seen, which is inferred to be associated with magnetic domain walls that pin history-dependent spin chirality and / or Fermi-arc surface states projected from the in-gap Weyl nodes. These exotic results place Ce$_3$TiSb$_5$ in a regime of highly-frustrated antiferromagnetic dense Kondo lattice with a nontrivial topology on an ``extended" global phase diagram, and highlight the interplay among electronic correlation, geometric frustration and topology.

cond-mat.str-el↗

arXiv2025

Floquet spin textures in optically pumped non-Hermitian surface states

Optical effects of quantum matter with interaction are key to physics and technology. The class of non-Hermitian (NH) phenomena is mostly explored in cold atoms, photonics, and metamaterials out of equilibrium. Effective NH systems due to interaction in equilibrium solids, however, provide a unique opportunity for realizing light-NH matter hybrids via periodic irradiation. Given NH topological surface states with magnetic disorder, here we reveal spectroscopically observable Floquet spin textures for this hybrid quantum matter: merged meron strings, dichroic skyrmions, and domain structure accompanying vortices in energy planes; Bloch lines and topologically twisted vortex rings distinct from Hopfions in energy-momentum space; topological selectiveness of linear polarization occurs besides circular dichroism. Spectroscopic energy evolution and chemical potential dependence are key ingredients of this open hybrid system. With spin-resolved photoemission spectroscopy, this scenario bears prime physical interest by reaching the crossroad between solid-state interaction effects, non-Hermiticity, and light-matter coupling.

cond-mat.mes-hall↗

arXiv2025

Mechanical resonant sensing of spin texture dynamics in a two-dimensional antiferromagnet

The coupling between the spin degrees of freedom and macroscopic mechanical motions, including striction, shearing, and rotation, has attracted wide interest with applications in actuation, transduction, and information processing. Experiments so far have established the mechanical responses to the long-range ordered or isolated single spin states. However, it remains elusive whether mechanical motions can couple to a different type of magnetic structure, the non-collinear spin textures, which exhibit nanoscale spatial variations of spin (domain walls, skyrmions, etc.) and are promising candidates to realize high-speed computing devices. Here, we report the detection of collective spin texture dynamics with nanoelectromechanical resonators made of two-dimensional antiferromagnetic (AFM) MnPS3 with $10^{-9}$ strain sensitivity. By examining radio frequency mechanical oscillations under magnetic fields, new magnetic transitions were identified with sharp dips in resonant frequency. They are attributed to the collective AFM domain wall motions as supported by the analytical modeling of magnetostriction and large-scale spin-dynamics simulations. Additionally, an abnormally large modulation in the mechanical nonlinearity at the transition field infers a fluid-like response due to the ultrafast domain motion. Our work establishes a strong coupling between spin texture and mechanical dynamics, laying the foundation for electromechanical manipulation of spin texture and developing quantum hybrid devices.

cond-mat.mes-hall↗

arXiv2024

This took us a Weyl: synthesis of a semimetallic Weyl ferromagnet with point Fermi surface

Quantum materials governed by emergent topological fermions have become a cornerstone of physics. Dirac fermions in graphene form the basis for moiré quantum matter, and Dirac fermions in magnetic topological insulators enabled the discovery of the quantum anomalous Hall effect. In contrast, there are few materials whose electromagnetic response is dominated by emergent Weyl fermions. Nearly all known Weyl materials are overwhelmingly metallic, and are largely governed by irrelevant, conventional electrons. Here we theoretically predict and experimentally observe a semimetallic Weyl ferromagnet in van der Waals (Cr,Bi)$_2$Te$_3$. In transport, we find a record bulk anomalous Hall angle $> 0.5$ along with non-metallic conductivity, a regime sharply distinct from conventional ferromagnets. Together with symmetry analysis, our data suggest a semimetallic Fermi surface composed of two Weyl points, with a giant separation $> 75\%$ of the linear dimension of the bulk Brillouin zone, and no other electronic states. Using state-of-the-art crystal synthesis techniques, we widely tune the electronic structure, allowing us to annihilate the Weyl state and visualize a unique topological phase diagram exhibiting broad Chern insulating, Weyl semimetallic and magnetic semiconducting regions. Our observation of a semimetallic Weyl ferromagnet offers an avenue toward novel correlated states and non-linear phenomena, as well as zero-magnetic-field Weyl spintronic and optical devices.

cond-mat.mes-hall↗

arXiv2024

Nonmonotonic Hall effect of Weyl semimetals under magnetic field

Hall effect of topological quantum materials often reveals essential new physics and possesses potential for application. Magnetic Weyl semimetal is one especially interesting example that hosts an interplay between the spontaneous time-reversal symmetry-breaking topology and the external magnetic field. However, it is less known beyond the anomalous Hall effect thereof, which is unable to account for plenty of magnetotransport measurements. We propose a new Hall effect characteristically nonmonotonic with respect to the external field, intrinsic to the three-dimensional Weyl topology and free from chemical potential fine-tuning. Two related mechanisms from the Landau level bending and chiral Landau level shifting are found, together with their relation to Shubnikov-de Hass effect. This field-dependent Hall response, universal to thin films and bulk samples, provides a concrete physical picture for existing measurements and is promising to guide future experiments.

cond-mat.mes-hall↗

arXiv2024

Surface spectroscopy and surface-bulk hybridization of Weyl semimetals

Weyl semimetal showing open-arc surface states is a prominent example of topological quantum matter in three dimensions. With the bulk-boundary correspondence present, nontrivial surface-bulk hybridization is inevitable but less understood. Spectroscopies have been often limited to verifying the existence of surface Fermi arcs, whereas its spectral shape related to the hybridization profile in energy-momentum space is not well studied. We present an exactly solvable formalism at the surface for a wide range of prototypical Weyl semimetals. The resonant surface state and the bulk influence coexist as a surface-bulk hybrid and are treated in a unified manner. Directly accessible to angle-resolved photoemission spectroscopy, we analytically reveal universal information about the system obtained from the spectroscopy of resonant topological states. We systematically find inhomogeneous and anisotropic singular responses around the surface-bulk merging borderline crossing Weyl points, highlighting its critical role in the Weyl topology. The response in scanning tunneling spectroscopy is also discussed. The results will provide much-needed insight into the surface-bulk-coupled physical properties and guide in-depth spectroscopic investigation of the nontrivial hybrid in many topological semimetal materials.

cond-mat.mes-hall↗

arXiv2024

Electrical switching of spin-polarized light-emitting diodes based on a 2D CrI3/hBN/WSe2 heterostructure

Spin-polarized light-emitting diodes (spin-LEDs) convert the electronic spin information to photon circular polarization, offering potential applications including spin amplification, optical communications, and advanced imaging. The conventional control of the emitted light's circular polarization requires a change in the external magnetic field, limiting the operation conditions of spin-LEDs. Here, we demonstrate an atomically thin spin-LED device based on a heterostructure of a monolayer WSe2 and a few-layer antiferromagnetic CrI3, separated by a thin hBN tunneling barrier. The CrI3 and hBN layers polarize the spin of the injected carriers into the WSe2. With the valley optical selection rule in the monolayer WSe2, the electroluminescence exhibits a high degree of circular polarization that follows the CrI3 magnetic states. Importantly, we show an efficient electrical tuning, including a sign reversal, of the electroluminescent circular polarization by applying an electrostatic field due to the electrical tunability of the few-layer CrI3 magnetization. Our results establish a new platform to achieve on-demand operation of nanoscale spin-LED and electrical control of helicity for device applications.

cond-mat.mes-hall↗

arXiv2024

Distinguishing Surface and Bulk Electromagnetism via Their Dynamics in an Intrinsic Magnetic Topological Insulator

The indirect exchange interaction between local magnetic moments via surface electrons has been long predicted to bolster the surface ferromagnetism in magnetic topological insulators (MTIs), which facilitates the quantum anomalous Hall effect. This unconventional effect is critical to determining the operating temperatures of future topotronic devices. However, the experimental confirmation of this mechanism remains elusive, especially in intrinsic MTIs. Here we combine time-resolved photoemission spectroscopy with time-resolved magneto-optical Kerr effect measurements to elucidate the unique electromagnetism at the surface of an intrinsic MTI MnBi2Te4. Theoretical modeling based on 2D Ruderman-Kittel-Kasuya-Yosida interactions captures the initial quenching of a surface-rooted exchange gap within a factor of two but over-estimates the bulk demagnetization by one order of magnitude. This mechanism directly explains the sizable gap in the quasi-2D electronic state and the nonzero residual magnetization in even-layer MnBi2Te4. Furthermore, it leads to efficient light-induced demagnetization comparable to state-of-the-art magnetophotonic crystals, promising an effective manipulation of magnetism and topological orders for future topotronics.

cond-mat.str-el↗

arXiv2024

$^{27}$Al NMR study of the magnetic Weyl semimetal CeAlGe

Motivated by the recent observations of electronic correlation effect [M. Corasaniti \textit{et al}., Phys. Rev. B \textbf{104}, L121112 (2021)] and topology-stabilized magnetic fluctuations [N. Drucker \textit{et al}., Nat. Commun. \textbf{14}, 5182 (2023)] in the noncentrosymmetric magnetic Weyl semimetal candidate CeAlGe, we performed systematic studies on the local static and dynamic spin susceptibilities by $^{27}$Al nuclear magnetic resonance. Due to the large spin susceptibility from Ce-$4f$ electrons, the theoretically predicted responses from Weyl fermions are overwhelmed. A Knight-shift anomaly is observed below $T^*\sim50$ K, a signature of the onset of coherent Kondo coupling. In addition, an anomalous peak is found in $1/T_1T$ near 15 K, well above the magnetic ordering temperature $T_N \approx 5$ K, which probably is a consequence of topology-stabilized magnetic fluctuations. These results highlight the interplay among electronic correlation, magnetism and band topology in this family of Kondo Weyl semimetals.

cond-mat.str-el↗

arXiv2023

Topological spin textures in electronic non-Hermitian systems

Non-Hermitian systems have been discussed mostly in the context of open systems and nonequilibrium. Recent experimental progress is much from optical, cold-atomic, and classical platforms due to the vast tunability and clear identification of observables. However, their counterpart in solid-state electronic systems in equilibrium remains unmasked although highly desired, where a variety of materials are available, calculations are solidly founded, and accurate spectroscopic techniques can be applied. We demonstrate that, in the surface state of a topological insulator with spin-dependent relaxation due to magnetic impurities, highly nontrivial topological soliton spin textures appear in momentum space. Such spin-channel phenomena are delicately related to the type of non-Hermiticity and correctly reveal the most robust non-Hermitian features detectable spectroscopically. Moreover, the distinct topological soliton objects can be deformed to each other, mediated by topological transitions driven by tuning across a critical direction of doped magnetism. These results not only open a solid-state avenue to exotic spin patterns via spin- and angle-resolved photoemission spectroscopy, but also inspire non-Hermitian dissipation engineering of spins in solids.

cond-mat.mes-hall↗

arXiv2023

Interplay of valley polarized dark trion and dark exciton-polaron in monolayer WSe2

The interactions between charges and excitons involve complex many-body interactions at high densities. The exciton-polaron model has been adopted to understand the Fermi sea screening of charged excitons in monolayer transition metal dichalcogenides. The results provide good agreement with absorption measurements, which are dominated by dilute bright exciton responses. Here we investigate the Fermi sea dressing of spin-forbidden dark excitons in monolayer WSe2. With a Zeeman field, the valley-polarized dark excitons show distinct p-doping dependence in photoluminescence when the carriers reach a critical density. This density can be interpreted as the onset of strongly modified Fermi sea interactions and shifts with increasing exciton density. Through valley-selective excitation and dynamics measurements, we also infer an intervalley coupling between the dark trions and exciton-polarons mediated by the many-body interactions. Our results reveal the evolution of Fermi sea screening with increasing exciton density and the impacts of polaron-polaron interactions, which lay the foundation for understanding electronic correlations and many-body interactions in 2D systems.

cond-mat.mes-hall↗

arXiv2023

Exciton-magnon splitting in van der Waals antiferromagnet MnPS$_3$ unveiled by second-harmonic generation

Ultrafast and coherent generation of magnons is of great significance for high-speed antiferromagnetic spintronics. One possible route is by exciton-magnon pairwise optical excitation. To date, such exciton-magnon transitions have been studied mostly by linear optical means in a limited number of conventional three-dimensional antiferromagnets. Here we investigate this correlated transition in van der Waals antiferromagnet MnPS$_3$ by using resonant second-harmonic generation spectroscopy, a nonlinear optical probe sensitive to the symmetry of electronic and magnetic excitations. Two exciton-magnon peaks are observed, in line with the exciton-induced splitting of magnon density of states predicted by a Koster-Slater type theory, indicating significant exciton-magnon interactions. In addition, a large linear magnetoelectric effect of excitons is observed. These findings provide renewed understandings on the correlation effects in two-dimensional magnets with enhanced quasiparticle scattering cross-sections, and point to potential coherent control among charge, spin and orbital degrees of freedom in two-dimensional magnets by optical means.

cond-mat.str-el↗